We demonstrate the ability to control quantum coherent Rabi-oscillations in a room-temperature quantum dot semiconductor optical amplifier (SOA) by shaping the light pulses that trigger them. The experiments described here show that when the excitation is resonant with the short wavelength slope of the SOA gain spectrum, a linear frequency chirp affects its ability to trigger Rabi-oscillations within the SOA: A negative chirp inhibits Rabi-oscillations whereas a positive chirp can enhance them, relative to the interaction of a transform limited pulse. The experiments are confirmed by a numerical calculation that models the propagation of the experimentally shaped pulses through the SOA.
Time Shaping of ultrashort visible pulses has been performed using a specially designed Acousto-Optic Programmable Dispersive Filter of 50% efficiency at the output of a two-stage noncollinear optical parametric amplifier. The set-up is compact and reliable. It provides a tunable shaped source in the visible with unique features: 4 ps shaping window with preserved tunability over 500-650 nm, and pulses as short as 30 fs. Several $μ$J output energy is easily obtained.
We demonstrate the Ramsey analogous experiment known as coherent control, taking place along an electrically-driven semiconductor optical amplifier operating at room temperature.
We describe a system for generating frequency-chirped and amplitude-shaped pulses on time scales from sub-nanosecond to ten nanoseconds. The system starts with cw diode-laser light at 780 nm and utilizes fiber-based electro-optical phase and intensity modulators, driven by an arbitrary waveform generator, to generate the shaped pulses. These pulses are subsequently amplified to several hundred mW with a tapered amplifier in a delayed double-pass configuration. Frequency chirps up to 5 GHz in 2 ns and pulse widths as short as 0.15 ns have been realized.
The ability to induce, observe and control quantum coherent interactions in room temperature, electrically driven optoelectronic devices is of outmost significance for advancing quantum science and engineering towards practical applications. We demonstrate here a quantum interference phenomena, Ramsey fringes, in an inhomogeneously broadened InAs/InP quantum dot (QD) ensemble in the form of a 1.5 mm long optical amplifier operating at room temperature. Observation of Ramsey fringes in semiconductor QD was previously achieved only at cryogenic temperatures and only in isolated single dot system…
We propose a scheme of an optical amplifier based on GaN and ZnO waveguides operating in the regime of strong coupling between photonic modes and excitonic resonances. Amplification of the guided exciton-polaritons is obtained by stimulated scattering from the excitonic reservoir, which is found to be fast enough compared with the large velocity of the guided polariton modes. We analyze the device parameters at different temperatures. We find that an 80 $μ$m-long amplifier can provide a gain of 10dB at room temperature, being supplied by 5 mA current in the $cw$ regime.
We report on the design and whole characterization of low-noise and affordable-cost Yb-doped double-clad fiber amplifiers operating at room temperature in the near-infrared spectral region at pulse repetition rate of 160 MHz. Two different experimental configurations are discussed. In the first one, a broadband seed radiation with a transform limited pulse duration of 71 fs, an optical spectrum of 20 nm wide at around 1040 nm, and 20 mW average power is adopted. In the second configuration, the seed radiation is constituted by stretched pulses with a time duration as long as 170 ps, with a 5-n…
In long-haul optical continuous-wave frequency transfer via fiber, remote bidirectional Er$^+$-doped fiber amplifiers are commonly used to mitigate signal attenuation. We demonstrate for the first time the ultrastable transfer of an optical frequency using a remote fiber Brillouin amplifier, placed in a server room along the link. Using it as the only means of remote amplification, on a 660 km loop of installed underground fiber we bridge distances of 250 km and 160 km between amplifications. Over several days of uninterrupted measurement we find an instability of the frequency transfer (Allan…
