We present calculations for the action of laser pulses on vibrational transfer within the H2+ and Na2 molecules in the presence of dissipation due to photodissociation of the molecule. The laser fields perform closed loops surrounding exceptional points in the laser parameter plane of intensity and wavelength. In principle the process should produce controlled vibrational transfers due to an adiabatic flip of the dressed eigenstates. We directly solve the Schrödinger equation with the complete time-dependent field instead of using the adiabatic Floquet formalism which initially suggested the design of the laser pulses. Results given by wavepacket propagations disagree with predictions obtained using the adiabatic hypothesis. Thus we show that there are large non-adiabatic exchanges and that the dissipative character of the dynamics renders the adiabatic flip very difficult to obtain. Using much longer durations than expected from previous studies, the adiabatic flip is only obtained for the Na2 molecule and with strong dissociation.
Exceptional points, the spectral degeneracy points in the complex parameter space, are fundamental to non-Hermitian quantum systems. The dynamics of non-Hermitian systems in the presence of exceptional points differ significantly from those of Hermitian ones. Here we investigate non-adiabatic transitions in non-Hermitian $\mathcal{P}\mathcal{T}$-symmetric systems, in which the exceptional points are driven through at finite speed which are quadratic or cubic functions of time. We identity different transmission dynamics separated by exceptional points, and derive analytical approximate formula…
Exceptional points, at which two or more eigenfunctions of a Hamiltonian coalesce, occur in non-Hermitian systems and lead to surprising physical effects. In particular, the behaviour of a system under parameter variation can differ significantly from the familiar Hermitian case in the presence of exceptional points. Here we analytically derive the probability of a non-adiabatic transition in a two-level system driven through two consecutive exceptional points at finite speed. The system is Hermitian far away from the exceptional points. In the adiabatic limit an equal redistribution between t…
Non-Hermitian quantum systems with explicit time dependence are of ever-increasing importance. There are only a handful of models that have been analytically studied in this context. Here, a PT-symmetric non-Hermitian $N$-level Landau-Zener type problem with two exceptional points of $N$th order is introduced. The system is Hermitian for asymptotically large times, far away from the exceptional points, and has purely imaginary eigenvalues between the exceptional points. The full Landau-Zener transition probabilities are derived, and found to show a characteristic binomial behaviour. In the adi…
The appearance of so-called exceptional points in the complex spectra of non-Hermitian systems is often associated with phenomena that contradict our physical intuition. One example of particular interest is the state-exchange process predicted for an adiabatic encircling of an exceptional point. In this work we analyse this and related processes for the generic system of two coupled oscillator modes with loss or gain. We identify a characteristic system evolution consisting of periods of quasi-stationarity interrupted by abrupt non-adiabatic transitions, and we present a qualitative and quant…
We study the behavior of the non-adiabatic population transfer between resonances at an exceptional point in the spectrum of the hydrogen atom. It is known that, when the exceptional point is encircled, the system always ends up in the same state, independent of the initial occupation within the two-dimensional subspace spanned by the states coalescing at the exceptional point. We verify this behavior for a realistic quantum system, viz. the hydrogen atom in crossed electric and magnetic fields. It is also shown that the non-adiabatic hypothesis can be violated when resonances in the vicinity …
The efficient transfer of excitations between different levels of a quantum system is a task with many applications. Among the various protocols to carry out such a state transfer in driven systems, rapid adiabatic passage (RAP) is one of the most widely used. Here we show both theoretically and experimentally that adding a suitable amount of loss to the driven Hamiltonian turns a RAP protocol into a scheme for encircling an exceptional point including the chiral state transfer associated with it. Our work thus discloses an intimate connection between a whole body of literature on RAP and rece…
Physical systems with loss or gain feature resonant modes that are decaying or growing exponentially with time. Whenever two such modes coalesce both in their resonant frequency and their rate of decay or growth, a so-called "exceptional point" occurs, around which many fascinating phenomena have recently been reported to arise. Particularly intriguing behavior is predicted to appear when encircling an exceptional point sufficiently slowly, like a state-flip or the accumulation of a geometric phase. Experiments dedicated to this issue could already successfully explore the topological structur…
We present a formal geometric framework for the study of adiabatic quantum mechanics for arbitrary finite-dimensional non-degenerate Hamiltonians. This framework generalizes earlier holonomy interpretations of the geometric phase to non-cyclic states appearing for non-Hermitian Hamiltonians. We start with an investigation of the space of non-degenerate operators on a finite-dimensional state space. We then show how the energy bands of a Hamiltonian family form a covering space. Likewise, we show that the eigenrays form a bundle, a generalization of a principal bundle, which admits a natural co…
We show a parameter-dependent $3\times 3$ non-Hermitian matrix that exhibits both degeneracy and coalescence of eigenvalues at an exceptional point (Hermitian and non-Hermitian degeneracies). This simple non-Hermitian model is suitable for the discussion of those concepts in an undergraduate or graduate course on quantum-mechanics. We also study the symmetry group responsible for the degeneracy.
