We consider ground state of electron-hole graphene bilayer composed of two independently doped graphene layers when a condensate of spatially separated electron-hole pairs is formed. In the weak coupling regime the pairing affects only conduction band of electron-doped layer and valence band of hole-doped layer, thus the ground state is similar to ordinary BCS condensate. At strong coupling, an ultrarelativistic character of electron dynamics reveals and the bands which are remote from Fermi surfaces (valence band of electron-doped layer and conduction band of hole-doped layer) are also affected by the pairing. The analysis of instability of unpaired state shows that s-wave pairing with band-diagonal condensate structure, described by two gaps, is preferable. A relative phase of the gaps is fixed, however at weak coupling this fixation diminishes allowing gapped and soliton-like excitations. The coupled self-consistent gap equations for these two gaps are solved at zero temperature in the constant-gap approximation and in the approximation of separable potential. It is shown that, if characteristic width of the pairing region is of the order of magnitude of chemical potential, then the value of the gap in the spectrum is not much different from the BCS estimation. However, if the pairing region is wider, then the gap value can be much larger and depends exponentially on its energy width.
We discuss the composite fermion pairing state in bilayer quantum Hall systems. After the evaluation of the range of the inter-layer separation in which the quantum Hall state is stabilized, we discuss the effect of inter-layer tunneling on the composite fermion pairing state at ν=1/2. We show that there is a cusp at the transition point between the Halperin (3,3,1) state and the Pfaffian state.
We study interacting GaAs bilayer hole systems, with very small interlayer tunneling, in a counterflow geometry where equal currents are passed in opposite directions in the two, independently contacted layers. At low temperatures, both the longitudinal and Hall counterflow resistances tend to vanish in the quantum Hall state at total bilayer filling $ν=1$, demonstrating the pairing of oppositely charged carriers in opposite layers. The temperature dependence of the counterflow Hall resistance is anomalous compared to the other transport coefficients: even at relatively high temperatures ($\si…
We study the pairing symmetry of the interlayer paired state of composite fermions in quantum Hall bilayers. Based on the Halperin-Lee-Read (HLR) theory, the effect of the long-range Coulomb interaction and the internal Chern-Simons gauge fluctuation is analyzed with the random-phase approximation beyond the leading order contribution in small momentum expansion, and we observe that the interlayer paired states with a relative angular momentum $l=+1$ are energetically favored for filling $ν=\frac{1}{2}+\frac{1}{2}$ and $\frac{1}{4}+\frac{1}{4}$. The degeneracy between states with $\pm l$ is li…
We report a theoretical study of the many-body effects of electron-electron interaction on the ground-state and spectral properties of double-layer graphene. Using a projector-based renormalization method we show that if a finite voltage difference is applied between the graphene layers electron-hole pairs can be formed and---at very low temperatures---an excitonic instability might emerge in a double-layer graphene structure. The single-particle spectral function near the Fermi surface exhibits a prominent quasiparticle peak, different from neutral (undoped) graphene bilayers. Away from the F…
We derive the effective Hamiltonian for the composite fermion in double-layer quantum Hall systems with inter-layer tunneling at total Landau-level filling factor $ν=1/m$, where $m$ is an integer. We find that the ground state is the triplet p-wave BCS pairing state of the composite fermions. At $ν=1/2$, the ground state of the system evolves from the Halperin $(3,3,1)$-state toward the Pfaffian-state with increasing the tunneling amplitude. On the other hand, at $ν=1$, the pairing state is uniquely determined independent of tunneling amplitude.
