We investigate the generation of entanglement (spin squeezing) in an optical-transition atomic clock through the coupling to a vacuum electromagnetic field that is enhanced by an optical cavity. We show that if each atom is prepared in a superposition of the ground state and a long-lived electronic excited state, and viewed as a spin-1/2 system, then the collective vacuum light shift entangles the atoms, resulting in a squeezed distribution of the ensemble collective spin. This scheme reveals that even a vacuum field can be a useful resource for entanglement and quantum manipulation. The method is simple and robust since it requires neither the application of light nor precise frequency control of the ultra-high-finesse cavity. Furthermore, the scheme can be used to implement two-axis twisting by rotating the spin direction while coupling to the vacuum, resulting in stronger squeezing.
When linearly polarized light propagates through a medium in which elliptically polarized light would undergo self-rotation, squeezed vacuum can appear in the orthogonal polarization. A simple relationship between self-rotation and the degree of vacuum squeezing is developed. Taking into account absorption, we find the optimum conditions for squeezing in any medium that can produce self-rotation. We then find analytic expressions for the amount of vacuum squeezing produced by an atomic vapor when light is near-resonant with a transition between various low-angular-momentum states. Finally, we …
We use the vacuum Rabi splitting to perform quantum nondemolition (QND) measurements that prepare a conditionally spin-squeezed state of a collective atomic psuedo-spin. We infer a 3.4(6) dB improvement in quantum phase estimation relative to the standard quantum limit for a coherent spin state composed of uncorrelated atoms. The measured collective spin is composed of the two-level clock states of nearly 10^6 Rb-87 atoms confined inside a low finesse F = 710 optical cavity. This technique may improve atomic sensor precision and/or bandwidth, and may lead to more precise tests of fundamental p…
We report the generation of optical squeezed vacuum states by means of polarization self-rotation in rubidium vapor following a proposal by Matsko et al. [Phys. Rev. A 66, 043815 (2002)]. The experimental setup, involving in essence just a diode laser and a heated rubidium gas cell, is simple and easily scalable. A squeezing of 0.85+-0.05 dB was achieved.
We study a squeezed vacuum field generated in hot Rb vapor via the polarization self-rotation effect. Our previous experiments showed that the amount of observed squeezing may be limited by the contamination of the squeezed vacuum output with higher-order spatial modes, also generated inside the cell. Here, we demonstrate that the squeezing can be improved by making the light interact several times with a less dense atomic ensemble. With optimization of some parameters we can achieve up to -2.6 dB of squeezing in the multi-pass case, which is 0.6 dB improvement compared to the single-pass expe…
We observed squeezed vacuum light at 795 nm in 87Rb vapor via resonant polarization self-rotation, and report noise sidebands suppression of ~1 dB below shot noise level spanning from acoustic (30 kHz) to MHz frequencies. This is the first demonstration of sub-MHz quadrature vacuum squeezing in atomic systems. The spectral range of observed squeezing matches well typical bandwidths of electromagnetically induced transparency (EIT) resonances, making this simple technique for generation of optical fields with non-classical statistics at atomic transitions wavelengths attractive for EIT-based qu…
The squeezing spectrum of the fluorescence field emitted from a four-level atom in $J=1/2$ to $J=1/2$ configuration driven by two coherent fields is studied. We find that the squeezing properties of the fluorescence radiation are significantly influenced by the presence of vacuum-induced coherence in the atomic system. It is shown that such coherence induces spectral squeezing in phase quadratures of the fluorescence light for both weak and strong driving fields. The dependence of the squeezing spectrum on the relative phase of the driving fields is also investigated. Effects such as enhanceme…
