The long-standing debate whether the phase transition in the Dicke model can be realized with dipoles in electromagnetic fields is yet an unsettled one. The well-known statement often referred to as the "no-go theorem", asserts that the so-called A-square term, just in the vicinity of the critical point, becomes relevant enough to prevent the system from undergoing a phase transition. At variance with this common belief, in this paper we prove that the Dicke model does give a consistent description of the interaction of light field with the internal excitation of atoms, but in the dipole gauge of quantum electrodynamics. The phase transition cannot be excluded by principle and a spontaneous transverse-electric mean field may appear. We point out that the single-mode approximation is crucial: the proper treatment has to be based on cavity QED, wherefore we present a systematic derivation of the dipole gauge inside a perfect Fabry-Pérot cavity from first principles. Besides the impact on the debate around the Dicke phase transition, such a cleanup of the theoretical ground of cavity QED is important because currently there are many emerging experimental approaches to reach strong or even ultrastrong coupling between dipoles and photons, which demand a correct treatment of the Dicke model parameters.
We investigate realistic experimental conditions under which the collective Dicke model can be implemented in ion-cavity QED context. We show how ideal subradiance and superradiance can be observed and we propose an experiment to generate entanglement exploiting the existence of the subradiant state. We explore the conditions to achieve optimal entanglement generation and we show that they are reachable with current experimental technology.
The Dicke model consisting of an ensemble of two-state atoms interacting with a single quantized mode of the electromagnetic field exhibits a zero-temperature phase transition at a critical value of the dipole coupling strength. We propose a scheme based on multilevel atoms and cavity-mediated Raman transitions to realise an effective Dicke system operating in the phase transition regime. Output light from the cavity carries signatures of the critical behavior which is analyzed for the thermodynamic limit where the number of atoms is very large.
We generalize the Power-Zineau-Woolley transformation to obtain a canonical Hamiltonian of cavity quantum electrodynamics for arbitrary geometry of boundaries. This Hamiltonian is free from the A-square term and the instantaneous Coulomb interaction between distinct atoms. The single-mode models of cavity QED (Dicke, Tavis-Cummings, Jaynes-Cummings) are justified by a term by term mapping to the proposed microscopic Hamiltonian. As one straightforward consequence, the basis of no-go argumentations concerning the Dicke phase transition with atoms in electromagnetic fields dissolves.
The Dicke model of cavity quantum electrodynamics is approximately realized in condensed matter when the cyclotron transition of a two-dimensional electron gas is nearly resonant with a cavity photon mode. We point out that in the strong coupling limit the Dicke model of cavity cyclotron resonance must be supplemented by a term that is quadratic in the cavity photon field and suppresses the model's transition to a super-radiant state. We develop the theory of graphene cavity cyclotron resonance and show that the quadratic term, which is absent in graphene's low-energy Dirac model Hamiltonian, …
We propose a scheme to create universal Dicke states of n largely detuned atoms through detecting the leaky photons from an optical cavity. The generation of entangled states in our scheme has quasi-unit success probability, so it has potential practicability based on current or near coming laboratory cavity QED technology.
We discuss a general physical mechanism for arbitrary control of the quantum states of multiple qubits in the symmetric Dicke subspace. The qubit-qubit coupling leads to unequal energy spacing in the symmetric Dicke subspace. This allows one to manipulate a prechosen transition with an external driving source, with other transitions remaining off-resonant. Any entangled state in the symmetric Dicke subspace can be created from the initial ground state by tuning the driving source. We illustrate the idea in cavity QED, but it should be applicable to other related systems.
We study effective light-matter interactions in a circuit QED system consisting of a single $LC$ resonator, which is coupled symmetrically to multiple superconducting qubits. Starting from a minimal circuit model, we demonstrate that in addition to the usual collective qubit-photon coupling the resulting Hamiltonian contains direct qubit-qubit interactions, which have a drastic effect on the ground and excited state properties of such circuits in the ultrastrong coupling regime. In contrast to a superradiant phase transition expected from the standard Dicke model, we find an opposite mechanism…
We propose the analog-digital quantum simulation of the quantum Rabi and Dicke models using circuit quantum electrodynamics (QED). We find that all physical regimes, in particular those which are impossible to realize in typical cavity QED setups, can be simulated via unitary decomposition into digital steps. Furthermore, we show the emergence of the Dirac equation dynamics from the quantum Rabi model when the mode frequency vanishes. Finally, we analyze the feasibility of this proposal under realistic superconducting circuit scenarios.
