Increasing the collection efficiency from solid-state emitters is an important step towards achieving robust single photon sources, as well as optically connecting different nodes of quantum hardware. A metallic substrate may be the most basic method of improving the collection of photons from quantum dots, with predicted collection efficiency increases of up to 50%. The established 'method-of-images' approach models the effects of a reflective surface for atomic and molecular emitters by replacing the metal surface with a second fictitious emitter which ensures appropriate electromagnetic boundary conditions. Here, we extend the approach to the case of driven solid-state emitters, where exciton-phonon interactions play a key role in determining the optical properties of the system. We derive an intuitive polaron master equation and demonstrate its agreement with the complementary half-sided cavity formulation of the same problem. Our extended image approach offers a straightforward route towards studying the dynamics of multiple solid-state emitters near a metallic surface.
We show how to create maximal entanglement between spectrally distinct solid-state emitters embedded in a waveguide interferometer. By revealing the rich underlying structure of multi-photon scattering in emitters, we show that a two-photon input state can generate deterministic maximal entanglement even for emitters with significantly different transition energies and line-widths. The optimal frequency of the input is determined by two competing processes: which-path erasure and interaction strength. We find that smaller spectral overlap can be overcome with higher photon numbers, and quasi-m…
The ability to entangle distant quantum nodes is essential for the construction of quantum networks and for quantum information processing. For solid-state quantum emitters used as qubits, it can be achieved by photon interference. When the emitter is subject to spectral diffusion, this process can become highly inefficient, impeding the achievement of scalable quantum technologies. We study two-photon interference in the context of a Hong-Ou-Mandel (HOM)-type experiment for two separate quantum emitters, with different detunings with respect to a specific target frequency. We evaluate the sec…
Coherent quantum optics, where the interaction of a photon with an emitter does not scramble phase coherence, lies at the heart of many quantum optical effects and emerging technologies. Solid-state emitters coupled to nanophotonic waveguides are a promising platform for quantum devices, as this combination is scalable. Yet, reaching full coherence in these systems is challenging due to the dynamics of the solid-state environment of the emitters. Here, we review progress towards coherent light-matter interactions with solid-state quantum emitters coupled to nanophotonic waveguides. We first la…
Purdue University（普渡大学）；Max Planck Institute of Quantum Optics（马克斯·普朗克量子光学研究所）；Munich Center for Quantum Science and Technology（慕尼黑量子科学与工程中心）；Virginia Tech（弗吉尼亚理工大学）；Northwestern University（西北大学）；University of Maryland, Baltimore County（马里兰大学巴尔的摩县分校）；Stanford University（斯坦福大学）
The ability to create large highly entangled `cluster' states is crucial for measurement-based quantum computing. We show that deterministic multi-photon entanglement can be created from coupled solid state quantum emitters without the need for any two-qubit gates and regardless of whether the emitters are identical. In particular, we present a general method for controlled entanglement creation by making direct use of the always-on exchange interaction, in combination with single-qubit operations. This is used to provide a recipe for the generation of two-dimensional, cluster-state entangled …
Coherent scattering of light by a single quantum emitter is a fundamental process at the heart of many proposed quantum technologies. Unlike atomic systems, solid-state emitters couple to their host lattice by phonons. Using a quantum dot in an optical nanocavity, we resolve these interactions in both time and frequency domains, going beyond the atomic picture to develop a comprehensive model of light scattering from solid-state emitters. We find that even in the presence of a cavity, phonon coupling leads to a sideband that is completely insensitive to excitation conditions, and to a non-mono…
It was shown by a study of the incoherent part of the low-frequency resonance fluorescence spectrum of the polar quantum emitter driven by semiclassical external laser field and damped by non-squeezed vacuum reservoir that the emitted fluorescence field is squeezed to some degree nevertheless. As was also found, a higher degree of squeezing could, in principle, be achieved by damping the emitter by squeezed vacuum reservoir.
