V. Akimkin, Ya. Pavlyuchenkov, A. Vasyunin, D. Wiebe, M. Kirsanova, Th. Henning
We study details of the UV radiation transfer in a protoplanetary disk, paying attention to the influence of dust growth and sedimentation on the disk density and temperature. Also, we show how the dust evolution affects photoreaction rates of key molecules, like CN and CS.
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Luminosity outbursts of the FUOri type stars, which have a magnitude of $\sim100 L_{\odot}$ and last for decades, may affect chemical composition of the surrounding protoplanetary disk. Using astrochemical modeling we analyze the changes induced by the outburst and search for species sensitive to the luminosity rise. Some changes in the disk molecular composition appear not only during the outburst itself but can also retain for decades after the end of the outburst. We analyze main chemical processes responsible for these effects and assess timescales at which chemically inert species return …
[Abridged] This review paper discussed which chemical effects may be at play in a planet-forming disk midplane, which effects are relevant under different conditions, and which tools are available for modelling chemical kinetics in a disk midplane. The review goes on to discuss some important efforts in the planet formation modelling community to treat chemical evolution, and, vice versa, efforts in the chemical modelling community to implement more physical effects related to planet formation into the chemical modelling. The aim of this review is both to outline some concepts related to plane…
Protoplanetary disks (PPDs) are characterized by different kinds of gas dynamics and chemistry, which are coupled via ionization, heating and cooling processes, as well as advective and turbulent transport. However, directly coupling gas dynamics with time-dependent chemistry is prohibitively computationally expensive when using comprehensive chemical reaction networks. In this paper, we evaluate the utility of a species-based network reduction method in different disk environments to produce small chemical networks that reproduce the abundances of major species found in large gas-phase chemis…
Giant planets can interact with multiple and chemically diverse environments in protoplanetary discs while they form and migrate to their final orbits. The way this interaction affects the accretion of gas and solids shapes the chemical composition of the planets and of their atmospheres. Here we investigate the effects of different chemical structures of the host protoplanetary disc on the planetary composition. We consider both scenarios of molecular (inheritance from the pre-stellar cloud) and atomic (complete chemical reset) initial abundances in the disc. We focus on four elemental tracer…
Comets provide a unique insight into the molecular composition and complexity of the material in the primordial solar nebula. Recent results from the Rosetta mission, currently monitoring comet 67P/Churyumov-Gerasimenko in situ, and ALMA (the Atacama Large Millimeter/submillimeter Array), have demonstrated a tantalising link between the chemical complexity now confirmed in disks (via the detection of gas-phase CH3CN; Oberg et al. 2015) and that confirmed on the surface of 67P (Goesmann et al. 2015), raising questions concerning the chemical origin of such species (cloud or inheritance versus d…
Recent surveys of protoplanetary disks show that substructure in dust thermal continuum emission maps is common in protoplanetary disks. These substructures, most prominently rings and gaps, shape and change the chemical and physical conditions of the disk, along with the dust size distributions. In this work, we use a thermochemical code to focus on the chemical evolution that is occurring within the gas-depleted gap and the dust-rich ring often observed behind it. The composition of these spatial locations are of great import, as the gas and ice-coated grains will end up being part of the at…
The chemical and physical evolution of primitive materials in protoplanetary disks are determined by the types of environments they are exposed to and their residence times within each environment. Here a method for calculating representative paths of materials in diffusive protoplanetary disks is developed and applied to understanding how the vertical trajectories that particles take impact their overall evolution. The methods are general enough to be applied to disks with uniform diffusivity, the so-called "constant-$α$" cases, and disks with a spatially varying diffusivity, such as expected…