We present a scheme to generate steady-state atomic spin squeezing in a cavity QED system using cavity-mediated Raman transitions to engineer effective atom-photon interactions, which include both linear and nonlinear (dispersive) atom-cavity couplings, on a potentially equal footing. We focus on a regime where the dispersive coupling is very large and find that the steady state of the system can in fact be a strongly spin-squeezed Dicke state, $|N/2,0\rangle$, of the atomic ensemble. These states offer Heisenberg-limited metrological properties and feature genuine multipartite entanglement am…
We consider the nonstationary circuit QED architecture in which a single-mode cavity interacts with N>1 identical qubits, and some system parameters undergo a weak external perturbation. It is shown that in the dispersive regime one can engineer the two-photon exchange interaction by adjusting the frequency of harmonic modulation to (approximately) $2|Δ_{-}|$, where $Δ_{-}$ is the average atom--field detuning. Closed analytic description is derived for the weak atom-field coupling regime, and numeric simulations indicate that the phenomenon can be observed in the present setups.
We propose a method to deterministically prepare a desired quantum state in a one-dimensional (1D) continuum by a shaped photon pulse. This method is based on time-reverse of the quantum emission process. We show that the desired quantum state such as Dicke or timed-Dicke state can be successfully prepared with very high fidelity even if the dissipation to the environment is nonnegligible and the pulse shaping is not perfect. We also show that large quantum entanglement between emitters can be created by just a single photon pulse. This method is experimentally feasible in 1D waveguide-QED or …
In order to examine whether or not the quantum phase transition of Dicke type exists in realistic systems, we revisit the model setup of the superconducting circuit QED from a microscopic many-body perspective based on the BCS theory with pseudo-spin presentation. By deriving the Dicke model with the correct charging terms from the minimum coupling principle, it is shown that the circuit QED system can exhibit superradiant quantum phase transition in the limit N\rightarrow\infty. The critical point could be reached at easiness by adjusting the extra parameters, the ratio of Josephson capacitan…
We revisit the derivation of Rabi- and Dicke-type models, which are commonly used for the study of quantum light-matter interactions in cavity and circuit QED. We demonstrate that the validity of the two-level approximation, which is an essential step in this derivation, depends explicitly on the choice of gauge once the system enters the ultrastrong coupling regime. In particular, while in the electric dipole gauge the two-level approximation can be performed as long as the Rabi frequency remains much smaller than the energies of all higher-lying levels, it can dramatically fail in the Coulom…
The Jaynes-Cummings model, with and without the rotating wave approximation, is expressed in the conjugate variable representation and solved numerically by wave packet propagation. Both cases are then cast into systems of two coupled harmonic oscillators, reminiscent of coupled bound electronic potential curves of diatomic molecules. Using the knowledge of such models, this approach of the problem gives new insight of the dynamics. The effect of the rotating wave approximation is discussed. The collapse-revival phenomenon is especially analyzed in a non-standard manner. Extensions of the meth…
Deterministic preparation of entangled Dicke states
Institute for Quantum Science and Engineering, Texas A&M University（德州农工大学量子科学与工程研究所）；Department of Biological and Agricultural Engineering, Texas A&M University（德州农工大学生物与农业工程系）
We propose a method for engineering spin dynamics in ensembles of integer-spin atoms confined within a high-finesse optical cavity. Our proposal uses cavity-assisted Raman transitions to engineer a Dicke model for integer-spin atoms, which, in a dispersive limit, reduces to effective atom-atom interactions within the ensemble. This scheme offers a promising and flexible new avenue for the exploration of a wide range of spinor many-body physics. As an example of this, we present results showing that this method can be used to generate spin-nematic squeezing in an ensemble of spin-1 atoms. With …
