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arXiv 1704.08477cond-mat.mes-hall
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揭示GaAs纳米级膜的大尺度均匀性和痕量杂质灵敏度

Revealing large-scale homogeneity and trace impurity sensitivity of GaAs nanoscale membranes

Z. Yang, A. Surrente, G. Tutuncuoglu, K. Galkowski, M. Cazaban-Carraze, F. Amaduzzi, P. Leroux, D. K. Maude, A. Fontcuberta i Morral, P. Plochocka

摘要:

III-V族纳米结构有可能彻底改变光电子学和能量收集。为了使这成为现实,应该解决诸如可再现性和对缺陷的敏感性等关键问题。通过讨论分子束外延生长的GaAs纳米膜的光学性质,我们强调了几个功能,使他们更接近大规模的应用。无帽膜表现出非常高的光学质量,表示为非常窄的中性激子发射,允许分辨率的更复杂的激子结构的第一次。用AlGaAs壳层覆盖膜导致发射强度的强烈增加,但也导致激子峰的移位和加宽。这归因于壳中存在超出MBE级质量的杂质,表明这些结构对杂质存在的高度敏感性。最后,发射性能在亚微米和亚毫米尺度下是相同的,证明了这些结构用于大规模应用的潜力。

英文摘要:

III-V nanostructures have the potential to revolutionize optoelectronics and energy harvesting. For this to become a reality, critical issues such as reproducibility and sensitivity to defects should be resolved. By discussing the optical properties of MBE grown GaAs nanomembranes we highlight several features that bring them closer to large scale applications. Uncapped membranes exhibit a very high optical quality, expressed by extremely narrow neutral exciton emission, allowing the resolution of the more complex excitonic structure for the first time. Capping of the membranes with an AlGaAs shell results in a strong increase of emission intensity but also to a shift and broadening of the exciton peak. This is attributed to the existence of impurities in the shell, beyond MBE-grade quality, showing the high sensitivity of these structures to the presence of impurities. Finally, emission properties are identical at the sub-micron and sub-millimeter scale, demonstrating the potential of these structures for large scale applications.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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