We report a theoretical study of the many-body effects of electron-electron interaction on the ground-state and spectral properties of double-layer graphene. Using a projector-based renormalization method we show that if a finite voltage difference is applied between the graphene layers electron-hole pairs can be formed and---at very low temperatures---an excitonic instability might emerge in a double-layer graphene structure. The single-particle spectral function near the Fermi surface exhibits a prominent quasiparticle peak, different from neutral (undoped) graphene bilayers. Away from the Fermi surface, we find that the charge carriers strongly interact with plasmons, thereby giving rise to a broad plasmaron peak in the angle-resolved photoemission spectrum.
We study the pairing symmetry of the interlayer paired state of composite fermions in quantum Hall bilayers. Based on the Halperin-Lee-Read (HLR) theory, the effect of the long-range Coulomb interaction and the internal Chern-Simons gauge fluctuation is analyzed with the random-phase approximation beyond the leading order contribution in small momentum expansion, and we observe that the interlayer paired states with a relative angular momentum $l=+1$ are energetically favored for filling $ν=\frac{1}{2}+\frac{1}{2}$ and $\frac{1}{4}+\frac{1}{4}$. The degeneracy between states with $\pm l$ is li…
We study bilayer fermionic cold atom systems with dipolar interactions, as well as a two-component tunable pseudopotential (TCTP) model which keeps only the zeroth and first Haldane pseudopotentials, at total Landau level filling factor 1/2. Our numerical results on the TCTP model indicates that Haldane-Rezayi state describes the critical point between strong and weak d-wave pairing quantum Hall phases. Further increasing the attractive zeroth pseudopotentials, the system transits from the strong-pairing phase to a stripe phase, and then to a cluster phase (or phase separation). The dipolar in…
Starting from a continuum-model description, we develop a microscopic weak-coupling theory for superconductivity in twisted double-bilayer graphene. We study both electron-phonon and entirely electronic pairing mechanisms. In each case, the leading superconducting instability transforms under the trivial representation, $A$, of the point group $C_3$ of the system, while the subleading pairing phases belong to the $E$ channel. We explicitly compute the momentum dependence of the associated order parameters and find that the leading state has no nodal points for electron-phonon pairing but exhib…
Triplon-mediated pairing and the superconducting gap structure in bilayer nickelates
National Laboratory of Solid State Microstructures and School of Physics, Nanjing University（南京大学固体微结构物理国家重点实验室和物理学院）；Collaborative Innovation Center of Advanced Microstructures, Nanjing University（南京大学先进微结构协同创新中心）；Max Planck Institute for Solid State Research（马克斯·普朗克固体研究所）
We investigate the twisted bilayer graphene by a two-orbital Hubbard model on the honeycomb lattice. The model is studied near 1/4 band filling by using the singular-mode functional renormalization group theory. Spin-triplet $f$-wave pairing is found from weak to moderate coupling limit of the local interactions, and is associated with the Hund's rule coupling and incommensurate spin fluctuations at moderate momenta.