In this paper,we present a rigorous demonstration and discussion of the quantum adiabatic theorem for systems having a non degenerate continuous spectrum. A new strategy is initiated by defining a kind of gap, "a virtual gap", for the continuous spectrum through the notion of eigendifferential (Weyl's packet) and using the differential projector operator. Finally we obtain the validity condition of the adiabatic approximation.
We revisit the complex time method for the application to quantum dynamics as an exceptional point is encircled in the parameter space of the Hamiltonian. The basic idea of the complex time method is using complex contour integration to perform the first-order adiabatic perturbation integral. In this way, the quantum dynamical problem is transformed to a study of singularities in the complex time plane -- transition points -- which represent complex degeneracies of the adiabatic Hamiltonian as the time-dependent parameters defining the encircling contour are analytically continued to complex p…
We study state conversion in parity-time (PT) symmetry broken non-Hermitian two level system. We construct a theory and explain underlying mechanism for state conversion and define adiabatic evolutions in non-Hermitian systems. The adiabatic theorem can be used if initial state is an instantaneous eigenstate in Hermitian systems. We show that the system can adiabatically follow the modulationally stable instantaneous eigenstate sooner or later, regardless of initial state if the system parameters are varied slowly in non-Hermitian systems. We discuss the topological feature of dynamical circli…
H$_2^+$ is an ideal candidate for a detailed study of strong field coherent control strategies inspired by basic mechanisms referring to some specific photodissociation resonances. Two of them are considered in this work, namely: Zero-width resonances (ZWR) on one hand, and coalescing pairs of resonances at exceptional points (EP) on the other hand. An adiabatic transport theory based on Floquet Hamiltonian formalism is developed within the challenging context of multiphoton dynamics involving nuclear continua. It is shown that a rigorous treatment is only possible for ZWRs, whereas adiabatic …
The correspondence between exotic quantum holonomy that occurs in families of Hermitian cycles, and exceptional points (EPs) for non-Hermitian quantum theory is examined in quantum kicked tops. Under a suitable condition, an explicit expressions of the adiabatic parameter dependencies of quasienergies and stationary states, which exhibit anholonomies, are obtained. It is also shown that the quantum kicked tops with the complexified adiabatic parameter have a higher order EP, which is broken into lower order EPs with the application of small perturbations. The stability of exotic holonomy again…
We consider the space of $n \times n$ non-Hermitian Hamiltonians ($n=2$, $3$, . . .) that are equivalent to a single $n\times n$ Jordan block. We focus on adiabatic transport around a closed path (i.e. a loop) within this space, in the limit as the time-scale $T=1/\varepsilon$ taken to traverse the loop tends to infinity. We show that, for a certain class of loops and a choice of initial state, the state returns to itself and acquires a complex phase that is $\varepsilon^{-1}$ times an expansion in powers of $\varepsilon^{1/n}$. The exponential of the term of $n$th order (which is equivalent t…
We consider an N-level non-Hermitian Hamiltonian with an exceptional point of order N. We define adiabatic equivalence in such systems and explore topological phase. We show that the topological exceptional states appear at the interface of topologically distinct systems. We discuss that topological states appear even in closed systems. We explore dynamical robustness of exceptional edge states.
