Nonclassical state is an essential resource for quantum-enhanced communication, computing and metrology to outperform their classical counterpart. The nonclassical states that can operate at high bandwidth and room temperature while being compatible with quantum memory are highly desirable to enable the scalability of quantum technologies. Here, we present a direct observation of broadband nonclasscal states in a room-temperature light-matter interface, where the atoms can also be controlled to store and interfere with photons. With a single coupling pulse and far off-resonance configuration, we are able to induce a multi-field interference between light and atoms to create the desired nonclassical states by spectrally selecting the two correlated photons out of seven possible emissions. We explicitly confirm the nonclassicality by observing a cross correlation up to 17 and a violation of Cauchy-Schwarz inequality with 568 standard deviations. Our results demonstrate the potential of a state-built-in, broadband and room-temperature light-matter interface for scalable quantum information networks.
Based on the measurement of quantum correlation functions, the quantum statistical properties of spectral measurements are studied for broadband radiation fields. The spectral filtering of light before its detection is compared with the direct detection followed by the spectral analysis of the recorded photocurrents. As an example, the squeezing spectra of the atomic resonance fluorescence are studied for both types of filtering procedures. The conditions for which the detection of the nonclassical signatures of the radiation is possible are analyzed. For the considered example, photocurrent f…
We observe at record-high speed the nonclassical nature of ultra-broadband bi-photons, reducing the measurement time by four orders of magnitude compared to standard techniques of Hong-Ou-Mandel interference or sum-frequency generation. We measure the quantum state of the broadband bi-photons, amplitude and phase, with a pairwise "Mach-Zehnder" quantum interferometer, where bi-photons that are generated in one nonlinear crystal are enhanced (constructive interference) or diminished (destructive interference) in another crystal, depending on the bi-photon phase. We verify the quantum nature of …
We report demonstrations of both quadrature squeezed vacuum and photon number difference squeezing generated in an integrated nanophotonic device. Squeezed light is generated via strongly driven spontaneous four-wave mixing below threshold in silicon nitride microring resonators. The generated light is characterized with both homodyne detection and direct measurements of photon statistics using photon number-resolving transition edge sensors. We measure $1.0(1)$~dB of broadband quadrature squeezing (${\sim}4$~dB inferred on-chip) and $1.5(3)$~dB of photon number difference squeezing (${\sim}7$…
Broadband quantum memories hold great promise as multiplexing elements in future photonic quantum information protocols. Alkali vapour Raman memories combine high-bandwidth storage, on-demand read-out, and operation at room temperature without collisional fluorescence noise. However, previous implementations have required large control pulse energies and suffered from four-wave mixing noise. Here we present a Raman memory where the storage interaction is enhanced by a low-finesse birefringent cavity tuned into simultaneous resonance with the signal and control fields, dramatically reducing the…
Quantum memory capable of stopping flying photons and storing their quantum coherence is essential for scalable quantum technologies. A room-temperature broadband quantum memory will enable the implementation of large-scale quantum systems for real-life applications. Due to either intrinsic high noises or short lifetime, it is still challenging to find a room-temperature broadband quantum memory beyond conceptual demonstration. Here, we present a far-off-resonance Duan-Lukin-Cirac-Zoller (FORD) protocol and demonstrate the broadband quantum memory in room-temperature atoms. We observe a low un…
We propose a scheme in which broadband nanostructures allow to generate squeezed light and entanglement of quantum emitters that are extremely far detuned. It is shown that the reduced fluctuations of the electromagnetic field arising from collective resonance fluorescence provide also a means to detect the entanglement between the emitters. Due to the near-field enhancement in the proposed hybrid systems, these nonclassical effects can be encountered outside both the extremely close separations limiting the observation in free space and narrow frequency bands in high-Q cavities. Our approach …
Nonclassical light sources are highly sought after as they are an integral part of quantum communication and quantum computation devices. Typical sources rely on bulk crystals that are not compact and have limited bandwidth due to phase-matching conditions. In this work, we demonstrate the generation of photon pairs from a free-standing lithium niobate microcube at the telecommunication wavelength through the spontaneous parametric down-conversion process. The maximum photon pair generation rate obtained from a single microcube with the size of ~4 microns is ~80 Hz, resulting in an efficiency …
We analyze the storage and retrieval of intense-broadband pulses with the added effects of Doppler broadening and detuning in a $Λ$ configuration. We compute analytical solutions via the inverse scattering technique and show how the signal field is transferred to a spin-wave in the atomic medium and later retrieved by the interaction of a control pulse. Due to the intensity of the pulses, the pulse area (as defined for self-induced transparency) plays a key role in the interaction, as it determines the location of the spin wave within the medium. Additionally, we compare our results to non-ide…
