Ligand-based transport resonances of single-molecule magnet spin filters: Suppression of the Coulomb blockade and determination of the orientation of the magnetic easy axis
We investigate single molecule magnet transistors (SMMTs) with ligands that support transport resonances. We find the lowest unoccupied molecular orbitals of Mn12-benzoate SMMs (with and without thiol or methyl-sulfide termination) to be on ligands, the highest occupied molecular orbitals being on the Mn12 magnetic core. We predict gate controlled switching between Coulomb blockade and coherent resonant tunneling in SMMTs based on such SMMs, strong spin filtering by the SMM in both transport regimes, and that if such switching is observed then the magnetic easy axis of the SMM is parallel to the direction of the current through the SMM.
The ligand-protected Au13 clusters have been synthesized by using meso-2,3-imercaptosuccinic acid as the reducing and stabilizing agent. Transmission electron microscopic analysis shows a size distribution of 0.6nm. Optical spectrum shows an absorbance peak at 390 nm. The electrical transport measurement devices are fabricated using the electro-migration method. Coulomb blockade is observed at the temperature of 1.6 K,revealing the formation of the tunneling junction. The Coulomb oscillation on-off ratio is nearly 5. Three peaks are extracted in the dI-dV data and attributed to the energy leve…
Scanning-probe magnetometry is a valuable experimental tool to investigate magnetic phenomena at the micro- and nanoscale. We theoretically analyze the possibility of measuring magnetic fields via the electrical current flowing through quantum dots. We characterize the shot-noise-limited magnetic-field sensitivity of two devices: a single dot in the Coulomb blockade regime, and a double dot in the Pauli blockade regime. Constructing such magnetometers using carbon nanotube quantum dots would benefit from the large, strongly anisotropic and controllable g tensors, the low abundance of nuclear s…
The total spin of correlated electrons in a quantum dot changes with magnetic field and this effect is generally linked to the change in the total angular momentum from one magic number to another, which can be understood in terms of an `electron molecule' picture for strong fields. Here we propose to exploit this fact to realize a spin blockade, i.e., electrons are prohibited to tunnel at specific values of the magnetic field. The spin-blockade regions have been obtained by calculating both the ground and excited states. In double dots the spin-blockade condition is found to be less stringent…
Based on the spin-blockade model for organic magnetoresistance we present an analytic expression for the polaron-bipolaron transition rate, taking into account the effective nuclear fields on the sites. We reveal the physics producing qualitatively different magnetoconductance line shapes as well as the ultrasmall magnetic field effect, and we study the role of the ratio between the intersite hopping rate and the typical magnitude of the nuclear fields. Our findings are in agreement with recent experiments and numerical simulations.
We analyze coherent spin phenomena in triple quantum dots in triangular configuration under crossed DC and AC magnetic fields. In particular, we discuss the interplay between Aharonov-Bohm current oscillations, coherent electron trapping and spin blockade under electron spin resonance conditions. We demonstrate that, for certain field frequencies, AC magnetic fields induce an antiresonant behavior in the current, allowing for both removal and restoration of entangled spin blockaded states by tuning the AC field frequency. Our theoretical predictions indicate how to manipulate spin qubits in a …
We consider statistical correlations between the heights of conductance peaks corresponding to two different levels in a Coulomb-blockaded quantum dot. Correlations exist for two peaks at the same magnetic field if the field does not fully break time-reversal symmetry as well as for peaks at different values of a magnetic field that fully breaks time-reversal symmetry. Our results are also relevant to Coulomb-blockade conductance peak height statistics in the presence of weak spin-orbit coupling in a chaotic quantum dot.
