The fate of entanglement of spins for two heavy constituents of a bound state moving in a strong laser field is analyzed within the semiclassical approach. The bound state motion as a whole is considered classically beyond the dipole approximation and taking into account the magnetic field effect by using the exact solution to the Newton equation. At the same time the evolution of constituent spins under the laser influence is studied quantum mechanically. The spin density matrix is determined as solution to the von Neumann equation with the effective Hamiltonian, describing spin-laser interaction along the bound state classical trajectory. Based on the solution, the dynamics of concurrence of spins is calculated for the maximally entangled Werner states as well as for an initially uncorrelated state.
We quantify the entanglement generated between an atom and a laser pulse in free space. We find that the entanglement calculated using a simple closed-system Jaynes-Cummings Hamiltonian is in remarkable agreement with a full open-system calculation, even though the free-space geometry is far from the strong coupling regime of cavity QED. We explain this result using a simple model in which the atom couples weakly to the laser while coupling strongly to the vacuum. Additionally we place an upper bound on the total entanglement between the atom and all paraxial modes using a quantum trajectories…
Inspired by laser operation, we address the question of whether stimulated emission into polarization entangled modes can be achieved. We describe a state produced by stimulated emission of the singlet Bell state and propose a setup for creating it. As a first important step towards an entangled-photon laser we demonstrate experimentally interference-enhanced polarization entanglement.
We show that an absolute coherent phase of a laser can be used to manipulate the entanglement of photon pairs of two-photon laser. Our focus is on the generation of a continuous source of entangled photon pairs in the double $Λ$ (or Raman) scheme. We study the dependence of steady state entanglement on the phase and laser parameters. We obtain a relationship between entanglement and two-photon correlation. We derive conditions that give steady state entanglement for the Raman-EIT scheme and use it to identify region of steady state macroscopic entanglement. No entanglement is found for the dou…
he dynamical properties of quantum entanglement in a time-dependent three-level-trapped ion interacting with a laser field are studied in terms of the reduced-density linear entropy considering two specific initial states of the field. Allowing the instantaneous position of the center-of-mass motion of the ion to be explicitly time-dependent, it is shown that either sudden death of entanglement or survivability of quantum entanglement can be obtained with a specific choice of the initial state parameters. The difference in evolution picture corresponding to the multi-quanta processes is discus…
We investigate the generation and the evolution of two-mode continuous-variable (CV) entanglement from system of a microwave-driven V-type atom in a quantum beat laser. By taking into account the effects of spontaneously generated quantum interference between two atomic decay channels, we show that the CV entanglement with large mean number of photons can be generated in our scheme, and the property of the filed entanglement can be adjusted by properly modulating the frequency detuning of the fields. More interesting, it is found that the entanglement can be significantly enhanced by the spont…
We discuss the dynamical behavior of the entanglement between the internal and the external degrees of freedom of a trapped atom in electromagnetically-induced transparency (EIT) laser cooling. It is shown that essential features of the intricate entanglement dynamics observed in full numerical simulations of the underlying quantum master equation can be understood in terms of a two-state model on the basis of Landau-Zener splittings in the atom-laser field Hamiltonian. An extension of this model to an effective non-Hermitian Hamiltonian is constructed which describes the decay of entanglement…
We study the effects of arbitrary laser pulse excitations on quantum correlation, entanglement and the role of quantum noise. The transient quantities are computed exactly using a method that provides exact solutions of the Langevin field operators for photon pairs produced by a double Raman atom driven by laser pulses. Short pulses with appropriate chirping, delay and/or detuning can generate broadband photon pairs and yield results that provide insights on how to generate very large nonclassical correlation. We find that short pulses are not favorable for entanglement. The quantity was previ…
The pairwise entanglement of an arbitrary atomic pair randomly extracted from a laser-driven dense multiqubit sample in the presence of quantum dissipation due to spontaneous emission is considered. The dipole-dipole interaction between the particles shifts the laser-qubit resonance frequency and consequently modifies the quantum entanglement. By means of an appropriate tuning of the laser frequency, one can optimize the entanglement in this system. For large ensembles, the maximum entanglement occurs near the laser parameters where the steady-state sample exhibits phase transition phenomena.
