Macroscopic quantum phenomena refer to quantum features in objects of `large' sizes, systems with many components or degrees of freedom, organized in ways where they can be identified as macroscopic objects. This emerging field is ushered in by several categories of definitive experiments in superconductivity, electromechanical systems, Bose-Einstein condensates and others. Yet this new field which is rich in open issues at the foundation of quantum and statistical physics remains little explored theoretically [1]. This talk summarizes our thoughts on attempting a systematic investigation into its foundation, with the goal of ultimately revealing or building a viable theoretical framework. Three major themes discussed in three intended essays are the large N expansion [2], the correlation hierarchy [3] and quantum entanglement [4]. We give a sketch of the first two themes and then discuss several key issues in the consideration of macro and quantum, namely, a) recognition that in a composite body there exist many 'levels of structure' characterized by collective variables. The quantum features of a macroscopic object can be captured by understanding how these collective variables function; b) 'quantum entanglement', an exclusively quantum feature [5], is known to persist to high temperatures [6] and large scales [7] under certain conditions, and may actually decrease with increased connectivity in a quantum network [8]. Here we use entanglement as a measure of quantumness and pick out these somewhat counter-intuitive examples to show that there are blind spots worthy of our attention and issues which we need to analyze closer. Our purpose is to try to remove the stigma that quantum only pertains to micro, in order to make way for deeper probes into the conditions whereby quantum features of macroscopic systems manifest.
From various points of view it is argued that one may find phenomena similar to the quantum effects also in macroscopic cases. This forces one to give up as a general requirement the assumption of realism as formulated by Gill and others. For any potential set of experiments on a limited set of units, we find it useful to introduce for these units the concept of a total parameter, a set of parameters which is so large that a joint value is meaningless.
Macroscopic quantum phenomena (MQP) is a relatively new research venue, with exciting ongoing experiments and bright prospects, yet with surprisingly little theoretical activity. What makes MQP intellectually stimulating is because it is counterpoised against the traditional view that macroscopic means classical. In this series of papers we report on a systematic investigation into some key foundational issues of MQP, with the hope of constructing a viable theoretical framework for this new endeavour. The three major themes discussed in these three essays are the large N expansion, the correla…
We explore in this paper ways to qualify and quantify the quantum entanglement $E(M)$ between two macroscopic objects by way of model studies. Knowing that a macroscopic object is a composite, how does one determine $E(M)$ in terms of the entanglements between its micro-constituents $E(μ)$? We assert that the notion of `levels of structure', the coupling strength between constituents in different levels, and the use of collective variables in each level are all pertinent factors. We consider two types of coupling, each constituent particle is coupled to only one other particle (1-to-1) versus …
Explaining how microscopic entities collectively produce macroscopic phenomena is a fundamental goal of many-body physics. Theory predicts that large-scale entanglement is responsible for exotic macroscopic phenomena, but observation of entangled particles in naturally occurring systems is extremely challenging. Synthetic quantum systems made of atoms in optical lattices have been con- structed with the goal of observing macroscopic quantum phenomena with single-atom resolution. Serious challenges remain in producing and detecting long-range quantum correlations in these systems, however. Here…
We present a new theoretical approach to describe the quantum behavior of a macroscopic system interacting with an external irradiation field, close to the resonant condition. Here we consider the extremely underdamped regime for a system described by a double well potential. The theory includes both: transitions from one well to the other and relaxation processes. We simulate resonant phenomena in a rf-SQUID, whose parameters lie in the range typically used in the experiments. The dependence of the transition probability W on the external drive of the system $ϕ_x$ shows three resonance peaks.…
H2O is one of the most important substances needed in sustaining life; but yet not much is known about its ground state. Here, a previously unidentified anomaly is identified in the form of a minimum in the imaginary part of the dielectric constant with respect to temperature near 20 K while the real part remains monotonic. Isothermal dispersion and absorption measurements show coinciding results. For the case of heavy ice (D2O), no anomaly was identified confirming an apparent isotope effect. Concerted quantum tunneling of protons is believed to be the main cause behind the reported anomaly. …