We study theoretically the spin-dependent transport in ferromagnet/normal-metal/ferromagnet double tunnel junctions by special attention to cotunneling in the Coulomb blockade region. The spin accumulation caused by cotunneling squeezes the Coulomb blockade region when the magnetizations in the ferromagnetic electrodes are antiparallel. Outside the squeezed Coulomb blockade region, we propose a new anomalous region, where the sequential tunneling in one of the spin bands is suppressed by the Coulomb blockade and that in the other is not. In this region, the tunnel magnetoresistance oscillates …
We report the observation of a giant positive magnetoresistance in millimetre scale hydrogenated graphene with magnetic field oriented in the plane of the graphene sheet. A positive magnetoresistance in excess of 200\% at a temperature of 300 mK was observed in this configuration, reverting to negative magnetoresistance with the magnetic field oriented normal to the graphene plane. We attribute the observed positive, in-plane, magnetoresistance to Pauli-blockade of hopping conduction induced by spin polarization. Our work shows that spin polarization in concert with electron-electron interacti…
We formulate the problem of electron transport through a single-molecule magnet (SMM) in the Coulomb blockade regime taking into account topological interference effects for the tunneling of the large spin of a SMM. The interference originates from spin Berry phases associated with different tunneling paths. We show that in the case of incoherent spin states it is essential to place the SMM between oppositely spin-polarized source and drain leads in order to detect the spin tunneling in the stationary current, which exhibits topological zeros as a function of the transverse magnetic field.
A magnet with precessing magnetization pumps a spin current into adjacent leads. As a special case of this spin pumping, a precessing macrospin (magnetization) can assist electrons in tunneling. In small systems, however, the Coulomb blockade effect can block the transport of electrons. Here, we investigate the competition between macrospin-assisted tunneling and Coulomb blockade for the simplest system where both effects meet; namely, for a single tunnel junction between a normal metal and a metallic ferromagnet with precessing magnetization. By combining Fermi's golden rule with magnetizatio…
We investigate the two-terminal nonlinear conductance of a Coulomb-blockaded quantum dot attached to chiral edge states. Reversal of the applied magnetic field inverts the system chirality and leads to a different polarization charge. As a result, the current--voltage characteristic is not an even function of the magnetic field. We show that the corresponding magnetic-field asymmetry arises from single-charge effects and vanishes in the limit of high temperature.
The distribution of Coulomb blockade peak heights as a function of magnetic field is investigated experimentally in a Ge-Si nanowire quantum dot. Strong spin-orbit coupling in this hole-gas system leads to antilocalization of Coulomb blockade peaks, consistent with theory. In particular, the peak height distribution has its maximum away from zero at zero magnetic field, with an average that decreases with increasing field. Magnetoconductance in the open-wire regime places a bound on the spin-orbit length ($l_{so}$ < 20 nm), consistent with values extracted in the Coulomb blockade regime ($l_{s…
We consider quantum transport and tunneling magnetoresistance (TMR) through an interacting quantum dot in the Coulomb blockade regime, attached to ferromagnetic leads. We show that there exist two kinds of anomalies of TMR, which have different origin. One type, associated with TMR sign change and appearing at conductance resonances, is of single particle origin. The second type, inducing a pronounced increase of TMR value far beyond 100%, is caused by electron correlations. It is manifested in-between Coulomb blockade conductance peaks. Both types of anomalies are discussed for zero and finit…
We have measured the critical current as a function of magnetic field in short and narrow superconducting aluminum nanowires. In the range of magnetic fields in which vortices can enter a nanowire in a single row, we find regular oscillations of the critical current as a function of magnetic field. The oscillations are found to correspond to adding a single vortex to the nanowire, with the number of vortices on the nanowire staying constant within each period of the oscillation. This effect can be thought of as a Weber blockade, and the nanowires act as quantum dots for vortices, analogous to …
We perform transport measurements on double quantum dots defined in Ge/Si core/shell nanowires and focus on Pauli spin blockade in the regime where tens of holes occupy each dot. We identify spin blockade through the magnetic field dependence of leakage current. We find both a dip and a peak in the leakage current at zero field. We analyze this behavior in terms of the quantum dot parameters such as coupling to the leads, interdot tunnel coupling as well as spin-orbit interaction. We find a lower bound for spin-orbit interaction with $l_{\rm so}=500$ nm. We also extract large and anisotropic e…
We study electron transport in a double quantum dot in the Pauli spin blockade regime, in the presence of strong spin-orbit coupling. The effect of spin-orbit coupling is incorporated into a modified interdot tunnel coupling. We elucidate the role of the external magnetic field, the nuclear fields in the dots, and spin relaxation. We find qualitative agreement with experimental observations, and we propose a way to extend the range of magnetic fields in which blockade can be observed.