A Josephson parametric amplifier (JPA) can create squeezed states of microwave light, lowering the noise associated with certain quantum measurements. We experimentally study how the JPA's pump influences the phase-sensitive amplification and deamplification of a coherent tone's amplitude when that amplitude is commensurate with vacuum fluctuations. We predict and demonstrate that by operating the JPA with a pump power greater than the value that maximizes gain, the amplifier distortion is reduced and consequently squeezing is improved. Optimizing the JPA's operation in this fashion, we direct…
In this paper, we theoretically investigate the displacement and momentum fluctuations spectra of the movable mirror in a standard optomechanical system driven by a finite bandwidth squeezed vacuum light accompanying a coherent laser field. Two cases in which the squeezed vacuum is generated by degenerated and non-degenerate parametric oscillators (DPO and NDPO) are considered. We find that for the case of finite bandwidth squeezed vacuum injection, the two spectra exhibit unique features, which strongly differ from those of broadband squeezing excitation. In particular, the spectra exhibit a …
It is commonly agreed that the electromagnetic vacuum is not empty but filled with virtual photons. This leads to effects like Lamb shift and spontaneous emission. Here we argue that if the vacuum has virtual photons it might mean that it is very weakly squeezed and therefore the electromagnetic field is not in its ground state (vacuum) but in an excited dark state. We suggest a stringent test relying on measuring various properties of the electromagnetic field to exclude this yet-untested squeezing hypothesis. This could be done by measuring the number of photons as a function of frequency an…
Three wave mixing vacuum squeezing generation in a SNAIL-based Traveling-Wave Parametric Amplifier with alternated flux polarity
CNR-SPIN（意大利国家研究委员会自旋物理中心）；Dipartimento di Fisica “Ettore Pancini”, Università di Napoli “Federico II,”（那不勒斯费德里科二世大学埃托雷·潘奇尼物理系）；Université Grenoble Alpes, CNRS, Grenoble INP, Institut Néel（格勒诺布尔阿尔卑斯大学）；Dipartimento di Ingegneria Civile e Meccanica (DICEM), Università di Cassino e Lazio Meridionale（卡西诺与拉齐奥南部大学土木机械工程系）；Dipartimento di Ingegneria Elettrica e delle Tecnologie dell’Informazione, Università degli Studi di Napoli Federico II（那不勒斯费德里科二世大学电气与信息技术工程系）
We present the observation of optical fields carrying squeezed vacuum states at sideband frequencies from 10Hz to above 35MHz. The field was generated with type-I optical parametric oscillation below threshold at 1064nm. A coherent, unbalanced classical modulation field at 40MHz enabled the generation of error signals for stable phase control of the squeezed vacuum field with respect to a strong local oscillator. Broadband squeezing of approximately -4dB was measured with balanced homodyne detection. The spectrum of the squeezed field allows a quantum noise reduction of ground-based gravitatio…
We present experimental and theoretical analysis of quantum fluctuation in a vacuum field in the presence of orthogonal linearly polarized pump field propagating through a Rb vapor cell. Previously reported theoretical and experimental studies provided somewhat contradictory conclusions regarding the possibility to observe the "squeezed vacuum" -- the reduction of vacuum fluctuations below standard quantum limit -- in this system. Here, using the D1 transitions of Rb in a cell without buffer as as an example, we demonstrate that vacuum squeezing is corrupted by incoherent processes (such as sp…
Spin squeezing by geometric focusing in vacuum Rabi oscillations
International Center for Quantum Materials, School of Physics, Peking University（北京大学物理学院量子材料中心）；Beijing Key Laboratory of Quantum Devices, Peking University（北京大学量子器件北京市重点实验室）；National Laboratory of Solid State Microstructures and School of Physics, Collaborative Innovation Center of Advanced Microstructures, Nanjing University（南京大学固体微结构物理国家重点实验室、物理学院、现代工程与应用科学协同创新中心）；MIT-Harvard Center for Ultracold Atoms and Research Laboratory of Electronics, Massachusetts Institute of Technology（麻省理工学院电子研究实验室与MIT-哈佛超冷原子中心）
We propose and demonstrate a system that produces squeezed vacuum using a pair of optical parametric amplifiers. This scheme allows the production of phase sidebands on the squeezed vacuum which facilitate phase locking in downstream applications. We observe strong, stably locked, continuous wave vacuum squeezing at frequencies as low as 220 kHz. We propose an alternative resonator configuration to overcome low frequency squeezing degradation caused by the optical parametric amplifiers.