In this sequel paper we explore how macroscopic quantum phenomena can be measured or understood from the behavior of quantum correlations which exist in a quantum system of many particles or components and how the interaction strengths change with energy or scale, under ordinary situations and when the system is near its critical point. We use the nPI (master) effective action related to the Boltzmann-BBGKY / Schwinger-Dyson hierarchy of equations as a tool for systemizing the contributions of higher order correlation functions to the dynamics of lower order correlation functions. Together wit…
In this paper we explore the quantum behaviour of a SQUID ring which has a significant Josephson coupling energy. We show that that the eigenfunctions of the Hamiltonian for the ring can be used to create macroscopic quantum superposition states of the ring. We also show that the ring potential may be utilised to squeeze coherent states. With the SQUID ring as a strong contender as a device for manipulating quantum information, such properties may be of great utility in the future. However, as with all candidate systems for quantum technologies, decoherence is a fundamental problem. In this pa…
When dealing with macroscopic objects one usually observes quasiclassical phenomena, which can be described in terms of quasiclassical (or classical) equations of motion. Recent development of the theory of quantum computation is based on implementation of the entangled states which do not have a classical analogy. Using a simple example of a paramagnetic spin system we show that the entangled states can be detected in standard macroscopic experiments as a sharp deviation from quasiclassical motion.
We explore a previously unknown connection between two important problems in physics, i.e., quantum macroscopicity and the quantum phase transition. We devise a general and computable measure of quantum macroscopicity that can be applied to arbitrary spin states. We find that a macroscopic quantum superposition of an extremely large size arises during the quantum phase transition of the transverse Ising model in contrast to some seeming macroscopic quantum phenomena such as superconductivity, superfluidity and Bose-Einstein condensates. Our result may be an important step forward in understand…
The experimental observation of quantum phenomena in mechanical degrees of freedom is difficult, as the systems become linear towards low energies and the quantum limit, and thus reside in the correspondence limit. Here we investigate how to access quantum phenomena in flexural nanomechanical systems which are strongly deflected by a voltage. Near a metastable point, one can achieve a significant nonlinearity in the electromechanical potential at the scale of zero point energy. The system could then escape from the metastable state via macroscopic quantum tunneling (MQT). We consider two model…
We theoretically investigate exciton relaxation dynamics in molecular aggregates based on model photosynthetic complexes under various conditions of incoherent excitation. We show that noise-induced quantum coherence is generated between spatially-separated exciton states which belong to the same or different energy transfer pathways, coupled via real and virtual transfer processes. Such quantum coherence effects may be used to improve light-harvesting efficiency and to reveal quantum phenomena in biology.
We analyze the weak-field limit of General Relativity with matter and its possible quantisations. This analysis aims towards a predictive quantum theory to provide a first-principles description of gravitational effects in macroscopic quantum systems. This includes recently proposed experiments on the generation of (Newtonian) gravitational forces from quantum distributions of matter, and phenomena like gravity-induced entanglement, gravitational cat states, gravity-induced Rabi oscillations, and quantum causal orderings of events. Our main results include: (i) The demonstration that these phe…
Macroscopic quantum phenomena such as lasers, Bose-Einstein condensates, superfluids, and superconductors are of great importance in foundations and applications of quantum mechanics. In particular, quantum superposition of a large number of spins in solids is highly desirable for both quantum information processing and ultrasensitive magnetometry. Spin ensembles in solids, however, have rather short collective coherence time (typically less than microseconds). Here we demonstrate that under realistic conditions it is possible to maintain macroscopic quantum superposition of a large spin ensem…
Entanglement-facilitated macroscopic cluster formation in quantum many-body dynamics
School of Physical and Chemical Sciences, Queen Mary University of London（伦敦大学玛丽女王学院物理与化学科学学院）；Department of Physics, Tsinghua University（清华大学物理系）；Clarendon Laboratory, University of Oxford（牛津大学克拉伦登实验室）；Queen Mary University of London（伦敦大学玛丽女王学院）；Tsinghua University（清华大学）；University of Oxford（牛津大学）
A two boundary quantum mechanics without time ordered causal structure is advocated as consistent theory. The apparent causal structure of usual "near future" macroscopic phenomena is attributed to a cosmological asymmetry and to rules governing the transition between microscopic to macroscopic observations. Our interest is a heuristic understanding of the resulting macroscopic physics.
