The presence of quasiparticles in superconducting qubits emerges as an intrinsic constraint on their coherence. While it is difficult to prevent the generation of quasiparticles, keeping them away from active elements of the qubit provides a viable way of improving the device performance. Here we develop theoretically and validate experimentally a model for the effect of a single small trap on the dynamics of the excess quasiparticles injected in a transmon-type qubit. The model allows one to evaluate the time it takes to evacuate the injected quasiparticles from the transmon as a function of trap parameters. With the increase of the trap size, this time decreases monotonically, saturating at the level determined by the quasiparticles diffusion constant and the qubit geometry. We determine the characteristic trap size needed for the relaxation time to approach that saturation value.
We study the effect of non-equilibrium quasiparticles on the operation of a superconducting device (a qubit or a resonator), including heating of the quasiparticles by the device operation. Focusing on the competition between heating via low-frequency photon absorption and cooling via photon and phonon emission, we obtain a remarkably simple non-thermal stationary solution of the kinetic equation for the quasiparticle distribution function. We estimate the influence of quasiparticles on relaxation and excitation rates for transmon qubits, and relate our findings to recent experiments.
We use radio-frequency reflectometry to measure quasiparticle tunneling rates in the single-Cooper-pair-transistor. Devices with and without quasiparticle traps in proximity to the island are studied. A $10^2$ to $10^3$-fold reduction in the quasiparticle tunneling rate onto the island is observed in the case of quasiparticle traps. In the quasiparticle trap samples we also measure a commensurate decrease in quasiparticle tunneling rate off the island.
Superconducting qubits probe environmental defects such as non-equilibrium quasiparticles, an important source of decoherence. We show that "hot" non-equilibrium quasiparticles, with energies above the superconducting gap, affect qubits differently from quasiparticles at the gap, implying qubits can probe the dynamic quasiparticle energy distribution. For hot quasiparticles, we predict a non-neligable increase in the qubit excited state probability P_e. By injecting hot quasiparticles into a qubit, we experimentally measure an increase of P_e in semi-quantitative agreement with the model and r…
Designing the spatial profile of the superconducting gap -- gap engineering -- has long been recognized as an effective way of controlling quasiparticles in superconducting devices. In aluminum films, their thickness modulates the gap; therefore, standard fabrication of Al/AlOx/Al Josephson junctions, which relies on overlapping a thicker film on top of a thinner one, always results in gap-engineered devices. Here we reconsider quasiparticle effects in superconducting qubits to explicitly account for the unavoidable asymmetry in the gap on the two sides of a Josephson junction. We find that di…
Quasiparticle tunneling across a Josephson junction sets a limit for the lifetime of a superconducting qubit state. We develop a general theory of the corresponding decay rate in a qubit controlled by a magnetic flux. The flux affects quasiparticles tunneling amplitudes, thus making the decay rate flux-dependent. The theory is applicable for an arbitrary quasiparticle distribution. It provides estimates for the rates in practically important quantum circuits and also offers a new way of measuring the phase-dependent admittance of a Josephson junction.
It is usually argued that the presence of gapless quasiparticle excitations at the nodes of the d-wave superconducting gap should strongly decohere the quantum states of a d-wave qubit, making quantum effects practically unobservable. Using a self-consistent linear response non-equilibrium quasiclassical formalism, we show that this is not necessarily true. We find quasiparticle conductance of a d-wave grain boundary junction to be strongly phase dependent. Midgap states as well as nodal quasiparticles contribute to the conductance and therefore decoherence. Quantum behavior is estimated to be…
As low-loss non-linear elements, Josephson junctions are the building blocks of superconducting qubits. The interaction of the qubit degree of freedom with the quasiparticles tunneling through the junction represent an intrinsic relaxation mechanism. We develop a general theory for the qubit decay rate induced by quasiparticles, and we study its dependence on the magnetic flux used to tune the qubit properties in devices such as the phase and flux qubits, the split transmon, and the fluxonium. Our estimates for the decay rate apply to both thermal equilibrium and non-equilibrium quasiparticles…
In many superconducting devices, including qubits, quasiparticle excitations are detrimental. A normal metal ($N$) in contact with a superconductor ($S$) can trap these excitations; therefore such a trap can potentially improve the devices performances. The two materials influence each other, a phenomenon known as proximity effect which has drawn attention since the '60s. Here we study whether this mutual influence places a limitation on the possible performance improvement in superconducting qubits. We first revisit the proximity effect in uniform $NS$ bilayers; despite the long history of th…
