Graphene superlattices (GSLs), formed by subjecting a monolayer graphene sheet to a periodic potential, can be used to engineer band structures and, from there, charge transport properties, but these are sensitive to the presence of disorder. The localization behavior of massless 2D Dirac particles induced by weak disorder is studied for both scalar-potential and vector-potential GSLs, computationally as well as analytically by a weak-disorder expansion. In particular, it is investigated how the Lyapunov exponent (inverse localization length) depends on the incidence angle to a 1D GSL. Delocalization resonances are found for both scalar and vector GSLs. The sharp angular dependence of the Lyapunov exponent may be exploited to realize disorder-induced filtering, as verified by full 2D numerical wave packet simulations.
We study the localization properties of disordered semiconductor superlattices driven by ac-fields. The localization length of the electrons in the superlattice increases when the frequency of the driving field is smaller than the miniband width. We show that there is an optimal value of the amplitude of the driving field for which the localization length of the system is maximal. This maximum localization length increases with the inverse of the driving frequency.
We study the conductance of disordered graphene superlattices with short-range structural correlations. The system consists of electron- and hole-doped graphenes of various thicknesses, which fluctuate randomly around their mean value. The effect of the randomness on the probability of transmission through the system of various sizes is studied. We show that in a disordered superlattice the quasiparticle that approaches the barrier interface almost perpendicularly transmits through the system. The conductivity of the finite-size system is computed and shown that the conductance vanishes when t…
Graphene has a high intrinsic thermal conductivity and a high electron mobility. The thermal conductivity of graphene can be significantly reduced when different carbon isotopes are mixed, which can enhance the performance of thermoelectric devices. Here we compare the thermal conductivities of isotopic c12/c13 random mixes with isotope superlattices with periods ranging from 46 to 225 nm. Raman Opto-Thermal conductivity measurements of these superlattice structures show an approximately 50% reduction in thermal conductivity compared to pristine c12 graphene. This average reduction is similar …
We theoretically investigate light propagation and Anderson localization in one-dimensional disordered superlattices composed of dielectric stacks with graphene sheets in between. Disorder is introduced either on graphene material parameters ({\it e.g.} Fermi energy) or on the widths of the dielectric stacks. We derive an analytic expression for the localization length $ξ$, and compare it to numerical simulations using transfer matrix technique; a very good agreement is found. We demonstrate that the presence of graphene may strongly attenuate the anomalously delocalised Breswter modes, and is…
The electronic transport properties of graphene-based superlattice structures are investigated. A graphene-based modulation-doped superlattice structure geometry is proposed and consist of periodically arranged alternate layers: InAs/graphene/GaAs/graphene/GaSb. Undoped graphene/GaAs/graphene structure displays relatively high conductance and enhanced mobilities at elevated temperatures unlike modulation-doped superlattice structure more steady and less sensitive to temperature and robust electrical tunable control on the screening length scale. Thermionic current density exhibits enhanced beh…
Using the transfer matrix method, we study the conductance of the chiral particles through a monolayer graphene superlattice with long-range correlated disorder distributed on the potential of the barriers. Even though the transmission of the particles through graphene superlattice with white noise potentials is suppressed, the transmission is revived in a wide range of angles when the potential heights are long-range correlated with a power spectrum $S(k)\sim1/k^β$. As a result, the conductance increases with increasing the correlation exponent values gives rise a metallic phase. We obtain a …
The specific rotational alignment of two-dimensional lattices results in a moiré superlattice with a larger period than the original lattices and allows one to engineer the electronic band structure of such materials. So far, transport signatures of such superlattices have been reported for graphene/hBN and graphene/graphene systems. Here we report moiré superlattices in fully hBN encapsulated graphene with both the top and the bottom hBN aligned to the graphene. In the graphene, two different moiré superlattices form with the top and the bottom hBN, respectively. The overlay of the two superl…
In this paper, we report on the controllable negative differential resistance (NDR) in a proposed planar graphene superlattice structure. High value of peak to valley ratio (PVR) is predicted. This is significant because of appearance of NDR with high PVR at low biases. Our finding is important since beside the other potential applications of the graphene, proposes implementation of the graphene based superlattice in electronic devices such as resonant tunneling diode and filters.
