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arXiv 1312.3554cond-mat.supr-con
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超导Eu(Fe0 .82Co0.18)2As 2的单晶中子衍射磁结构

Magnetic structure of superconducting Eu(Fe0.82Co0.18)2As2 as revealed by single-crystal neutron diffraction

W. T. Jin, S. Nandi, Y. Xiao, Y. Su, O. Zaharko, Z. Guguchia, Z. Bukowski, S. Price, W. H. Jiao, G. H. Cao, Th. Brueckel

摘要:

超导体Eu(Fe0.82Co0.18)2As 2的磁结构由单晶中子衍射明确确定。在低于磁相变温度Tc = 17 K时,Eu ~(2+)磁矩沿c方向呈现长程铁磁有序.此外,虽然Fe自旋密度波(SDW)阶和结构相变的转变温度分别被显著抑制到Tn = 70 K和Ts = 90 K,但Fe 2+磁矩的反铁磁性仍然存在,并且还观察到四方晶到正交晶的结构相变。通过与母体化合物EuFe_2As_2的比较,给出了超导晶体中Eu铁磁性(FM)和Fe-SDW共存的微观证据。Eu(Fe_(0.82)Co_(0.18))_2As_2的超导电性与Fe-SDW的超导电性存在竞争关系。此外,Eu(Fe_(1-x)Co_(0.18))_2As_2与Ba(Fe_(1-x)Co_(0.18))_2As_2的比较表明,稀土元素Eu对Fe亚晶格的磁性有很大的影响。

英文摘要:

The magnetic structure of superconducting Eu(Fe0.82Co0.18)2As2 is unambiguously determined by single-crystal neutron diffraction. A long-range ferromagnetic order of the Eu2+ moments along the c-direction is revealed below the magnetic phase transition temperature Tc = 17 K. In addition, the antiferromagnetism of the Fe2+ moments still survives and the tetragonal-to-orthorhombic structural phase transition is also observed, although the transition temperatures of the Fe-spin density wave (SDW) order and the structural phase transition are significantly suppressed to Tn = 70 K and Ts = 90 K, respectively, compared to the parent compound EuFe2As2.We present the microscopic evidences for the coexistence of the Eu-ferromagnetism (FM) and the Fe-SDW in the superconducting crystal. The superconductivity (SC) competes with the Fe-SDW in Eu(Fe0.82Co0.18)2As2.Moreover, the comparison between Eu(Fe1-xCox)2As2 and Ba(Fe1-xCox)2As2 indicates a considerable influence of the rare-earth element Eu on the magnetism of the Fe sublattice.

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