We investigate phonon-mediated Cooper pairing in flat electronic band systems by solving the full-bandwidth multiband Eliashberg equations for superconductivity in magic angle twisted bilayer graphene using a realistic tight-binding model. We find that Cooper pairing away from the Fermi level contributes decisively to superconductivity by enhancing the critical temperature and ensures a robust finite superfluid density. We show that this pairing yields particle-hole asymmetric superconducting domes in the temperature-gating phase diagram and gives rise to distinct spectroscopic signatures in t…
Motivated by recent experimental studies that have found signatures of a correlated insulator phase and tuning superconductivity in twisted bilayer graphene, we study the temperature-dependent conductivity, the spin correlation and the superconducting pairing correlation within a two-orbital Hubbard model on an emergent honeycomb lattice. The evaluation of the temperature dependence of the conductivity demonstrates that there is a metal-insulator transition, and the Mott phase at strong coupling is accompanied by antiferromagnetic order. The electronic correlation drives a $d+id$ superconducti…
The pairing symmetry of an effective Hamiltonian for interacting fermions on a twisted bilayer graphene superlattice is studied with the determinant quantum Monte Carlo method. The model has the symmetry of a triangle lattice and a nearly-flat low energy band, features which underlie the magic-angle twisted bilayer graphene superlattice. We show that the low temperature phase is insulating at half-filling, even for relatively weak interactions. The natures of the spin and pairing correlations upon doping are determined, and exhibit an electron-hole asymmetry consistent with experiment. Among t…
In this work, we study the magnetic-impurity resonance states in superconducting phase of twisted bilayer graphene for different pairing symmetries. Using the two-orbital model proposed by Yuan and Fu in [Phys. Rev. B 98, 045103 (2018)], we find that when the impurity is located at one site of the emergent honeycomb lattice, the spacial distributions of the resonance states will break both the threefold and twofold rotation symmetries of $D_3$ group for pairing symmetries which belong to the irreducible representations of this point group. When the magnetic impurity is located at the center of…
Pairing Symmetry Crossover from $d$-wave to $s_{\pm}$-wave in a Bilayer Nickelate Driven by Hund's Coupling and Crystal Field Splitting
School of Physics and Astronomy, Beijing Normal University（北京师范大学物理学院）；Key Laboratory of Multiscale Spin Physics (Ministry of Education), Beijing Normal University（北京师范大学多尺度自旋物理教育部重点实验室）
Half-filled Landau levels admit the theoretically powerful fermion-vortex duality but longstanding puzzles remain in their experimental realization as $ν_T=1$ quantum Hall bilayers, further complicated by Zheng et al's recent numerical discovery of an unknown phase at intermediate layer spacing. Here we propose that half-filled quantum Hall bilayers ($ν_T=1$) at intermediate values of the interlayer distance $d/\ell_B$ enter a phase with \textit{paired exciton condensation}. This phase shows signatures analogous to the condensate of interlayer excitons (electrons bound to opposite-layer holes)…
We consider the pairing between conduction band electrons, and the valence band holes in the neutral bilayer-type structures. By employing the bilayer Hubbard model, we show the possibility of the inter-plane exciton formation in the system without applied external field. The in-plane and inter-plane Coulomb interaction effects on the pairing mechanism are considered, and the role of the in-plane particle hopping asymmetry on the gap behavior is analyzed in the paper. We show that both Frenkel-type pairing channel and Wannier-Mott-type excitonic pairings are present in the considered system. W…
We study the superconducting pairing symmetry in twisted bilayer graphene by solving the Bogoliubov-de Gennes equation for all electrons in moiré supercells. With increasing the pairing potential, the system evolves from the mixed nontopological $d+id$ and $p+ip$ phase to the $s+p+d$ phase via the first-order phase transition. In the time-reversal symmetry breaking $d+id$ and $p+ip$ phase, vortex and antivortex lattices accompanying spontaneous supercurrent are induced by the twist. The superconducting order parameter is nonuniform in the moiré unit cell. Nevertheless, the superconducting gap …
Interacting many-body systems combining confined and extended dimensions, such as ladders and few layer systems are characterized by enhanced quantum fluctuations, which often result in interesting collective properties. Recently two-dimensional bilayer systems, such as twisted bilayer graphene or ultracold atoms, have sparked a lot of interest because they can host rich phase diagrams, including unconventional superconductivity. Here we present a theoretical proposal for realizing high temperature pairing of fermions in a class of bilayer Hubbard models. We introduce a general, highly efficie…