We calculate the chemical evolution of protoplanetary disks considering radial viscous accretion, vertical turbulent mixing and vertical disk winds. We study the effects on the disk chemical structure when different models for the formation of molecular hydrogen on dust grains are adopted. Our gas-phase chemistry is extracted from the UMIST Database for Astrochemistry (Rate06) to which we have added detailed gas-grain interactions. We use our chemical model results to generate synthetic near- and mid-infrared LTE line emission spectra and compare these with recent Spitzer observations. Our res…
The bulk composition of the Earth is dramatically carbon poor compared to that of the interstellar medium, and this phenomenon extends to the asteroid belt. To interpret this carbon deficit problem, the carbonaceous component in grains must have been converted into the gas-phase in the inner regions of protoplanetary disks prior to planetary formation. We examine the effect of carbon grain destruction on the chemical structure of disks by calculating the molecular abundances and distributions using a comprehensive chemical reaction network. When carbon grains are destroyed and the elemental ab…
[Abridged] With a growing number of molecules observed in many comets, and an improved understanding of chemical evolution in protoplanetary disk midplanes, comparisons can be made between models and observations that could potentially constrain the formation histories of comets. A $χ^{2}$-method was used to determine maximum likelihood surfaces for 14 different comets that formed at a given time (up to 8 Myr) and place (out to beyond the CO iceline) in the pre-solar nebula midplane. This was done using observed volatile abundances for the 14 comets and the evolution of volatile abundances fro…
Circumstellar discs may become warped or broken into distinct planes if there is a stellar or planetary companion with an orbit that is misaligned with respect to the disc. There is mounting observational evidence for protoplanetary discs with misaligned inner discs and warps that may be caused by such interactions with a previously undetected companion, giving us a tantalising indication of possible planets forming there. Hydrodynamical and radiative transfer models indicate that the temperature varies azimuthally in warped discs due to the variable angle at which the disc surface faces the s…
The origins of planets, and perhaps life itself, is intrinsically linked to the chemistry of planet formation. In this chapter we will attempt to explore the chemistry of planet-forming disks from the perspective of knowledge gained from decades of solar system study, combined with our rapidly growing knowledge of extra-solar protoplanetary disks. Our aim is not to provide a comprehensive survey of the literature, but rather to present the chemical and physical tools that are used to explore chemical evolution during the earliest stages of planet formation. We include a discussion of observati…
We present the next step in a series of papers devoted to connecting the composition of the atmospheres of forming planets with the chemistry of their natal evolving protoplanetary disks. The model presented here computes the coupled chemical and dust evolution of the disk and the formation of three planets per disk model. Our three canonical planet traps produce a Jupiter near 1 AU, a Hot Jupiter and a Super-Earth. We study the dependency of the final orbital radius, mass, and atmospheric chemistry of planets forming in disk models with initial disk masses that vary by 0.02 $M_\odot$ above an…
Gas dynamics around a Jupiter mass planet: II. Chemical evolution of circumplanetary material
本研究通过后处理嵌入木星质量行星的三维流体模拟，揭示气体坠入行星引力势阱时升温释冰并生成SO、SO$_2$、CS等独特分子，且柱密度与观测相符。
chemcomp: Modeling the chemical composition of planets formed in protoplanetary disks
本研究开源了chemcomp代码，该工具可模拟黏性原行星盘中行星的形成及化学组成演化，支持学界开展行星形成模型与观测约束的对比研究。
The size and density of dust grains determine their response to gas drag in protoplanetary discs. Aerodynamical (size x density) sorting is one of the proposed mechanisms to explain the grain properties and chemical fractionation of chondrites. However, the efficiency of aerodynamical sorting and the location in the disc in which it could occur are still unknown. Although the effects of grain sizes and growth in discs have been widely studied, a simultaneous analysis including dust composition is missing. In this work we present the dynamical evolution and growth of multicomponent dust in a pr…
