Optical forces allow manipulation of small particles and control of nanophotonic structures with light beams. Here, we describe a counter-intuitive lateral optical force acting on particles placed above a substrate, under uniform plane wave illumination without any field gradients. We show that under circularly-polarized illumination, nanoparticles experience a lateral force as a result of dipolar, spin-sensitive scattering, with a magnitude comparable to other optical forces. To this end, we rigorously calculate the force experienced by a circularly polarized dipole radiating above a surface. Unlike for linearly-polarized dipoles, force components parallel to the surface can exist, caused by the recoil of unidirectional guided modes excited at the surface and/or by dipole-dipole interactions with the induced image dipole. These results were presented and discussed in conferences [1] and [2].
Wide-field fluorescence microscopy, while much faster than confocal microscopy, suffers from a lack of optical sectioning and poor axial resolution. 3D structured illumination microscopy (SIM) has been demonstrated to provide optical sectioning and to double the achievable resolution both laterally and axially, but even with this the axial resolution is still worse than the lateral resolution of unmodified wide-field detection. Interferometric schemes using two high numerical aperture objectives, such as 4Pi confocal and I5S microscopy, have improved the axial resolution beyond that of the lat…
We demonstrate arbitrary helicity control of circularly polarized light (CPL) emitted at room temperature from the cleaved side-facet of a lateral-type spin-polarized light-emitting diode (spin-LED) with two ferromagnetic electrodes in an anti-parallel magnetization configuration. Driving alternate currents through the two electrodes results in polarization switching of CPL with frequencies up to 100 kHz. Furthermore, tuning the current density ratio in the two electrodes enables manipulation of the degree of circular polarization. These results demonstrate arbitrary electrical control of pola…
This paper aims to maximize optical force and torque on arbitrary micro- and nano-scale objects using numerically optimized structured illumination. By developing a numerical framework for computer-automated design of 3d vector-field illumination, we demonstrate a 20-fold enhancement in optical torque per intensity over circularly polarized plane wave on a model plasmonic particle. The nonconvex optimization is efficiently performed by combining a compact cylindrical Bessel basis representation with a fast boundary element method and a standard derivative-free, local optimization algorithm. We…
Chirality is at the origin of life and is ubiquitous in nature. An object is deemed chiral if it is non-superimposable with its own mirror image. This relates to how circularly polarized light interacts with such object, a circular dichroism, the differential absorption of right and left circularly polarized light. According to the common understanding in biology, chemistry and physics, the circular dichroism results from an internal chiral structure or external symmetry breaking by illumination. We show that circular dichroism is possible with simple symmetric optical nanoantennas at symmetri…
Dark-field illumination is shown to make planar chiral nanoparticle arrangements exhibit circular dichroism in extinction analogous to true chiral scatterers. Circular dichrosim is experimentally observed at the maximum scattering of single oligomers consisting rotationally symmetric arrangements of gold nanorods, with strong agreement to numerical simulation. A dipole model is developed to show that this effect is caused by a difference in the geometric projection of a nanorod onto the handed orientation of electric fields created by a circularly polarized dark-field that is normally incident…
When circularly polarized wave scatters off a sphere, the scattered field forms a vortex with spiraling energy flow. This is due to the transformation of spin angular momentum into orbital one. Here we demonstrate that during this scattering an anomalous force can be induced that acts in a direction perpendicular to the propagation of incident wave. The appearance of this lateral force is made possible by the presence of an interface in the vicinity of scattering object. Besides radiation pressure and tractor-beam pulling forces, this lateral force is another type of non-conservative force tha…
Application of circularly polarized beams in interferometric illumination of colloid sphere monolayers enables the direct fabrication of rectangular patterns consisting of circular nanohole miniarrays in metal films. The spectral and near-field effects of complex rectangular patterns made of a central nanoring and slightly rotated satellite nanocrescents were studied in azimuthal orientations promoting the localized and propagating plasmon's coupling. To inspect the localized modes separately, spectral responses and near-field phenomena of hexagonal patterns composed of uniform nanorings and n…
One of the main advantages of reciprocal bianisotropic metasurfaces is their capability to produce asymmetric scattering depending from which side they are illuminated and on the handedness of circularly polarized illuminations. For most applications, these metasurfaces are designed for illumination by a single source at a time. The resulting bianisotropic metasurface has a specific and usually complex geometrical structure that ensures the expected scattering produced under various illuminations. Here we show that geometrical asymmetry of metasurfaces can be emulated by using non-bianisotropi…