Solid-state quantum emitters are promising candidates for the realization of quantum networks, owing to their long-lived spin memories, high-fidelity local operations, and optical connectivity for long-range entanglement. However, due to differences in local environment, solid-state emitters typically feature a range of distinct transition frequencies, which makes it challenging to create optically mediated entanglement between arbitrary emitter pairs. We propose and demonstrate an efficient method for entangling emitters with optical transitions separated by many linewidths. In our approach, …
We use the scattering matrix formalism to analyze photon blockade in coherently-driven CQED systems with a weak drive. By approximating the weak coherent drive by an input single- and two-photon Fock state, we reduce the computational complexity of the transmission and the two-photon correlation function from exponential to polynomial in the number of emitters. This enables us to easily analyze cavity-based systems containing $\sim$50 quantum emitters with modest computational resources. Using this approach we study the coherence statistics of polaritonic photon blockade while increasing the n…
In this work, dissipative effects from a phonon bath on the resonance fluorescence of a solid state two level system embedded in a high quality semiconductor microcavity and driven by an intense laser, are investigated. Within the density operator formalism, we derive a variational master equation valid for broader ranges of temperatures, pumping rates, and radiation-matter couplings, than previous studies. From the obtained master equation, fluorescence spectra for various thermal and exciting conditions are numerically calculated, and compared to those computed from weak coupling and polaron…
We give an overview of our recent theoretical studies of the thermodynamics of excitons, and other solid-state qubits, driven by time-dependent laser fields. We consider a single such emitter and describe how the formation of strong-field dressed states allows the emitter to absorb or emit acoustic phonons in a controlled way. We present results for the heat absorption, and show that the form of the driving field can be tailored to produce different thermodynamic processes, including both reversible and irreversible heat absorption. We discuss these effects from the perspective of quantum ther…
Coherent interactions between quantum emitters in tailored photonic structures is a fundamental building block for future quantum technologies, but remains challenging to observe in complex solid-state environments, where the role of decoherence must be considered. Here, we investigate the optical interaction between two quantum emitters mediated by one-dimensional waveguides in a realistic solid-state environment, focusing on the creation, population and detection of a sub-radiant state, in the presence of dephasing. We show that as dephasing increases, the signatures of sub-radiance quickly …
One important building block for future integrated nanophotonic devices is the scalable on-chip interfacing of single photon emitters and quantum memories with single optical modes. Here we present the deterministic integration of a single solid-state qubit, the nitrogen-vacancy (NV) center, with a photonic platform consisting exclusively of SiO$_2$ grown thermally on a Si substrate. The platform stands out by its ultra-low fluorescence and the ability to produce various passive structures such as high-Q microresonators and mode-size converters. By numerical analysis an optimal structure for t…
Scalable photonic quantum computing architectures pose stringent requirements on photonic processing devices. The need for low-loss high-speed reconfigurable circuits and near-deterministic resource state generators are some of the most challenging requirements. Here we develop an integrated photonic platform based on thin-film lithium niobate and interface it with deterministic solid-state single-photon sources based on quantum dots in nanophotonic waveguides. The generated photons are processed with low-loss circuits programmable at speeds of several GHz. We realize a variety of key photonic…
Solid-state quantum emitters have emerged as a leading quantum memory for quantum networking applications. However, standard optical characterization techniques are neither efficient nor repeatable at scale. In this work, we introduce and demonstrate spectroscopic techniques that enable large-scale, automated characterization of color centers. We first demonstrate the ability to track color centers by registering them to a fabricated machine-readable global coordinate system, enabling systematic comparison of the same color center sites over many experiments. We then implement resonant photolu…
Bell states are the most prominent maximally entangled photon states. In a typical four-level emitter, like a semiconductor quantum dot, the photon states exhibit only one type of Bell state entanglement. By adding an external driving to the emitter system, also other types of Bell state entanglement are reachable without changing the polarization basis. In this paper, we show under which conditions the different types of entanglement occur and give analytical equations to explain these findings. We further identify special points, where the concurrence, being a measure for the degree of entan…
Single photon emitters (SPEs) are critical building blocks needed for quantum science and technology. For practical applications, large-scale room-temperature solid-state platforms are required. Color centers in layered hexagonal boron nitride (hBN) have recently been found to be ultra-bright and stable SPEs at room temperature. Yet, to scale up solid-state quantum information processing, large tuning range of single photon energy is demanded for wavelength division multiplexing quantum key distribution, where indistinguishability is not required, and for indistinguishable single-photon produc…
We study the dynamics of a mechanical resonator parametrically coupled to a driven dissipative quantum emitter in the ultra-strong coupling regime. We show that this regime is fully compatible with a semi-classical treatment, and we derive master equations for the emitter and the resonator. We show that the fluctuations of the driven emitter's population induce the non-symmetrical scattering of the mechanical quadratures. At long timescales, such scattering back-acts on the emitter, which eventually decouples from the driving light. This optical noise at the quantum limit is observable with st…
Cooperative Emission from Quantum Emitters in Hexagonal Boron Nitride Layers
Institute for Quantum Electronics, ETH Zurich（苏黎世联邦理工学院量子电子研究所）；Faculty of Electrical and Computer Engineering, Technion - Israel Institute of Technology（以色列理工学院电气与计算机工程学院）；Helen Diller Quantum Center, Technion - Israel Institute of Technology（以色列理工学院海伦·迪勒量子中心）；School of Electrical and Electronic Engineering, Nanyang Technological University（南洋理工大学电气与电子工程学院）；Research Center for Electronic and Optical Materials, National Institute for Materials Science, NIMS（日本物质材料研究机构电子与光学材料研究中心）；Research Center for Materials Nanoarchitectonics, National Institute for Materials Science, NIMS（日本物质材料研究机构材料纳米结构研究中心）
Solid-state single-photon emitters are attractive for realization of integrated quantum systems due to their experimental convenience and scalability. Unfortunately, however, their complex mesoscopic environments cause photons from different emitters to be spectrally distinguishable. Here we demonstrate spectral alignment of two solid-state single-photon emitters by utilizing the strain gradient. Multiple germanium vacancy (GeV) color centers in diamond are created in fabricated diamond microcantilevers using focused ion beam implantation. The strain response of the electronic energy levels of…
Controlling and manipulating individual quantum systems in solids underpins the growing interest in development of scalable quantum technologies. Recently, hexagonal boron nitride has garnered significant attention in quantum photonic applications due to its ability to host optically stable quantum emitters. However, the large band gap of hBN and the lack of efficient doping inhibits electrical triggering and limits opportunities to study electrical control of emitters. Here, we show an approach to electrically modulate quantum emitters in n hBN graphene van der Waals heterostructure. We show …
