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arXiv 1409.8474cond-mat.str-elcond-mat.mtrl-sci
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Ising磁体SmPt2Si2磁有序态中可能存在部分无序Sm离子的单晶研究

Possible Existence of Partially Disordered Sm Ions in Magnetically Ordered State of Ising Magnet SmPt2Si2: a Single Crystal Study

Kengo Fushiya, Tatsuma D. Matsuda, Ryuji Higashinaka, Kazuhiro Akiyama, Yuji Aoki

摘要:

我们已经成功地生长SmPt 2Si 2单晶,并进行了电阻率,磁化强度和比热测量。磁化率表明SmPt_2Si_2为Ising磁体,晶场基态为Jz=+-3/2。我们发现存在两个磁有序态,即,反铁磁(AFM)有序相(I)设置在TN= 5.1K和场诱导磁化平台相(II)。在第一阶段,不同于通常的AFM状态,一个明显的居里-外斯贡献仍然在磁化率,表明存在的“部分无序”的Sm离子。相I中的Sommerd系数(350 mJ/K ~ 2 mol)的大幅度提高可归因于部分无序Sm离子中重准粒子形成的Kondo亚晶格。这些发现可能反映了SmPt 2Si 2固有的大量磁挫折。

英文摘要:

We have succeeded in growing single crystals of SmPt2Si2 and have performed electrical resistivity, magnetization and specific heat measurements. The magnetic susceptibility shows that SmPt2Si2 is an Ising magnet with the crystalline-electric-field ground state of Jz=+-3/2. We have found the existence of two magnetically ordered states, i.e., an antiferromagnetically (AFM) ordered phase (I) setting in at TN=5.1 K and a field-induced magnetization plateau phase (II). In the phase I, unlike the usual AFM states, a pronounced Curie-Weiss contribution remains in magnetic susceptibility, indicating the existence of "partially disordered" Sm ions. Largely enhanced Sommerfeld-coefficient (350 mJ/K2mol) in the phase I can be attributed to formation of Kondo sublattice with heavy quasiparticles in the partially disordered Sm ions. These findings may reflect substantial magnetic frustrations inherent in SmPt2Si2.

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