Nonclassical phenomena of quantum mechanics such as anticorrelation and photonic de Broglie waves (PBWs) have been recently understood as a special case of coherence optics with a particular phase relation between orthogonal bases composing a classical system. Such a macroscopic understanding of nonclassical features has also been confirmed experimentally for a coherence version of PBWs in a doubly-coupled Mach-Zehnder interferometer (MZI). Here, a multi-coupled MZI system is analyzed and discussed to obtain a general understanding of the nonclassical feature using tensor products of binary ba…
Macroscopic realism is a classical worldview that a macroscopic system is always determinately in one of the two or more macroscopically distinguishable states available to it, and so is never in a superposition of these states. The question of whether there is a fundamental limitation on the possibility to observe quantum phenomena at the macroscopic scale remains unclear. Here we implement a strict and simple protocol to test macroscopic realism in a light-matter interfaced system. We create a micro-macro entanglement with two macroscopically distinguishable solid-state components and rule o…
We present a scheme to deterministically prepare non-classical quantum states of a massive mirror including highly non-Gaussian states exhibiting sizeable negativity of the Wigner function. This is achieved by exploiting the non-linear light-matter interaction in an optomechanical cavity by driving the system with optimally designed frequency patterns. Our scheme reveals to be resilient against mechanical and optical damping, as well as mechanical thermal noise and imperfections in the driving scheme. Our proposal thus opens a promising route for table-top experiments to explore and exploit ma…
We review recent progress in utilizing ultrafast light-matter interaction to control the macroscopic properties of quantum materials. Particular emphasis is placed on photoinduced phenomena that do not result from ultrafast heating effects but rather emerge from microscopic processes that are inherently nonthermal in nature. Many of these processes can be described as transient modifications to the free-energy landscape resulting from the redistribution of quasiparticle populations, the dynamical modification of coupling strengths and the resonant driving of the crystal lattice. Other pathways…
For the purpose of understanding the quantum behavior such as quantum decoherence, fluctuations, dissipation, entanglement and teleportation of a mesoscopic or macroscopic object interacting with a general environment, we derive here a set of exact master equations for the reduced density matrix of $N$ interacting harmonic oscillators in a heat bath with arbitrary spectral density and temperature. Two classes of problems of interest to us which these equations can be usefully applied to are that of the quantum dynamics of nanoelectromechanical oscillators and the entanglement evolution of mult…
Macroscopic quantum vacuum and modern theories of gravitation share the strong interplay between geometry and physical phenomena. We review selected issues related to the accuracy of the measurement of Casimir forces with particular emphasis on the implications for the search of non-Newtonian gravitational forces in the micrometer range. We then discuss the interplay of the Higgs particle with gravitation, arguing that spectroscopic shifts in atomic transitions due to the modifications of the vacuum expectation value of the Higgs field in regions with strong curvature of space-time may be of c…
We propose the quantum mechanical description of complex systems should be performed using two types of causality relation: the ordering relation ($x\prec y$) and the subset relation ($A\subseteq B$). The structures with two ordering operations, called the causal sites, have been already proposed in context of quantum gravity (Christensen and Crane, 2005). We suggest they are also common to biological physics and may describe how the brain works. In the spirit of the Penrose ideas we identify the geometry of the space-time with universal field of consciousness. The latter has its evident count…
Macroscopic Quantum Electrodynamics with Gain: Modified Fluctuations and Their Consequences
RIKEN Centre for Advanced Photonics, RIKEN（RIKEN先进光子学中心）；Instituto Superior Técnico—University of Lisbon and Instituto de Telecomunicações（里斯本高等理工学院与电信研究所）；The Blackett Laboratory, Imperial College London（帝国理工学院布莱克特实验室）