We propose and demonstrate a coherent control scheme for stable phase locking of squeezed vacuum fields. We focus on sideband fields at frequencies from 10Hz to 10kHz which is a frequency regime of particular interest in gravitational wave detection and for which conventional control schemes have failed so far. A vacuum field with broadband squeezing covering this entire band was produced using optical parametric oscillation and characterized with balanced homodyne detection. The system was stably controlled over long periods utilizing two coherent but frequency shifted control fields. In orde…
In a 3-wave mixing process occurring in some nonlinear optical medium when }$a_{1}^{\dagger}${\small mode interacts with both }$a_{2}^{\dagger}% ${\small mode and }$a_{3}^{\dagger}${\small mode, we theoretically study the squeezing effect generated by the operator }$S_{3}\equiv \exp[μ(a_{1}% a_{2}-a_{1}^{\dagger}a_{2}^{\dagger})+ν(a_{1}a_{3}-a_{1}^{\dagger}% a_{3}^{\dagger})]${\small . The new 3-mode squeezed vacuum state in Fock space is derived, and the uncertainty relation for it is demonstrated, It turns out that }$S_{3}${\small may exhibit enhanced squeezing. By virtue of the technique of…
We report on efficient generation of second harmonic laser and single-mode vacuum squeezed light of 795 nm with periodically poled KTiOPO4 (PPKTP) crystals. We achieved 111 mW of ultra-violet (UV) light at 397.5 nm from 191 mW of fundamental light with a PPKTP crystal in a doubling cavity, corresponding to a conversion efficiency of 58.1%. Using the UV light to pump an optical parametric oscillator with a PPKTP crystal, we realized -5.6 dB of a maximum squeezing. We analyzed the pump power dependence of the squeezing level and concluded that the UV light induced losses limit the improvement of…
We present a theoretical study of an ensemble of X-like 4-level atoms placed in an optical cavity driven by a linearly polarized field. We show that the self-rotation (SR) process leads to polarization switching (PS). Below the PS threshold, both the mean field mode and the orthogonal vacuum mode are squeezed. We provide a simple analysis of the phenomena responsible for the squeezing and trace the origin of vacuum squeezing not to SR, but to crossed Kerr effect induced by the mean field. Last, we show that this vacuum squeezing can be interpreted as polarization squeezing.
We have considered a cavity mode driven by coherent light and interacting with a three-level atom available in an open cavity coupled to a vacuum reservoir. We have carried out our analysis by putting the noise operators associated with the vacuum reservoir in normal order. We have also considered the interaction of the three-level atom with the vacuum reservoir outside the cavity. It is found that the squeezing occurs in both the plus and the minus quadratures and the maximum quadrature squeezing happens to be 52.08% and 33.32% below the vacuum state level, respectively. We have established t…
Dissipative generation of spin squeezing in the resolved vacuum Rabi splitting limit
JILA, University of Colorado and National Institute of Standards and Technology（科罗拉多大学与美国国家标准与技术研究院联合JILA研究所）；Department of Physics, University of Colorado（科罗拉多大学物理系）；Center for Theory of Quantum Matter, University of Colorado（科罗拉多大学量子物质理论中心）；T.C.M. Group, Cavendish Laboratory, University of Cambridge（剑桥大学卡文迪许实验室TCM小组）；Institute of Physics（物理研究所）
We have considered the interaction of subharmonic light modes with a three-level atom in a closed cavity coupled to a vacuum reservoir. We carry out analysis by normally ordering the vacuum reservoir noise operators. It so happens that there is perfect quadrature squeezing under certain conditions.