Starting from a continuum-model description, we develop a microscopic weak-coupling theory for superconductivity in twisted double-bilayer graphene. We study both electron-phonon and entirely electronic pairing mechanisms. In each case, the leading superconducting instability transforms under the trivial representation, $A$, of the point group $C_3$ of the system, while the subleading pairing phases belong to the $E$ channel. We explicitly compute the momentum dependence of the associated order parameters and find that the leading state has no nodal points for electron-phonon pairing but exhib…
Transitions from a paired quantum Hall state to another quantum Hall state in bilayer systems are discussed in the framework of the edge theory. Starting from the edge theory for the Haldane-Rezayi state, it is shown that the charging effect of a bilayer system which breaks the SU(2) symmetry of the pseudo-spin shifts the central charge and the conformal dimensions of the fermionic fields which describe the pseudo-spin sector in the edge theory. This corresponds to the transition from Haldane-Rezayi state to Halperin's 331 state, or singlet d-wave to triplet p-wave ABM type paired state in the…
Cooper pairing of spatially separated electrons and holes in graphene bilayer is studied beyond the mean-field approximation. Suppression of the screening at large distances, caused by appearance of the gap, is considered self-consistently. A mutual positive feedback between appearance of the gap and enlargement of the interaction leads to a sharp transition to correlated state with greatly increased gap above some critical value of the coupling strength. At coupling strength below the critical, this correlation effect increases the gap approximately by a factor of two. The maximal coupling st…
Half-filled Landau levels admit the theoretically powerful fermion-vortex duality but longstanding puzzles remain in their experimental realization as $ν_T=1$ quantum Hall bilayers, further complicated by Zheng et al's recent numerical discovery of an unknown phase at intermediate layer spacing. Here we propose that half-filled quantum Hall bilayers ($ν_T=1$) at intermediate values of the interlayer distance $d/\ell_B$ enter a phase with \textit{paired exciton condensation}. This phase shows signatures analogous to the condensate of interlayer excitons (electrons bound to opposite-layer holes)…
We study the proximity-induced superconducting state in a general bilayer -- conventional $s$-wave superconductor hybrid structure. For the bilayer we include a general parabolic dispersion, Rashba spin-orbit coupling, and finite layer tunneling as well as the possibility to apply a bias potential and a magnetic Zeeman field, in order to address experimentally relevant bilayer systems, ranging from topological insulator thin films to generic double quantum well systems. By extracting the proximity-induced anomalous Green's function in the bilayer we show on a very rich structure for the superc…
Identifying the microscopic mechanism for superconductivity in magic-angle twisted bilayer graphene (MATBG) is an outstanding open problem. While MATBG exhibits a rich phase-diagram, driven partly by the strong interactions relative to the electronic bandwidth, its single-particle properties are unique and likely play an important role in some of the phenomenological complexity. Some of the salient features include an electronic bandwidth smaller than the characteristic phonon bandwidth and a non-trivial structure of the underlying Bloch wavefunctions. We perform a theoretical study of the coo…
The topological nature of Weyl semimetals (WSMs) is corroborated by the presence of chiral surface states, which connect the projections of the bulk Weyl points by Fermi arcs (FAs). We study a bilayer structure realized by introducing a thin insulating spacer into a bulk WSM. Employing a self-consistent mean-field description of the interlayer Coulomb interaction, we propose that this system can develop an interlayer electron-hole pair condensate. The formation of this excitonic condensate leads to partial gapping of the FA dispersion. We obtain the dependence of the energy gap and the critica…
We provide numerical evidence for composite fermion pairing in quantum Hall bilayer systems at filling $ν=1/2 + 1/2$ for intermediate spacing between the layers. We identify the phase as $p_x + i p_y$ pairing, and construct high accuracy trial wavefunctions to describe the groundstate on the sphere. For large distances between the layers, and for finite systems, a competing "Hund's rule" state, or composite fermion liquid, prevails for certain system sizes. We argue that for larger systems, the pairing phase will persist to larger layer spacing.
