We discuss the nonlinear Andreev current of an interacting quantum dot coupled to spin-polarized and superconducting reservoirs when voltage and temperature biases are applied across the nanostructure. Due to the particle-hole symmetry introduced by the superconducting (S) lead, the subgap spin current vanishes identically. Nevertheless, the Andreev charge current depends on the degree of polarization in the ferromagnetic (F) contact since the shift of electrostatic internal potential of the conductor depends on spin orientation of the charge carrier. This spin-dependent potential shift characterizes nonlinear responses in our device. We show how the subgap current versus the bias voltage or temperature difference depends on the lead polarization in two cases, namely (i) S-dominant case, when the dot-superconductor tunneling rate ($Γ_R$) is much higher than the ferromagnet-dot tunnel coupling ($Γ_L$), and (ii) F-dominant case, when $Γ_L\gg Γ_R$. For the ferromagnetic dominant case the spin-dependent potential shows a nonmonotonic behavior as the dot level is detuned. Thus the subgap current can also exhibit interesting behaviors such as current rectification and the maximization of thermocurrents with smaller thermal biases when the lead polarization and the quantum dot level are adjusted.
We theoretically describe a thermoelectric effect that is entirely due to Andreev processes involving the formation of Cooper pairs through the coupling of electrons and holes. The Andreev thermoelectric effect can occur in ballistic ferromagnet-superconductor junctions with a dominant superconducting proximity effect on the ferromagnet, and it is very sensitive to surface states emerging in unconventional superconductors. We consider hybrid junctions in two and three dimensions to demonstrate that the thermoelectric current is always reversed in the presence of low-energy Andreev bound states…
We investigate thermoelectric transport through Andreev interferometers. We show that the ratio of the thermal and the charge conductance exhibits large oscillations with the phase difference $ϕ$ between the two superconducting contacts, and that the Wiedemann-Franz law holds only when $ϕ=π$. A large average thermopower furthermore emerges whenever there is an asymmetry in the dwell times to reach the superconducting contacts. When this is the case, the thermopower is odd in $ϕ$. In contrast, when the average times to reach either superconducting contact are the same, the average thermopower i…
We discuss the phase dependent nonlocal thermoelectric effect in a topological Josephson junction in contact with a normal-metal probe. We show that, due to the helical nature of topological edge states, nonlocal thermoelectricity is generated by a purely Andreev interferometric mechanism. This response can be tuned by imposing a Josephson phase difference, through the application of a dissipationless current between the two superconductors, even without the need of applying an external magnetic field. We discuss in detail the origin of this effect and we provide also a realistic estimation of…
We realized point contact spectroscopy experiment on ferromagnet/superconductor bilayers. Differential conductance curves show several features that we explained within Bogoliubov-de Gennes formalism considering the presence of two interfaces in the normal-metal-tip/ferromagnet/superconductor device. We demonstrate that such configuration is suitable as local probe of the spin polarization and thickness of ferromagnetic layer, directly on bilayer areas. This is due to the high sensitivity of the Andreev surface states to the physical properties of the ferromagnetic interlayer.
Ferromagnetic-insulator (FI) based Josephson junctions are promising candidates for a coherent superconducting quantum bit as well as a classical superconducting logic circuit. Recently the appearance of an intriguing atomic-scale 0-pi transition has been theoretically predicted. In order to uncover the mechanism of this phenomena, we numerically calculate the spectrum of Andreev bound states in a FI barrier by diagonalizing the Bogoliubov-de Gennes equation. We show that Andreev spectrum drastically depends on the parity of the FI-layer number L and accordingly the pi (0) state is always more…
We study charge transport through a metallic dot coupled to a superconducting and a ferromagnetic lead with a precessing magnetization due to ferromagnetic resonance. Using the quasiclassical theory, we find that the magnetization precession induces a dc current in the subgap regime even in the absence of a bias voltage. This effect is due to the rectification of the ac spin currents at the interface with the ferromagnet; it exists in the absence of spin current in the superconductor. When the dot is strongly coupled to the superconductor, we find a strong enhancement in a wide range of parame…