We show that the inability of a quantum Otto cycle to reach a limit cycle is connected with the propagator of the cycle being non-compact. For a working fluid consisting of quantum harmonic oscillators, the transition point in parameter space where this instability occurs is associated with a non-hermitian degeneracy (exceptional point) of the eigenvalues of the propagator. In particular, a third-order exceptional point is observed at the transition from the region where the eigenvalues are complex numbers to the region where all the eigenvalues are real. Within this region we find another exc…
Spontaneous symmetry breaking has revolutionized the understanding in numerous fields of modern physics. Here, we theoretically demonstrate the spontaneous time-reversal symmetry breaking in a cavity quantum electrodynamics system in which an atomic ensemble interacts coherently with a single resonant cavity mode. The interacting system can be effectively described by two coupled oscillators with positive and negative mass when the two-level atoms are prepared in their excited states. The occurrence of symmetry breaking is controlled by the atomic detuning and the coupling to the cavity mode, …
We develop perturbative methods to study and control dynamical phenomena related to exceptional points in Non-Hermitian systems. In particular, we show how to find perturbative solutions based on the Magnus expansion that accurately describe the evolution of non-Hermitian systems when encircling an exceptional point. This allows us to use the recently proposed Magnus-based strategy for control to design fast non-reciprocal, topological operations whose fidelity error is orders of magnitude smaller than their much slower adiabatic counterparts.
Non-Hermitian classical and open quantum systems near an exceptional point (EP) are known to undergo strong deviations in their dynamical behavior under small perturbations or slow cycling of parameters as compared to Hermitian systems. Such a strong sensitivity is at the heart of many interesting phenomena and applications, such as the asymmetric breakdown of the adiabatic theorem, enhanced sensing, non-Hermitian dynamical quantum phase transitions and photonic catastrophe. Like for Hermitian systems, the sensitivity to perturbations on the dynamical evolution can be captured by Loschmidt ech…
We study theoretically the population transfer in two-level atoms driven by chirped lasers. It is known that in the Hermitian case, the rapid adiabatic passage (RAP) is stable for an above-critical chirp below which the final populations of states Rabi oscillate with varying laser power. We show that if the excited state is represented by a resonance, the separatrix marking this critical phenomenon in the space of the laser pulse parameters emanates from an exceptional point (EP) -- a non-Hermitian singularity formed in the atomic system by the fast laser field oscillations and encircled due t…
We investigate the parameter estimation in a magnon-cavity-magnon coupled system. PT symmetrical two magnons system can be formed in the gain magnetic materials by the adiabatic elimination of the cavity field mode. We show that the optimal estimation will not appear at the exceptional point due to that the quantum fluctuations are the strongest at the exceptional point. Moreover, we demonstrate that the measurements at the exceptional point tend to be optimal with the increase of prepared time. And the direct photon detection is the optimal measurement for the initial state in the vacuum inpu…
We consider the geometric phase and quantum tunneling in vicinity of diabolic and exceptional points. We show that the geometric phase associated with the degeneracy points is defined by the flux of complex magnetic monopole. In weak-coupling limit the leading contribution to the real part of geometric phase is given by the flux of the Dirac monopole plus quadrupole term, and the expansion for its imaginary part starts with the dipolelike field. For a two-level system governed by the generic non-Hermitian Hamiltonian, we derive a formula to compute the non-adiabatic complex geometric phase by …
With a specific choice of laser parameters resulting into a so-called exceptional point in the wavelength-intensity plane, it is possible to produce the coalescence of two Floquet resonances describing the photodissociation of the molecule Na$_2$, which is one of the candidates for molecular cooling. Appropriately tuning laser parameters, following a contour around the exceptional point, the resonances exchange their labels. This represents a laser control of the vibrational transfer from one field-free state to another, through an adiabatic transport involving these resonances. The proportion…
We report on the experimental study of an exceptional point (EP) in a dissipative microwave billiard with induced time-reversal invariance (T) violation. The associated two-state Hamiltonian is non-Hermitian and non-symmetric. It is determined experimentally on a narrow grid in a parameter plane around the EP. At the EP the size of T violation is given by the relative phase of the eigenvector components. The eigenvectors are adiabatically transported around the EP, whereupon they gather geometric phases and in addition geometric amplitudes different from unity.