We study the simplest optomechanical system in the presence of laser phase noise using the covariance matrix formalism. We show that the destructive effect of the phase noise is especially strong in the bistable regime. This explains why ground state cooling is still possible in the presence of phase noise, as it happens far away from the bistable regime. On the other hand, the optomechanical entanglement is strongly affected by phase noise.
We show that the generation of entanglement of two heavily macroscopic mirrors with masses of up to several kilograms are feasible with state of the art techniques of high-precision laser interferometry. The basis of such a demonstration would be a Michelson interferometer with suspended mirrors and simultaneous homodyne detections at both interferometer output ports. We present the connection between the generation of entanglement and the Standard Quantum Limit (SQL) for a free mass. The SQL is a well-known reference limit in operating interferometers for gravitational-wave detection and prov…
We address an experimental scheme to analyze the optical bistability and the entanglement of two movable mirrors coupled to a two-mode laser inside a doubly resonant cavity. With this aim we investigate the master equations of the atom-cavity subsystem in conjunction with the quantum Langevin equations that describe the interaction of the mirror cavity. The parametric amplification-type coupling induced by the two-photon coherence on the optical bistability of the intracavity mean photon numbers is found and investigated. Under this condition, the optical intensities exhibit bistability for al…
Effectiveness of using laser field to produce entanglement between two dipole-interacting identical two-level atoms is considered in detail. The entanglement is achieved by driving the system with a carefully designed laser pulse transferring the system's population to one of the maximally entangled Dicke states in a way analogous to population inversion by a resonant $π$-pulse in a two-level atom. It is shown that for the optimally chosen pulse frequency, power and duration, the fidelity of generating a maximally entangled state approaches unity as the distance between the atoms goes to zero.
We calculate the emission spectra, the Glauber $g^{(2)}$ function, and the entanglement of formation for a few two-level emitters coupled to a single cavity mode and subject to an external laser-excitation. To evaluate these quantities we couple the system to environmental degrees of freedom which leads to dissipative dynamics. Because of the periodic time-dependence of the system Hamiltonian, the coefficients of the (Markovian) master equation are constant if Floquet states are used as the computational basis. Studying the emission spectra we show that the dynamic Stark effect, i.e., the shif…
We present a new scheme to generate high dimensional entanglement between two photonic systems. The idea is based on parametric down conversion with a sequence of pump pulses generated by a mode-locked laser. We prove experimentally the feasibility of this scheme by performing a Franson-type Bell test using a 2-way interferometer with path-length difference equal to the distance between 2 pump pulses. With this experiment, we can demonstrate entanglement for a two-photon state of at least dimension D=11. Finally, we propose a feasible experiment to show a Fabry-Perot like effect for a high dim…
Optical entanglement is a key requirement for many quantum communication protocols. Conventionally entanglement is formed between two distinct beams, with the quantum correlations being measured at separate locations. We show entanglement between the modes within one beam. Our technique is particularly elegant and a major advance towards practical systems with minimum complexity. We demonstrate three major experimental achievements: (i) only one source is required to produce squeezed light in two orthogonal spatial modes, (ii) the entanglement is formed through lenses and beam rotation, withou…
We consider the creation of polarization entangled light from parametric down- conversion driven by an intense pulsed pump inside a cavity. The multi-photon states produced are close approximations to singlet states of two very large spins. A criterion is derived to quantify the entanglement of such states. We study the dynamics of the system in the presence of losses and other imperfections, concluding that the creation of strongly entangled states with photon numbers up to a million seems achievable.