Spin squeezing is a form of entanglement that can improve the stability of quantum sensors operating with multiple particles, by inducing inter-particle correlations that redistribute the quantum projection noise. Previous analyses of potential metrological gain when using spin squeezing were performed on theoretically ideal states, without incorporating experimental imperfections or inherent limitations which result in non-unitary quantum state evolution. Here, we show that potential gains in clock stability are substantially reduced when the spin squeezing is non-unitary, and derive analytic…
We study the interaction of a nearly resonant linearly polarized laser beam with a cloud of cold cesium atoms in a high finesse optical cavity. We show theoretically and experimentally that the cross-Kerr effect due to the saturation of the optical transition produces quadrature squeezing on both the mean field and the orthogonally polarized vacuum mode. An interpretation of this vacuum squeezing as polarization squeezing is given and a method for measuring quantum Stokes parameters for weak beams via a local oscillator is developed.
It was shown by a study of the incoherent part of the low-frequency resonance fluorescence spectrum of the polar quantum emitter driven by semiclassical external laser field and damped by non-squeezed vacuum reservoir that the emitted fluorescence field is squeezed to some degree nevertheless. As was also found, a higher degree of squeezing could, in principle, be achieved by damping the emitter by squeezed vacuum reservoir.
One of the most fundamental quantum states of light is squeezed vacuum, in which noise in one of the quadratures is less than the standard quantum noise limit. Significant progress has been made in the generation of optical squeezed vacuum and its utilization for numerous applications. However, it remains challenging to generate, manipulate, and measure such quantum states in nanophotonics with performances required for a wide range of scalable quantum information systems. Here, we overcome this challenge in lithium niobate nanophotonics by utilizing ultrashort-pulse phase-sensitive amplifiers…
We analyze spin squeezing via Rydberg dressing in optical lattice clocks with random fractional filling. We compare the achievable clock stability in different lattice geometries, including unity-filled tweezer clock arrays and fractionally filled lattice clocks with varying dimensionality. We provide practical considerations and useful tools in the form of approximate analytical expressions and fitting functions to aid in the experimental implementation of Rydberg-dressed spin squeezing. We demonstrate that spin squeezing via Rydberg dressing in one-, two-, and three-dimensional optical latti…
We have developed a quantum memory technique that is completely compatible with current quantum information processing for continuous variables of light, where arbitrary frequency sidebands of a squeezed vacuum can be stored and retrieved using bichromatic electromagnetic induced transparency. 2MHz sidebands of squeezed vacuum pulses with temporal widths of 470ns and a squeezing level of -1.78 +- 0.02dB were stored for 3us in the laser-cooled 87Rb atoms. -0.44 +- 0.02dB of squeezing was retrieved, which is the highest squeezing ever reported for a retrieved pulse.