We propose a method to adiabatically control an atomic ensemble using a decoherence-free subspace (DFS) within a dissipative cavity. We can engineer a specific eigenstate of the system's Lindblad jump operators by injecting a field into the cavity which deconstructively interferes with the emission amplitude of the ensemble. In contrast to previous adiabatic DFS proposals, our scheme creates a DFS in the presence of collective decoherence. We therefore have the ability to engineer states that have high multi-particle entanglements which may be exploited for quantum information science or metro…
Non-orientable Exceptional Points in Twisted Boundary Systems
Institute for Basic Science (IBS)（基础科学研究所）；Korea University of Science and Technology (UST)（韩国科学技术院）；Korea Advanced Institute of Science and Technology (KAIST)（韩国科学技术高等研究院）；Hanyang University（汉阳大学）；Pukyong National University（釜庆国立大学）
The time evolution of a single particle in a harmonic trap with time dependent frequency omega(t) is well studied. Nevertheless here we show that, when the harmonic trap is opened (or closed) as function of time while keeping the adiabatic parameter mu = [d omega(t)/dt]/omega(t)^2 fixed, a sharp transition from an oscillatory to a monotonic exponential dynamics occurs at mu = 2. At this transition point the time evolution has a third-order exceptional point (EP) at all instants. This situation, where an EP of a time-dependent Hermitian Hamiltonian is obtained at any given time, is very differe…
A short resume is given about the nature of exceptional points (EPs) followed by discussions about their ubiquitous occurrence in a great variety of physical problems. EPs feature in classical as well as in quantum mechanical problems. They are associated with symmetry breaking for ${\cal PT}$-symmetric Hamiltonians, where a great number of experiments have been performed in particular in optics, and to an increasing extent in atomic and molecular physics. EPs are involved in quantum phase transition and quantum chaos, they produce dramatic effects in multichannel scattering, specific time dep…
Universidad Politécnica Metropolitana de Hidalgo（伊达尔戈都会理工大学）；University of Texas Rio Grande Valley（德克萨斯大学里奥格兰德河谷分校）；Technical University of Munich（慕尼黑工业大学）
本文提出了一种基于 sl(3, C) 的非厄米特三模耦合器框架，通过代数对角化揭示几何相位，并分析了三腿光束分离器的传播动力学。
The technique of stimulated Raman adiabatic passage (STIRAP), which allows efficient and selective population transfer between quantum states without suffering loss due to spontaneous emission, was introduced in 1990 (Gaubatz \emph{et al.}, J. Chem. Phys. \textbf{92}, 5363, 1990). Since then STIRAP has emerged as an enabling methodology with widespread successful applications in many fields of physics, chemistry and beyond. This article reviews the many applications of STIRAP emphasizing the developments since 2000, the time when the last major review on the topic was written (Vitanov \emph{et…
An interplay of an exotic quantum holonomy and exceptional points is examined in one-dimensional Bose systems. The eigenenergy anholonomy, in which Hermitian adiabatic cycle induces nontrivial change in eigenenergies, can be interpreted as a manifestation of eigenenergy's Riemann surface structure, where the branch points are identified as the exceptional points which are degeneracy points in the complexified parameter space. It is also shown that the exceptional points are the divergent points of the non-Abelian gauge connection for the gauge theoretical formulation of the eigenspace anholono…
We show here that due to non-adiabatic couplings in decaying systems applying the same time-dependent protocol in the forward and reverse direction to the same mixed initial state leads to different final pure states. In particular, in laser driven molecular systems applying a specifically chosen positively chirped laser pulse or an equivalent negatively chirped laser pulse yields entirely different final vibrational states. This phenomenon occurs when the laser frequency and intensity are slowly varied around an exceptional point (EP) in the laser intensity and frequency parameter space where…
The Constrained Adiabatic Trajectory Method (CATM) is reexamined as an integrator for the Schrödinger equation. An initial discussion places the CATM in the context of the different integrators used in the literature for time-independent or explicitly time-dependent Hamiltonians. The emphasis is put on adiabatic processes and within this adiabatic framework the interdependence between the CATM, the wave operator, the Floquet and the (t,t') theories is presented in detail. Two points are then more particularly analysed and illustrated by a numerical calculation describing the $H_2^+$ ion submit…
Observation of Restored Adiabatic State Transfer in Time-Modulated Non-Hermitian Systems
Beijing Computational Science Research Center（北京计算科学研究中心）；Joint Laboratory of Optics of Palacký University and Institute of Physics of CAS, Faculty of Science, Palacký University（帕尔卡大学与捷克科学院物理研究所联合光学实验室，帕尔卡大学理学院）；School of Physics, Southeast University（东南大学物理学院）；Quantum Information Physics Theory Research Team, Quantum Computing Center, RIKEN（理研量子计算中心量子信息物理理论研究组）
For an arbitrary possibly non-Hermitian matrix Hamiltonian H, that might involve exceptional points, we construct an appropriate parameter space M and the lines bundle L^n over M such that the adiabatic geometric phases associated with the eigenstates of the initial Hamiltonian coincide with the holonomies of L^n. We examine the case of 2 x 2 matrix Hamiltonians in detail and show that, contrary to claims made in some recent publications, geometric phases arising from encircling exceptional points are generally geometrical and not topological in nature.