Superlattice in graphene generates extra Dirac points in the band structure and their number depends on the superlattice potential strength. Here, we have created a lateral superlattice in a graphene device with a tunable barrier height using a combination of two gates. In this Letter, we demonstrate the use of lateral superlattice to modify the band structure of graphene leading to the emergence of new Dirac cones. This controlled modification of the band structure persists up to 100 K.
A scalable tight-binding model is applied for large-scale quantum transport calculations in clean graphene subject to electrostatic superlattice potentials, including two types of graphene superlattices: moiré patterns due to the stacking of graphene and hexagonal boron nitride (hBN) lattices, and gate-controllable superlattices using a spatially modulated gate capacitance. In the case of graphene/hBN moiré superlattices, consistency between our transport simulation and experiment is satisfactory at zero and low magnetic field, but breaks down at high magnetic field due to the adopted simple m…
Van der Waals heterostructures of graphene and hexagonal boron nitride feature a moiré superlattice for graphene's Dirac electrons. Here, we review the effects generated by this superlattice, including a specific miniband structure featuring gaps and secondary Dirac points, and a fractal spectrum of magnetic minibands known as Hofstadter's butterfly.
In tight binding approximation the explicit form of the electron energy in graphene superlattice was derived. The possibility of propagation of the cnoidal waves in graphene superlattice was discussed. The direct current induced perpendicularly to the superlattice axis by cnoidal and sinusoidal electromagnetic waves under the presence of longitudinal constant electric field was calculated. Such direct current was shown to change its direction when the intensity of longitudinal electric field changes its absolute value.
We study a novel type of graphene-based superlattices formed owing to a periodic modulation of the Fermi surface. Such a modulation is possible for graphene deposited on a striped substrate made of materials with substantially different values of the dc permittivity. Similar superlattices appear also in graphene sheets applied over substrates with a periodic array of parallel grooves. We suggest a model describing such superlattices. Using the transfer-matrix technique, we determine the dispersion relation and calculate the energy spectrum of these superlattices. We also analyze at a qualitati…
We show that, if graphene is subjected to the potential from an external superlattice, a band gap develops at the Dirac point provided the superlattice potential has broken inversion symmetry. As a numerical example, we calculate the band structure of graphene in the presence of an external potential due to periodically patterned gates arranged in a triangular graphene superlattice (TGS) with broken inversion symmetry, and find that a band gap is created at both the original and "second generation" Dirac point. The gap can be controlled, in principle, by changing the external potential and the…
General properties of long wavelength triangular graphene superlattice are studied. It is shown that Dirac points with and without gaps can arise at a number of high symmetry points of the Brillouin Zone. The existence of gaps can lead to insulating behavior at commensurate fillings. Strain and magnetic superlattices are also discussed.
Electronic properties of two-dimensional graphene superlattice made with partial hydrogenation were thoroughly studied via Density Functional Tight Binding approach (DFTB) which incorporates the tight-binding method into the density functional formalism. The two-dimensional (2-d) pattern of hydrogen atoms on graphene was found to have great effects on electronic structures of graphene superlattice. In particular, the edges of the 2-d pattern, armchair or zigzag, are essential for the energy band gap opening, and the energy band gap sensitively depends on the shape, size, and the 2-d periodicit…
Electronic band gap and transport in quasi-periodic graphene superlattice of double-periodic sequence have been investigated. It is found that such quasi-periodic structure can possess a zero-averaged wave number (zero-$\bar{k}$) gap which associated with an unusual Dirac point. Different from Bragg gap, the zero-$\bar{k}$ gap is less sensitive to the incidence angle, and robust against the lattice constants. The locations of Dirac point and multi-Dirac-points in the graphene superlattices of various sequences are also compared. The control of electron transport over the zero-$\bar{k}$ band ga…
Superlattices are artificial periodic nanostructures which can control the flow of electrons. Their operation typically relies on the periodic modulation of the electric potential in the direction of electron wave propagation. Here we demonstrate transparent graphene superlattices which can manipulate infrared photons utilizing the collective oscillations of carriers, i.e., plasmons of the ensemble of multiple graphene layers. The superlattice is formed by depositing alternating wafer-scale graphene sheets and thin insulating layers, followed by patterning them all together into 3-dimensional …
An exact expression of the transmission probability through a finite graphene superlattice with an arbitrary number of potential barriers $n$ is derived in two cases of the periodic potential: rectangular electric potential and $δ$-function magnetic potential. Obtained transmission probabilities show two types of resonance energy: barrier-induced resonance energies unchanged as $n$ varies and well-induced resonance energies undergone the $(n - 1)$-fold splitting as $n$ increases. Supported by numerical calculations for various types of graphene superlattices, these analytical findings are assu…
