We perform frequency- and time-resolved all-optical switching of a GaAs-AlAs micropillar cavity using an ultrafast pump-probe setup. The switching is achieved by two-photon excitation of free carriers. We track the cavity resonances in time with a high frequency resolution. The pillar modes exhibit simultaneous frequency shifts, albeit with markedly different maximum switching amplitudes and relaxation dynamics. These differences stem from the non-uniformity of the free carrier density in the micropillar, and are well understood by taking into account the spatial distribution of injected free carriers, their spatial diffusion and surface recombination at micropillar sidewalls.
Optical bistability of exciton polaritons in semiconductor microcavities is a promising platform for digital optical devices. Steady states of coherently driven polaritons can be toggled in tens of picoseconds by a short external pulse of appropriate amplitude and phase. We have analyzed the switching behavior of polaritons depending on the pulse amplitude, phase, and duration. The switches are found to change dramatically when the inverse pulse duration becomes comparable to the frequency detuning between the driving field and polariton resonance. If the detuning is large compared to the pola…
We experimentally investigate a nonlinear switching mechanism in a dual-core highly nonlinear optical fiber. We focus the input beam of femtosecond pulses on one core only, to identify transitions between inter-core oscillations, self-trapping in the cross core, and self-trapping of the pulse in the straight core. A model based in the system of coupled nonlinear Schrodinger equations provides surprisingly good agreement with the experimental findings.
Ultrafast control of light-matter interactions constitutes a crucial feature in view of new technological frontiers of information processing. However, conventional optical elements are either static or feature switching speeds that are extremely low with respect to the timescales at which it is possible to control light. Here, we exploit high-quality-factor engineered epsilon-near-zero (ENZ) modes of a metal-insulator-metal nanocavity to realize an all-optical ultrafast modulation of the reflectance of light at a tailored wavelength. Our approach is based on the presence of the two, spectrall…
We demonstrate ultrafast soliton-based nonlinear balancing of dual-core asymmetry in highly nonlinear photonic crystal fiber at sub-nanojoule pulse energy level. The effect of fiber asymmetry was studied experimentally by selective excitation and monitoring of individual fiber cores at different wavelengths between 1500 nm and 1800 nm. Higher energy transfer rate to non-excited core was observed in the case of fast core excitation due to nonlinear asymmetry balancing of temporal solitons, which was confirmed by the dedicated numerical simulations based on the coupled generalized nonlinear Schr…
All-optical switches have attracted attention because they can potentially overcome the speed limitation of electric switches. However, ultrafast, energy-efficient all-optical switches have been challenging to realize due to the intrinsically small optical nonlinearity in existing materials. As a solution, we propose graphene-loaded deep-subwavelength plasmonic waveguides (30 nm x 20 nm). Thanks to extreme light confinement, we have significantly enhanced optical nonlinear absorption in graphene, and achieved ultrafast all-optical switching with a switching energy of 35 fJ and a switching time…
To enhance the efficiency of next-generation ferroelectric (FE) electronic devices, new techniques for controlling ferroelectric polarization switching are required. While most prior studies have attempted to induce polarization switching via the excitation of phonons, these experimental techniques required intricate and expensive terahertz sources and have not been completely successful. Here, we propose a new mechanism for rapidly and efficiently switching the FE polarization via laser-tuning of the underlying dynamical potential energy surface. Using time-dependent density functional calcul…
Next-generation communication networks require > Tbit/s single-channel data transfer and processing with sub-picosecond switches and routers at network nodes. Materials enabling ultrafast all-optical switching have high potential to solve the speed limitations of current optoelectronic circuits. Chromoproteins have been shown to exhibit a fast light-controlled refractive index change much larger than that induced by the optical Kerr effect due to a purely electronic nonlinearity, alleviating the driving energy requirements for optical switching. Here, we report femtosecond transient grating ex…