Quantum phenomena appear in a macroscopic scale in Bose-Einstein condensates. The Gross-Pitaevskii (GP) equation describes the dynamics of the weakly interacting Bose-Einstein condensates. The GP equation has a form of the Schroedinger equation with self-interaction. The coupled Gross-Pitaevskii equations are used to describe some mixtures of Bose-Einstein condensates. In this paper, we will show some numerical results of coupled Gross-Pitaevskii equations without self-interaction, which has a form of nonlinearly-coupled Schroedinger equations. We demonstrate that the macroscopic oscillation a…
Quantum fluctuations and chaos in fully connected spin models
Institute of Physics, Johannes Gutenberg University Mainz（美因茨约翰内斯·古腾堡大学物理研究所）；School of Physics and Astronomy, University of St Andrews（圣安德鲁斯大学物理与天文学学院）；Department of Physics, University of Konstanz（康斯坦茨大学物理系）
We theoretically study classical thermal activation (TA) and macroscopic quantum tunneling (MQT) for a YBCO Josephson junction coupled with an LC circuit. The TA and MQT escape rate are calculated by taking into account the two-dimensional nature of the classical and quantum phase dynamics. We find that the MQT escape rate is largely suppressed by the coupling to the LC circuit. On the other hand, this coupling leads to the slight reduction of the TA escape rate. These results are relevant for the interpretation of a recent experiment on the MQT and TA phenomena in YBCO bi-epitaxial Josephson …
Macroscopic fields like electromagnetic, MHD, acoustic or gravitational waves are usually described by classical wave equations with possible additional damping terms and coherent sources. The aim of this paper is to develop a complete macroscopic formalism including random/thermal sources, dissipation and random scattering of waves by environment. The proposed reduced state of field (RSF) combines averaged field with the two-point correlation function called single-particle density matrix. The evolution equations for RSF is obtained by reduction of the generalized quasi-free dynamical semigro…
This paper summarises the results of our research on macroscopic entanglement in spin systems and free Bosonic gases. We explain how entanglement can be observed using entanglement witnesses which are themselves constructed within the framework of thermodynamics and thus macroscopic observables. These thermodynamical entanglement witnesses result in bounds on macroscopic parameters of the system, such as the temperature, the energy or the susceptibility, below which entanglement must be present. The derived bounds indicate a relationship between the occurrence of entanglement and the establish…
Quantum mechanics predicts microscopic phenomena with undeniable success. Nevertheless, current theoretical and experimental efforts still do not yield conclusive evidence that there is, or not, a fundamental limitation on the possibility to observe quantum phenomena at the macroscopic scale. This question prompted several experimental efforts producing quantum superpositions of large quantum states in light or matter. Here we report on the observation of entanglement between a single photon and an atomic ensemble. The certified entanglement stems from a light-matter micro-macro entangled stat…
We investigate classical thermal activation (TA) and macroscopic quantum tunneling (MQT) for a Josephson junction coupled with an LC circuit theoretically. The TA and MQT escape rate are calculated analytically by taking into account the two-dimensional nature of the classical and quantum phase dynamics. We find that the MQT escape rate is largely suppressed by the coupling to the LC circuit. On the other hand, this coupling gives rise to slight reduction of the TA escape rate. These results are relevant for the interpretation of a recent experiment on the MQT and TA phenomena in grain boundar…
Quantum physics challenges our understanding of the nature of physical reality and of space-time and suggests the necessity of radical revisions of their underlying concepts. Experimental tests of quantum phenomena involving massive macroscopic objects would provide novel insights into these fundamental questions. Making use of the unique environment provided by space, MAQRO aims at investigating this largely unexplored realm of macroscopic quantum physics. MAQRO has originally been proposed as a medium-sized fundamental-science space mission for the 2010 call of Cosmic Vision. MAQRO unites tw…