We explore and develop the mathematics of the two multi-level ions. In particular, we describe some new features of quantum entanglement in two three-level trapped ions confined in a one-dimensional harmonic potential, allowing the instantaneous position of the center-of-mass motion of the ions to be explicitly time-dependent. By solving the exact dynamics of the system, we show how survivability of the quantum entanglement is determined by a specific choice of the initial state settings.
The entanglement dynamics of a laser-pumped two-level quantum dot pair is investigated in the steady-state. The closely spaced two-level emitters, embedded in a semiconductor substrate, interact with both the environmental vacuum modes of the electromagnetic field reservoir as well as with the lattice vibrational phonon thermostat. We have found that the entanglement among the pair's components is substantially enhanced due to presence of the phonon subsystem. The reason is phonon induced decay among the symmetrical and antisymmetrical two-qubit collective states and, consequently, the populat…
We show that the quantum interference between downconverted photon pairs and photons from coherent laser light can produce a maximally path entangled N-photon output component with a fidelity greater than 90% for arbitrarily high photon numbers. A simple beam splitter operation can thus transform the 2-photon coherence of down-converted light into an almost optimal N-photon coherence.
We investigate the time-evolution of quantum entanglement between an electron, liberated by a strong few-cycle laser pulse, and its parent ion-core. Since the standard procedure is numerically prohibitive in this case, we propose a novel way to quantify the quantum correlation in such a system: we use the reduced density matrices of the directional subspaces along the polarization of the laser pulse and along the transverse directions as building blocks for an approximate entanglement entropy. We present our results, based on accurate numerical simulations, in terms of several of these entropi…
A detailed study of the effects of phase fluctuation and dephasing on the dynamics of the entanglement generated from a coherently pumped correlated emission laser is presented. It is found that the time evolution of the entanglement is significantly reliant on the phase fluctuation and dephasing, particularly, at early stages of the lasing process. In the absence of external driving radiation, the degree of entanglement and intensity turns out to attain a maximum value just before starting to exhibit oscillation which dies at longer time scale. However, in case the driving mechanism is on, th…
We study the entanglement between the internal electronic and the external vibrational degrees of freedom of a trapped atom which is driven by two lasers into electromagnetically-induced transparency. It is shown that basic features of the intricate entanglement dynamics can be traced to Landau-Zener splittings (avoided crossings) in the spectrum of the atom-laser field Hamiltonian. We further construct an effective Hamiltonian that describes the behavior of entanglement under dissipation induced by spontaneous emission processes. The proposed approach is applicable to a broad range of scenari…
The effect of a coupling laser field on the entanglement of a three-level quantum system and its spontaneous emission is investigated via reduced quantum entropy. We consider two schemes, the upper- and lower-level couplings. By calculating the degree of entanglement (DEM) for both systems, it is shown that the entanglement between atom and its spontaneous emission can be controlled by the coupling laser field. This field, however, affects the entanglement differently in the two schemes; it is only the lower-level coupling scheme that shows a nonzero steady state DEM which can be controlled by…
We investigate theoretically the optical properties of an atomic gas which has been cooled by the laser cooling method velocity-selective coherent population trapping. We demonstrate that the application of a weak laser pulse gives rise to a backscattered pulse, which is a direct signal for the entanglement in the atomic system, and which leads to single-particle entanglement on the few-photon level. If the pulse is applied together with the pump lasers, it also displays the phenomenon of electromagnetically induced transparency. We suggest that the effect should be observable in a gas of Rubi…
We introduce a scheme for creating continuous variable entanglement between an atomic beam and an optical field, by using squeezed light to outcouple atoms from a BEC via a Raman transition. We model the full multimode dynamics of the atom laser beam and the squeezed optical field, and show that with appropriate two-photon detuning and two-photon Rabi frequency, the transmitted light is entangled in amplitude and phase with the outcoupled atom laser beam. The degree of entanglement is controllable via changes in the two-photon Rabi frequency of the outcoupling process.