The Josephson current is investigated in a superconducting graphene bilayer where pristine graphene sheets can make in-plane or out-of-plane displacements with respect to each other. The superconductivity can be of an intrinsic nature, or due to a proximity effect. The results demonstrate that the supercurrent responds qualitatively differently to relative displacement if the superconductivity is due to either intralayer or interlayer spin-singlet electron-electron pairing, thus providing a tool to distinguish between the two mechanisms. Specifically, both the AA and AB stacking orders are stu…
In n-p bilayer systems an exotic phase-coherent state emerges due to Coulomb pairing of n-layer electrons with p-layer holes. Unlike Josephson junctions, the order parameter phase may be locked by matrix elements of interlayer tunneling in n-p bilayers. Here we show how the phase locking phenomenon specifies the response of the electron-hole condensate to interlayer voltages. In the absence of an applied magnetic field, the phase is steady-state (locked) at low interlayer voltages, V<V_c, however the phase increases monotonically with time (is unlocked) at V>V_c. The change in the system dynam…
We find exact analytic expressions for the energies and wavefunctions of the charged and neutral excitations above the exact ground states (at rational filling per unit cell) of projected Coulomb Hamiltonians in twisted bilayer graphene. Our exact expressions are valid for any form of the Coulomb interaction and any form of $AA$ and $AB/BA$ tunneling. The single charge excitation energy is a convolution of the Coulomb potential with a quantum geometric tensor of the TBG bands. The neutral excitations are (high-symmetry group) magnons, and their dispersion is analytically calculated in terms of…
We investigate the many-body instabilities of electrons interacting near Van Hove singularities arising in monolayer and twisted bilayer graphene. We show that a pairing instability must be dominant over the tendency to magnetic order as the Fermi level is tuned to the Van Hove singularity in the conduction band of graphene. As a result of the extended character of the saddle points in the dispersion, we find that the pairing of the electrons takes place preferentially in a channel of f-wave symmetry, with an order parameter vanishing at the position of the saddle points along the Fermi line. …
Magic-angle twisted bilayer graphene exhibits a panoply of many-body phenomena that are intimately tied to the appearance of narrow and well-isolated electronic bands. The microscopic ingredients that are responsible for the complex experimental phenomenology include electron-electron (phonon) interactions and non-trivial Bloch wavefunctions associated with the narrow bands. Inspired by recent experiments, we focus on two independent quantities that are considerably modified by Coulomb interaction driven band renormalization, namely the density of states and the minimal spatial extent associat…
In this paper, we consider the spectral properties of the bilayer graphene with the local excitonic pairing interaction between the electrons and holes. We consider the generalized Hubbard model, which includes both intralayer and interlayer Coulomb interaction parameters. The solution of the excitonic gap parameter is used to calculate the electronic band structure, single-particle spectral functions, the hybridization gap, and the excitonic coherence length in the bilayer graphene. We show that the local interlayer Coulomb interaction is responsible for the semimetal-semiconductor transition…
We show how the pairing symmetry of superconducting states in twisted bilayer graphene can be experimentally identified by theoretically studying effects of externally applied in-plane magnetic field and strain. In the low field regime, superconducting critical temperature $T_c$ is suppressed by in-plane magnetic field $\boldsymbol{B}_{\parallel}$ in singlet channels, but is enhanced by weak $\boldsymbol{B}_{\parallel}$ in triplet channels, providing an important distinction. The in-plane angular dependence of the critical $\boldsymbol{B}_{\parallel, c}$ has a six-fold rotational symmetry, whi…
We develop a theory for interlayer pairing of chiral electrons in graphene materials which results in an unconventional superconducting (S) state with s-wave spin-triplet order parameter. In a pure bilayer graphene, this superconductivity exhibits a gapless property with an exotic effect of temperature-induced condensation causing an increase of the pairing amplitude (PA) with increasing temperature. We find that a finite doping opens a gap in the excitation spectrum and weakens this anomalous temperature-dependence. We further explore the possibility of realizing variety of pairing patterns w…
