The Nernst coefficient for the quasi-one-dimensional metal, Li(0.9)Mo(6)O(17), is found to be among the largest known for metals (~500 microV/KT at T~20K), and is enhanced in a broad range of temperature by orders of magnitude over the value expected from Boltzmann theory for carrier diffusion. A comparatively small Seebeck coefficient implies that Li(0.9)Mo(6)O(17) is bipolar with large, partial Seebeck coefficients of opposite sign. A very large thermomagnetic figure of merit, ZT~0.5, is found at high field in the range T~35-50K.
We report the study of Nernst effect in quasi-low dimensional tungsten bronze P4W12O44 showing a sequence of Peierls instabilities. We demonstrate that both condensation of the electronic carriers in the CDW state and the existence of high-mobility electrons and holes originating from the small pockets remaining in the incompletely nested Fermi surface give rise to a Nernst effect of a magnitude similar to that observed in heavy fermion compounds.
We present a study of Nernst and Seebeck coefficients in the heavy-fermion compound URu$_{2}$Si$_{2}$, which hosts a phase transition of unsettled origin. A giant Nernst signal of unprecedented magnitude was found to emerge in the ordered state. Moreover, our analysis of the Seebeck and Hall data indicates that the ordering leads to a sudden increase in the entropy per itinerant electron and to a drastic decrease in the scattering rate.
We reveal a novel source of giant Nernst response exhibiting strong non-linear temperature and magnetic field dependence including the mysterious tilted-hill temperature profile observed in a pleiad of materials. The phenomenon results directly from the formation of a chiral ground state, e.g. a chiral d-density wave, which is compatible with the eventual observation of diamagnetism and is distinctly different from the usual quasiparticle and vortex Nernst mechanisms. Our picture provides a unified understanding of the anomalous thermoelectricity observed in materials as diverse as hole doped …
The "failed Kondo insulator" CeNiSn has long been suspected to be a nodal metal, with a node in the hybridization matrix elements. Here we carry out a series of Nernst effect experiments to delineate whether the severely anisotropic magnetotransport coefficients do indeed derive from a nodal metal or can simply be explained by a highly anisotropic Fermi surface. Our experiments reveal that despite an almost 20-fold anisotropy in the Hall conductivity, the large Nernst signal is isotropic. Taken in conjunction with the magnetotransport anisotropy, these results provide strong support for an iso…
The strange-metal state is a crucial problem in condensed matter physics highlighted by its ubiquity in almost all major correlated systems[1-7]. Its understanding could provide important insight into high-Tc superconductivity[2] and quantum criticality[8]. However, with the Fermi liquid theory failing in strange metals, understanding the highly unconventional behaviors has been a long-standing challenge. Fundamental aspects of strange metals remain elusive, including the nature of their charge carriers[1]. Here, we report the observation of a giant Nernst response in the strange-metal state i…
The giant anomalous Hall and Nernst effects in Kagome permanent magnets RCo5
School of Physics & Astronomy and Center for Advanced Quantum Studies, Beijing Normal University（北京师范大学物理与天文学学院及先进量子研究中心）；Key Laboratory of Multiscale Spin Physics (Ministry of Education), Beijing Normal University（北京师范大学多尺度自旋物理教育部重点实验室）
We present a detailed study of the Nernst effect N$_{zx}$ in (TMTSF)$_2$PF$_6$ as a function of temperature, magnetic field magnitude and direction and pressure. As previously reported there is a large resonant-like structure as the magnetic field is rotated through crystallographic directions, the Lebed Magic Angles. These Nernst effect resonances strongly suggest that the transport of the system is effectively ``coherent'' only in crystallographic planes along or close to the applied field direction. We also present analytical and numerical calculations of the conductivity and thermoelectric…
We present a study of Nernst and Seebeck coefficients of the heavy-fermion superconductor CeCoIn$_{5}$. Below 18 K, concomitant with a field-dependent Seebeck coefficient, a large sub-linear Nernst signal emerges with a magnitude drastically exceeding what is expected for a multi-band Fermi-liquid metal. In the mixed state, in contrast with all other superconductors studied before, this signal overwhelms the one associated with the motion of superconducting vortices. The results point to a hitherto unknown source of transverse thermoelectricity in strongly interacting electrons.