We study the spectrum and the transport properties of two identical, vertically coupled quantum dots in a perpendicular magnetic field. We find correlation-induced energy crossings in a magnetic field sweep between states differing only in the vertical degree of freedom. Considering the influence of a slight asymmetry between the dots caused by the applied source-drain voltage in vertical transport experiments these crossings convert to anticrossings accompanied by the build-up of charge polarization which is tunable by the perpendicular magnetic field. The polarization strongly affects the ve…
We consider a quantum dot in the regime of the quantum Hall effect, particularly in Laughlin states and non-Abelian Read-Rezayi states. We find the location of the Coulomb blockade peaks in the conductance as a function of the area of the dot and the magnetic field. When the magnetic field is fixed and the area of the dot is varied, the peaks are equally spaced for the Laughlin states. In contrast, non-Abelian statistics is reflected in modulations of the spacing which depend on the magnetic field.
We present a new mechanism for a spin blockade effect associated with a change in the type of magnetic anisotropy over oxidation state in a single molecule transistor, by taking an example of an individual Eu$_{2}$(C$_{8}$H$_{8}$)$_{3}$ molecule weakly coupled to non-magnetic electrodes without linker groups. The molecule switches its magnetization direction from in-plane to out-of-plane when it is charged. In other words, the magnetic anisotropy of the molecule changes from easy plane to easy axis when the molecule is charged. By solving the master equation based on model Hamiltonian, we find…
We review the peculiarities of transport through a quantum dot caused by the spin transition in its ground state. Such transitions can be induced by a magnetic field. Tunneling of electrons between the dot and leads mixes the states belonging to the ground state manifold of the dot. Unlike the conventional Kondo effect, this mixing, which occurs only at the singlet-triplet transition point, involves both the orbital and spin degrees of freedom of the electrons. We present theoretical and experimental results that demonstrate the enhancement of the conductance through the dot at the transition …
Magnetotransport through cylindrical topological insulator (TI) nanowires is governed by the interplay between quantum confinement and geometric (Aharonov-Bohm and Berry) phases. Here, we argue that the much broader class of TI nanowires with varying radius -- for which a homogeneous coaxial magnetic field induces a varying Aharonov-Bohm flux that gives rise to a non-trivial mass-like potential along the wire -- is accessible by studying its simplest member, a TI nanocone. Such nanocones allow to observe intriguing mesoscopic transport phenomena: While the conductance in a perpendicular magnet…
Signatures of "mesoscopic Coulomb blockade" are reported for quantum dots with one fully transmitting point-contact lead, T1 = 1, T2 << 1. Unlike Coulomb blockade (CB) in weak-tunneling devices (T1, T2 << 1), one-channel CB is a mesoscopic effect requiring quantum coherence. Several distinctive features of mesoscopic CB are observed, including a reduction in CB upon breaking time-reversal symmetry with a magnetic field, relatively large fluctuations of peak position as a function of magnetic field, and strong temperature dependence on the scale of the quantum level spacing.