The impact of rates of reactions with cosmic ray induced photons on chemical composition of protoplanetary discs
本研究利用ANDES模型探讨宇宙射线诱导光子反应速率与尘埃尺寸上限增加对原行星盘化学组成的影响，发现该速率显著改变2至20天文单位间的冰质量分数，但对盘内电离度影响甚微。
Investigating the Sulfur Mystery in Protoplanetary Disks Through Chemical Modeling
本研究更新二维时变原行星盘化学模型，纳入新含硫物种与反应，探究围绕太阳质量T Tauri恒星的盘中硫的分子形式，发现高C/O比可解释相关观测现象，初始硫形式影响盘冰丰度。
Effective reaction temperatures of irreversible dust chemical reactions in a protoplanetary disk
本研究通过三维蒙特卡洛模拟推导原行星盘尘埃不可逆反应有效反应温度的半解析公式，验证其精度后应用于硅酸盐结晶与氧同位素交换，解释了原太阳盘尘埃独特氧同位素组成的成因。
Volatiles are compounds with low sublimation temperatures, and they make up most of the condensible mass in typical planet-forming environments. They consist of relatively small, often hydrogenated, molecules based on the abundant elements carbon, nitrogen and oxygen. Volatiles are central to the process of planet formation, forming the backbone of a rich chemistry that sets the initial conditions for the formation of planetary atmospheres, and act as a solid mass reservoir catalyzing the formation of planets and planetesimals. This growth has been driven by rapid advances in observations and …
Chemical footprints of giant planet formation. Role of planet accretion in shaping the C/O ratio of protoplanetary disks
本研究提出巨行星吸积会在原行星盘留下化学足迹，通过模拟发现吸积行星可升华富碳有机物提升局地气相C/O比，解释了ALMA观测到的谱线发射环现象，建立了巨行星吸积与行星盘化学的新关联。
The composition of gas and solids in protoplanetary discs sets the composition of planets that form out of them. Recent chemical models have shown that the composition of gas and dust in discs evolves on Myr time-scales, with volatile species disappearing from the gas phase. However, discs evolve due to gas accretion and radial drift of dust on time-scales similar to these chemical time-scales. Here we present the first model coupling the chemical evolution in the disc mid-planes with the evolution of discs due to accretion and radial drift of dust. Our models show that transport will always o…
Observations of protoplanetary disks have revealed them to be complex and dynamic, with vertical and radial transport of gas and dust occurring simultaneously with chemistry and planet formation. Previous models of protoplanetary disks focused primarily on chemical evolution of gas and dust in a static disk, or dynamical evolution of solids in a chemically passive disk. In this paper, we present a new 1D method for modelling pebble growth and chemistry simultaneously. Gas and small dust particles are allowed to diffuse vertically, connecting chemistry at all elevations of the disk. Pebbles are…
Distribution of Chemically-Processed Dust in a Viscously Evolving Protoplanetary Disk: Application to Crystalline Silicates in Comets
研究原行星盘中尘埃化学反应，通过蒙特卡罗模拟扩展反应线公式到粘性盘，分析反应尘埃时空分布受反应线与停滞线位置影响，评估出与彗星结晶硅酸盐相符的盘条件，揭示原太阳盘特性。
The composition of a protoplanetary disk is set by a combination of interstellar inheritance and gas and grain surface chemical reactions within the disk. The survival of inherited molecules, as well as the disk in situ chemistry depends on the local temperature, density and irradiation environment, which can change over time due to stellar and disk evolution, as well as transport in the disk. We address one aspect of this coupling between the physical and chemical evolution in disks by following accretion streamlines of gas and small grains in the disk midplane, while simultaneously taking th…
Tracking the Chemical Evolution of Hydrocarbons Through Carbon Grain Supply in Protoplanetary Disks
本文通过42个单细胞模型研究原行星盘内部区域不同C/O比和化学驱动条件下碳氢化合物的演化，揭示碳汇分布、关键物种生成对初始水丰度的强依赖性及CH$_4$和C的瞬态供体作用。
Impact of photoevaporative winds in chemical models of externally irradiated protoplanetary disks
本研究利用DALI后处理外部辐照原行星盘的辐射流体动力学模拟，发现光致蒸发风通过长波热再辐射改变盘体加热与挥发物丰度，并主导数量级的谱线流量差异。
The physical and chemical processes in protoplanetary disks: constraints on the composition of comets
该研究综述原行星盘观测与理论进展，结合ALMA等多波段观测揭示气尘结构、分子分布及动力学特征，指出元素丰度非均匀性或源于气尘解耦，为彗星组成研究提供约束。
Unveiling the Chemical Complexity and C/O Ratio of the HD 163296 Protoplanetary Disk: Constraints from Multi-line ALMA Observations of Organics, Nitriles, Sulfur-bearing, and Deuterated Molecules
本研究利用多波段ALMA观测及DRive、PEGASIS代码，约束HD 163296原行星盘分子分布与C/O比（最佳值1.1），揭示DCO+三环亚结构，给出NH2CHO和HNCO柱密度上限，为行星形成化学提供关键数据。
Protoplanetary Disk Chemistry
本文综述了原行星盘中挥发性元素HOCNSP的化学及相关观测与理论方法，指出盘化学组成受继承与原位化学共同影响，且与物理动力学过程紧密交织，为探测盘演化和行星形成提供了化学探针。