We have theoretically investigated the properties of electronic transport in graphene heterostructures, which are consisted of two different graphene superlattices with one-dimensional periodic potentials. It is found that such heterostructures possess an unusual tunneling state occurring inside the original forbidden gaps, and the electronic conductance is greatly enhanced and Fano factor is strongly suppressed near the energy of the tunneling state. Finally we present the matching condition of the impedance of the pseudospin wave for occuring the tunneling state by using the Bloch-wave expan…
We review recent work on superlattices in monolayer and bilayer graphene. We highlight the role of the quasiparticle chirality in generating new Dirac fermion modes with tunable anisotropic velocities in one dimensional (1D) superlattices in both monolayer and bilayer graphene. We discuss the structure of the Landau levels and magnetotransport in such superlattices over a wide range of perpendicular (orbital) magnetic fields. In monolayer graphene, we show that an orbital magnetic field can reverse the anisotropy of the transport imposed by the superlattice potential, suggesting possible switc…
We theoretically investigate gate-defined graphene superlattices with broken inversion symmetry as a platform for realizing tunable valley dependent transport. Our analysis is motivated by recent experiments [C. Forsythe et al., Nat. Nanotechnol. 13, 566 (2018)] wherein gate-tunable superlattice potentials have been induced on graphene by nanostructuring a dielectric in the graphene/patterneddielectric/gate structure. We demonstrate how the electronic tight-binding structure of the superlattice system resembles a gapped Dirac model with associated valley dependent transport using an unfolding …
We develop a theory of interaction effects in graphene superlattices, where tunable superlattice periodicity can be used as a knob to control the gap at the Dirac point. Applied to graphene on hexa-boron-nitride (G/h-BN), our theory predicts substantial many-body enhancement of this gap. Tunable by the moire superlattice periodicity, a few orders of magnitude enhancement is reachable under optimal conditions. The Dirac point gap enhancement can be much larger than that of the minigaps opened by Bragg scattering at principal superlattice harmonics. This naturally explains the conundrum of large…
A so-called artificial graphene is an artificial material whose low-energy carriers are described by the massless Dirac equation. Applying a periodic potential with triangular symmetry to a two-dimensional electron gas is one way to make such a material. According to recent experimental results, it is now possible to realize an artificial graphene in the lab and to even apply an additional lateral, one-dimensional periodic potential to it. We name the latter system an artificial graphene superlattice in order to distinguish it from a genuine graphene superlattice made from graphene. In this st…
Based on first-principles calculations we predict that periodically repeated junctions of armchair graphene nanoribbons of different widths form superlattice structures. In these superlattice heterostructures the width and the energy gap are modulated in real space and specific states are confined in certain segments. Orientation of constituent nanoribbons, their width and length, the symmetry of the junction are the structural parameters to engineer electronic properties of these quantum structures. Not only the size modulation, but also composition modulation, such as periodically repeated, …
A model for energy spectrum of superlattice on the base of graphene placed on the striped dielectric substrate is proposed. A direct current component which appears in that structure perpendicularly to pulling electric field under the influence of elliptically polarized electromagnetic wave was derived. A transverse current density dependence on pulling field magnitude and on magnitude of component of elliptically polarized wave directed along the axis of a superlattice is analyzed.
We study the existence of edge modes in gapped Moiré superlattices in graphene monolayer ribbons. We find that the superlattice bands acquire finite Chern numbers, which lead to a Valley Hall Effect. The presence of dispersive edge modes is confirmed by calculations of the band structure of realistic nanoribbons using tight binding methods. These edge states are only weakly sensitive to disorder, as short-range scattering processes lead to mean free paths of the order of microns. The results explain the existence of edge currents when the chemical potential lies within the bulk superlattice ga…
Motivated by recent experimental findings on the low-energy spectrum of Kekulé-patterned graphene, the optoelectronic signatures of graphene superlattices with a spatial modulation that triples the size of the unit cell and folds the valleys to the center of the Brillouin zone are studied. For superlattices like those visualized in recent experiments, the optoelectronic response reveals multiple species of carriers distinguished by their effective masses or Fermi velocities. Their signatures are similar to those of systems hosting multifold fermions in which different frequency intervals are d…
The energy spectrum of planar polytype graphene-based superlattices has been investigated. It is shown that their energy spectrum undergoes pseudospin splitting due to the asymmetry of quantum wells forming the superlattice potential profile.