Superconducting circuits have attracted growing interest in recent years as a promising candidate for fault-tolerant quantum information processing. Extensive efforts have always been taken to completely shield these circuits from external magnetic field to protect the integrity of superconductivity. Surprisingly, here we show vortices can improve the performance of superconducting qubits by reducing the lifetimes of detrimental single-electron-like excitations known as quasiparticles. Using a contactless injection technique with unprecedented dynamic range, we quantitatively distinguish betwe…
Extending the qubit coherence times is a crucial task in building quantum information processing devices. In the three-dimensional cavity implementations of circuit QED, the coherence of superconducting qubits was improved dramatically due to cutting the losses associated with the photon emission. Next frontier in improving the coherence includes the mitigation of the adverse effects of superconducting quasiparticles. In these lectures, we review the basics of the quasiparticles dynamics, their interaction with the qubit degree of freedom, their contribution to the qubit relaxation rates, and …
Controlling quasiparticle dynamics can improve the performance of superconducting devices. For example, it has been demonstrated effective in increasing lifetime and stability of superconducting qubits. Here we study how to optimize the placement of normal-metal traps in transmon-type qubits. When the trap size increases beyond a certain characteristic length, the details of the geometry and trap position, and even the number of traps, become important. We discuss for some experimentally relevant examples how to shorten the decay time of the excess quasiparticle density. Moreover, we show that…
Nonequilibrium quasiparticles represent a significant source of decoherence in superconducting quantum circuits. Here we investigate the mechanism of quasiparticle poisoning in devices subjected to local quasiparticle injection. We find that quasiparticle poisoning is dominated by the propagation of pair-breaking phonons across the chip. We characterize the energy dependence of the timescale for quasiparticle poisoning. Finally, we observe that incorporation of extensive normal metal quasiparticle traps leads to a more than order of magnitude reduction in quasiparticle loss for a given injecte…
We present experiments on the dynamics of a two-state parametric fluctuator in a superconducting flux qubit. In spectroscopic measurements, the fluctuator manifests itself as a doublet line. When the qubit is excited in resonance with one of the two doublet lines, the correlation of readout results exhibits an exponential time decay which provides a measure of the fluctuator transition rate. The rate increases with temperature in the interval 40 to 158 mK. Based on the magnitude of the transition rate and the doublet line splitting we conclude that the fluctuation is induced by quasiparticle t…
Quasiparticles represent an intrinsic source of perturbation for superconducting qubits, leading to both dissipation of the qubit energy and dephasing. Recently, it has been shown that normal-metal traps may efficiently reduce the quasiparticle population and improve the qubit lifetime, provided the trap surpasses a certain characteristic size. Moreover, while the trap itself introduces new relaxation mechanisms, they are not expected to harm state-of-the-art transmon qubits under the condition that the traps are not placed too close to extremal positions where electric fields are high. Here, …
We have observed that the supercurrent across phase-biased, highly transmitting atomic size contacts is strongly reduced within a broad phase interval around π. We attribute this effect to quasiparticle trapping in one of the discrete sub-gap Andreev bound states formed at the contact. Trapping occurs essentially when the Andreev energy is smaller than half the superconducting gap Δ, a situation in which the lifetime of trapped quasiparticles is found to exceed 100 \mus. The origin of this sharp energy threshold is presently not understood.
The performance of many superconducting devices is degraded in presence of non-equilibrium quasiparticles in the superconducting part. One promising approach towards their evacuation is the use of normal-metal quasiparticle traps, where normal metal is brought into good metallic contact with the superconductor. A voltage biased normal-metal--insulator--superconductor junction equipped with such a trap is used to investigate on the trapping performance and the part played by the superconducting proximity effect therein. This involves an appropriate one-dimensional model of the junction and the …
Quasiparticle excitations adversely affect the performance of superconducting devices in a wide range of applications. They limit the sensitivity of photon detectors in astronomy, the accuracy of current sources in metrology, the cooling power of micro-refrigerators, and could break the topological protection of Majorana qubits. In superconducting circuits for quantum information processing, tunneling of quasiparticles across Josephson junctions constitutes a decoherence mechanism. As relaxation and pure dephasing times of transmon-type charge qubits now reach 100 microseconds, understanding w…
The Josephson quasiparticle (JQP) cycle in a voltage-biased superconducting single-electron transistor (SSET) combines coherent Cooper pair tunneling with incoherent quasiparticle decay. We have measured the influence of current flow through an independently-biased SSET on the JQP cycle when the two SSET's have a strong mutual capacitive coupling. We find, among other effects, that the JQP current in one SSET is enhanced by the presence of a quasiparticle current in the other SSET. A simplified model of the coupled-SSET system is presented which reproduces the enhancement effect.