The existence of quantum tricriticality and exotic phases are found in a Dicke triangle (TDT) where three cavities, each one containing an ensemble of three-level atoms, are connected to each other through the action of an artificial magnetic field. The conventional superradiant phase (SR) is connected to the normal phase through first- and second-order boundaries, with tricritical points located at the intersection of such boundaries. Apart from the SR phase, a chiral superradiant (CSR) phase is found by tuning the artificial magnetic field. This phase is characterized by a nonzero photon cur…
We study the effect of spontaneous emission and incoherent atomic pumping on the nonlinear semiclassical dynamics of the unbalanced Dicke model -- a generalization of the Dicke model that features independent coupling strengths for the co- and counter-rotating interaction terms. As well as the ubiquitous superradiant behavior the Dicke model is well-known for, the addition of spontaneous emission combined with the presence of strong counter-rotating terms creates laser-like behavior termed counter-lasing. These states appear in the semiclassical model as stable periodic orbits. We perform a co…
Recently, the authors of the commented PRL presented the $ N=\infty $ solution of the $ U(1)/Z_2 $ Dicke model studied by us previously. Here we point out that (1) The authors missed an important transformation relating the two parameter regimes, so their separate discussions on the two regimes is redundant. (2) Both $ N=\infty $ classical limit and $ 1/N $ quantum fluctuations have been achieved in two of our previously published papers. It is the $ 1/N $ quantum fluctuations which lead to the non-trivial new quantum phenomena. In view of only a few $ N=2\sim 9 $ qubits inside a circuit QED m…
We introduce an extended Dicke model with controllable long-range atom-atom interaction to simulate topologically ordered states and achieve decoherence-protected qubits. We illustrate our idea in an experimentally feasible circuit quantum electrodynamics scenario. Due to the intrinsic competition with the atom-field coupling strength, we first demonstrate that this atom-atom interaction can exhibit a novel topological quantum interference effect arising from the instanton and anti-instanton tunneling paths. As a consequence, this proposed model only with a few odd-number of atoms has a two-fo…
Circuit QED on a chip has become a powerful platform for simulating complex many-body physics. In this report, we realize a Dicke-Ising model with an antiferromagnetic nearest-neighbor spin-spin interaction in circuit QED with a superconducting qubit array. We show that this system exhibits a competition between the collective spin-photon interaction and the antiferromagnetic nearest-neighbor spin-spin interaction, and then predict four quantum phases, including: a paramagnetic normal phase, an antiferromagnetic normal phase, a paramagnetic superradiant phase, and an antiferromagnetic superrad…
The interaction of a quantized electromagnetic field in a cavity with a set of two-level atoms inside can be described with algebraic Hamiltonians of increasing complexity, from the Rabi to the Dicke models. Their algebraic character allows, through the use of coherente states, a semiclassical description in phase space, where the non-integrable Dicke model has regions associated with regular and chaotic motion. The appearance of classical chaos can be quantified calculating the largest Lyapunov exponent in the whole available phase space for a given energy. In the quantum regime, employing ef…
Cavity quantum electrodynamics (C-QED) effects, such as Rabi splitting, Rabi oscillations and superradiance, have been demonstrated with nitrogen vacancy center spins in diamond in microwave resonators at cryogenic temperature. In this article we explore the possibility to realize strong collective coupling and the resulting C-QED effects with ensembles of spins at room temperature. Thermal excitation of the individual spins by the hot environment leads to population of collective Dicke states with low symmetry and a reduced collective spin-microwave field coupling. However, we show with simul…
We consider a generalized Dicke model with U(1) symmetry, which can undergo a transition to a superradiant state that spontaneously breaks this symmetry. By exploiting the difference in timescale between atomic and cavity dynamics, one may eliminate the cavity dynamics, providing an atom-only theory. We show that the standard Redfield theory cannot describe the transition to the superradiant state, but including higher-order corrections does recover the transition. Our work reveals how the forms of effective theories must vary for models with continuous symmetry, and provides a template to dev…