We investigate the impact of photochemistry and X-ray ionization on the molecular composition of, and ionization fraction in, a protoplanetary disk surrounding a typical T Tauri star. We use a sophisticated physical model, which includes a robust treatment of the radiative transfer of UV and X-ray radiation, and calculate the time-dependent chemical structure using a comprehensive chemical network. In previous work, we approximated the photochemistry and X-ray ionization, here, we recalculate the photoreaction rates using the explicit UV wavelength spectrum and wavelength-dependent reaction cr…
CO is the most widely used gas tracer of protoplanetary disks. Its abundance is usually assumed to be an interstellar ratio throughout the warm molecular layer of the disk. But recent observations of low CO gas abundance in many protoplanetary disks challenge our understanding of physical and chemical evolutions in disks. Here we investigate the CO abundance structures in four well-studied disks and compare their structures with predictions of chemical processing of CO and transport of CO ice-coated dust grains in disks. We use spatially resolved CO isotopologue line observations and detailed …
The gas-phase CO abundance (relative to hydrogen) in protoplanetary disks decreases by up to 2 orders of magnitude from its ISM value ${\sim}10^{-4}$, even after accounting for freeze-out and photo-dissociation. Previous studies have shown that while local chemical processing of CO and the sequestration of CO ice on solids in the midplane can both contribute, neither of these processes appears capable of consistently reaching the observed depletion factors on the relevant timescale of $1{-}3\mathrm{~Myr}$. In this study, we model these processes simultaneously by including a compact chemical n…
This is the second paper in a series where we study the influence of transport processes on the chemical evolution of protoplanetary disks. Our analysis is based on a flared alpha-model of the DM Tau system, coupled to a large gas-grain chemical network. To account for production of complex molecules, the chemical network is supplied with an extended set of surface reactions and photo-processes in ice mantles. Our disk model covers a wide range of radii, 10-800 AU (from a Jovian planet-forming zone to the outer disk edge). Turbulent transport of gases and ices is implicitly modeled in full 2D …
The processes that transform gas and dust in circumstellar disks into diverse exoplanets remain poorly understood. One key pathway is to study exoplanets as they form in their young ($\sim$few~Myr) natal disks. Extremely Large Telescopes (ELTs) such as GMT, TMT, or ELT, can be used to establish the initial chemical conditions, locations, and timescales of planet formation, via (1)~measuring the physical and chemical conditions in protoplanetary disks using infrared spectroscopy and (2)~studying planet-disk interactions using imaging and spectro-astrometry. Our current knowledge is based on a l…
Size-dependent charging of dust particles in protoplanetary disks Can turbulence cause charge separation and lightning?
本文利用 ProDiMo 二维热化学模型研究原行星盘中不同尺寸尘埃颗粒的带电行为与电荷平衡，识别出中平面低层温暖区域最可能产生闪电，但湍流诱导电场远低于临界电场，表明该机制难以引发闪电。
Ices are an important constituent of protoplanetary disks. New observational facilities, notably the James Webb Space Telescope (JWST), will greatly enhance our view of disk ices by measuring their infrared spectral features. We present a suite of models to complement these upcoming observations. Our models use a kinetics-based gas-grain chemical evolution code to simulate the distribution of ices in a disk, followed by a radiative transfer code using a subset of key ice species to simulate the observations. We present models reflecting both molecular inheritance and chemical reset initial con…
[Abridged] Chemical evolution in the protoplanetary disk midplane can modify the composition of ices and gases. We have investigated if and how chemical evolution affects the abundances and distributions of key volatile species in the midplane of a protoplanetary disk in the 0.2-30 AU range. A full chemical network including gas-phase, gas-grain interactions and grain-surface chemistry is used to evolve chemistry in time, for 1 Myr. Great diversity is observed in the relative abundance ratios of the main considered species: H2O, CO, CO2, CH4, O2, NH3 and N2. The choice of ionisation level, the…
