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arXiv 1202.0184physics.atom-ph
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通过402 nm共振线的双光子laser激发俘获的232 Th+离子

Two-photon laser excitation of trapped 232Th+ ions via the 402 nm resonance line

O. A. Herrera-Sancho, M. V. Okhapkin, K. Zimmermann, Chr. Tamm, E. Peik, A. V. Taichenachev, V. I. Yudin, P. Glowacki

摘要:

报道了在射频离子阱中用单光子和双光子激光激发~(232)Th ~+离子的实验。作为第一个激发步骤,通过来自扩展腔二极管激光器的辐射驱动在402 nm处从6d^2 7s J=3/2基态到24874 cm^{-1}处的6d 7s 7 p J=5/2态的最强共振线。中间态的自发衰变填充了许多低的亚稳态,从而限制了连续激光激发可获得的激发态数量和荧光信号。我们研究了氦、氩和氮缓冲气体的碰撞猝灭效率,以及从三个最低亚稳能级再泵浦激光激发的效果。实验结果进行了比较与四个级别的速率方程模型,使我们能够推断这些缓冲气体的猝灭率。第二步使用399 nm的激光辐射,我们证明了双光子激发到49960 cm^{-1}的状态,在Th+的最高分类能级中。这是一个有趣的测试情况下,在55000 cm^{-1}以上的范围内,可以共振增强激发的229 Th+核共振通过一个反双光子电子桥过程中寻找更高的水平。

英文摘要:

Experiments on one- and two-photon laser excitation of 232Th+ ions in a radiofrequency ion trap are reported. As the first excitation step, the strongest resonance line at 402 nm from the 6d^2 7s J=3/2 ground state to the 6d7s7p J=5/2 state at 24874 cm^{-1} is driven by radiation from an extended cavity diode laser. Spontaneous decay of the intermediate state populates a number of low-lying metastable states, thus limiting the excited state population and fluorescence signal obtainable with continuous laser excitation. We study the collisional quenching efficiency of helium, argon, and nitrogen buffer gases, and the effect of repumping laser excitation from the three lowest-lying metastable levels. The experimental results are compared with a four-level rate equation model, that allows us to deduce quenching rates for these buffer gases. Using laser radiation at 399 nm for the second step, we demonstrate two-photon excitation to the state at 49960 cm^{-1}, among the highest-lying classified levels of Th+. This is of interest as a test case for the search for higher-lying levels in the range above 55000 cm^{-1} which can resonantly enhance the excitation of the 229Th+ nuclear resonance through an inverse two-photon electronic bridge process.

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