We investigate theoretically the cavity quantum electrodynamics of the cyclotron transition for Dirac fermions in graphene. We show that the ultrastrong coupling regime characterized by a vacuum Rabi frequency comparable or even larger than the transition frequency can be obtained for high enough filling factors of the graphene Landau levels. Important qualitative differences occur with respect to the corresponding physics of massive electrons in a semiconductor quantum well. In particular, an instability for the ground state analogous to the one occuring in the Dicke-model is predicted for in…
We discuss the simulation of non-perturbative cavity-QED effects using systems of trapped ions. Specifically, we address the implementation of extended Dicke models with both collective dipole-field and direct dipole-dipole interactions, which represent a minimal set of models for describing light-matter interactions in the ultrastrong and deep-strong coupling regime. We show that this approach can be used in state-of-the-art trapped ion setups to investigate excitation spectra or the transition between sub- and superradiant ground states, which are currently not accessible in any other physic…
We investigate theoretically how the spectroscopy of an ancillary qubit can probe cavity (circuit) QED ground states containing photons. We consider three classes of systems (Dicke, Tavis-Cummings and Hopfield-like models), where non-trivial vacua are the result of ultrastrong coupling between N two-level systems and a single-mode bosonic field. An ancillary qubit detuned with respect to the boson frequency is shown to reveal distinct spectral signatures depending on the type of vacua. In particular, the Lamb shift of the ancilla is sensitive to both ground state photon population and correlat…
Gauge invariance is the cornerstone of modern quantum field theory. Recently, it has been shown that the quantum Rabi model, describing the dipolar coupling between a two-level atom and a quantized electromagnetic field, violates this principle. This widely used model describes a plethora of quantum systems and physical processes under different interaction regimes. In the ultrastrong coupling regime, it provides predictions which drastically depend on the chosen gauge. This failure is attributed to the finite-level truncation of the matter system. We show that a careful application of the gau…
In cavity quantum electrodynamics (QED), the interaction between an atomic transition and the cavity field is measured by the vacuum Rabi frequency $Ω_0$. The analogous term "circuit QED" has been introduced for Josephson junctions, because superconducting circuits behave as artificial atoms coupled to the bosonic field of a resonator. In the regime with $Ω_0$ comparable to the two-level transition frequency, "superradiant" quantum phase transitions for the cavity vacuum have been predicted, e.g. within the Dicke model. Here, we prove that if the time-independent light-matter Hamiltonian is co…
We study a generic cavity-QED system where a set of (artificial) two-level dipoles is coupled to the electric field of a single-mode LC resonator. This setup is used to derive a minimal quantum mechanical model for cavity QED, which accounts for both dipole-field and direct dipole-dipole interactions. The model is applicable for arbitrary coupling strengths and allows us to extend the usual Dicke model into the non-perturbative regime of QED, where the dipole-field interaction can be associated with an effective finestructure constant of order unity. In this regime, we identify three distinct …
Jahn-Teller systems and the Jahn-Teller effect are discussed in terms of cavity QED models. By expressing the field modes in a quadrature representation, it is shown that certain setups of a two-level system interacting with a bimodal cavity is described by the Jahn-Teller $E\timesε$ Hamiltonian. We identify the corresponding adiabatic potential surfaces and the conical intersection. The effects of a non-zero geometrical Berry phase, governed by encircling the conical intersection, are studied in detail both theoretically and numerically. The numerical analysis is carried out by applying a wav…
We investigate the possibility of a Dicke-type superradiant phase transition of an atomic gas with an extended model which takes into account the short-range depolarizing interactions between atoms approaching each other as close as the atomic size scale, which interaction appears in a regularized electric-dipole picture of the QED of atoms. By using a mean field model, we find that a critical density does indeed exist, though the atom-atom contact interaction shifts it to a higher value than it can be obtained from the bare Dicke-model. We argue that the system, at the critical density, trans…