Aims. With the large amount of molecular emission data from (sub)millimeter observatories and incoming James Webb Space Telescope infrared spectroscopy, access to fast forward models of the chemical composition of protoplanetary disks is of paramount importance. Methods. We used a thermo-chemical modeling code to generate a diverse population of protoplanetary disk models. We trained a K-nearest neighbors (KNN) regressor to instantly predict the chemistry of other disk models. Results. We show that it is possible to accurately reproduce chemistry using just a small subset of physical condition…
Chemistry in Protoplanetary Disks
本文综述了原行星盘中的化学过程，总结了从近红外到毫米波长的分子谱线观测，讨论了化学反应类型与化学建模进展，并重点介绍了雪线位置、碳氧氮主要载体丰度及复杂有机分子研究的最新成果，最后探讨了结合盘化学与行星形成过程追溯行星形成历史的努力。
We present high resolution spectroscopy of mid-infrared molecular emission from two very active T Tauri stars, AS 205 N and DR Tau. In addition to measuring high signal-to-noise line profiles of water, we report the first spectrally resolved mid-infrared line profiles of HCN emission from protoplanetary disks. The similar line profiles and temperatures of the HCN and water emission indicate that they arise in the same volume of the disk atmosphere, within 1-2AU of the star. The results support the earlier suggestion that the observed trend of increasing HCN/water emission with disk mass is a c…
(English) In this lecture I discuss recent progress in the understanding of the chemical evolution of protoplanetary disks that resemble our Solar system during the first ten million years. At the verge of planet formation, strong variations of temperature, density, and radiation intensities in these disks lead to a layered chemical structure. In hot, dilute and heavily irradiated atmosphere only simple radicals, atoms, and atomic ions can survive, formed and destroyed by gas-phase processes. Beneath the atmosphere a partly UV-shielded, warm molecular layer is located, where high-energy radiat…
[Abridged] Planet formation is expected to be enhanced around snowlines in protoplanetary disks, in particular around the water snowline. However, the close proximity of the water snowline to the host star and water in the Earth's atmosphere makes a direct detection of the water snowline in protoplanetary disks challenging. Following earlier work on protostellar envelopes, the aim of this research is to investigate the validity of HCO$^+$ and H$^{13}$CO$^+$, as tracers of the water snowline in protoplanetary disks, as HCO$^+$ is destroyed by gas-phase water. Two small chemical networks are use…
The chemical influence of luminosity outbursts on the environments of young solar-type stars is explored. Species are categorised into several types according to their response to the outburst. The first and second types imply chemical changes only during the outburst (with slightly different behaviours). These response types are mostly observed close to the star and are caused by icy mantle evaporation. However, mantles recover after the outburst almost immediately. A notable exception is benzene ice, which is accumulated on dust surfaces during and after the outburst, so that its abundance e…
The gas temperature in protoplanetary disks (PPDs) is determined by a combination of irradiation heating and accretion heating, with the latter conventionally attributed to turbulent dissipation. However, recent studies have suggested that the inner disk (a few AU) is largely laminar, with accretion primarily driven by magnetized disk winds, as a result of nonideal magnetohydrodynamic (MHD) effects from weakly ionized gas, suggesting an alternative heating mechanism by Joule dissipation. We perform local stratified MHD simulations including all three nonideal MHD effects (ohmic, Hall, and ambi…
We study the influence of different metallicities on the physical, thermal, and chemical properties of protoplanetary disks, and in particular on the formation and destruction of carbon-based molecules. With the thermo-chemical code ProoDIMO we investigate the impact of lower metallicities on the radiation field, disk temperature, and the abundance of different molecules (H$_2$O, CH$_4$, CO, CO$_2$, HCN, CN, HCO$^+$ and N$_2$H$^+$). We use a fiducial disk model as a reference model and produce two models with lower metallicity. The resulting influence on different chemical species is studied b…
The composition of planets may be largely determined by the chemical processing and accretion of icy pebbles in protoplanetary disks. Recent observations of protoplanetary disks hint at wide-spread depletion of gaseous carbon. The missing volatile carbon is likely frozen in CO and/or CO$_2$ ice on grains and locked into the disk through pebble trapping in pressure bumps or planetesimals. We present the results of the first successful ACA (Atacama Compact Array) [C I] $J$ = 1-0 mini-survey of seven protoplanetary disks. Using tailored azimuthally symmetric DALI (Dust And LInes) thermo-chemical …