We show that two groups of slow two-level atoms in a weak resonant laser field, are entangled. The considered groups can be separated by a macroscopic distance, and be parts of a larger atomic ensemble. In a dilute regime, for two very distant groups of atoms, in a plane wave laser beam, we determine the maximum attainable entanglement negativity, and a laser intensity below which they are certainly entangled. They both decrease with increasing distance between the two groups, but increase with enlarging groups sizes. As a consequence, for given laser intensity, far separated groups of atoms a…
The entanglement of two dipole-coupled atoms with nondegenerate two-photon transitions interacting with two-mode field in lossless cavity has been investigated. It shows that the entanglement is dependent on the initial atomic states. The possibility of considerable growth of atomic entanglement due atomic coherence and dipole-dipole interaction is shown in the case of great mean values of thermal photons.
The dynamical behavior of entanglement between the atomic ensemble and the spontaneous emission is investigated by applying the femtosecond Gaussian pulses in double- lambda quantum system. In fact by solving the density matrix equations of motion in such a system and by using the von Neumann entropy, the degree of entanglement (DEM) could be measured in semi classical regime and in the multi-photon resonance condition. We interested in investigating the maximum value for DEM and controlled the DEM via relative phase. At first we consider three laser fields as CW optical laser fields and one f…
The conventional approach to perform two-qubit gate operations in trapped ions relies on exciting the ions on motional sidebands with laser light, which is an inherently slow process. One way to implement a fast entangling gate protocol requires a suitable pulsed laser to increase the gate speed by orders of magnitude. However, the realization of such a fast entangling gate operation presents a big technical challenge, as such the required laser source is not available off-the-shelf. For this, we have engineered an ultrafast entangling gate source based on a frequency comb. The source generate…
We generate high-dimensional time-bin entanglement using a mode-locked laser and analyze it with a 2-photon Fabry-Perot interferometer. The dimension of the entangled state is limited only by the phase coherence between subsequent pulses and is practically infinite. In our experiment a pico-second mode-locked laser at 532 nm pumps a non-linear potassium niobate crystal to produce photon pairs by spontaneous parametric down-conversion at 810 and 1550 nm.
We propose an experimentally feasible scheme to generate Greenberger-Horne-Zeilinger (GHZ) type of maximal entanglement between many atomic ensembles based on laser manipulation and single-photon detection. The scheme, with inherent fault tolerance to the dominant noise and efficient scaling of the efficiency with the number of ensembles, allows to maximally entangle many atomic ensemble within the reach of current technology. Such a maximum entanglement of many ensembles has wide applications in demonstration of quantum nonlocality, high-precision spectroscopy, and quantum information process…
We study the time evolution of quantum entanglement between an electron and its parent ion during the rescattering due to a strong few-cycle laser pulse. Based on a simple one-dimensional model, we compute the Neumann entropy during the process for several values of the carrier-envelope phase. The local maxima of the oscillations in the Neumann entropy coincide with the zero crossings of the electric field of the laser pulse. We employ the Wigner function to qualitatively explain the quantum dynamics of rescattering in the phase space.
We have investigated the dynamics of entanglement between two spin-1/2 qubits that are subject to independent kick and Gaussian pulse type external magnetic fields analytically as well as numerically. Dyson time ordering effect on the dynamics is found to be important for the sequence of kicks. We show that "almost-steady" high entanglement can be created between two initially unentangled qubits by using carefully designed kick or pulse sequences.
Entanglement of remote atom lasers is obtained via quantum state transfer technique from lights to matter waves in a five-level $M$-type system. The considered atom-atom collisions can yield an effective Kerr susceptibility for this system and lead to the self- and cross- phase modulation between the two output atom lasers. This effect results in generation of entangled states of output fields. Particularly, under different conditions of space-dependent control fields, the entanglement of atom lasers and of atom-light fields can be obtained, respectively. Furthermore, based on the Bell-state m…
An experimental scheme is suggested that permits a direct measure of entanglement in a two-qubit cavity system. It is realized in the cavity-QED technology utilizing atoms as flying qubits. With this scheme we generate two different measures of entanglement, namely logarithmic negativity and concurrence. The phenomenon of sudden death entanglement (ESD) in a bipartite system subjected to dissipative environment is examined. We show that the sudden death time of the entangled states depends on the initial preparation of the entangled state and the temperature of the reservoir.
