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arXiv 1403.4166cond-mat.str-elcond-mat.mtrl-sci
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Dy2BaNiO5的磁和介电性质中的重入现象及外加磁场的影响

A reentrant phenomenon in magnetic and dielectric properties of Dy2BaNiO5 and an intriguing influence of external magnetic field

Tathamay Basu, P. L. Paulose, Kartik K Iyer, Kiran Singh, N. Mohapatra, S. Chowki, Babu Gonde, E. V. Sampathkumaran

摘要:

我们报道了自旋链化合物Dy_2BaNiO_5在低于58K的Neel温度下表现出磁电耦合,在低温(<10K)下表现出很强的交流磁化率频率依赖行为和复杂的介电性质,类似于“重入”多玻璃现象。这种行为在未掺杂的化合物中是未知的。在多铁性领域的一个新发现是,在磁场(H)存在时,低温下的特征磁性向高温移动,而相应的介电特征则向低温移动,这与T_N附近的情况不同。这一观察结果表明,外部磁场对自旋的排列倾向于抑制类似玻璃的慢电偶极子动力学,至少在这个系统中,这可能是由磁结构的特殊性引起的。

英文摘要:

We report that the spin-chain compound Dy2BaNiO5 recently proven to exhibit magnetoelectric coupling below its Neel temperature (T_N) of 58 K, exhibits strong frequency-dependent behavior in ac magnetic susceptibility and complex dielectric properties at low temperatures (<10K), mimicking 'reentrant' multiglass phenomenon. Such a behavior is not known among undoped compounds. A new finding in the field of multiferroics is that the characteristic magnetic feature at such low temperatures moves towards higher temperatures in the presence of a magnetic-field (H), whereas the corresponding dielectric feature shifts towards lower temperatures with H, unlike the situation near T_N. This observation indicates that the alignment of spins by external magnetic fields tends to inhibit glassy-like slow electric-dipole dynamics, at least in this system, possibly arising from peculiarities in the magnetic structure.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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