We investigate a silicon single-electron transistor (SET) in a metal-oxide-semiconductor (MOS) structure by applying a magnetic field perpendicular to the sample surface. The quantum dot is defined electrostatically in a point contact channel and by the potential barriers from negatively charged interface traps. The magnetic field dependence of the excitation spectrum is primarily driven by the Zeeman effect. In the two-electron singlet-triplet (ST) transition, electron-electron Coulomb interaction plays a significant role. The evolution of Coulomb blockade peaks with magnetic field B is also …
A Weyl semimetal with broken time-reversal symmetry has a minimum of two species of Weyl fermions, distinguished by their opposite chirality, in a pair of Weyl cones at opposite momenta $\pm K$ that are displaced in the direction of the magnetization. Andreev reflection at the interface between a Weyl semimetal in the normal state (N) and a superconductor (S) that pairs $\pm K$ must involve a switch of chirality, otherwise it is blocked. We show that this "chirality blockade" suppresses the superconducting proximity effect when the magnetization lies in the plane of the NS interface. A Zeeman …
We present a theoretical study of the spin-valley blockade transport effect in a double quantum dot defined in a straight carbon nanotube. We find that intervalley scattering due to short-range impurities completely lifts the spin-valley blockade and induces a large leakage current in a certain confined range of the external magnetic field vector. This current hot spot emerges due to different effective magnetic fields acting on the spin-valley qubit states of the two quantum dots. Our predictions are compared to a recent measurement [F. Pei et al., Nat. Nanotech. 7, 630 (2012)]. We discuss th…
We study electron transport in nanostructures patterned in bilayer graphene patches grown epitaxially on SiC as a function of doping, magnetic field, and temperature. Away from charge neutrality transport is only weakly modulated by changes in carrier concentration induced by a local side-gate. At low n-type doping close to charge neutrality, electron transport resembles that in exfoliated graphene nanoribbons and is well described by tunnelling of single electrons through a network of Coulomb-blockaded islands. Under the influence of an external magnetic field, Coulomb blockade resonances flu…
Spin-orbit coupling is key to all-electrical control of quantum-dot spin qubits, and is frequently stronger for holes than for electrons. Here we investigate Pauli spin blockade for two heavy holes in a gated double quantum dot in an in-plane magnetic field. The interplay of the complex Zeeman and spin-orbit couplings causes a blockade leakage current anisotropic in the field direction. The period of the anisotropic leakage is critically dependent on the relative magnitude of Zeeman interaction terms linear and cubic in the magnetic field. The current and singlet-triplet exchange splitting can…
We performed ab initio computations of the magnetic properties of simple iron oxide clusters and slabs. We considered an iron oxide cluster functionalized by a molecule or glued to a gold cluster of the same size. We also considered a magnetite slab coated by cobalt oxide or a mixture of iron oxide and cobalt oxide. The changes in magnetic behavior were explored using constrained magnetic calculations. A possible value for the surface anisotropy was estimated from the fit of a classical Heisenberg model on ab initio results. The value was found to be compatible with estimations obtained by oth…
Pauli spin blockade (PSB) in double quantum dots (DQDs) has matured into a prime technique for precise measurements of nanoscale system parameters. In this work we demonstrate that systems with site-dependent g-tensors and spin-polarized leads allow for a complete characterization of the g-tensors in the dots by magnetotransport experiments alone. Additionally, we show that special polarization configurations can enhance the often elusive magnetotransport signal, rendering the proposed technique robust against noise in the system, and inducing a giant magnetoresistance effect. Finally, we inco…
We report on magnetotransport measurements of nanoconstricted (Ga,Mn)As devices showing very large resistance changes that can be controlled by both an electric and a magnetic field. Based on the bias voltage and temperature dependent measurements down to the millikelvin range we compare the models currently used to describe transport through (Ga,Mn)As nanoconstrictions. We provide an explanation for the observed spin-valve like behavior during a magnetic field sweep by means of the magnetization configurations in the device. Furthermore, we prove that Coulomb-blockade plays a decisive role fo…
We predict that singly-occupied carrier traps, produced by electrical stress or irradiation within organic semiconductors, can cause spin blockades and the large room-temperature magnetoresistance known as organic magnetoresistance. The blockade occurs because many singly-occupied traps can only become doubly occupied in a spin-singlet configuration. Magnetic-field effects on spin mixing during transport dramatically modify the effects of this blockade and produce magnetoresistance.We calculate the quantitative effects of these traps on organic magnetoresistance from percolation theory and fin…