We consider graphene superlattice miniband fermions probed by electronic interferometry in magneto-transport experiments. By decoding the observed Fabry-Pérot interference patterns together with our corresponding quantum transport simulations, we find that the Dirac quasiparticles originating from the superlattice minibands do not undergo conventional cyclotron motion but follow more subtle trajectories. In particular, dynamics at low magnetic fields is characterized by peculiar, straight trajectory segments. Our results provide new insights into superlattice miniband fermions and open up nove…
The hybridization of $σ$ and $π$ orbitals of carbon atoms in graphene depends on the surface curvature. Considering a single junction between flat and rippled graphene subsystems, it is found an accumulation of charge in the rippled subsystem due to Klein penetration phenomenon that gives rise to n-p junction. Using this fact, we show that the momentum distribution of electrons in ballisitically propagating beam can be selective without a waveguide, or external electric, and/or magnetic fields in graphene strip under experimentally feasible one-dimensional periodic potential. Such a potential …
The eigen energy and the conductivity of a graphene sheet subject to a one-dimensional cosinusoidal potential and in the presence of a magnetic field are calculated. Such a graphene superlattice presents three distinct magnetic miniband structures as the magnetic field increases. They are, respectively, the triply degenerate Landau level spectrum, the nondegenerate minibands with finite dispersion and the same Landau level spectrum with the pristine graphene. The ratio of the magnetic length to the period of the potential function is the characteristic quantity to determine the electronic stru…
A model of a superlattice consisting of alternating strips of single-layer and bilayer graphene is proposed, whose parameters of the energy spectrum can be controlled by changing the external electric field perpendicular to the surface of the sample. Using the Kronig-Penney model, the dispersion equation is obtained, based on the analysis of which the energy spectrum of a graphene superlattice is studied depending on the ratio of the strip widths of single-layer and bilayer graphene. The results of the analytical solution are compared with the results of modeling by methods of the theory of th…
Flat bands emerging in buckled monolayer graphene superlattices have been recently shown to realize correlated states analogous to those observed in twisted graphene multilayers. Here, we demonstrate the emergence of valley topology driven by competing electronic correlations in buckled graphene superlattices. We show, both by means of atomistic models and a low-energy description, that the existence of long-range electronic correlations leads to a competition between antiferromagnetic and charge density wave instabilities, that can be controlled by means of screening engineering. Interestingl…
We theoretically study the occurrence of Bloch oscillations in biased hybrid graphene systems with spin-dependent superlattices. The spin-dependent potential is realized by a set of ferromagnetic insulator strips deposited on top of a gapped graphene nanoribbon, which induce a proximity exchange splitting of the electronic states in the graphene monolayer. We numerically solve the Dirac equation and study Bloch oscillations in the lowest conduction band of the spin-dependent superlattice. While the Bloch frequency is the same for both spins, we find the Bloch amplitude to be spin dependent. Th…
Plasmon collective excitations are studied in a planar graphene superlattice formed by periodically alternating regions of gapless graphene and of its gapped modification. The plasmon dispersion law is determined both for the quasi-one-dimensional case (the Fermi level is located within the minigap) and for the quasi-two-dimensional case (the Fermi level is located within the miniband). The problem concerning the absorption of modulated electromagnetic radiation at the excitation of plasmons is also considered.
