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arXiv 1408.0930cond-mat.mes-hall
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量子点中Mn自旋与单个空穴耦合的动力学

Dynamics of a Mn spin coupled to a single hole confined in a quantum dot

B. Varghese, H. Boukari, L. Besombes

摘要:

以带正电荷的激子发射为探针,分析了Ⅱ-Ⅵ族半导体量子点中Mn自旋交换耦合与受限空穴自旋耦合的光抽运动力学和弛豫动力学.在自旋极化载流子的光注入下,空穴Mn自旋可以在几十个$ns$中有效地初始化。我们表明,这种光泵浦过程及其动力学控制的电子锰触发器内带正电的激子锰复合物。在理论上描述了抽运机制及其磁场依赖性的模型,包括在激发态的电子锰复合物的动力学和空穴锰复合物的动力学在基态的正电荷的量子点。我们测量在零磁场的自旋弛豫时间的空穴-Mn自旋在$μs$范围内或更短。这种空穴-Mn自旋弛豫是由自组装量子点中存在的价带混合引起的。

英文摘要:

Using the emission of the positively charged exciton as a probe, we analyze the dynamics of the optical pumping and the dynamics of the relaxation of a Mn spin exchange-coupled with a confined hole spin in a II-VI semiconductor quantum dot. The hole-Mn spin can be efficiently initialized in a few tens of $ns$ under optical injection of spin polarized carriers. We show that this optical pumping process and its dynamics are controlled by electron-Mn flip-flops within the positively charged exciton-Mn complex. The pumping mechanism and its magnetic field dependence are theoretically described by a model including the dynamics of the electron-Mn complex in the excited state and the dynamics of the hole-Mn complex in the ground state of the positively charged quantum dot. We measure at zero magnetic field a spin relaxation time of the hole-Mn spin in the $μs$ range or shorter. This hole-Mn spin relaxation is induced by the presence of valence band mixing in self-assembled quantum dots.

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