In a recent Letter, Serbyn et al. [A] investigated thermomagnetic effects above the superconducting transition and generalized previous works for arbitrary magnetic fields and temperatures. While the results of [A] have been confirmed in [B], we have strong objections: (i) According to our results [C], the linear response calculation does not require any correction from the magnetization currents; (ii) The result of [A,B] is giant, because unlike the normal Fermi liquid, it is of zero order in the particle-hole asymmetry. Changing the interaction constant in the Cooper channel leads to ridicul…
Giant anomalous Hall and Nernst effects in a heavy fermion ferromagnet
International Center for Quantum Materials, School of Physics, Peking University（北京大学量子材料科学中心物理学院）；Department of Physics, Southern University of Science and Technology（南方科技大学物理系）；Wuhan National High Magnetic Field Center and School of Physics, Huazhong University of Science and Technology（华中科技大学物理学院武汉国家高磁场实验室）；Department of Physics, School of Science, Tianjin University（天津大学理学院物理系）；Interdisciplinary Institute of Light-Element Quantum Materials and Research Center for Light-Element Advanced Materials, Peking University（北京大学轻元素量子材料交叉研究中心及轻元素先进材料研究中心）；Hefei National Laboratory（合肥国家实验室）
Motivated by the observation of a giant Nernst effect in URu_2Si_2, the thermoelectric response of the related system UPt_2Si_2 was investigated using thermal and electric transport properties such as the Nernst and Seebeck effects, thermal conductivity, Hall effect and electrical resitivity. Unlike URu_2Si_2, UPt_2Si_2 is neither superconducting nor exhibits a ``hidden-order'' state. Nevertheless a pronounced Nernst effect anomaly is found to coincide with the onset of the antiferromagnetic order in UPt_2Si_2. Although the absolute values are substantially lower, its appearance and characteri…
The Nernst effect is known to be a sensitive probe of the scattering mechanisms. Large Nernst effects, a decade ago a topic mainly in vortex dynamics in superconductors, have recently attracted interest in correlated systems like cuprate metals and heavy fermion systems. However, it has been found that these ``giant" Nernst signals stay within one order of magnitude of the classical Sondheimer formula for a Fermi liquid. It therefore seems that a large Nernst effect neither relies on nor is sensitive to strong correlations. This might, however, be different in some recently studied supposedly …
The topological Hall effect (THE) and its thermoelectric counterpart, the topological Nernst effect (TNE), are hallmarks of the skyrmion lattice phase (SkL). We observed the giant TNE of the SkL in centrosymmetric Gd$_2$PdSi$_3$, comparable in magnitude to the largest anomalous Nernst signals in ferromagnets. Significant enhancement (suppression) of the THE occurs when doping electrons (holes) to Gd$_2$PdSi$_3$. On the electron-doped side, the topological Hall conductivity approaches the characteristic threshold $\sim 1000\,\left(\mathrm{Ωcm}\right)^{-1}$ for the intrinsic regime. We use the f…
We examine an unusual phenomenon where, in tilted magnetic fields near magic angles parallel to crystallographic planes, a "giant" resonant Nernst signal has been observed by Wu et al.[Phys. Rev. Lett. 91 56601(2003)] in the metallic state of an organic conducting Bechgaard salt. We show that this effect appears to be a general feature of these materials, and is also present in the field induced spin density wave phase with even larger amplitude. Our results place new restrictions on models that treat the metallic state as an unconventional density wave or as a state with finite Cooper pairing…
A giant Nernst signal was recently observed for fields near crystallographic directions in (TMTSF)$_2$PF$_6$. Such large Nernst signals are most naturally associated with the motion of pancake vortices. We propose a model in which phase coherence is destroyed throughout the sample except in planes closely aligned with the applied field $\bf H$. A small tilt above or below the plane changes the direction and density of the penetrating vortices and leads to a Nernst signal that varies with the tilt angle of $\bf H$ as observed. The resistance notches at magic angles are understood in terms of fl…
We report the observation of a universal scaling of the Nernst coefficient over a wide intermediate temperature range in heavy fermion materials, including the superconductors CeCu$_2$Si$_2$, CeCoIn$_5$, and Ce$_2$PdIn$_8$, the ferromagnetic Kondo lattice Ce$_3$RhSi$_3$, the nonmagnetic CeRu$_2$Si$_2$, the intermediate valent YbAl$_3$, and the hidden order compound URu$_2$Si$_2$, that cover a broad spectrum of heavy fermion materials with different crystal, valence and ground state properties. The scaling formula follows exactly the magnetic susceptibility of emergent heavy quasiparticles as p…
Motived by time-reversal symmetry breaking and giant anomalous Hall effect in kagome superconductor \textit{A}V$_3$Sb$_5$ (\textit{A} = Cs, K, Rb), we carried out the thermal transport measurements on CsV$_3$Sb$_5$. In addition to the anomalous Hall effect, the anomalous Nernst effect and the anomalous thermal Hall effect emerge. Interestingly, the longitudinal thermal conductivity $κ_{xx}$ largely deviates from the electronic contribution obtained from the longitudinal conductivity $σ_{xx}$ by the Wiedemann-Franz law. In contrast, the thermal Hall conductivity $κ_{xy}$ is roughly consistent w…
Angle dependent magnetoresistance (ADMR) and giant Nernst effect are hallmarks of unconventional density waves (UDW). Here these transport properties for d-wave density wave (d-DW) are computed for quasi-two-dimensional systems. The present theory describes ADMR observed in the pseudogap phase of Y_0.68Pr_0.32Ba_2Cu_3O_7 and CeCoIn_5 single crystals very satisfactorily.