Spin-orbit interactions of light are ubiquitous in multiple branches of nanophotonics, including optical wave localization. In that framework, it is widely accepted that circularly polarized beams lead to spin-dependent apparent shifts of dipolar targets commonly referred to as optical mirages. In contrast, these optical mirages vanish when the illumination comes from a spinless beam such as a linearly polarized wave. Here we show that optical localization errors emerge for particles sustaining electric and magnetic dipolar response under the illumination of spinless beams. As an example, we c…
Illumination of colloid sphere monolayers by circularly polarized beams enables the fabrication of concave patterns consisting of circular nanohole miniarrays that can be transferred into convex metal nanoparticle patterns via a lift-off procedure. Unique spectral and near-field properties are achievable by tuning the geometry of the central nanoring and quadrumer of slightly rotated satellite nanocrescents and by selecting those azimuthal orientations that promote localized plasmon resonances. The spectral and near-field effects of hexagonal patterns made of uniform gold nanorings and nanocre…
We theoretically investigate the optical force exerted on an isotropic particle illuminated by a superposition of plane waves. We derive explicit analytical expressions for the exerted force up to quadrupolar polarizabilities. Based on these analytical expressions, we demonstrate that an illumination consisting of two tilted plane waves can provide a full control on the optical force. In particular, optical pulling, pushing and lateral forces can be obtained by the proper tuning of illumination parameters. Our findings might unlock multiple applications based on a deterministic control of the …
Measuring the three dimension nanoscale organization of protein or cellular structures is challenging, especially when the structure is dynamic. Owing to the informative total internal reflection fluorescence (TIRF) imaging under varied illumination angles, multi-angle (MA) TIRF has been examined to offer a nanoscale axial and a sub-second temporal resolution. However, conventional MA-TIRF still performs badly in lateral resolution and fail to characterize the depth-image in densely-distributed regions, leaving a huge contrast between the nanoscale axial resolution and the diffraction limited …
Modern optical microscopy methods have been advanced to provide super resolution at high imaging speed, but not chirality discriminative. We recently proposed chiral structured-illumination microscopy (SIM) method to image chiral fluorescent domains at sub-wavelength resolution. Chiral SIM is suitable for imaging chiral domains at sub-wavelength resolution but loses the high spatial frequency of the achiral ones. In order to obtain the full picture of all fluorescent domains at sub-wavelength resolution, we propose an advanced version of chiral SIM, termed double SIM, which enables simultaneou…
We discuss optical forces exerted on particles, either dielectric or metallic, near a subwavelength slit illuminated by a photonic nanojet. We compare those cases in which the Mie resonances are or are not excited. The configurations on study are 2D, hence those particles are infinite cylinders and, in order to obtain extraordinary transmission, the illuminating beam is p-polarized. We show the different effects of these particle resonances on the optical forces: while whispering gallery modes under those illumination conditions weaken the force strength, this latter is enhanced by localized p…
The focal field properties of radially/azimuthally polarized Zernike polynomials are studied. A method to design the pupil field in order to shape the focal field of radially or azimuthally polarized phase vortex is introduced. With this method, we are able to obtain a pupil field to achieve a longitudinally polarized hollow spot with a depth of focus up to $12λ$ and $0.14λ$ lateral resolution for a optical system with numerical aperture 0.99; A pupil field to generate 8 circularly polarized focal spots along the optical axis is also obtained with this method.
A circularly polarized plane-wave is known to have no angular momentum when examined through Maxwell's equations. This, however, contradicts the experimentally observed facts, where finite segments of plane waves are known to be capable of imparting angular momentum to birefringent platelets. Using a superposition of four plane-waves propagating at slightly different angles to a common direction, we derive an expression for the angular momentum density of a single plane-wave in the limit when the propagation directions of the four beams come into alignment. We proceed to use this four-beam tec…
Configurations capable of maximizing both absorptance and polarization contrast were determined for 1550 nm polarized light illumination of different plasmonic structure integrated superconducting nanowire single-photon detectors (SNSPDs) consisting of p=264 nm and P=792 nm periodic niobium-nitride (NbN) patterns on silica substrate. Global NbN absorptance maxima appear in case of p/s-polarized light illumination in S/P-orientation (gamma=90 azimuthal angle) and the highest polarization contrast is attained in S-orientation of all devices. Common nanophotonical origin of absorptance enhancemen…
Label-free observation of nanoparticles by far-field optical microscopy is challenging because their ability to scatter or absorb light dramatically diminishes with decreasing size. Surface plasmon resonance (SPR) and localized surface plasmon resonance (LSPR) imaging have shown promises and respective limitations. For instance, it is challenging to achieve diffraction-limited resolution in SPR imaging; its refractive index sensitivity is not as localized as desired. LSPR imaging is typically employed with dark-field microscopy on sparse noble metal nanostructures, leading to low light through…