Sign-changing interactions constitute a crucial ingredient in the creation of frustrated many-body systems such as spin glasses. We present here the demonstration of a photon-mediated sign-changing interaction between Bose-Einstein condensed (BEC) atoms in a confocal cavity. The interaction between two atoms is of an unusual, nonlocal form proportional to the cosine of the inner product of the atoms' position vectors. This interaction arises from the differing Gouy phase shifts of the cavity's degenerate modes. Moreover, these Gouy phase anomalies induce an extra pattern of Z_2-symmetry-breaki…
Discrete time crystals are a recently proposed and experimentally observed out-of-equilibrium dynamical phase of Floquet systems, where the stroboscopic evolution of a local observable repeats itself at an integer multiple of the driving period. We address this issue in a driven-dissipative setup, focusing on the modulated open Dicke model, which can be implemented by cavity or circuit QED systems. In the thermodynamic limit, we employ semiclassical approaches and find rich dynamical phases on top of the discrete time-crystalline order. In a deep quantum regime with few qubits, we find clear s…
Starting from a general material system of $N$ particles coupled to a cavity, we use a coherent-state path integral formulation to produce a non-perturbative effective theory for the material degrees of freedom. We tackle the effects of image charges, the $A^2$ term and a multimode arbitrary-geometry cavity. The resulting (non-local) action has the photonic degrees of freedom replaced by an effective position-dependent interaction between the particles. In the large-$N$ limit, we discuss how the theory can be cast into an effective Hamiltonian where the cavity induced interactions are made exp…
Systems of strongly interacting atoms and photons, that can be realized wiring up individual cavity QED systems into lattices, are perceived as a new platform for quantum simulation. While sharing important properties with other systems of interacting quantum particles here we argue that the nature of light-matter interaction gives rise to unique features with no analogs in condensed matter or atomic physics setups. By discussing the physics of a lattice model of delocalized photons coupled locally with two-level systems through the elementary light-matter interaction described by the Rabi mod…
In this work, we study the $ U(1)/Z_2 $ Dicke model at a finite $ N $ by using the $ 1/J $ expansion and exact diagonization. This model includes the four standard quantum optics model as its various special limits. The $ 1/J $ expansions is complementary to the strong coupling expansion used by the authors in arXiv:1512.08581 to study the same model in its dual $ Z_2/U(1) $ representation. We identify 3 regimes of the system's energy levels: the normal, $ U(1) $ and quantum tunneling (QT) regime. The system's energy levels are grouped into doublets which consist of scattering states and Schro…
We study dynamical phase transitions (DPT) in the driven and damped Dicke model, realizable for example by a driven atomic ensemble collectively coupled to a damped cavity mode. These DPTs are characterized by non-analyticities of certain observables, primarily the overlap of time evolved and initial state. Even though the dynamics is dissipative, this phenomenon occurs for a wide range of parameters and no fine-tuning is required. Focusing on the state of the 'atoms' in the limit of a bad cavity, we are able to asymptotically evaluate an exact path integral representation of the relevant over…
We realize the dynamical 1D spin-orbit-coupling (SOC) of a Bose-Einstein condensate confined within an optical cavity. The SOC emerges through spin-correlated momentum impulses delivered to the atoms via Raman transitions. These are effected by classical pump fields acting in concert with the quantum dynamical cavity field. Above a critical pump power, the Raman coupling emerges as the atoms superradiantly populate the cavity mode with photons. Concomitantly, these photons cause a back-action onto the atoms, forcing them to order their spin-spatial state. This SOC-inducing superradiant Dicke p…
The quantum Rabi model describing the fundamental interaction between light and matter is a cornerstone of quantum physics. It predicts exotic phenomena like quantum phase transitions and ground-state entanglement in the ultrastrong-coupling (USC) regime, where coupling strengths are comparable to subsystem energies. Despite progress in many experimental platforms, the few experiments reaching USC have been limited to spectroscopy: demonstrating USC dynamics remains an outstanding challenge. Here, we employ a circuit QED chip with moderate coupling between a resonator and transmon qubit to rea…