We investigate spin states of few electrons in a double quantum dot by coupling them weakly to a magnetic field resilient NbTiN microwave resonator. We observe a reduced resonator transmission if resonator photons and spin singlet states interact. This response vanishes in a magnetic field once the quantum dot ground state changes from a spin singlet into a spin triplet state. Based on this observation, we map the two-electron singlet-triplet crossover by resonant spectroscopy. By measuring the resonator only, we observe Pauli spin blockade known from transport experiments at finite source-dra…
Silicon quantum dots are attractive candidates for the development of scalable, spin-based qubits. Pauli spin blockade in double quantum dots provides an efficient, temperature independent mechanism for qubit readout. Here we report on transport experiments in double gate nanowire transistors issued from a CMOS process on 300 mm silicon-on-insulator wafers. At low temperature the devices behave as two few-electron quantum dots in series. We observe signatures of Pauli spin blockade with a singlet-triplet splitting ranging from 0.3 to 1.3 meV. Magneto-transport measurements show that transition…
We detect in real time inter-dot tunneling events in a weakly coupled two electron double quantum dot in GaAs. At finite magnetic fields, we observe two characteristic tunneling times, T_d and T_b, belonging to, respectively, a direct and a blocked (spin-flip-assisted) tunneling. The latter corresponds to lifting of a Pauli spin blockade and the tunneling times ratio eta=T_b/T_d characterizes the blockade efficiency. We find pronounced changes in the behavior of eta upon increasing the magnetic field, with eta increasing, saturating and increasing again. We explain this behavior as due to the …
The magnetopolaronic generalization of a Majorana-resonant-level (MRL) model is considered for a single-level vibrating quantum dot coupled to two half-infinite $g=1/2$ Tomonaga-Luttinger liquid (TLL) leads. A qualitatively new non-trivial formula for the effective transmission coefficient and differential conductance for resonant magnetopolaron-assisted tunneling is obtained under the assumption about a fermion-boson factorization of corresponding averages. This approach is valid for the case of weak magnetopolaronic coupling in a system. Surprisingly, it is found that despite a supposed weak…
We develop a theory of the reversible switching of the magnetic state of the ferromagnet-insulator-normal metalferromagnet (FINF) nanostructure. The switching is controlled by tuning the Coulomb blockade strength via the gate voltage on the normal metal granule. The proposed mechanism allows for realizing the switching without passing a dissipative current through the structure.
We investigate current fluctuations in a three-terminal quantum dot in the sequential tunneling regime. Dynamical spin blockade can be induced when the spin-degeneracy of the dot states is lifted by a magnetic field. This results in super-Poissonian shot noise and positive zero-frequency cross-correlations. Our proposed setup can be realized with semiconductor quantum dots.
The influence of electron-electron (e-e) interactions on the transmission through a quantum dot is investigated numerically for the Coulomb blockade regime. For vanishing magnetic fields, the conductance peak height statistics is found to be independent of the interactions strength. It is identical to the statistics predicted by constant interaction single electron random matrix theory and agrees well with recent experiments. However, in contrast to these random matrix theories, our calculations reproduces the reduced sensitivity to magnetic flux observed in many experiments. The relevant phys…
It is known that the quantum-mechanical ground state of a nano-scale junction has a significant impact on its electrical transport properties. This becomes particularly important in transistors consisting of a single molecule. Due to strong electron-electron interactions and the possibility to access ground states with high spins, these systems are eligible hosts of a current-blockade phenomenon called ground-state spin blockade. This effect arises from the inability of a charge carrier to account for the spin difference required to enter the junction, as that process would violate the spin se…
We discuss the angular momentum blockade in small d-wave superconducting grains in an external field. We find that abrupt changes in angular momentum state of the condensate, angular momentum blockade, occur as a result of changes in the angular momentum of the condensate in an external magnetic field. The effect rep- resents a direct analogy with the Coulomb blockade. We use the Ginzburg-Landau formalism to illustrate how a magnetic field induces a deviation from the d-wave symmetry which is described by a (d + id')-order parameter. We derive the behavior of the volume magnetic susceptibility…
We find the leakage current through a double quantum dot in the Pauli spin blockade regime accounting for inelastic (spin-flip) cotunneling processes. Taking the energy-dependence of this spin-flip mechanism into account allows for an accurate description of the current as a function of applied magnetic fields, gate voltages, and an inter-dot tunnel coupling. In the presence of an additional local dephasing process or nonuniform magnetic field, we obtain a simple closed-form analytical expression for the leakage current giving the full dependence on an applied magnetic field and energy detunin…
