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arXiv 1802.04152physics.app-phcond-mat.mes-hall
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基于硅基锗纳米天线的中红外非线性等离子体

Mid Infrared Nonlinear Plasmonics using Germanium Nanoantennas on Silicon Substrates

Marco P. Fischer, Aaron Riede, Kevin Gallacher, Jacopo Frigerio, Giovanni Pellegrini, Michele Ortolani, Douglas J. Paul, Giovanni Isella, Alfred Leitenstorfer, … 展开作者

Marco P. Fischer, Aaron Riede, Kevin Gallacher, Jacopo Frigerio, Giovanni Pellegrini, Michele Ortolani, Douglas J. Paul, Giovanni Isella, Alfred Leitenstorfer, Paolo Biagioni, Daniele Brida

摘要:

我们展示了三次谐波产生等离子体天线制成的高掺杂锗和设计在中红外共振。由于近场增强,结果是在硅衬底上的3和5微米波长之间可调谐的超快、亚衍射、相干光源。为了观察在这个具有挑战性的光谱区域的非线性,一个高功率飞秒激光系统配备参数频率转换与全反射共焦显微镜设置相结合。我们显示了空间分辨地图的线性散射截面和非线性发射的单个隔离天线结构。清晰的三阶功率依赖性以及中红外发射光谱证明了光发射的非线性性质。模拟结果支持了所观察到的双杆天线的谐振长度,并表明天线材料内部的场增强是造成非线性频率混合的原因。

英文摘要:

We demonstrate third harmonic generation in plasmonic antennas made of highly doped germanium and designed to be resonant in the mid infrared. Owing to the near-field enhancement, the result is an ultrafast, sub-diffraction, coherent light source tunable between 3 and 5 micrometer wavelength on a silicon substrate. To observe nonlinearity in this challenging spectral region, a high-power femtosecond laser system equipped with parametric frequency conversion in combination with an all-reflective confocal microscope setup is employed. We show spatially resolved maps of the linear scattering cross section and the nonlinear emission of single isolated antenna structures. A clear third order power dependence as well as the mid-infrared emission spectra prove the nonlinear nature of the light emission. Simulations support the observed resonance length of the double rod antenna and demonstrate that the field enhancement inside the antenna material is responsible for the nonlinear frequency mixing.

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