All-optical devices are essential for next generation ultrafast, ultralow-power and ultrahigh bandwidth information processing systems. Silicon microring resonators (SiMRR) provide a versatile platform for all-optical switching and CMOS-compatible computing, with added advantages of high Q-factor, tunability, compactness, cascadability and scalability. A detailed theoretical analysis of ultrafast all-optical switching 2 x 2 SiMRRs has been carried out incorporating the effects of two photon absorption induced free-carrier injection and thermo optic effect. The results have been used to design …
We consider light scattering by a coated magneto-plasmonic nanoparticle (MPNP) with a Kerr-type nonlinear plasmonic shell and a magneto-optic core. Such structure features two plasmon dipole modes, associated with electronic oscillations on the inner and outer surfaces of the shell. Driven in a nonlinear regime, each mode exhibits a bistable response. Bistability of an inner plasmon leads to switching between this state and a Fano resonance (Fano switching). Once the external light intensity exceeds the critical value, the bistability zones of both eigen modes overlap yielding optical tristabi…
Achieving ultrafast all-optical switching in a silicon waveguide geometry is a key milestone on the way to an integrated platform capable of handling the increasing demands for higher speed and higher capacity for information transfer. Given the weak electro-optic and thermo-optic effects in silicon, there has been intense interest in hybrid structures in which that switching could be accomplished by integrating another material into the waveguide, including the phase-changing material, vanadium dioxide (VO2). It has long been known that the phase transition in VO2 can be triggered by ultrafas…
Transient Pauli blocking in a InN film as a mechanism for broadband ultrafast optical switching
Global Center for Science and Engineering (GCSE), Faculty of Science and Engineering, Waseda University（早稻田大学理工学部）；Graduate School of Advanced Science and Engineering, Waseda University（早稻田大学先进理工学研究科）；Graduate School of Science and Engineering, Aoyama Gakuin University（青山学院大学理工学府）；Institute for Molecular Science（分子科学研究所）；The Graduate University for Advanced Studies (SOKENDAI)（综合研究大学院大学）；National Metrology Institute of Japan (NMIJ), National Institute of Advanced Industrial Science and Technology (AIST)（产业技术综合研究所国家计量标准研究所）
We propose a novel ultrafast electronic switching device based on dual-graphene electron waveguides, in analogy to the optical dual-channel waveguide device. The design utilizes the principle of coherent quantum mechanical tunneling of Rabi oscillations between the two graphene electron waveguides. Based on a modified coupled mode theory, we construct a theoretical model to analyse the device characteristics, and predict that the swtiching speed is faster than 1 ps. Due to the long mean free path of electrons in graphene at room temperature, the proposed design avoids the limitation of low tem…
Networks inside current data centers comprise a hierarchy of power-hungry electronic packet switches interconnected via optical fibers and transceivers. As the scaling of such electrically-switched networks approaches a plateau, a power-efficient solution is to implement a flat network with optical circuit switching (OCS), without electronic switches and a reduced number of transceivers due to direct links among servers. One of the promising ways of implementing OCS is by using tunable lasers and arrayed waveguide grating routers. Such an OCS-network can offer high bandwidth and low network la…
Optical nonlinear functions are crucial for various applications in integrated photonics, such as all-optical information processing, photonic neural networks and on-chip ultrafast light sources. Due to the weak nonlinearities in most integrated photonic platforms, realizing optical nonlinear functions typically requires large driving energies in the picojoules level or beyond, thus imposing a barrier for most applications. Here, we tackle this challenge and demonstrate an integrated nonlinear splitter device in lithium niobate nano-waveguides by simultaneous engineering of the dispersion and …
We exploit the nonlinearity arising from the spin-photon interaction in an InAs quantum dot to demonstrate phase shifts of scattered light pulses at the single-photon level. Photon phase shifts of close to 90 degrees are achieved using a charged quantum dot in a micropillar cavity. We also demonstrate a photon phase switch by using a spin-pumping mechanism through Raman transitions in an in-plane magnetic field. The experimental findings are supported by a theoretical model which explores the dynamics of the system. Our results demonstrate the potential of quantum dot-induced nonlinearities fo…