Dynamical error suppression techniques are commonly used to improve coherence in quantum systems. They reduce dephasing errors by applying control pulses designed to reverse erroneous coherent evolution driven by environmental noise. However, such methods cannot correct for irreversible processes such as energy relaxation. In this work, we investigate a complementary, stochastic approach to reducing errors: instead of deterministically reversing the unwanted qubit evolution, we use control pulses to shape the noise environment dynamically. In the context of superconducting qubits, we implement…
We study a superconducting artificial atom which is represented by a single Josephson junction or a Josephson junction chain, capacitively coupled to a coherently driven transmission line, and which contains exactly one residual quasiparticle (or up to one quasiparticle per island in a chain). We study the dissipation in the atom induced by the quasiparticle tunneling, taking into account the quasiparticle heating by the drive. We calculate the transmission coefficient in the transmission line for drive frequencies near resonance and show that, when the artificial atom spectrum is nearly harmo…
We investigate subgap quasiparticles of a single level quantum dot coupled to the superconducting and normal leads, whose energy level is periodically driven by external potential. Using the Floquet formalism we determine the quasienergies and analyze redistribution of their spectral weights between individual harmonics upon varying the frequency and amplitude of the driving potential. We also propose feasible spectroscopic methods for probing the in-gap quasiparticles observable in the differential conductance of the charge current averaged over a period of oscillations.
Spin ordering and its effect on low energy quasiparticles in a p-wave superconducting liquid are investigated. We show that there is a new 2D p-wave superconducting liquid where the ground state is rotation invariant. In quantum spin disordered liquids, the low energy quasiparticles are bound states of the bare Bogolubov- De Gennes (${\em BdeG}$) quasiparticles and zero energy skyrmions, which are charge neutral bosons at the low energy limit. Further more, spin collective excitations are fractionalized ones carrying a half spin and obeying fermionic statistics. In thermally spin disordered li…
We have measured the number of quasiparticles and their lifetime in aluminium superconducting microwave resonators. The number of excess quasiparticles below 160 mK decreases from 72 to 17 $μ$m$^{-3}$ with a 6 dB decrease of the microwave power. The quasiparticle lifetime increases accordingly from 1.4 to 3.5 ms. These properties of the superconductor were measured through the spectrum of correlated fluctuations in the quasiparticle system and condensate of the superconductor, which show up in the resonator amplitude and phase respectively. Because uncorrelated noise sources vanish, fluctuatio…
We predict 'heating' of quasiparticles driven by order parameter oscillations in the resistive state of short superconducting microbridges. The finite relaxation time of the magnitude of the order parameter $|Δ|$ and the dependence of the spectral functions both on $|Δ|$ and the supervelocity $Q$ are the origin of this effect. Our result is opposite to those of Aslamazov and Larkin (Zh. Eks. Teor. Fiz. {\bf 70}, 1340 (1976)) and Schmid, Schon and Tinkham (Phys. Rev. B {\bf 21} 5076 (1980)) where 'cooling' of quasiparticles was found.