Proposals for solid state quantum computing are extremely promising as they can be used to built room temperature quantum computers. If such a quantum computer is ever built it would require in-built sources of nonclassical states required for various quantum information processing tasks. Possibilities of generation of such nonclassical states are investigated here for a physical system composed of a monochromatic light coupled to a two-band semiconductor with direct band gap. The model Hamiltonian includes both photon-exciton and exciton-exciton interactions. Time evolution of the relevant bo…
This article reviews recent progress in quasi-phasematched $χ^{(2)}$ nonlinear nanophotonics, with a particular focus on dispersion-engineered nonlinear interactions. Throughout this article, we establish design rules for the bandwidth and interaction lengths of various nonlinear processes, and provide examples for how these processes can be engineered in nanophotonic devices. In particular, we apply these rules towards the design of sources of non-classical light and show that dispersion-engineered devices can outperform their conventional counterparts. Examples include ultra-broadband optica…
We theoretically consider wave mixing under the irradiation of a single qubit by two photon fields. The first signal is a classical monochromatic drive, while the second one is a nonclassical light. Particularly, we address two examples of a nonclassical light: (i) a broadband squeezed light and (ii) a periodically excited quantum superposition of Fock states with 0 and 1 photons. The mixing of classical and nonclassical photon fields gives rise to side peaks due to the elastic multiphoton scattering. We show that side peaks structure is distinct from the situation when two classical fields ar…
A key question of quantum optics is how nonclassical bi-photon correlations at low power evolve into classical coherence at high-power. Direct observation of the crossover from quantum to classical behavior is desirable, but difficult due to the lack of adequate experimental techniques that cover the ultra-wide dynamic range in photon flux from the single photon regime to the classical level. We investigate bi-photon correlations within the spectrum of light generated by broadband four-wave mixing (FWM) over a \emph{large dynamic range of $\sim80dB$ in photon flux} across the classical-to-quan…
Ensembles of alkali or noble-gas atoms at room temperature and above are widely applied in quantum optics and metrology owing to their long-lived spins. Their collective spin states maintain nonclassical nonlocal correlations, despite the atomic thermal motion in the bulk and at the boundaries. Here we present a stochastic, fully-quantum description of the effect of atomic diffusion in these systems. We employ the Bloch-Heisenberg-Langevin formalism to account for the quantum noise originating from diffusion and from various boundary conditions corresponding to typical wall coatings, thus mode…
Semiconductor quantum dots embedded in hybrid circular Bragg gratings are a promising platform for the efficient generation of nonclassical light. The scalable fabrication of multiple devices with similar performance is highly desirable for their practical use as sources of single and entangled photons, while the ability to operate at telecom wavelength is essential for their integration with the existing fiber infrastructure. In this work we combine the promising properties of broadband hybrid circular Bragg gratings with a membrane-transfer process performed on 3" wafer scale. We develop and…
A quantum state light-storage, using a virtual magnetic field through the ac Stark effect is proposed to combine the high overall storage efficiency and large bandwidth employing room temperature atomic vapor. In this approach, which was called the ac Stark Gradient Echo Memory (ASGEM), it has been shown the possibility to employ about a nanosecond ac Stark pulse far detuned (about 127 THz) from D1 line of rubidium and create an atomic media with the possibility to store a photon with about a GHz bandwidth with storage and retrieval efficiency of more than 90%. A contour plot of efficiency as …
We report on the broadband measurement of quantum radiation pressure noise (QRPN) in an optomechanical cavity at room temperature over a broad range of frequencies relevant to gravitational-wave detectors. We show that QRPN drives the motion of a high-reflectivity single-crystal microresonator, which serves as one mirror of a Fabry-Perot cavity. In our measurements QRPN dominates over all other noise between 10 kHz and 50 kHz and scales as expected with the circulating power inside the cavity. The thermal noise of the microresonator, the largest noise source next to the QRPN, is measured and s…
In this paper we experimentally demonstrated a broadband microwave scheme suitable for the multiresonator quan- tum memory-interface. The microwave scheme consists of the system of composed mini-resonators strongly inter- acting with a common broadband resonator coupled with the external microwave waveguide. We have implemented the controllable tuning of the mini-resonator frequencies and coupling of the common resonator with the external waveguide for the implementation of the impedance matched quantum storage. The storage of microwave pulses with an efficiency of 16.3% has been shown experim…