In this work the effects of defects in the superconducting phases of the twisted bilayer graphene (TBG) are investigated. A will-accepted low energy effective model and a non-magnetic impurity potential to mimic defects are employed. Different superconducting pairing symmetries, including $s$-wave, $(d+id)$-wave and $(p+ip)$-wave pairing, are considered. In single impurity case, the local density of states (DOS) are calculated for the pairing symmetries above. For different pairing symmetries the number and property of bound states induced by defects are different. In multi-impurity case, the …
PH Pfaffian topological phase may exist in a uniform system due to strong Landau level (LL) mixing according to theoretical predictions based on the Son - Dirac composite fermion theory. Numerical investigations in the presence of large LL mixing are limited due to numerical complexities, when taking into account at least one more LL. Because of this, we apply the same field theoretical approach to the quantum Hall bilayer at total filling factor equal to one, for which many numerical studies exist. The most recent work in the torus geometry predicts an intermediate phase (for intermediate dis…
Microscopic details such as interactions and Fermiology determine the structure of superconducting pairing beyond the spatial symmetry classification along irreducible point group representations. From the effective pairing vertex, the pairing wave function related to superconducting order unfolds in its orbital-resolved Fourier profile which we call the harmonic fingerprint (HFP). The HFP allows to formulate a concise connection between microsopic parameter changes and their impact on superconductivity. From a random phase approximation analysis of twisted bilayer graphene (TBG) involving $d+…
A strong low-temperature enhancement of the tunneling conductance between graphene bilayers has been reported recently, and interpreted as a signature of equilibrium electron-hole pairing, first predicted in bilayers more than forty years ago but previously unobserved. Here we provide a detailed theory of conductance enhanced by fluctuating electron-hole Cooper pairs, which are a precursor to equilibrium pairing, that accounts for specific details of the multi-band double graphene bilayer system which supports several different pairing channels. Above the equilibrium condensation temperature, …
Using a Green's function approach, we study phonon-mediated superconducting pairing symmetries that may arise in bilayer graphene where the monolayers are displaced in-plane with respect to each other. We consider a generic coupling potential between the displaced graphene monolayers, which is applicable to both shifted and commensurate twisted graphene layers; study intralayer and interlayer phonon-mediated BCS pairings; and investigate AA and AB(AC) stacking orders. Our findings demonstrate that at the charge neutrality point, the dominant pairings in both AA and AB stackings with intralayer…
The superconducting critical temperature $T_C$ of a superconductor/ferromagnet (S/F) bilayer with spin-flip scatterings at the interface is calculated as a function of the ferromagnet thickness $d_F$ in the dirty limit employing the Usadel equation. The appropriate boundary conditions from the spin-flip scatterings at the S/F interface are derived for the Usadel equation which includes the spin triplet pairing components as well as the spin singlet one. The spin-flip processes induce the spin triplet pairing components with s-wave in momentum and odd symmetry in frequency from the s-wave singl…
The existence of spin-triplet superconductivity in non-collinear magnetic heterostructures with superconductors is by now well established. This observation lays the foundation of superconducting spintronics with the aim to create a low-power consuming devices in order to replace the conventional electronics limited by heating. From a fundamental point of view the investigation of the structure and properties of spin-triplet Cooper pairs continues. Recently, spectroscopic evidence has shown to offer more detailed insights in the structure of triplet Cooper pairs than the supercurrent. Hence, w…
We theoretically demonstrate the formation of a new type of unconventional superconductivity in graphene materials, which exhibits gapless property. The studied superconductivity is based on an interlayer pairing of chiral electrons in bilayer graphene, which results in an exotic s-wave spin-triplet condensate order with anomalous thermodynamic properties. These include the possibility of a temperature induced condensation causing an increase of the pairing gap with increasing temperature, and an entropy of the stable superconducting state which can be higher than its value in the normal state…
Layer-Asymmetry-Induced Topological Superconductivity in High-T$_c$ Bilayer Nickelates