Ultrafast manipulation of magnetic order has challenged our understanding the fundamental and dynamic properties of magnetic materials. So far single shot magnetic switching has been limited to ferrimagnetic alloys and multilayers. In ferromagnetic (FM)/antiferromagnetic (AFM) bilayers, exchange bias (He) arises from the interfacial exchange coupling between the two layers and reflects the microscopic orientation of the antiferromagnet. Here we demonstrate the possibility of single shot switching of the antiferromagnet (change of the sign and amplitude of He) with a single femtosecond laser pu…
Ultrafast control of magnetization on the nanometer length scale, in particular all-optical switching, is key to putting ultrafast magnetism on the path towards future technological application in data storage technology. However, magnetization manipulation with light on this length scale is challenging due to the wavelength limitations of optical radiation. Here, we excite transient magnetic gratings in a GdFe alloy with a periodicity of 87 nm by interference of two coherent femtosecond light pulses in the extreme ultraviolet spectral range at the free electron laser facility FERMI. The subse…
Optically induced ultrafast switching of single photons is demonstrated by rotating the photon polarization via the Kerr effect in a commercially available single mode fiber. A switching efficiency of 97\% is achieved with a $\sim1.7$\,ps switching time, and signal-to-noise ratio of $\sim800$. Preservation of the quantum state is confirmed by measuring no significant increase in the second-order autocorrelation function $g^{(2)}(0)$. These values are attained with only nanojoule level pump energies that are produced by a laser oscillator with 80\,MHz repetition rate. The results highlight a si…
Ultrafast All-Optical Switching via a Supersolid Phase Transition of Light
GoLP/Instituto de Plasmas e Fusão Nuclear, Instituto Superior Técnico, Universidade de Lisboa（里斯本大学高等技术学院等离子体与核聚变研究所）；Instituto Superior de Engenharia de Lisboa, Instituto Politécnico de Lisboa（里斯本理工学院里斯本高等工程学院）
We present a laboratory system for single-shot magneto-optical (MO) imaging of ultrafast magnetization dynamics with high-sensitivity of MO rotation. We create a stack of MO images repeatedly employing a single pair of a pump and defocused probe pulses to induce and visualize MO changes in the sample. Both laser beams are independently wavelength-tunable allowing for a flexible, resonant adjustable two-color pump and probe scheme. To increase the MO contrast the probe beam is spatially filtered. We performed the all-optical switching experiment in Co-doped yttrium iron garnet films (YIG:Co) to…
The quest to improve density, speed and energy efficiency of magnetic memory storage has led to exploration of new ways of optically manipulating magnetism at the ultrafast time scale, in particular in ferrimagnetic alloys. While all-optical magnetization switching is well-established on the femtosecond timescale, lateral nanoscale confinement and thus potential significant reduction of the size of the magnetic element remains an outstanding challenge. Here we employ resonant electromagnetic energy-funneling plasmon nanoantennas to influence the demagnetization dynamics of a ferrimagnetic TbCo…
Bistability is widely exploited to demonstrate all-optical signal processing and light-based computing. The standard paradigm of switching between two steady states corresponding to '0" and '1" bits is based on the rule that a transition occurs when the signal pulse intensity overcomes the bistability threshold, and otherwise, the system remains in the initial state. Here, we break with this concept by revealing the phenomenon of indefinite switching in which the eventual steady state of a resonant bistable system is transformed into a nontrivial function of signal pulse parameters for moderat…
Active Control of Topological Exceptional Points in Non-Hermitian Metasurfaces
Indian Institute of Technology Bombay (IITB)（印度理工学院孟买分校）；Nanyang Technological University（南洋理工大学）；University of Notre Dame（圣母大学）；Jawaharlal Nehru Centre for Advanced Scientific Research (JNCASR)（贾瓦哈拉尔·尼赫鲁高级科学研究中心）
Future information technology demands ultimately fast, low-loss quantum control. Intense light fields have facilitated important milestones, such as inducing novel states of matter, accelerating electrons ballistically, or coherently flipping the valley pseudospin. These dynamics leave unique signatures, such as characteristic bandgaps or high-order harmonic radiation. The fastest and least dissipative way of switching the technologically most important quantum attribute - the spin - between two states separated by a potential barrier is to trigger an all-coherent precession. Pioneering experi…