On-chip photon sources carrying orbital angular momentum (OAM) are in demand for high-capacity optical information processing in both classical and quantum regimes. However, currently-exploited integrated OAM sources have been primarily limited to the classical regime. Herein, we demonstrate a room-temperature on-chip integrated OAM source that emits well-collimated single photons, with a single-photon purity of g(2)(0) = 0.22, carrying entangled spin and orbital angular momentum states and forming two spatially separated entangled radiation channels with different polarization properties. The…
We present the reduction and manipulation of quantum radiation pressure noise (QRPN) in an optomechanical cavity with the injection of squeezed light. The optomechanical system consists of a high-reflectivity single-crystal microresonator which serves as one mirror of a Fabry-Perot cavity. The experiment is performed at room temperature and is QRPN dominated between 10 kHz and 50 kHz, frequencies relevant to gravitational wave observatories. We observed a reduction of 1.2 dB in the measurement noise floor with the injection of amplitude squeezed light generated from a below-threshold degenerat…
We demonstrate coherent storage and retrieval of pulsed light using the atomic frequency comb quantum memory protocol in a room temperature alkali vapour. We utilise velocity-selective optical pumping to prepare multiple velocity classes in the $F=4$ hyperfine ground state of caesium. The frequency spacing of the classes is chosen to coincide with the $F'=4 - F'=5$ hyperfine splitting of the $6^2$P$_{3/2}$ excited state resulting in a broadband periodic absorbing structure consisting of two usually Doppler-broadened optical transitions. Weak coherent states of duration $2\,\mathrm{ns}$ are map…
An ensemble of noble-gas nuclear spins is a unique quantum system that could maintain coherence for many hours at room temperature and above, owing to exceptional isolation from the environment. This isolation, however, is a mixed blessing, limiting the ability of these ensembles to interface with other quantum systems coherently. Here we show that spin-exchange collisions with alkali-metal atoms render a quantum interface for noble-gas spins without impeding their long coherence times. We formulate the many-body theory of the hybrid system and reveal a collective mechanism that strongly coupl…
Hanbury Brown-Twiss interference with massively parallel spectral multiplexing for broadband light
Czech Technical University（捷克理工大学）；Technology Innovation Institute（技术创新研究所）；École polytechnique fédérale de Lausanne（洛桑联邦理工学院）；Institute of Physics of Czech Academy of Sciences（捷克科学院物理研究所）；Florida International University（佛罗里达国际大学）
Quantum memory capable of storage and retrieval of flying photons on demand is crucial for developing quantum information technologies. However, the devices needed for long-distance links are quite different from those envisioned for local processing. Here, we present the first hybrid quantum memory enabled network by demonstrating the interconnection and simultaneous operation of two types of quantum memory: an atomic-ensemble-based memory and an all-optical loop memory. The former generates and stores single atomic excitations that can then be converted to single photons; and the latter maps…
Quantum Noise Spectroscopy of Nanoscale Charge Defects in Silicon Carbide at Room Temperature
School of Biomedical Engineering, Division of Life Sciences and Medicine, University of Science and Technology of China（中国科学技术大学生命科学与医学部生物医学工程学院）；Laboratory of Spin Magnetic Resonance, School of Physical Sciences, Anhui Province Key Laboratory of Scientific Instrument Development and Application, University of Science and Technology of China（中国科学技术大学物理学院自旋磁共振实验室、安徽省科学仪器开发与应用重点实验室）；Suzhou Institute for Advanced Research, University of Science and Technology of China（中国科学技术大学苏州高等研究院）；Hefei National Laboratory, University of Science and Technology of China（中国科学技术大学合肥国家实验室）
The generation of nonclassical states of light in miniature chips is a crucial step towards practical implementations of future quantum technologies. Semiconductor materials are ideal to achieve extremely compact and massively parallel systems and several platforms are currently under development. In this context, spontaneous parametric down conversion in AlGaAs devices combines the advantages of room temperature operation, possibility of electrical injection and emission in the telecom band. Here we report on a chip-based AlGaAs source, producing indistinguishable and energy-time entangled ph…
High-order correlations and ultrafast Wigner negativities in bright-squeezed-vacuum-driven high-harmonic generation
Max Planck Institute for the Structure and Dynamics of Matter（马普固体与结构研究所）；Guangdong Technion-Israel Institute of Technology（广东以色列理工学院）；Technion–Israel Institute of Technology（以色列理工学院）；Initiative for Computational Catalysis (ICC), Flatiron Institute（Flatiron研究所计算催化倡议）
Laboratoire Matériaux et Phénomènes Quantiques, Université Paris Cité（量子物质与现象实验室，巴黎西岱大学）；Centre de Nanosciences et Nanotechnologies, Université Paris-Saclay（纳米科学与纳米技术研究中心，巴黎萨克雷大学）；STMicroelectronics（意法半导体）
Characterizing the nitrogen-vacancy center singlet transition and its phonon sideband for absorption-based room-temperature magnetometry
Fraunhofer Institute for Applied Solid State Physics IAF（弗劳恩霍夫应用固体物理研究所）；School of Science, RMIT University（皇家墨尔本理工大学理学院）；College of Staten Island (CUNY)（石溪学院（纽约市立大学））；National Institutes for Quantum Science and Technology (QST)（量子科学技术研究机构）；Physikalisches Institut, Universität Heidelberg（海德堡大学物理研究所）