We investigate transport and thermoelectric properties of hybrid systems based on a single-level quantum dot and one superconducting lead. The other lead is generally normal-metallic ferromagnet. In the latter case single-particle transport is spin-polarized. Our main interest is in the interplay of Andreev tunneling of Cooper pairs and single-particle tunneling. The latter is responsible for relatively large thermopower and figure of merit due to a diverging density of single-particle states at the superconducting gap edges. System with ferromagnetic and superconducting leads can also reveal …
We investigate the thermoelectric properties of a quantum dot coupled to ferromagnetic and superconducting electrodes. The combination of spin polarized tunneling at the ferromagnetic-quantum dot interface and the application of an external magnetic field that Zeeman splits the dot energy level leads to large values of the thermopower (Seebeck coefficient). Importantly, the thermopower can be tuned with an external gate voltage connected to the dot. We compute the figure of merit that measures the efficiency of thermoelectric conversion and find that it attains high values. We discuss the diff…
Superconducting spintronics is based on the creation of spin-triplet Cooper pairs in ferromagnet-superconductor (F-S) hybrid junctions. Previous proposals to manipulate spin-polarized supercurrents on-demand typically require the ability to carefully control magnetic materials. We, instead, propose a quantum heat engine that generates equal-spin Cooper pairs and drives supercurrents on-demand without manipulating magnetic components. We consider a S-F-S junction, connecting two leads at different temperatures, on top of the helical edge of a two-dimensional topological insulator. Heat and char…
In an unconventional superconductor, the interplay of scattering off impurities and Andreev processes may lead to different scattering times for electronlike and holelike quasiparticles. Such electron-hole asymmetry appears when the impurity scattering phase shift is intermediate between the Born and unitary limits and leads to an expectation for large thermoelectric effects. Here, we examine the thermoelectric response of a $d$-wave superconductor connected to normal-metal reservoirs under a temperature bias using a fully self-consistent quasiclassical theory. The thermoelectrically induced q…
We describe a simple hybrid superconductor$|$ferromagnetic-insulator structure manifesting spin-resolved Andreev bound states in which dynamic magnetization is employed to probe spin related physics. We show that, at low bias and below $T_c$, the transfer of spin angular momentum pumped by an externally driven ferromagnetic insulator is greatly affected by the formation of spin-resolved Andreev bound states. Our results indicate that these bound states capture the essential physics of condensate-facilitated spin flow. For finite thicknesses of the superconducting layer, comparable to the coher…
We discuss the nonlinear current of an interacting quantum dot coupled to normal and superconducting reservoirs with applied voltage and temperature differences. Due to the particle-hole symmetry introduced by the superconducting lead, the pure (subgap) thermoelectric response vanishes. However, we show that the Andreev bound states shift as the thermal gradient increases. As a consequence, the $I$--$V$ characteristic can be tuned with a temperature bias if the system is simultaneously voltage biased. This is a cross effect that occurs beyond linear response only. Furthermore, we emphasize the…
We present thermoelectric measurements of the heat dissipated due to ferromagnetic resonance of a Permalloy strip. A microwave magnetic field, produced by an on-chip coplanar strip waveguide, is used to drive the magnetization precession. The generated heat is detected via Seebeck measurements on a thermocouple connected to the ferromagnet. The observed resonance peak shape is in agreement with the Landau-Lifshitz-Gilbert equation and is compared with thermoelectric finite element modeling. Unlike other methods, this technique is not restricted to electrically conductive media and is therefore…
Co$_3$Sn$_2$S$_2$ has recently emerged as a ferromagnetic Weyl semi-metal. Theoretical investigation of the spin-split bands predicted half metalicity in the compound. Here, we report the detection of a spin polarized supercurrent through a Nb/Co$_3$Sn$_2$S$_2$ point contact where Andreev reflection is seen to be large indicating a large deviation from half metallicity. In fact, analysis of the Andreev reflection spectra reveals only 50\% spin polarization at the Fermi level of Co$_3$Sn$_2$S$_2$. Our theoretical calculations of electronic Density of States (DOS) reveal a spin depolarizing effe…
We present a semiclassical theory of spin-diffusion in a ferromagnetic metal subject to a temperature gradient. Spin-flip scattering can generate pure thermal spin currents by short-circuiting spin channels while suppressing spin accumulations. A thermally induced spin density is locally generated when the energy dependence of the density of states is spin polarized.