We investigate the dynamics of entanglement given by the concurrence of a two-qubit system in the non-Markovian setting. A quantum master equation is derived which is solved in the eigen basis of the system Hamiltonian for X-type initial states. A closed formula for time evolution of concurrence is presented for a pure state. It is shown that under the influence of dissipation that non-zero entanglement is created in unentangled two qubit states which decay in the same way as pure entangled states. We also show that under real circumstances, the decay rate of concurrence is strongly modified b…
Entanglement and non-locality are non-classical global characteristics of quantum states important to the foundations of quantum mechanics. Recent investigations have shown that environmental noise, even when it is entirely local in influence, can destroy both of these properties in finite time despite giving rise to full quantum state decoherence only in the infinite time limit. These investigations, which have been carried out in a range of theoretical and experimental situations, are reviewed here.
Interference of laser pulses is an essential ingredient of quantum randomness; therefore, probabilistic properties of laser pulses gains new relevance. Here, we consider in detail the combined influence of the three effects - chirp, jitter and relaxation oscillations - on the probability density function of the interference of pulses from a gain-switched semiconductor laser. We develop a rigorous model based on laser rate equations and demonstrate that only consideration of all these three effects together allows describing the interference statistics properly. We supplement our theoretical ca…
A scheme for preparation of coherent superposition of Fock states of electromagnetic field is constructed. The superposition state is created inside the cavity via a strong interaction of a four-level atom with quantum field of the cavity and classic laser fields. We demonstrate the possibility to create desired arbitrary superposition of the cavity Fock states just by changing the relative delay of the fields. Then, as another application of our model, we study a means of creating entanglement of neutral four-level atoms using different sequences of interactions with the cavity and laser fiel…
The influence of a repump laser on a nearly degenerate four-wave-mixing (NDFWM) spectrum was investigated. We found the amplitude and line shape of the NDFWM depended strongly on the detuning of the repump field. A five-peak structure was observed. And at some certain repump detuning a dip appeared at the central peak. A rough analysis was proposed to explain this effect.
Distributing entangled photon pairs over noisy channels is an important task for various quantum information protocols. Encoding an entangled state in a decoherence-free subspace (DFS) formed by multiple photons is a promising way to circumvent the phase fluctuations and polarization rotations in optical fibres. Recently, it has been shown that the use of a counter-propagating coherent light as an ancillary photon enables us to faithfully distribute entangled photon with success probability proportional to the transmittance of the optical fibres. Several proof-of-principle experiments have bee…
We study the effect of laser phase noise on the generation of stationary entanglement between an intracavity optical mode and a mechanical resonator in a generic cavity optomechanical system. We show that one can realize robust stationary optomechanical entanglement even in the presence of non-negligible laser phase noise. We also show that the explicit form of the laser phase noise spectrum is relevant, and discuss its effect on both optomechanical entanglement and ground state cooling of the mechanical resonator.
Crossovers between Time-Bin and Energy-Time Entanglement in Homodyned Resonance Fluorescence
Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）；Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；University of Chinese Academy of Sciences（中国科学院大学）
We propose a simple model for the nondegenerate parametric inter- action that takes into account the finite spectral bandwidth of the pump wave. The Heisenberg equations of motion are solved exactly and we show that the bosonic operators obey to a generalized Bogoliubov transforma- tion, where the degree of squeezing depends on the spectral bandwidth. The average number of photons produced in the interaction, the degree of squeezing as well as the degree of entanglement are computed showing that they decrease with increasing spectral bandwidth.