Hong Kong University of Science and Technology（香港科技大学）；RIKEN Interdisciplinary Theoretical and Mathematical Sciences (iTHEMS)（理化学研究所交叉理论与数学科学中心）；Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所）；CAS Key Laboratory of Theoretical Physics, Institute of Theoretical Physics, Chinese Academy of Sciences（中国科学院理论物理研究所理论物理重点实验室）；School of Physics, Beijing Institute of Technology（北京理工大学物理学院）
We investigate hybrid structures based on a bilayer quantum spin Hall system in proximity to an s-wave superconductor as a platform to mimic time-reversal symmetric topological superconductors. In this bilayer setup, the induced pairing can be of intra- or inter-layer type, and domain walls of those different types of pairing potentials host Kramers partners (time-reversal conjugate pairs) of Majorana bound states. Interestingly, we discover that such topological interfaces providing Majorana bound states can also be achieved in an otherwise homogeneous system by a spatially dependent inter-la…
Topological flat bands, valley polarization, and interband superconductivity in magic-angle twisted bilayer graphene with proximitized spin-orbit couplings
Ferroelectric Hysteresis in Superconducting Bilayer Td-MoTe2
State Key Laboratory of Quantum Functional Materials, School of Physical Science and Technology, ShanghaiTech University（上海科技大学物理科学与技术学院量子功能材料国家重点实验室）；ShanghaiTech Laboratory for Topological Physics, ShanghaiTech University（上海科技大学拓扑物理实验室）
Superfluidity has recently been reported in double electron-hole bilayer graphene. The multiband nature of the bilayers is important because of the very small band gaps between conduction and valence bands. The long range nature of the superfluid pairing interaction means that screening must be fully taken into account. We have carried out a systematic mean-field investigation that includes (i) contributions to screening from both intraband and interband excitations, (ii) the low-energy band structure of bilayer graphene with its small band gap and flattened Mexican hat-like low-energy bands, …
We present a systematic classification and analysis of possible pairing instabilities in graphene-based moiré superlattices. Motivated by recent experiments on twisted double-bilayer graphene showing signs of triplet superconductivity, we analyze both singlet and triplet pairing separately, and describe how these two channels behave close to the limit where the system is invariant under separate spin rotations in the two valleys, realizing an SU(2)$_+$ $\times$ SU(2)$_-$ symmetry. Further, we discuss the conditions under which singlet and triplet can mix via two nearly degenerate transitions, …
Motivated by experiments on twisted bilayer graphene, we study the emergence of superconductivity from $\textit{weak}$ repulsive interactions in the Hubbard model on a honeycomb lattice, with both spin and orbital degeneracies, and with the filling treated as a tunable control parameter. The attraction is generated through the Kohn-Luttinger mechanism. We find, similar to old studies of single layer graphene, that the leading superconducting instability is in a $d$-wave pairing channel close to Van Hove filling, and is in an $f$-wave pairing channel away from Van Hove filling. The $d$-wave pai…
Bilayer transition metal dichalcogenides (TMDs) belong to a class of materials with two unique features, the coupled spin-valley-layer degrees of freedom and the crystal structure that is globally centrosymmetric but locally non-centrosymmetric. In this work, we will show that the combination of these two features can lead to a rich phase diagram for unconventional superconductivity, including intra-layer and inter-layer singlet pairings and inter-layer triplet pairings, in bilayer superconducting TMDs. In particular, we predict that the inhomogeneous Fulde-Ferrell-Larkin-Ovchinnikov state can…
Coulomb screening of superconductivity in magic-angle twisted bilayer graphene
School of Physics & Astronomy, University of Manchester（曼彻斯特大学物理与天文学学院）；National Graphene Institute, University of Manchester（曼彻斯特大学国家石墨烯研究所）；Department of Physics, Washington University in St. Louis（华盛顿大学圣路易斯分校物理系）；Department of Physics and Astronomy, University of Pennsylvania（宾夕法尼亚大学物理与天文学系）；Department of Physics, University of Antwerp（安特卫普大学物理系）；Henry Royce Institute for Advanced Materials, The University of Manchester（曼彻斯特大学亨利·罗伊斯先进材料研究所）；National Institute for Materials Science（国立材料研究所）；Department of Materials Science and Engineering, National University of Singapore（新加坡国立大学材料科学与工程系）；Department of Physics, National University of Singapore（新加坡国立大学物理系）
I study the possible phase transitions when two layers at filling factor $ν_t=1$ are gradually separated. In the bosonic case the system should undergo a pairing transition from a Fermi liquid to an incompressible state. In the Fermionic case, the state evolves from an incompressible $(1,1,1)$ state to a Fermi liquid. I speculate that there is an intermediate phase involving charge two quasiparticles.