We study thermal and charge transport in a three-terminal setup consisting of one superconducting and two ferromagnetic contacts. We predict that the simultaneous presence of spin filtering and of spin- dependent scattering phase shifts at each of the two interfaces will lead to very large nonlocal thermo- electric effects both in clean and in disordered systems. The symmetries of thermal and electric transport coefficients are related to fundamental thermodynamic principles by the Onsager reciprocity. Our results show that a nonlocal version of the Onsager relations for thermoelectric current…
Thermoelectric effects through a serial double quantum dot system weakly coupled to ferromagnetic leads are analyzed. Formal expressions of electrical conductance, thermal conductance, and thermal coefficient are obtained by means of Hubbard operators. The results show that although the thermopower is independent of the polarization of the leads, the figure of merit is reduced by an increase of polarization. The influences of temperature and interdot tunneling on the figure of merit are also investigated, and it is observed that increase of the interdot tunneling strength results in reduction …
The Andreev transport through a quantum dot coupled to two external ferromagnetic leads and one superconducting lead is studied theoretically by means of the real-time diagrammatic technique in the sequential and cotunneling regimes. We show that the tunnel magnetoresistance (TMR) of the Andreev current displays a nontrivial dependence on the bias voltage and the level detuning, and can be described by analytical formulas in the zero temperature limit. The cotunneling processes lead to a strong modification of the TMR, which is most visible in the Coulomb blockade regime. We find a zero-bias a…
By investigating the nonequilibrium transport across a metal/superconductor junction in both nonrelativistic and relativistic cases, we reveal that the asymmetric Andreev reflection with anisotropic superconductors is able to induce the electric and thermal Hall-like effect, in the absence of magnetic field. That is, a longitudinal electric voltage or temperature bias can induce transverse electric or thermal currents merely through the asymmetric Andreev reflection, respectively. In particular, a transverse thermoelectric effect, i.e., the Ettingshausen-like effect, is identified, although th…
Using ab-initio methods we calculate thermoelectric and spin thermoelectric properties of silicene nanoribbons with bare, mono-hydrogenated and di-hydrogenated edges. Asymmetric structures, in which one edge is either bare or di-hydrogenated while the other edge is mono-hydrogenated (0H-1H and 2H-1H nanoribbons) have ferromagnetic ground state and display remarkable conventional and spin thermoelectric properties. Strong enhancement of the thermoelectric efficiency, both conventional and spin ones, results from a very specific band structure of such nanoribbons, where one spin channel is block…
A detailed investigation of the non-equilibrium steady-state electric and thermoelectric transport properties of a quantum dot coupled to the normal metallic and s-wave superconducting reservoirs (N-QD-S) are provided within the Coulomb blockade regime. Using non-equilibrium Keldysh Green's function formalism, initially, various model parameter dependence of thermoelectric transport properties are analysed within the linear response regime. It is observed that the single-particle tunnelling close to the superconducting gap edge can generate a relatively large thermopower and figure of merit. M…
Using the Bogoliubov de-Gennes formalism, we investigate the charge and spin-dependent thermoelectric effects in superconductor graphene junctions. Results demonstrate that despite normal-superconductor junctions, there is a temperature-dependent spin thermopower both in the graphene-based ferromagnetic-superconductor (F-S) and ferromagnetic-Rashba spin-orbit region-superconductor (F-RSO-S) junctions. It is also shown that in the presence of Rashba spin-orbit interaction, the charge and spin-dependent Seebeck coefficients can reach to their maximum up to 3.5$k_B/e$ and 2.5$k_B/e$, respectively…
In this work, it is considered a nanostructure composed by a quantum dot coupled to two ferromagnets and a superconductor. The transport properties of this system are studied within a generalized mean-field approximation taking into account proximity effects and spin-flip correlations within the quantum dot. It is shown that the zero-bias transmittance for the co-tunneling between the ferromagnetic leads presents a dip whose height depends on the relative orientation of the magnetizations. When the superconductor is coupled to the system, electron-hole correlations between different spin state…
The thermoelectric performance of a topological Josephson nonlocal heat engine is thoroughly investigated. The nonlocal response is obtained by using a normal metal probe coupled with only one of the proximized helical edges in the middle of the junction. In this configuration, we investigate how the flux bias and the phase bias trigger the nonlocal thermoelectric effects under the application of a thermal difference between the superconducting terminals. Possible experimental nonidealities such as asymmetric proximized superconducting gaps are considered showing how the nonlocal response can …
Crossed Andreev reflection in a lateral spin valve geometry device is an aspect of considerable recent interest, particularly with regards to Cooper pair splitting experiments to realize solid state quantum entanglement. In this work, devices are fabricated consisting of two ferromagnetic permalloy (Py) electrodes contacted by a overlaid perpendicular superconducting Ta electrode, of variable lateral in-plane offset within the expected BCS superconducting coherence length $ξ_0$. Experimental electrical transport measurements are presented of local and nonlocal conduction, showing characteristi…
We report on large thermoelectric effects in superconductor-ferromagnet tunnel junctions in proximity contact with the ferromagnetic insulator europium sulfide. The combination of a spin-splitting field and spin-polarized tunnel conductance in these systems breaks the electron-hole symmetry and leads to spin-dependent thermoelectric currents. We show that the exchange splitting induced by the europium sulfide boosts the thermoelectric effect in small applied fields and can therefore eliminate the need to apply large magnetic fields, which might otherwise impede applications in thermometry or c…
Thermoelectric transport across normal-metal/helical-multiferroic/ferromagnetic heterojunctions is theoretically investigated. We find a anisotropic charge and spin thermopower with a $C_{2v}$ symmetry. The angular dependence on the magnetization orientation of the ferromagnetic layer is substantiated by a phenomenological theory based on the symmetry of the effective spin-orbit interaction induced by the topology of the spiral magnetic order in the multiferroic barrier.