Tunable lasers emitting at a 2-3 $μ$m wavelength range and compatible with photonic integration platforms are of great interest for sensing applications. To this end, combining GaSb-based semiconductor gain chips with Si$_3$N$_4$ photonic integrated circuits offers an attractive platform. Herein, we exploit the low-loss features of Si$_3$N$_4$ waveguides and demonstrate a hybrid laser comprising a GaSb gain chip with an integrated tunable Si$_3$N$_4$ Vernier mirror. At room temperature, the laser exhibited a maximum output power of 15 mW and a tuning range of 80 nm (1937-2017 nm). The low-loss…
The influence of low temperatures on the performance of a high-power single-frequency fiber laser amplifier is evaluated with a numerical simulation. Cooling the fiber can allow to take advantage of both higher damping of the acoustic waves in the silica glass, and higher laser efficiency. We first report on the measurement of the stimulated Brillouin scattering (SBS) threshold in a silica fiber as a function of the temperature from 300~K down to 77~K. We then present the measurements of small-signal absorption and gain spectra of an erbium doped alumino-phosphosilicate fiber, at room temperat…
We report what we believe to be the first radiation-balanced fiber amplifier - a device that provides optical gain while experiencing no temperature rise. The gain medium is a silica fiber with a 21 um-diameter core highly doped with Yb3+ (2.52 wt.%) and co doped with 2.00 wt.% Al to reduce concentration quenching. The amplifier was core-pumped with 1040 nm light to create anti-Stokes fluorescence (ASF) cooling and gain in the core at 1064 nm. Using a custom slow-light FBG sensor with mK resolution, temperature measurements were performed at multiple locations along the amplifier fiber. A 4.35…
All-optical signal processing is envisioned as an approach to dramatically decrease power consumption and speed up performance of next-generation optical telecommunications networks. Nonlinear optical effects, such as four-wave mixing (FWM) and parametric gain, have long been explored to realize all-optical functions in glass fibers. An alternative approach is to employ nanoscale engineering of silicon waveguides to enhance the optical nonlinearities by up to five orders of magnitude, enabling integrated chip-scale all-optical signal processing. Previously, strong two-photon absorption (TPA) o…
Superfluorescence as a cooperative amplifier of hidden anisotropy in a ferroelectric hybrid perovskite
Physikalisch-Chemisches Institut, Universität Heidelberg（海德堡大学物理化学研究所）；Institute for Molecular Systems Engineering and Advanced Materials, Universität Heidelberg（海德堡大学分子系统工程与先进材料研究所）
We study the interplay between coherent light-matter interactions and non-resonant pulse propagation effects when ultra-short pulses propagate in room-temperature quantum-dot (QD) semiconductor optical amplifiers (SOAs). The signatures observed on a pulse envelope after propagating in a transparent SOA, when coherent Rabi-oscillations are absent, highlight the contribution of two-photon absorption (TPA), and its accompanying Kerr-like effect, as well as of linear dispersion, to the modification of the pulse complex electric field profile. These effects are incorporated into our previously deve…
Realization of a room-temperature ultra-fast photon-number-resolving (PNR) quantum nondemolition (QND) measurement would have significant implications for photonic quantum information processing (QIP), enabling, e.g., deterministic quantum computation in discrete-variable architectures, but the requirement for strong coupling has hampered the development of scalable implementations. In this work, we propose and analyze a nonlinear-optical route to PNR QND using quadratic (i.e., $χ^{(2)}$) nonlinear interactions. We show that the coherent pump field driving a phase-mismatched optical parametric…
Using a computational approach based on the driven diffusion equation for dipolariton wave packets, we simulate the diffusive dynamics of dipolaritons in an optical microcavity embedded with a transition-metal dichalcogenide (TMDC) heterogeneous bilayer encompassing a Ψ-shaped channel. By considering exciton-dipolaritons, which are a three way superposition of direct excitons, indirect excitons and cavity photons, we are able to drive the dipolaritons in our system by the use of an electric voltage and investigate their diffusive properties. More precisely, we study the propagation of dipolari…