We present measurements on spin blockade in a laterally integrated quantum dot. The dot is tuned into the regime of strong Coulomb blockade, confining ~ 50 electrons. At certain electronic states we find an additional mechanism suppressing electron transport. This we identify as spin blockade at zero bias, possibly accompanied by a change in orbital momentum in subsequent dot ground states. We support this by probing the bias, magnetic field and temperature dependence of the transport spectrum. Weak violation of the blockade is modelled by detailed calculations of non-linear transport taking i…
Two distinct types of magnetoresistance oscillations are observed in two electronic Fabry-Perot interferometers of different sizes in the integer quantum Hall regime. Measuring these oscillations as a function of magnetic field and gate voltages, we observe three signatures that distinguish the two types. The oscillations observed in a 2.0 square micron device are understood to arise from the Coulomb blockade mechanism, and those observed in an 18 square micron device from the Aharonov-Bohm mechanism. This work clarifies, provides ways to distinguish, and demonstrates control over, these disti…
We present transport measurements on a lateral double dot produced by combining local anodic oxidation and electron beam lithography. We investigate the tunability of our device and demonstrate, that we can switch between capacitive and tunnel coupling. In the regime of capacitive coupling we observe the phenomenon of spin blockade in a magnetic field and analyze the influence of capacitive interdot coupling on this effect.
A tunable directional coupler based on Coulomb Blockade effect is presented. Two electron waveguides are coupled by a quantum dot to an injector waveguide. Electron confinement is obtained by surface Schottky gates on single GaAs/AlGaAs heterojunction. Magneto-electrical measurements down to 350 mK are presented and large transconductance oscillations are reported on both outputs up to 4.2 K. Experimental results are interpreted in terms of Coulomb Blockade effect and the relevance of the present design strategy for the implementation of an electronic multiplexer is underlined.
We report the observation of Coulomb blockade in a quantum dot contacted by two quantum point contacts each with a single fully-transmitting mode, a system previously thought to be well described without invoking Coulomb interactions. At temperatures below 50 mK we observe a periodic oscillation in the conductance of the dot with gate voltage that corresponds to a residual quantization of charge. From the temperature and magnetic field dependence, we infer the oscillations are Mesoscopic Coulomb Blockade, a type of Coulomb blockade caused by electron interference in an otherwise open system.
The magnetic properties of metal-organic complexes are strongly influenced by conformational changes in the ligand. The flexibility of Fe-tetra-pyridyl-porphyrin molecules leads to different adsorption configurations on a Au(111) surface. By combining low-temperature scanning tunneling spectroscopy and atomic force microscopy, we resolve a correlation of the molecular configuration with different spin states and magnitudes of magnetic anisotropy. When the macrocycle exhibits a laterally-undistorted saddle shape, the molecules lie in a S=1 state with axial anisotropy arising from a square-plana…
Spin-bearing molecules can be stabilized on surfaces and in junctions with desirable properties such as a net spin that can be adjusted by external stimuli. Using scanning probes, initial and final spin states can be deduced from topographic or spectroscopic data, but how the system transitioned between these states is largely unknown. Here we address this question by manipulating the total spin of magnetic cobalt hydride complexes on a corrugated boron nitride surface with a hydrogen- functionalized scanning probe tip by simultaneously tracking force and conductance. When the additional hydro…
We propose a general capacitive model for an antidot, which has two localized edge states with different spins in the quantum Hall regime. The capacitive coupling of localized excess charges, which are generated around the antidot due to magnetic flux quantization, and their effective spin fluctuation can result in Coulomb blockade, h/(2e) Aharonov-Bohm oscillations, and the Kondo effect. The resultant conductance is in qualitative agreement with recent experimental data.
We study the magneto-conductance of a $1.4~\mathrm{μm}$-wide quantum dot in the fractional quantum Hall regime. For a filling factor $\approx 2/3$ and $\gtrsim 1/3$ in the quantum dot the observed Coulomb resonances show a periodic modulation in magnetic field. This indicates a non-trivial reconstruction of the 2/3 fractional quantum Hall state in the quantum dot. We present a model for the charge stability diagram of the system assuming two compressible regions separated by an incompressible stripe of filling factor $2/3$ and $1/3$, respectively. From the dependence of the magnetic field peri…
We study the charge of a small normal island connected by a tunnel junction to a superconducting lead. Unlike the N-I-N case, the steps of the Coulomb staircase remain sharp even if the conductance of the tunneling barrier exceeds e^2/h. One can observe the transition from sharp steps to the smeared ones by applying magnetic field to destroy the superconductivity.