Identifying the microscopic mechanism for superconductivity in magic-angle twisted bilayer graphene (MATBG) is an outstanding open problem. While MATBG exhibits a rich phase-diagram, driven partly by the strong interactions relative to the electronic bandwidth, its single-particle properties are unique and likely play an important role in some of the phenomenological complexity. Some of the salient features include an electronic bandwidth smaller than the characteristic phonon bandwidth and a non-trivial structure of the underlying Bloch wavefunctions. We perform a theoretical study of the coo…
We investigate the interplay of magnetic fluctuations and Cooper pairing in twisted bilayer graphene from a purely microscopic model within a large-scale tight-binding approach resolving the Ångström scale. For local onsite repulsive interactions and using the random-phase approximation for spin fluctuations, we derive a microscopic effective pairing interaction that we use for self-consistent solutions of the Bogoliubov-de-Gennes equations of superconductivity. We study the predominant pairing types as function of interaction strength, temperature and band filling. For large regions of this p…
Decoupled interband pairing in a bilayer iron-based superconductor evidenced by ultrahigh-resolution ARPES
Shanghai Jiao Tong University（上海交通大学）；Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所）；University of Chinese Academy of Sciences（中国科学院大学）；Zhejiang University（浙江大学）
The Josephson current is investigated in a superconducting graphene bilayer where pristine graphene sheets can make in-plane or out-of-plane displacements with respect to each other. The superconductivity can be of an intrinsic nature, or due to a proximity effect. The results demonstrate that the supercurrent responds qualitatively differently to relative displacement if the superconductivity is due to either intralayer or interlayer spin-singlet electron-electron pairing, thus providing a tool to distinguish between the two mechanisms. Specifically, both the AA and AB stacking orders are stu…
One of the most dominant candidates for the paired quantum Hall (QH) state at filling factor $ν=5/2$ is the Moore-Read (MR) Pfaffian state. A salient problem, however, is that it does not occur exactly at the Coulomb interaction, but rather at a modified interaction, which favors particle-hole symmetry breaking. In an effort to find a better state, in this work, we investigate the possible connection between the paired QH state and the antisymmetrized bilayer ground state, which is inspired by the intriguing identity that the MR Pfaffian state is entirely equivalent to the antisymmetrized proj…
We find exact analytic expressions for the energies and wavefunctions of the charged and neutral excitations above the exact ground states (at rational filling per unit cell) of projected Coulomb Hamiltonians in twisted bilayer graphene. Our exact expressions are valid for any form of the Coulomb interaction and any form of $AA$ and $AB/BA$ tunneling. The single charge excitation energy is a convolution of the Coulomb potential with a quantum geometric tensor of the TBG bands. The neutral excitations are (high-symmetry group) magnons, and their dispersion is analytically calculated in terms of…
Magic-angle twisted bilayer graphene exhibits a panoply of many-body phenomena that are intimately tied to the appearance of narrow and well-isolated electronic bands. The microscopic ingredients that are responsible for the complex experimental phenomenology include electron-electron (phonon) interactions and non-trivial Bloch wavefunctions associated with the narrow bands. Inspired by recent experiments, we focus on two independent quantities that are considerably modified by Coulomb interaction driven band renormalization, namely the density of states and the minimal spatial extent associat…
In this paper, we consider the spectral properties of the bilayer graphene with the local excitonic pairing interaction between the electrons and holes. We consider the generalized Hubbard model, which includes both intralayer and interlayer Coulomb interaction parameters. The solution of the excitonic gap parameter is used to calculate the electronic band structure, single-particle spectral functions, the hybridization gap, and the excitonic coherence length in the bilayer graphene. We show that the local interlayer Coulomb interaction is responsible for the semimetal-semiconductor transition…
In the present paper, we consider the excitonic effects on the single particle normal density of states (DOS) in the bilayer graphene (BLG). The local interlayer Coulomb interaction is considered between the particles on the non-equivalent sublattice sites in different layers of the BLG. We show the presence of the excitonic shift of the neutrality point, even for the noninteracting layers. Furthermore, for the interacting layers, a very large asymmetry in the DOS structure is shown between the particle and hole channels. At the large values of the interlayer hopping amplitude, a large number …