We derive ground state wave functions of superconducting instabilities on the honeycomb lattice induced by nearest-neighbor attractive interactions. They reflect the Dirac nature of electrons in the low-energy limit. For the order parameter that is the same irrespective of the direction to any of the nearest neighbors we find weak pairing (slowly decaying) behavior in the orbital part of the Cooper pair with no angular dependence. At the neutrality point, in the spin-singlet case, we recover a strong pairing behavior. We also derive ground state wave functions for the superconductivity on the …
We consider the optical properties of the half-filled AB-stacked bilayer graphene with the excitonic pairing and condensation between the layers. Both intra and interlayer local Coulomb interaction effects have been taken into account and the role of the exact Fermi energy has been discussed in details. We have calculated the absorption coefficient, refractive index, dielectric response functions and the electron energy loss spectrum for different interlayer Coulomb interaction regimes and for different temperatures. Considering the full four-band model for the interacting AB bilayer graphene,…
Superfluidity in e-h bilayers in graphene and GaAs has been predicted many times but not observed. A key problem is how to treat the screening of the Coulomb interaction for pairing. Different mean-field theories give dramatically different conclusions, and we test them against diffusion Monte-Carlo calculations. We get excellent agreement with the mean-field theory that uses screening in the superfluid state, but large discrepancies with the others. The theory predicts no superfluidity in existing devices and gives pointers for new devices to generate superfluidity.
Layered bosonic dipolar fluids have been suggested to host a condensate of interlayer molecular bound states. However, its experimental observation has remained elusive. Motivated by two recent experimental works [Hubert et al., Phys. Rev. X 9, 021026 (2019) and D. J. Choksy et al., Phys. Rev. B 103 045126 (2021)], we theoretically study, using numerically exact quantum Monte Carlo calculations, the experimental signatures of collective interlayer pairing in vertically stacked indirect exciton (IX) layers. We find that IX energy shifts associated with each layer evolve non trivially as a funct…
The superconducting pairing of electrons in doped graphene due to in-plane and out-of-plane phonons is considered. It is shown that the structure of the order parameter in the valley space substantially affects conditions of the pairing. Electron-hole pairing in graphene bilayer in the strong coupling regime is also considered. Taking into account retardation of the screened Coulomb pairing potential shows a significant competition between the electron-hole direct attraction and their repulsion due to virtual plasmons and single-particle excitations.
Recently, a Dirac (particle-hole symmetric) description of composite fermions in the half-filled quantum Hall system was proposed [D. T. Son, Phys. Rev. X 5, 031027 (2015)], and we study its possible consequences on BCS (Cooper) pairing of composite fermions (CF's). One of the main consequences is the existence of anisotropic states in single and bilayer systems, which was previously suggested in Ref. [J. S. Jeong and K. Park, Phys. Rev. B 91, 195119 (2015)]. We argue that in the half-filled single layer the gapped states may sustain anisotropy, because isotropic pairings may coexist with anis…
We present a unified description of zitterbewegung-like phenomena for electron and hole systems showing Rashba spin splitting as well as for electrons in single-layer and bilayer graphene. The former class of systems can be interpreted as "nonrelativistic" whereas the latter are often called "ultrarelativistic" so that our unified description indicates an interesting connection between these two opposite limits.