We present a comprehensive theoretical framework for the Andreev bound state population dynamics in superconducting weak links. Contrary to previous works, our approach takes into account the generated nonequilibrium distribution of the continuum quasiparticle states in a self-consistent way. As application of our theory, we show that the coupling of the superconducting contact to environmental phase fluctuations induces a charge imbalance of the continuum quasiparticle population. This imbalance is due to the breaking of the left-right symmetry in the rates connecting continuum quasiparticles…
Identifying, quantifying, and suppressing decoherence mechanisms in qubits are important steps towards the goal of engineering a quantum computer or simulator. Superconducting circuits offer flexibility in qubit design; however, their performance is adversely affected by quasiparticles (broken Cooper pairs). Developing a quasiparticle mitigation strategy compatible with scalable, high-coherence devices is therefore highly desirable. Here we experimentally demonstrate how to control quasiparticle generation by downsizing the qubit, capping it with a metallic cover, and equipping it with suitabl…
In superconducting qubits, the interaction of the qubit degree of freedom with quasiparticles defines a fundamental limitation for the qubit coherence. We develop a theory of the pure dephasing rate Γ_ϕ caused by quasiparticles tunneling through a Josephson junction and of the inhomogeneous broadening due to changes in the occupations of Andreev states in the junction. To estimate Γ_ϕ, we derive a master equation for the qubit dynamics. The tunneling rate of free quasiparticles is enhanced by their large density of states at energies close to the superconducting gap. Nevertheless, we find that…
Hybrid Superconductor/Ferromagnet structures have been investigated recently to address the interplay between ferromagnetism and superconductivity. They also open up new routes for the investigation of out of equilibrium superconductivity. Here, we show how it is possible for out of equilibrium excitations produced in a superconducting thin film (S) to be localized in a ferromagnetic trap (F). Specifically, a ferromagnetic nano-volume in good contact with S represents a potential well for the quasiparticles (QPs) at the gap edge. As the superconducting proximity effect is highly suppressed in …
We present a full theoretical and experimental study of the dynamics and energy distribution of non-equilibrium quasiparticles in superconducting tunnel junctions (STJs). STJs are often used for single-photon spectrometers, where the numbers of quasiparticles excited by a photon provide a measure of the photon energy. The magnitude and fluctuations of the signal current in STJ detectors are in large part determined by the quasiparticle dynamics and energy distribution during the detection process. We use this as motivation to study the transport and energy distribution of non-equilibrium quasi…
The quasiparticle relaxation time in superconducting films has been measured as a function of temperature using the response of the complex conductivity to photon flux. For tantalum and aluminium, chosen for their difference in electron-phonon coupling strength, we find that at high temperatures the relaxation time increases with decreasing temperature, as expected for electron-phonon interaction. At low temperatures we find in both superconducting materials a saturation of the relaxation time, suggesting the presence of a second relaxation channel not due to electron-phonon interaction.
Within the kinetic energy driven superconducting mechanism, we study the interplay between superconductivity and the nodal and antinodal superconducting quasiparticle coherences in cuprate superconductors, and find the s-wave superconducting transition temperature is heavily suppressed by the antinodal superconducting quasiparticle coherence, while the d-wave superconducting transition temperature is enhanced, therefore the antinodal superconducting quasiparticle coherence plays a more crucial role in superconductivity of cuprate superconductors.
Quasiparticles are an important decoherence mechanism in superconducting qubits, and can be described with a complex admittance that is a generalization of the Mattis-Bardeen theory. By injecting non-equilibrium quasiparticles with a tunnel junction, we verify qualitatively the expected change of the decay rate and frequency in a phase qubit. With their relative change in agreement to within 4% of prediction, the theory can be reliably used to infer quasiparticle density. We describe how settling of the decay rate may allow determination of whether qubit energy relaxation is limited by non-equ…
Evanescent quasiparticles entering a superconductor and propagating over distances larger than the coherence length give rise to intermediate states induced by double Andreev scattering on disorder.The resulting effective attractive interaction between evanescent quasiparticles is retarded at the extremely slow frequency of the applied bias voltage. The non-BCS out-of-equilibrium mesoscopic condensate is compatible with a recent experiment [S. Russo et al., Phys. Rev. Lett. 95, 027002 (2005)]. Microscopic theory is discussed in the random phase approximation.
Propagation and relaxation of nonequilibrium quasiparticles in superconductors are of key importance for functioning of numerous nanoscale devices, enabling operation of some of them, and limiting the performance of the others. The quasiparticles heated above lattice temperature may relax locally via phonon or photon emission channels, or diffuse over appreciable distances in a nanostructure altering the functionality of their remote components. Tracing quasiparticles experimentally in real-time domain has remained the challenging task owing to their rapid dynamics. With electronic nanothermom…
We report an experimentally observed anomalous doubly split spectrum and its split-width fluctuation in an ultrastrongly coupled superconducting qubit and resonator. From an analysis of Rabimodel and circuit model Hamiltonians, we found that the doubly split spectrum and split-width fluctuation are caused by discrete charge hops due to quasiparticle tunnelings and a continuous background charge fluctuation in islands of a flux qubit. During 70 hours in the spectrum measurement, split width fluctuates but the middle frequency of the split is constant. This result indicates that quasiparticles i…
We report on nonlocal spin transport in mesoscopic superconducting aluminum wires in contact with the ferromagnetic insulator europium sulfide. We find spin injection and long-range spin transport in the regime of the exchange splitting induced by europium sulfide. Our results demonstrate that spin transport in superconductors can be manipulated by ferromagnetic insulators, and opens a new path to control spin currents in superconductors.