Despite several different measures of efficiency that are applicable to the photosynthetic systems, a precise degree of efficiency of these systems is not completely determined. Introducing an efficient model for the dynamics of light-harvesting complexes in biological environments is a major purpose in investigating such systems. Here, we investigate the effect of macroscopic quantum behavior of a system of two pigments on the transport phenomena in this system model which interacts with an oscillating environment. We use the second-order perturbation theory to calculate the time-dependent po…
Speed of state transitions in macroscopic systems is a crucial concept for foundations of nonequilibrium statistical mechanics as well as various applications in quantum technology represented by optimal quantum control. While extensive studies have made efforts to obtain rigorous constraints on dynamical processes since Mandelstam and Tamm, speed limits that provide tight bounds for macroscopic transitions have remained elusive. Here, by employing the local conservation law of probability, the fundamental principle in physics, we develop a general framework for deriving qualitatively tighter …
Many technologies emerging from quantum information science heavily rely upon the generation and manipulation of entangled quantum states. Here, we propose and demonstrate a new class of quantum interference phenomena that arise when states are created in and coherently converted between the propagating modes of an optical microcavity. The modal coupling introduces several new creation pathways to a nonlinear optical process within the device, which quantum mechanically interfere to drive the system between states in the time domain. The coherent conversion entangles the generated biphoton sta…
The investigation of macroscopic quantum phenomena is a current active area of research that offers significant promise to advance the forefronts of both fundamental and applied quantum science. Utilizing the exquisite precision and control of quantum optics provides a powerful toolset for generating such quantum states where the types and 'size' of the states that can be generated are set by the resourcefulness of the protocol applied. In this work we present a new scheme for 'growing' macroscopic superposition states of motion of a mechanical oscillator via cavity quantum optomechanics. The …
The quantum coherence of electronic quasiparticles underpins many of the emerging transport properties of conductors at small scales. Novel electronic implementations of quantum optics devices are now available with perspectives such as 'flying' qubit manipulations. However, electronic quantum interferences in conductors remained up to now limited to propagation paths shorter than $30\,μ$m, independently of the material. Here we demonstrate strong electronic quantum interferences after a propagation along two $0.1\,$mm long pathways in a circuit. Interferences of visibility as high as $80\%$ a…
To help resolve stubborn aporias in quantum mechanics, Kastner, Kauffman and Epperson have recently proposed a new interpretation of Heisenbergs ontological duality of res extensa and res potentia. In related work, Khrennikov and Aerts and their respective associates have explored the intermediate domain of mesoscopic phenomena in which quantum-like behavior can be observed and formalized. We generalize this work to define a third domain, one of macroscopic, interactive processes to which quantum concepts, but not quantum formalism apply. We show that they follow the non-standard logic propose…
We present an overview of the framework of macroscopic quantum electrodynamics from a quantum nanophotonics perspective. Particularly, we focus our attention on three aspects of the theory which are crucial for the description of quantum optical phenomena in nanophotonic structures. First, we review the light-matter interaction Hamiltonian itself, with special emphasis on its gauge independence and the minimal and multipolar coupling schemes. Second, we discuss the treatment of the external pumping of quantum-optical systems by classical electromagnetic fields. Third, we introduce an exact, co…
The combination of different quantum systems may allow the exploration of the distinctive features of each system for the investigation of fundamental phenomena as well as for quantum technologies. In this work we consider a setup consisting of an atomic ensemble enclosed within a laser-driven optomechanical cavity, having the moving mirror further (capacitively) coupled to a low frequency LC circuit. This constitutes a four-partite optoelectromechanical quantum system containing three macroscopic quantum subsystems of a different nature, viz, the atomic ensemble, the massive mirror and the LC…
