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arXiv 1703.04573cond-mat.str-elcond-mat.stat-mech
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受抑铁磁自旋- $1/2$海森堡链的热力学:链间耦合的作用

Thermodynamics of frustrated ferromagnetic spin-$1/2$ Heisenberg chains: The role of inter-chain coupling

P. Müller, J. Richter, D. Ihle

摘要:

用自旋转动不变格林函数方法研究了耦合阻挫铁磁链的热力学。我们考虑了一个各向同性的海森堡自旋半系统,其最近邻之间存在铁磁链内耦合$J_1<0$,而次近邻链内存在反铁磁链内耦合$J_2>0$。我们专注于中等强度的挫折$J_2 < |J_1|/4$,使链中的自旋自旋相关主要是铁磁性。我们考虑两个链间耦合(IC)$J_{\perp,y}$和$J_{\perp,z}$,对应于两个轴垂直于链,铁磁以及反铁磁IC考虑。我们讨论了阻挫效应对反铁磁集成电路基态性质的影响,其中基态是量子性质的。我们研究的主要部分是致力于有限温度特性。我们计算的临界温度$T_{c}$作为竞争交换耦合$J_{2},J_{\perp,y}, J_{\perp,z}$的函数。我们发现,对于固定的IC $T_c$单调减少增加挫折$J_2$,其中作为$J_2 \to |J_1|/4$的$T_c(J_2)$曲线迅速下降。为了表征$T_c$上下的磁序,我们计算了自旋-自旋关联函数$\langle {\bf S}_0 {\bf S}_{\bf R} \rangle$、磁序参数$M$、均匀静态磁化率$χ_0$以及关联长度$ξ$ .此外,我们还讨论了比热$C_V$和激发光谱$ω_{\mathbf{q}}$的温度依赖性。随着温度的升高,$J_2 \to |J_1|/4$的链内自旋刚度(铁磁IC)和链内自旋波速度(反铁磁IC)都增加。

英文摘要:

The thermodynamics of coupled frustrated ferromagnetic chains is studied within a spin-rotation-invariant Green's function approach. We consider an isotropic Heisenberg spin-half system with a ferromagnetic in-chain coupling $J_1<0$ between nearest neighbors and a frustrating antiferromagnetic next-nearest neighbor in-chain coupling $J_2>0$. We focus on moderate strength of frustration $J_2 < |J_1|/4$ such that the in-chain spin-spin correlations are predominantly ferromagnetic. We consider two inter-chain couplings (ICs) $J_{\perp,y}$ and $J_{\perp,z}$, corresponding to the two axis perpendicular to the chain, where ferromagnetic as well as antiferromagnetic ICs are taken into account. We discuss the influence of frustration on the ground-state properties for antiferromagnetic ICs, where the ground state is of quantum nature. The major part of our study is devoted to the finite-temperature properties. We calculate the critical temperature $T_{c}$ as a function of the competing exchange couplings $J_{2},J_{\perp,y}, J_{\perp,z}$. We find that for fixed ICs $T_c$ monotonically decreases with increasing frustration $J_2$, where as $J_2 \to |J_1|/4$ the $T_c(J_2)$-curve drops down rapidly. To characterize the magnetic ordering below and above $T_c$ we calculate the spin-spin correlation functions $\langle {\bf S}_0 {\bf S}_{\bf R} \rangle$, the magnetic order parameter $M$, the uniform static susceptibility $χ_0$ as well as the correlation length $ξ$. Moreover, we discuss the specific heat $C_V$ and the temperature dependence of the excitation spectrum $ω_{\mathbf{q}}$. As $J_2 \to |J_1|/4$ some unusual frustration-induced features were found, such as an increase of the in-chain spin stiffness (in case of ferromagnetic ICs) or of the in-chain spin-wave velocity (in case of antiferromagnetic ICs) with growing temperature.

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