We present a microscopic theory of transport through quantum dot set-ups coupled to superconducting leads. We derive a master equation for the reduced density matrix to lowest order in the tunneling Hamiltonian and focus on quasiparticle tunneling. For high enough temperatures transport occurs in the subgap region due to thermally excited quasiparticles, which can be used to observe excited states of the system for low bias voltages. On the example of a double quantum dot we show how subgap transport spectroscopy can be done. Moreover, we use the single level quantum dot coupled to a normal an…
It is shown that there are a significant number of quasiparticles present in the superconductor even at the temperature far below the transition temperature and that those quasiparticles seriously contribute to the characteristics of superconducting thin-film resonators.
A superconducting tunnel junction is used to directly extract quasiparticles from one of the leads of a single-Cooper-pair-transistor. The consequent reduction in quasiparticle density causes a lower rate of quasiparticle tunneling onto the device. This rate is directly measured by radio-frequency reflectometry. Local cooling may be of direct benefit in reducing the effect of quasiparticles on coherent superconducting nanostructures.
Quasiparticle properties in the superconducting state are masked by the superfluid and are not directly accessible to infrared spectroscopy. We show how one can use a Kramers--Kronig transformation to separate the quasiparticle from superfluid response and extract intrinsic quasiparticle properties in the superconducting state. We also address the issue of a narrow quasiparticle peak observed in microwave measurements, and demonstrate how it can be combined with infrared measurements to obtain unified picture of electrodynamic properties of cuprate superconductors.
Vortices trapped in thin-film superconducting microwave resonators can have a significant influence on the resonator performance. Using a variable-linewidth geometry for a weakly coupled resonator we are able to observe the effects of a single vortex trapped in the resonator through field cooling. For resonant modes where the vortex is near a current antinode, the presence of even a single vortex leads to a measurable decrease in the quality factor and a dispersive shift of the resonant frequency. For modes with the vortex located at a current node, the presence of the vortex results in no det…
Spin/magnetisation relaxation and coherence times, respectively T_1 and T_2, initially defined in the context of nuclear magnetic resonance (NMR), are general concepts applicable to a wide range of systems, including quantum bits [1-4]. At first glance, these ideas might seem to be irrelevant to conventional Bardeen-Cooper-Schrieffer (BCS) superconductors, as the BCS superconducting ground state is a condensate of Cooper pairs of electrons with opposite spins (in a singlet state) [5]. It has recently been demonstrated, however, that a non-equilibrium magnetisation can appear in the quasipartic…
We directly observe low-temperature non-equilibrium quasiparticle tunneling in a pair of charge qubits based on the single Cooper-pair box. We measure even- and odd-state dwell time distributions as a function of temperature, and interpret these results using a kinetic theory. While the even-state lifetime is exponentially distributed, the odd-state distribution is more heavily weighted to short times, implying that odd-to-even tunnel events are not described by a homogenous Poisson process. The mean odd-state dwell time increases sharply at low temperature, which is consistent with quasiparti…
Scanning tunneling spectroscopy measurements of superconducting thin lanthanum films grown on a normal metal tungsten substrate reveal an extraordinarily large broadening of the coherence peaks. The observed broadening corresponds to very short electron-like quasiparticle lifetimes in the tunneling process. A thorough analysis considering the different relaxation processes reveals that the dominant mechanism is an efficient quasiparticle relaxation at the interface between the superconducting film and the underlying substrate. This process is of general relevance to scanning tunneling spectros…
We study impurity scattering in the normal and d-wave superconducting states of line nodal semimetals and show that, due to additional scattering phase space available for impurities on the surface, the quasiparticle interference pattern acquires an extended character instead of a discrete collection of delta function peaks. Moreover, using the T-matrix formalism, we demonstrate that the conventional behavior of a scalar impurity in a d-wave superconductor breaks down on the surface of a line nodal semimetal in the quasi flat band limit.
In a superconductor absorption of photons with an energy below the superconducting gap leads to redistribution of quasiparticles over energy and thus induces a strong non-equilibrium quasiparticle energy distribution. We have measured the electrodynamic response, quality factor and resonant frequency, of a superconducting aluminium microwave resonator as a function of microwave power and temperature. Below 200 mK, both the quality factor and resonant frequency decrease with increasing microwave power, consistent with the creation of excess quasiparticles due to microwave absorption. Counterint…