Hierarchical structure of primary and hybridization-induced superconducting correlations in bilayer nickelates
College of Industrial Technology, Nihon University（日本大学工业技术学部）；Research Organization of Science and Technology, Ritsumeikan University（立命馆大学科学技术研究院）；Faculty of Engineering, Tottori University（鸟取大学工学部）；Department of Physics, The University of Osaka（大阪大学物理学系）
Fully occupied or unoccupied bands in a solid are often considered inert and irrelevant to a material's low-energy properties. But the discovery of enhanced superconductivity in heavily electron-doped FeSe-derived superconductors poses questions about the possible role of incipient bands (those laying close to but not crossing the Fermi level) in pairing. To answer this question, researchers have studied pairing correlations in the bilayer Hubbard model, which has an incipient band for large interlayer hopping $t_\perp$, using many-body perturbation theory and variational methods. They have ge…
PH Pfaffian topological phase may exist in a uniform system due to strong Landau level (LL) mixing according to theoretical predictions based on the Son - Dirac composite fermion theory. Numerical investigations in the presence of large LL mixing are limited due to numerical complexities, when taking into account at least one more LL. Because of this, we apply the same field theoretical approach to the quantum Hall bilayer at total filling factor equal to one, for which many numerical studies exist. The most recent work in the torus geometry predicts an intermediate phase (for intermediate dis…
One of the outstanding questions in the study of twisted bilayer graphene -- from both experimental and theoretical points of view -- is the nature of its superconducting phase. In this work we perform a comprehensive synthesis of existing experiments, and argue that experimental constraints are strong enough to allow the structure of the superconducting order parameter to be nearly uniquely determined. In particular, we argue that the order parameter is nodal, and is formed from an admixture of spin-singlet and spin-triplet Cooper pairs. This argument is made on phenomenological grounds, with…
Based on our revised perturbational-band theory, we study possible pairing states driven by interaction in the electron-doped quasicrystal 30\degree-twisted bilayer graphene. Our mean-field study on the related t-J model predicts that, the beneath-van-Hove and beyond-van-Hove low doping regimes are covered by the chiral $d+id$ and $g+ig$ topological superconductivities (TSCs) respectively. The $g+ig$-TSC possesses a pairing angular momentum 4, and hence following each effective $C_{12}$- rotation by $Δϕ=nπ/6$, the pairing phase changes $4Δϕ$. This intriguing TSC is novel, as it belongs to a sp…
In the present paper, we describe the antiferromagnetic and excitonic correlations in the AA-stacked bilayer graphene. We consider the applied external electric field potential to the structure which leads to the electronic charge imbalance between the layers in the system. By using the generalized two-layer Hubbard Hamiltonian, we consider different particle filling regimes in the layers. We calculate the important energy scales in the system and we establish the conditions for the appearance of the antiferromagnetic order in the system. We consider both large and small Coulomb interaction li…
We show that unconventional nematic superconductors with multi-component order parameter in lattices with three-fold and six-fold rotational symmetries support a charge-$4e$ vestigial superconducting phase above $T_c$. The charge-$4e$ state, which is a condensate of four-electron bound states that preserve the rotational symmetry of the lattice, is nearly degenerate with a competing vestigial nematic state, which is non-superconducting and breaks the rotational symmetry. This robust result is the consequence of a hidden discrete symmetry in the Ginzburg-Landau theory, which permutes quantities…
The evolution of pairing correlation with $3d_{z^{2}}$ electron filling in a bilayer two-orbital model for La$_3$Ni$_2$O$_7$
Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education), School of Physics and Astronomy, Shanghai Jiao Tong University（上海交通大学物理与天文学院人工结构与量子控制教育部重点实验室）；State Key Laboratory of Quantum Functional Materials, School of Physical Science and Technology, ShanghaiTech University（上海科技大学物理科学与技术学院量子功能材料国家重点实验室）；Tsung-Dao Lee Institute, Shanghai Jiao Tong University（上海交通大学李政道研究所）；Hefei National Laboratory（合肥国家实验室）
Using a Green's function approach, we study phonon-mediated superconducting pairing symmetries that may arise in bilayer graphene where the monolayers are displaced in-plane with respect to each other. We consider a generic coupling potential between the displaced graphene monolayers, which is applicable to both shifted and commensurate twisted graphene layers; study intralayer and interlayer phonon-mediated BCS pairings; and investigate AA and AB(AC) stacking orders. Our findings demonstrate that at the charge neutrality point, the dominant pairings in both AA and AB stackings with intralayer…