The time evolution of electron waves in graphene superlattices is studied using both microscopic and 'effective medium' formalisms. The numerical simulations reveal that in a wide range of physical scenarios it is possible to neglect the granularity of the superlattice and characterize the electron transport using a simple effective Hamiltonian. It is verified that as general rule the continuum approximation is rather accurate when the initial state is less localized than the characteristic spatial period of the superlattice. This property holds even when the microsocopic electric potential ha…
We theoretically investigate electron transport through corrugated graphene ribbons and show how the ribbon curvature leads to an electronic superlattice with a period set by the corrugation wave length. Transport through the ribbon depends sensitively on the superlattice band structure which, in turn, strongly depends on the geometry of the deformed sheet. In particular, we find that for ribbon widths where the transverse level separation is comparable to the the band edge energy, a strong current switching occurs as function of an applied backgate voltage. Thus, artificially corrugated graph…
We report the experimental study of resonant Rayleigh scattering in GaAs-AlGaAs superlattices with ordered and intentionally disordered potential profiles (correlated and uncorrelated) in the growth direction z. We show that the intentional disorder along z modify markedly the energy dispersion of the dephasing rates of the excitons. The application of an external magnetic field in the same direction allows the continuous tuning of the in plane exciton localization and to study the interplay between the in plane and vertical disorder.
In this paper, the electronic band structures and its transport properties in the gapped graphene superlattices, with one-dimensional (1D) periodic potentials of square barriers, are systematically investigated. It is found that a zero averaged wave-number (zero-$\overline{k}$ ) gap is formed inside the gapped graphene-based superlattices, and the condition for obtaining such a zero-$\overline{k}$ gap is analytically presented. The properties of this zero-$\overline{k}$ gap including its transmission, conductance and Fano factor are studied in detail. Finally it is revealed that the properties…
We have studied the electronic excitation spectrum in periodically rippled graphene on Ru(0001) and flat, commensurate graphene on Ni(111) by means of high-resolution electron energy loss spectroscopy and a combination of density functional theory and tight-binding approaches. We show that the periodic moiré superlattice originated by the lattice mismatch in graphene/Ru(0001) induces the emergence of an extra mode, which is not present in graphene/Ni(111). Contrary to the ordinary intra-band plasmon of doped graphene, the extra mode is robust in charge-neutral graphene/metal contacts, having i…
The dispersion relation for magnetoplasmons in a planar superlattice with periodically alternating regions of gapless and gapped modications of graphene has been derived within the frame of the random-phase approximation. The contribution of virtual transitions between the lower electron miniband and the upper hole miniband to the polarization operator has been taken into account in addition to the contribution of virtual intra-miniband transitions.
Most studies on moiré superlattices formed from a stack of h-BN and graphene have focused on single layer graphene; graphene with multiple layers is less understood. Here, we show that a moiré superlattice of multilayer graphene shows new features arising from the anisotropic Fermi surface affected by the superlattice structure. The moiré superlattice of a h-BN/AB-stacked tetralayer graphene heterostructure exhibited resistivity peaks showing a complicated dependence on the perpendicular electric field. The peaks were not due to secondary Dirac cones forming, but rather opening of the energy g…
A graphene-based superlattice formed due to the periodic modulation of the band gap has been investigated. Such a modulation is possible in graphene deposited on a strip substrate made of silicon oxide and hexagonal boron nitride. The advantages and some possible problems in the superlattice under consideration are discussed. A model describing such a superlattice is proposed and the dispersion relation between the energy and momentum of carriers has been obtained using the transfer matrix method within this model.