Scanning near-field field optical microscopy (SNOM) is a technique, which allows sub-wavelength optical imaging of photonic structures. While the electric field components of light can be routinely obtained, imaging of the magnetic components has only recently become of interest. This is so due to the development of artificial materials, which enhance and exploit the typically weak magnetic light-matter interactions to offer extraordinary optical properties. Consequently, both sources and detectors of the magnetic field of light are now required. In this paper, assisted by finite-difference ti…
Plasmonics is based on surface plasmon polariton (SPP) modes which can be laterally confined below the diffraction limit, thereby enabling ultracompact optical components. In order to exploit this potential, the fundamental bottleneck of poor light-SPP coupling must be overcome. In established SPP sources (using prism, grating} or nanodefect coupling) incident light is a source of noise for the SPP, unless the illumination occurs away from the region of interest, increasing the system size and weakening the SPP intensity. Back-side illumination of subwavelength apertures in optically thick met…
The emerging optical multiplexing within nanoscale shows super-capacity in encoding information by using the time-domain fingerprints from uniform nanoparticles. However, the optical diffraction limit compromises the decoding throughput and accuracy of the nanoparticles during wide-field imaging. This, in turn, challenges the quality of nanoparticles to afford the modulated excitation condition, and further to retain the multiplexed optical fingerprints for super-resolution multiplexing. Here we report a tailor-made time-domain super-resolution method with the lifetime-engineered upconversion …
Speckle photography can be used to monitor deformations of solid surfaces. The measuring characteristics, such as range or lateral resolution depend heavily on the optical recording and illumination set-up. This paper shows how, by the addition of two suitably perforated masks, the optical aperture of the system may vary from point to point, accordingly adapting the range and resolution to local requirements. Furthermore, by illuminating narrow areas, speckle size can be chosen independently from the optical aperture, thus lifting an important constraint on its choice. The new technique in des…
Light scattering and spin-orbit angular momentum coupling phenomena from subwavelength objects, with electric and magnetic dipolar responses, are receiving an increasing interest. Under illumination by circularly polarized light, spin-orbit coupling effects have been shown to lead to significant shifts between the measured and actual position of particles. Here we show that the remarkable angular dependence of these "optical mirages" and those of the intensity, degree of circular polarization (DoCP), and spin and orbital angular momentum of scattered photons, are all linked and fully determine…
Local Chiral Optical Responses in Phthalocyanine Molecular Assemblies Revealed by Photoinduced Force Microscopy
Kwansei Gakuin University（关西学院大学）；Osaka Metropolitan University（大阪公立大学）；Ritsumeikan University（立命馆大学）；Osaka Research Institute of Industrial Science and Technology（大阪市立工业技术研究所）；Ritsumeikan Semiconductor Application research center (RISA)（立命馆半导体应用研究中心）
The recoil optical force that acts on emitters near a surface or waveguide relies on near-field directionality and conservation of momentum. It features desirable properties uncommon in optical forces, such as the ability to produce it via wide-area illumination of vast numbers of particles without the need for focusing, or being dynamically switchable via the polarization of light. Unfortunately, these recoil forces are usually very weak and have not been experimentally observed in small dipolar particles. Some works theoretically demonstrate orders-of-magnitude enhancement of these forces vi…
Circular dichroism (CD) caused by the response of a chiral object to circularly polarized light has been well established, and the strong CD of plasmonic meta-molecules has also become of interest in recent years; however, their response if the light also has orbital angular momentum is unclear. In this paper, the dichroism of a plasmonic cuboid-protuberance chiral structure under the illumination of a light beam with both orbital and spin angular momentums is numerically investigated. Distinguished spectra are observed under the different momentums. The circular dichroism under the combinatio…
Matter manipulation with optical forces has become commonplace in a wide range of research fields and is epitomized by the optical trap. Calculations of optical forces on small illuminated particles typically neglect multiple scattering on nearby structures. However, this scattering can result in large recoil forces, particularly when the scattering includes directional near-field excitations. Near-field recoil forces have been studied in the case of electric, magnetic and circularly polarized dipoles, but they exist for any type of directional near-field excitation. We use the force angular s…
The quest to improve density, speed and energy efficiency of magnetic memory storage has led to exploration of new ways of optically manipulating magnetism at the ultrafast time scale, in particular in ferrimagnetic alloys. While all-optical magnetization switching is well-established on the femtosecond timescale, lateral nanoscale confinement and thus potential significant reduction of the size of the magnetic element remains an outstanding challenge. Here we employ resonant electromagnetic energy-funneling plasmon nanoantennas to influence the demagnetization dynamics of a ferrimagnetic TbCo…
