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arXiv 1503.00824physics.optics
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单脉冲飞秒激光诱导周期性表面结构形成的时间分辨测量

Time-resolved measurement of single pulse femtosecond laser-induced periodic surface structure formation

K. R. P. Kafka, D. R. Austin, H. Li, A. Yi, J. Cheng, E. A. Chowdhury

AI总结:

本研究利用时间分辨衍射显微观测单飞秒脉冲作用于Cu表面纳米沟槽后的LIPSS形成过程,并以电子加热与SPP激发模型解释其0–1200 ps动力学。

摘要:

时间分辨衍射显微技术已被用于观察激光诱导周期性表面结构(LIPSS)的形成,该结构源于单个飞秒激光脉冲(泵浦)与单晶Cu衬底上机械形成的纳米尺度沟槽之间的相互作用。通过采用无限共轭显微装置,使一个经过时间延迟的倍频脉冲从泵浦诱导的新生LIPSS形成过程中发生衍射,从而捕捉了0–1200 ps的相互作用动力学。观察到LIPSS波纹从沟槽边缘开始依次向外形成,第一道波纹在50 ps后形成。一个关于入射激光脉冲与沟槽边缘相互作用所诱导的电子加热和表面等离激元极化激元(SPP)激发的一维解析模型,定性解释了LIPSS形成的时间演化。

英文摘要:

Time-resolved diffraction microscopy technique has been used to observe the formation of laser-induced periodic surface structures (LIPSS) from the interaction of a single femtosecond laser pulse (pump) with a nano-scale groove mechanically formed on a single-crystal Cu substrate. The interaction dynamics (0-1200 ps) was captured by diffracting a time-delayed, frequency-doubled pulse from nascent LIPSS formation induced by the pump with an infinity-conjugate microscopy setup. The LIPSS ripples are observed to form sequentially outward from the groove edge, with the first one forming after 50 ps. A 1-D analytical model of electron heating and surface plasmon polariton (SPP) excitation induced by the interaction of incoming laser pulse with the groove edge qualitatively explains the time-evloution of LIPSS formation.

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