We present an exhaustive study of Andreev crystals (ACs) -- quasi-one-dimensional superconducting wires with a periodic distribution of magnetic regions. The exchange field in these regions is assumed to be much smaller than the Fermi energy. Hence, the transport through the magnetic region can be described within the quasiclassical approximation. In the first part of the paper, by assuming that the separation between the magnetic regions is larger than the coherence length, we derive the effective nearest-neighbour tight-binding equations for ACs with a helical magnetic configuration. The spe…
We report on the experimental observation of nonlocal spin-dependent thermoelectric effects in superconductor-ferromagnet multiterminal structures. Our samples consist of a thin superconducting aluminum wire with several ferromagnetic tunnel junctions attached to it. When a thermal excitation is applied to one of the junctions in the presence of a Zeeman splitting of the density of states of the superconductor, a thermoelectric current is observed in remote junctions at distances exceeding $10~\mathrm{μm}$. The results can be explained by recent theories of coupled spin and heat transport in h…
We investigate the nonlocal thermoelectric transport in a Cooper-pair splitter based on a double-quantum-dot-superconductor three-terminal hybrid structure. We find that the nonlocal coupling between the superconductor and the quantum dots gives rise to nonlocal thermoelectric effects which originate from the nonlocal particle-hole breaking of the system. We show that Cooper-pair splitting induces the generation of a thermo-current in the superconducting lead without any transfer of charge between the two normal metal leads. Conversely, we show that a nonlocal heat exchange between the normal …
We investigate the charge and spin transport of a voltage-biased superconducting point contact coupled to a nanomagnet. The magnetization of the nanomagnet is assumed to precess with the Larmor frequency, $ω_L$, due to ferromagnetic resonance. The interplay between the ac Josephson current and the magnetization dynamics leads to spin-polarized Shapiro steps at voltages $|V|=\hbar ω_L/2en$ for $n=1,2,...$ and the subharmonic steps with $n>1$ are a consequence of multiple Andreev reflection (MAR). Moreover, the spin-precession-assisted MAR generates quasiparticle scattering amplitudes that, due …
The accurate and proper form of electron-hole excitations and corresponding Dirac-like spinors of monolayer molybdenum disulfide superconductor are exactly obtained. Andreev reflection and resulting subgap conductance in a $MoS_2$-based ferromagnetic superconducting (F/S) junction is accurately investigated in terms of dynamical characteristics of system. Due to spin-splitting energy gap in the valence band and nondegenerate $K$ and $K'$ valleys, the ferromagnetic exchange energy $σh$ can cause a distinct behavior of Andreev process between spin-up and spin-down charge carriers belonging to di…
We study a periodic arrangement of magnetic regions in a one-dimensional superconducting wire. Due to the local exchange field, each region supports Andreev bound states that hybridize forming Bloch bands in the subgap spectrum of what we call the Andreev crystal (AC). As an illustration, ACs with ferromagnetic and antiferromagnetic alignment of the magnetic regions are considered. We relate the spectral asymmetry index of a spin-resolved Hamiltonian to the spin polarization and identify it as the observable that quantifies the closing and reopening of the excitation gap. In particular, antife…
We investigate the current cross-correlations in a double quantum dot based Cooper pair splitter coupled to one superconducting and two ferromagnetic electrodes. The analysis is performed by assuming a weak coupling between the double dot and ferromagnetic leads, while the coupling to the superconductor is arbitrary. Employing the perturbative real-time diagrammatic technique, we study the Andreev transport properties of the device, focusing on the Andreev current cross-correlations, for various parameters of the model, both in the linear and nonlinear response regimes. Depending on parameters…
We study the spin-resolved subgap transport in a triple quantum-dot system coupled to one superconducting and two ferromagnetic leads. We examine the Andreev processes in the parallel and antiparallel alignments of ferromagnets magnetic moments in both the linear and nonlinear response regimes. The emphasis is put on the analysis of the current cross-correlations between the currents flowing through the left and right arms of the device and relevant electron waiting time distributions. We show that both quantities can give an important insight into the subgap transport processes and their anal…
Spin-polarized transport through a double quantum dot system attached to a common superconducting lead and two ferromagnetic electrodes (fork geometry) is investigated theoretically. The key objective of the analysis is to describe the influence of electrodes' ferromagnetism on the Andreev tunneling. Both direct and crossed Andreev tunneling processes are considered, in general. The other objective is a detailed analysis of the role of Coulomb interaction and its impact on the Andreev tunneling processes.