We study the squeezing as well as the statistical properties of the output radiation from a degenerate parametric oscillator coupled to a squeezed vacuum reservoir employing the stochastic differential equations associated with the normal ordering. It is found that the degree of squeezing of the output radiation is less than the corresponding cavity radiation. However, for output radiation the correlation of the quadrature operators evaluated at different times also exhibits squeezing, which is the reason for quenching of the overall noise in one of the quadrature components of the squeezing s…
Applying stochastic differential equations, we study the squeezing and statistical properties of the cavity and output modes of a degenerate three-level laser whose cavity contains a parametric amplifier and coupled to a squeezed vacuum reservoir. We consider the case in which the top and bottom levels of the three-level cascade atoms injected into the cavity are coupled by the pump mode emerging from the parametric amplifier. It turns out that the presence of the squeezed vacuum reservoir and the parametric amplifier contribute considerably to the mean photon number and the degree of squeezin…
A completely quantum description of Raman process is used to investigate the nonclassical properties of the modes in the stimulated, spontaneous and partially spontaneous Raman process. Both coherent scattering (where all the initial modes are coherent) and chaotic scattering (where initial phonon mode is chaotic and all the other modes are coherent) are studied. Nonclassical character of Raman process is observed by means of intermodal entanglement, single mode and intermodal squeezing of vacuum fluctuations, sub-shot noise and wave variances. Joint photon-phonon number and integrated-intensi…
Using squeezed states it is possible to surpass the standard quantum limit of measurement uncertainty by reducing the measurement uncertainty of one property at the expense of another complementary property. Squeezed states were first demonstrated in optical fields and later with ensembles of pseudo spin-1/2 atoms using non-linear atom-light interactions. Recently, collisional interactions in ultracold atomic gases have been used to generate a large degree of quadrature spin squeezing in two-component Bose condensates. For pseudo spin-1/2 systems, the complementary properties are the different…
Employing the quantum Hamiltonian describing the interaction of two-mode light (signal-idler modes) generated by a nondegenerate parametric oscillator (NDPO) with two uncorrelated squeezed vacuum reservoirs (USVR), we derive the master equation. The corresponding Fokker-Planck equation for the Q-function is then solved employing a propagator method developed in Ref. \cite{1}. Making use of this Q-function, we calculate the quadrature fluctuations of the optical system. From these results we infer that the signal-idler modes are in squeezed states and the squeezing occurs in the first quadratur…
We report an interaction that controls spin squeezing in a collection of spin 1/2 particles. We describe how spin squeezing can be generated and maintained in time. Our scheme can be applied to control the spin squeezing in a Bose condensate with two internal spin states.
A complete set of generalized spin-squeezing inequalities is derived for an ensemble of particles with an arbitrary spin. Our conditions are formulated with the first and second moments of the collective angular momentum coordinates. A method for mapping the spin-squeezing inequalities for spin-1/2 particles to entanglement conditions for spin-j particles is also presented. We apply our mapping to obtain a generalization of the original spin-squeezing inequality to higher spins. We show that, for large particle numbers, a spin-squeezing parameter for entanglement detection based on one of our …
We consider the superpositions of spin coherent states and study the coherence properties and spin squeezing in these states. The spin squeezing is examined using a new version of spectroscopic squeezing criteria. The results show that the antibuching effect can be enhanced and spin squeezing can be generated in the superpositions of two spin coherent states.
We investigate spin squeezing of a two-mode boson system with a Josephson coupling. An exact relation between the squeezing and the single-particle coherence at the maximal-squeezing time is discovered, which provides a more direct way to measure the squeezing by readout the coherence in atomic interference experiments. We prove explicitly that the strongest squeezing is along the $J_z$ axis, indicating the appearance of atom number-squeezed state. Power laws of the strongest squeezing and the optimal coupling with particle number $N$ are obtained based upon a wide range of numerical simulatio…
Conditional homodyne detection of quadrature squeezing is compared with standard nonconditional detection. Whereas the latter identifies nonclassicality in a quantitative way, as a reduction of the noise power below the shot noise level, conditional detection makes a qualitative distinction between vacuum state squeezing and squeezed classical noise. Implications of this comparison for the realistic interpretation of vacuum fluctuations (stochastic electrodynamics) are discussed.
We study spin squeezing, negative correlations, and concurrence in the quantum kicked top model. We prove that the spin squeezing and negative correlations are equivalent for spin systems with only symmetric Dicke states populated. We numerically analyze spin squeezing parameters and concurrence in this model, and find that the maximal spin squeezing direction, which refers to the minimal pairwise correlation direction, is strongly influenced by quantum chaos. Entanglement (spin squeezing) sudden death and sudden birth occur alternatively for the periodic and quasi-periodic cases, while only e…
In this study we investigate the spin squeezing in superposition of a Biaxial state [1,2] and Bell state. Numerical and analytical solutions for the length of mean spin, mean spin direction and spin squeezing are given. It is shown that both the mean spin direction and spin squeezing parameter are determined by the coefficients of superposition and the relative phase.