Singlet-triplet spin blockade in a few-electron lateral double quantum dot is investigated using simultaneous transport and charge-sensing measurements. Transport from the (1,1) to the (0,2) electron occupancy states is strongly suppressed relative to the opposite bias [(0,2) to (1,1)]. At large bias, spin blockade ceases as the (0,2) triplet state enters the transport window, giving a direct measure of exchange splitting as a function of magnetic field. A simple model for current and steady-state charge distribution in spin-blockade conditions is developed and found to be in excellent agreeme…
Double quantum dot systems in the spin blockade regime exhibit leakage currents that have been attributed to the Hyperfine interaction. We model weakly coupled double-dot transport using a rate equation approach which accounts for Hyperfine flip-flop transitions. The rate equations allow us to obtain self-consistently the time evolution for electronic charge occupations and for the nuclei polarizations in each dot. We analyze the current in the spin blockade region as a function of magnetic field and observe hysteretic behavior for fields corresponding to the crossing between triplet and singl…
We investigate spin relaxation in a silicon double quantum dot via leakage current through Pauli blockade as a function of interdot detuning and magnetic field. A dip in leakage current as a function of magnetic field on a \sim 40 mT field scale is attributed to spin-orbit mediated spin relaxation. On a larger (\sim 400 mT) field scale, a peak in leakage current is seen in some, but not all, Pauli-blocked transitions, and is attributed to spin-flip cotunneling. Both dip and peak structure show good agreement between theory and experiment.
We study the effect of spin-orbit scattering on the statistics of the conductance of a quantum dot for Coulomb blockade peaks and valleys. We find the distribution function of the peak heights for strong spin-orbit scattering in the presence and absence of time reversal symmetry. We find that the application of a magnetic field suppresses the average peak height, similar to the antilocalizaion in the bulk systems. For the valleys, we consider the elastic cotunneling contribution to the conductance and calculate its moments at the crossover between ensembles of various symmetries.
We investigate vibron-assisted electron transport in single-molecule transistors containing an individual Fe4 Single-Molecule Magnet. We observe a strong suppression of the tunneling current at low bias in combination with vibron-assisted excitations. The observed features are explained by a strong electron-vibron coupling in the framework of the Franck-Condon model supported by density-functional theory.
We study mesoscopic fluctuations of the differential capacitance of a dot connected to a lead by a single-mode quantum channel with adjustable conductance G. We show that the amplitude of the fluctuations reaches maximum at a partially opened channel, G\lesssim e^2/π\hbar. Parametric correlations of fluctuations at different values of the applied voltage and magnetic field can be studied experimentally, and we find the corresponding correlation functions for the differential capacitance.
Low-temperature transport spectroscopy measurements on a quantum dot lithographically defined in a multiwall $\mathrm{MoS}_2$ nanotube are demonstrated. At $T=300\,\mathrm{mK}$, clear Coulomb blockade is observed, with charging energies in the range of 1 meV. In single-electron tunneling, discrete conductance resonances are visible at finite bias. Additionally, a magnetic field perpendicular to the nanotube axis reveals clear indications of quantum state transitions, with effective $g$ factors consistent with published theoretical predictions.
Magnetic Weyl semimetals (WSMs) have been presumed to be immune to proximity-induced spin-singlet superconducting pairing due to a chirality blockade of the regular Andreev reflection. In this work we study all possible superconducting pairing induced in a WSM sandwiched between two conventional superconductors in a Josephson junction setup. We confirm that, while conventional intra-orbital $s$-wave pairing is present on the surface of the WSM, it cannot propagate into the bulk due to the chirality blockade. However, inter-orbital $s$-wave pairing, with both even-frequency spin-singlet and odd…