One-dimensional (1D) graphene superlattices have been predicted to exhibit zero-energy modes a decade ago, but an experimental proof has remained missing. Motivated by a recent experiment that could possibly shed light on this, here we perform quantum transport simulations for 1D graphene superlattices, considering electrostatically simulated potential profiles as realistic as possible. Combined with the analysis on the corresponding miniband structures, we find that the zero modes generated by the 1D superlattice potential can be further cloned to higher energies, which are also accessible by…
Dirac electrons in graphene have a valley degree of freedom that is being explored as a carrier of information. In that context of "valleytronics" one seeks to coherently manipulate the valley index. Here we show that reflection from a superlattice potential can provide a valley switch: Electrons approaching a pristine-graphene--superlattice-graphene interface near normal incidence are reflected in the opposite valley. We identify the topological origin of this valley switch, by mapping the problem onto that of Andreev reflection from a topological superconductor, with the electron-hole degree…
Recent experimental studies on graphene on hexagonal Boron Nitride (hBN) have demonstrated that hBN is not only a passive substrate that ensures superb electronic properties of graphene's carriers, but that it actively modifies their massless Dirac fermion character through a periodic moiré potential. In this work we present a theory of the plasmon excitation spectrum of massless Dirac fermions in a moiré superlattice. We demonstrate that graphene-hBN stacks offer a rich platform for plasmonics in which control of plasmon modes can occur not only via electrostatic gating but also by adjusting …
We have investigated theoretically the resonance splitting effect of Dirac electrons through graphene superlattices with periodic potentials of square barriers. It is found that each resonance peak in the transmission gap presents (N-1)-fold resonance splitting for N-barriers, which is the analogy of the case in semiconductor superlattices. The resonance splitting effect depends on the incidence angle rather than the height and width of potential. However, there is no explicit splitting rule for the conductance and shot noise, which is different from the magnetic case. These properties may lea…
Non-trivial Berry phase of graphene leads to unusual quantum correction to the conductivity. Berry phase of pi in single layer graphene (SLG) and 2pi in bi-layer graphene (BLG) is expected to reveal weak anti-localization (WAL) and weak localization (WL), respectively. However, experimentally both WAL and WL have been observed in graphene devices depending on the strength of different scattering mechanisms. Graphene superlattice having multiple Dirac cones is expected to exhibit pi to 2pi Berry phase transition from primary Dirac cone (PDC) to cloned Dirac cone (CDC). However, its effect on lo…
Interactions between stacked two-dimensional (2D) atomic crystals can radically change their properties, leading to essentially new materials in terms of the electronic structure. Here we show that monolayers placed on an atomically flat substrate can be forced to undergo a buckling transition, which results in periodically strained superlattices. By using scanning tunneling microscopy and spectroscopy and support from numerical simulations, we show that such lateral superlattices in graphene lead to a periodically modulated pseudo-magnetic field, which in turn creates a post-graphene material…
Graphene on hexagonal boron nitride (hBN) can exhibit a topological phase via mutual crystallographic alignment. Recent measurements of nonlocal resistance ($R_{nl}$) near the secondary Dirac point (SDP) in ballistic graphene/hBN superlattices have been interpreted as arising due to the quantum valley Hall state. We report hBN/graphene/hBN superlattices in which $R_{nl}$ at SDP is negligible, but below 60 K approaches the value of $h/2e^{2}$ in zero magnetic field at the primary Dirac point with a characteristic decay length of 2 $μ$m. Furthermore, nonlocal transport transmission probabilities…
We report on transport properties in dual-gated hexagonal boron nitride (hBN)/bilayer-graphene (BLG) superlattices. Here, BLG is nontwisted, i.e., plain. This paper focuses on the charge neutrality point (CNP) for a plain BLG. Under a perpendicular magnetic field, transitions between two insulating phases at the CNP are detected by varying a displacement field with the study on the resistance-temperature characteristics and the magnetoresistance. This work opens avenues for exploring the global phase diagram of the hBN/BLG superlattices beyond the CNP.
Ordered atomic-scale superlattices on surface hold great interest both for basic science and for potential applications in advanced technology. However, controlled fabrication of superlattices down to atomic scale has proven exceptionally challenging. Here we demonstrate the segregation-growth and self-organization of ordered S atomic superlattices confined at the interface between graphene and S-rich Cu substrates. Scanning tunneling microscope (STM) studies show that, by finely controlling the growth temperature, we obtain well-ordered S (sub)nanometer-cluster superlattice and monoatomic sup…
Energy band structure of the bilayer graphene superlattices with $δ$-function magnetic barriers and zero average magnetic flux is studied within the four-band continuum model, using the transfer matrix method. The periodic magnetic potential effects on the zero-energy Dirac point of pristine bilayer graphene are exactly analyzed. Magnetic potential is shown also to generate finite-energy Dirac points at the edges of Brillouin zone the positions of which and the related dispersions are determined in the case of symmetric potentials.
We study the band structure of graphene's Dirac-Weyl quasi-particles in a one-dimensional magnetic superlattice formed by a periodic sequence of alternating magnetic barriers. The spectrum and the nature of the states strongly depend on the conserved longitudinal momentum and on the barrier width. At the center of the superlattice Brillouin zone we find new Dirac points at finite energies where the dispersion is highly anisotropic, in contrast to the dispersion close to the neutrality point which remains isotropic. This finding suggests the possibility of collimating Dirac-Weyl quasi-particles…