We evaluate the spin squeezing dynamics of N independent spin-1/2 particles with exchange symmetry. Each spin interacts with its own reservoir, and the reservoirs are independently and identical. The spin squeezing parameter is analytically calculated with different kinds of decoherence. The spin squeezing property vanishes with evolution time under the Markovian decoherence. Whereas coupled to the non-Markovian decoherence channels, the spin squeezing property collapses and revives with time. As spin squeezing can be regarded as a witness of multipartite entanglement, thus our scheme shows th…
The celebrated Majorana representation is exploited to investigate spin squeezing in different classes of pure symmetric states of N qubits with two distinct spinors, namely the Dicke-class of states. On obtaining a general expression for spin squeezing parameter, the variation of squeezing for different configurations is studied in detail.It is shown that the states in the Dicke-class, characterized by two-distinct non-orthogonal spinors, exhibit squeezing.
We report the suitability of an Einstein-Podolsky-Rosen (EPR) entanglement source for gaussian continuous-variable quantum key distribution at 1550 nm. Our source is based on a single continuous-wave squeezed vacuum mode combined with a vacuum mode at a balanced beam splitter. Extending a recent security proof, we characterize the source by quantifying the extractable length of a composable secure key from a finite number of samples under the assumption of collective attacks. We show that distances in the order of 10 km are achievable with this source for a reasonable sample size despite the f…
We study relations between bosonic quadrature squeezing and atomic spin squeezing, and find that the latter reduces to the former in the limit of a large number of atoms for even and odd states. We demonstrate this reduction by treating even and odd spin coherent states, for which analytical solutions are readily obtained, and prove that even spin coherent states always exhibit spin squeezing, whereas odd spin coherent states do not, analogous to the squeezing characteristic of even and odd bosonic coherent states. Finally, we examine the squeezing transfer between photons and atoms via the Di…
We study entanglement and spin squeezing in the ground state of three qubits interacting via the transverse Ising model. We give analytical results for the entanglement and spin squeezing, and a quantitative relation between the concurrence, quantifying the entanglement of two spins, and the spin squeezing parameter, measuring the degree of squeezing. Finally, by appropriately choosing the exchange interaction and strengths of the transverse field, we propose a scheme for generating entangled W state from an unentangled initial state with all spins down.
We analyze the relation between the entanglement and spin-squeezing parameter in the two-atom Dicke model and identify the source of the discrepancy recently reported by Banerjee and Zhou et al that one can observe entanglement without spin squeezing. Our calculations demonstrate that there are two criteria for entanglement, one associated with the two-photon coherences that create two-photon entangled states, and the other associated with populations of the collective states. We find that the spin-squeezing parameter correctly predicts entanglement in the two-atom Dicke system only if it is a…
Weak squeezed vacuum light, especially resonant to the atomic transition, plays an important role in quantum storage and generation of various quantum sources. However, the general homodyne detection (HD) cannot determine weak squeezing due to the low signal to noise ratio and the limited resolution of the HD system. Here we provide an alternative method based on photon statistics measurement to determine the weak squeezing of the squeezed vacuum light generated from an optical parametric oscillator working far below the threshold. The approach is established the relationship between the squee…
We propose a new spin squeezing criterion for arbitrary multi-qubit states that is invariant under local unitary operations. We find that, for arbitrary pure two-qubit states, spin squeezing is equivalent to entanglement, and multi-qubit states are entangled if this new spin squeezing parameter is less than 1.
We study the dynamics of a general multi-emitter system coupled to the squeezed vacuum reservoir and derive a master equation for this system based on the Weisskopf-Wigner approximation. In this theory, we include the effect of positions of the squeezing sources which is usually neglected in the previous studies. We apply this theory to a quasi-one-dimensional waveguide case where the squeezing in one dimension is experimentally achievable. We show that while dipole-dipole interaction induced by ordinary vacuum depends on the emitter separation, the two-photon process due to the squeezed vacuu…