The entanglement, purity and energy of two isolated two-level atoms which are initially prepared in Bell state and each interacts with a thermal cavity field are investigated by considering the atomic motion and the field-mode structure. We achieve the analytical solutions of the atomic qubits by using the algebraic dynamical approach and the influences of the field-mode structure parameter, the strength of the thermal field and the detuning on the entanglement, purity and energy are discussed. We also investigate the state evolution of the atomic qubits based on the entanglement-purity-energy…
We investigate the characteristics of entanglement teleportation of a two-qubit Heisenberg XYZ model under different Dzyaloshinskii-Moriya interaction with intrinsic decoherence taken into account. The comparison of the two different Dzyaloshinskii-Moriya interaction, the effects of the initial state and the inputting state on the entanglement teleportation are presented. The results reveal that the dynamics of entanglement is a symmetry function about for the system, whereas it is not for the system. The ferromagnetic case is superior to the antiferromagnetic case for restrain decoherence whe…
We investigate how the polarization correlations of entangled photons described by wave packets are modified when measured by moving detectors. For this purpose, we analyze the Clauser-Horne-Shimony-Holt Bell inequality as a function of the apparatus velocity. Our analysis is motivated by future experiments with entangled photons designed to use satellites. This is a first step towards the implementation of quantum information protocols in a global scale.
Orientation states of two coupled polar molecules controlled by laser pulses are studied theoretically. By varying the period of a series of periodically applied laser pulse, transition from regular to chaotic behavior may occur. Schmidt decomposition is used to measure the degree of entanglement. It is found that the entanglement can be enhanced by increasing the strength of laser pulse.
Entangled states of two coupled polar molecules controlled by laser pulses are studied theoretically. Schmidt decomposition is used to measure the degree of entanglement. By varying the pulse shape of the applied laser, transition from regular to chaotic behavior may occur. This quantum feature is due to the inference of different phases. Moreover, the entanglement is also found to be enhanced by increasing the strength of the laser pulses.
We theoretically investigate how the initial state influence the entanglement dynamics between two and three two-level atoms with dipole-dipole interaction (DDI) coupled to a whispering-gallery-mode (WGM) microtoroidal cavity. Two different cases, where the two atoms are coupled symmetrically or asymmetrically to the two WGMs through evanescent fields, are discussed in detail. Considering two types of initial states between the atoms and the symmetric regime, we show that for the initial entangled state, the sudden death and birth, as well as the freezing of the entanglement, can be obtained b…
Strong correlations in two conjugate variables are the signature of quantum entanglement and have played a key role in the development of modern physics. Entangled photons have become a standard tool in quantum information and foundations. An impressive example is position-momentum entanglement of photon pairs, explained heuristically through the correlations implied by a common birth zone and momentum conservation. However, these arguments entirely neglect the importance of the `quantumness', i.e. coherence, of the driving force behind the generation mechanism. We study theoretically and expe…
While many-particle entanglement can be found in natural solids and strongly interacting atomic and molecular gases, generating highly entangled states between weakly interacting particles in a controlled and scalable way presents a significant challenge. We describe here a one-step method to generate entanglement in a dilute gas of cold polar molecules. For molecules in optical traps separated by a few micrometers, we show that maximally entangled states can be created using the strong off-resonant pulses that are routinely used in molecular alignment experiments. We show that the resulting a…
We report on the generation of time-bin entangled photon pairs from a semiconductor quantum dot via pulsed resonant biexciton generation. Based on theoretical modeling we optimized the duration of the excitation pulse to minimize the laser-induced dephasing and increase the biexciton-to-background single exciton occupation probability. This results in a high degree of entanglement with a concurrence of up to 0.78(6) and a 0.88(3) overlap with a maximally entangled state. Theoretical simulations also indicate a power dependent nature of the dephasing during the laser excitation that limits the …
