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arXiv 1402.4040cond-mat.mtrl-scicond-mat.str-el
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揭示了SrTiO3反铁畸变相变对La0. 7 Sr 0. 3 MnO 3薄膜磁性能的影响

Unravelling the effect of SrTiO3 antiferrodistortive phase transition on the magnetic properties of La0.7Sr0.3MnO3 thin films

D. A. Mota, Y. Romaguera Barcelay, A. M. R. Senos, C. M. Fernandes, P. B. Tavares, I. T. Gomes, P. Sá, L. Fernandes, B. G. Almeida, F. Figueiras, P. Mirzadeh Va… 展开作者

D. A. Mota, Y. Romaguera Barcelay, A. M. R. Senos, C. M. Fernandes, P. B. Tavares, I. T. Gomes, P. Sá, L. Fernandes, B. G. Almeida, F. Figueiras, P. Mirzadeh Vaghefi, V. S. Amaral, A. Almeida, J. Pérez de la Cruz, J. Agostinho Moreira

摘要:

采用脉冲激光沉积法在(100)取向的钛酸锶(STO)衬底上制备了20 ~ 330 nm的La 0. 7Sr 0. 3 MnO 3(LSMO)外延薄膜,并在室温下对其结构和形貌进行了表征。磁和电输运性质的处理后的薄膜揭示了在反铁畸变STO相变(TSTO)以下的温度依赖的磁化强度M(T)的异常行为,也在相同的温度附近的磁电阻和电阻率的异常。高达100 nm的LSMO薄膜,在过量的磁化强度和显着的变化,证明了通过界面介导的磁弹性耦合与反铁畸变畴壁运动发生低于TSTO。相反,对于较厚的LSMO薄膜,在100 nm以上,观察到缺陷内磁化。通过高分辨率透射电子显微镜观察到,在膜的上层中出现了松弛存储在膜中的弹性能所需的分支结构,这导致随机取向的磁畴重构,可以理解这种相反的行为。对于足够高的施加的磁场,当达到热力学平衡时,发生对异常磁化的完全抑制,其中磁化的温度依赖性开始遵循预期的布里渊行为。

英文摘要:

Epitaxial La0.7Sr0.3MnO3 (LSMO) thin films, with different thickness ranging from 20 nm up to 330 nm, were deposited on (100)-oriented strontium titanate (STO) substrates by pulsed laser deposition, and their structure and morphology characterized at room temperature. Magnetic and electric transport properties of the as-processed thin films reveal an abnormal behavior in the temperature dependent magnetization M(T) below the antiferrodistortive STO phase transition (TSTO) and also an anomaly in the magnetoresistance and electrical resistivity close to the same temperature. Up to 100 nm LSMO thin films, an in-excess magnetization and pronounced changes in the coercivity are evidenced, achieved through the interface-mediated magnetoelastic coupling with antiferrodistortive domain wall movement occurring below TSTO. Contrarily, for thicker LSMO thin films, above 100 nm, an in-defect magnetization is observed. This reversed behavior can be understood within the emergence in the upper layer of the film, observed by high resolution transmission electron microscopy, of a branched structure needed to relax elastic energy stored in the film which leads to randomly oriented magnetic domain reconstructions. For enough high-applied magnetic fields, as thermodynamic equilibrium is reached, a fully suppression of the anomalous magnetization occurs, wherein the temperature dependence of the magnetization starts to follow the expected Brillouin behavior.

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