We present in this work a quasi-continuous-wave (CW) pentacene maser operating at 1.45 GHz in the Earth's magnetic field at room temperature with a duration of $\sim$4 ms and an output power of up to -25 dBm. The maser is optically pumped by a cerium-doped YAG (Ce:YAG) luminescent concentrator (LC) whose wedge-shaped output is embedded inside a 0.1% pentacene-doped para-terphenyl (Pc:Ptp) crystal. The pumped crystal is located inside a ring of strontium titanate (STO) that supports a TE$_{01δ}$ mode of high magnetic Purcell factor. Combined with simulations, our results indicate that CW operat…
Metastable wurtzite crystal phases of semiconductors comprise enormous potential for high-performance electro-optical devices, owed to their extended tunable direct band gap range. However, synthesizing these materials in good quality and beyond nanowire size constraints has remained elusive. In this work, the epitaxy of wurtzite InP microdisks and related geometries on insulator for optical applications is explored. This is achieved by an elaborate combination of selective area growth of fins and a zipper-induced epitaxial lateral overgrowth, which enables co-integration of diversely shaped c…
In 2003 Bergman and Stockman introduced the spaser, a quantum amplifier of surface plasmons by stimulated emission of radiation [1]. They argued that, by exploiting a metal/dielectric composite medium, it should be possible to construct a nano-device, where a strong coherent field is built up in a spatial region much smaller than the wavelength [1,2]. V-shaped metallic inclusion, combined with a collection of semiconductor quantum dots were discussed as a possible realization of the spaser [1]. Here we introduce a further development of the spaser concept. We show that by combining the metamat…
We present a micro-mechanical terahertz (THz) detector fabricated on a silicon on insulator (SOI) substrate and operating at room-temperature. The device is based on a U-shaped cantilever of micrometric size, on top of which two aluminum half-wave dipole antennas are deposited. This produces an absorption extending over the $\sim 2-3.5$THz frequency range. Due to the different thermal expansion coefficients of silicon and aluminum, the absorbed radiation induces a deformation of the cantilever, which is read out optically using a $1.5μ$m laser diode. By illuminating the detector with an amplit…
Optomechanical SiN nano-oscillators in high-finesse Fabry-Perot cavities can be used to investigate the interaction between mechanical and optical degree of freedom for ultra-sensitive metrology and fundamental quantum mechanical studies. In this work we present a nano-oscillator made of a high-stress round-shaped SiN membrane with an integrated on-chip 3D seismic filter properly designed to reduce mechanical losses. This oscillator works in the 200 kHz - 5 MHz range and features a mechanical quality factor of $Q\simeq10^7$ and a Q-frequency product in excess of $6.2 \times 10^{12}$ Hz at room…
We present a system of room-temperature extended-cavity grating-diode lasers (ECDL) for production of light in the range 760-790nm. The extension of the tuning range towards the blue is permitted by the weak feedback in the cavity: the diodes are anti-reflection coated, and the grating has just 10% reflectance. The light is then amplified using semiconductor tapered amplifiers to give more than 400mW of power. The outputs are shown to be suitable for atomic physics experiments with potassium (767nm), rubidium (780nm) or both, of particular relevance to doubly-degenerate boson-fermion mixtures.
Room-temperature cavity exciton-polariton condensation in perovskite quantum dots
IBM Research Europe – Zurich（IBM欧洲苏黎世研究中心）；ETH Zurich（苏黎世联邦理工学院）；Institute of Materials Science of Sevilla, Consejo Superior de Investigaciones Científicas − Universidad de Sevilla (CSIC-US)（塞维利亚材料科学研究所，西班牙国家研究委员会-塞维利亚大学）；Laboratory of Inorganic Chemistry, Department of Chemistry and Applied Biosciences, ETH Zürich（苏黎世联邦理工学院化学与应用生物科学学院无机化学实验室）；Empa − Swiss Federal Laboratories for Materials Science and Technology（瑞士联邦材料科学与技术研究院）