Gas kinematics are an important part of the planet formation process. Turbulence influences planetesimal growth and migration from the scale of sub-micron dust grains through gas-giant planets. Radio observations of resolved molecular line emission can directly measure this non-thermal motion and, taking advantage of the layered chemical structure of disks, different molecular lines can be combined to map the turbulence throughout the vertical extent of a protoplanetary disk. Here we present ALMA observations of three molecules (DCO$^+$(3-2), C$^{18}$O(2-1) and CO(2-1)) from the disk around HD…
Chemical Evolution of Complex Organic Molecules in Turbulent Protoplanetary Disks: Effect of stochastic UV irradiation
本研究通过气体-冰化学网络模拟，发现湍流原行星盘中紫外辐射的时间变化显著影响复杂有机分子丰度，且含氧与含氮分子对辐射通量的响应不同。
In this paper, we model the chemical evolution of a 0.25 M$_{\odot}$ protoplanetary disc surrounding a 1 M$_{\odot}$ star that undergoes fragmentation due to self-gravity. We use Smoothed Particle Hydrodynamics including a radiative transfer scheme, along with time-dependent chemical evolution code to follow the composition of the disc and resulting fragments over approximately 4000 yrs. Initially, four quasi-stable fragments are formed, of which two are eventually disrupted by tidal torques in the disc. From the results of our chemical modelling, we identify species that are abundant in the f…
Chemical transformation of CO in evolving protoplanetary discs across stellar masses: a route to C-rich inner regions
本文通过一维盘演化模型研究不同恒星质量原行星盘中CO化学转化对C/O升高的作用，发现需结合气相CO破坏、气体平流和径向漂移才能在极低质量恒星盘中实现C/O显著高于1，并指出电离率是关键控制因素。
This paper introduces a new disk code, called ProDiMo, to calculate the thermo-chemical structure of protoplanetary disks and to interpret gas emission lines from UV to sub-mm. We combine frequency-dependent 2D dust continuum radiative transfer, kinetic gas-phase and UV photo-chemistry, ice formation, and detailed non-LTE heating & cooling balance with the consistent calculation of the hydrostatic disk structure. We include FeII and CO ro-vibrational line heating/cooling relevant for the high-density gas close to the star, and apply a modified escape probability treatment. The models are chara…
Molecular lines observed towards protoplanetary disks carry information about physical and chemical processes associated with planet formation. We present ALMA Band 6 observations of C2H, HCN, and C18O in a sample of 14 disks spanning a range of ages, stellar luminosities, and stellar masses. Using C2H and HCN hyperfine structure fitting and HCN/H13CN isotopologue analysis, we extract optical depth, excitation temperature, and column density radial profiles for a subset of disks. C2H is marginally optically thick (τ~1-5) and HCN is quite optically thick (τ~ 5-10) in the inner 200 AU. The extra…
Protoplanetary disks (PPDs) surrounding young stars are short-lived (~0.3-10 Myr), compact (~10-1000 AU) rotating reservoirs of gas and dust. PPDs are believed to be birthplaces of planetary systems, where tiny grains are assembled into pebbles, then rocks, planetesimals, and eventually planets, asteroids, and comets. Strong variations of physical conditions (temperature, density, ionization rate, UV/X-rays intensities) make a variety of chemical processes active in disks, producing simple molecules in the gas phase and complex polyatomic (organic) species on the surfaces of dust particles. In…
Interstellar comets offer direct samples of volatiles from distant protoplanetary disks. 2I/Borisov is the first notably active interstellar comet discovered in our solar system[1]. Comets are condensed samples of the gas, ice, and dust that were in a star's protoplanetary disk during the formation of its planets and inform our understanding on how chemical compositions and abundances vary with distance from the central star. Their orbital migration moves volatiles[2], organic material, and prebiotic chemicals in their host system[3]. In our solar system, hundreds of comets have been observed …
The cosmochemistry of planetary systems
本文综述了利用太阳系物质的化学和同位素组成约束类地行星形成路径，提出流动不稳定性和卵石吸积模型可解释观测特征，并影响行星宜居性。
Oxygen Isotope Constraints on the Importance of Photochemical Processing in Protoplanetary Disks
研究通过分析氧同位素组成，探讨原行星盘中光化学处理对行星构成块的影响，发现其对太阳系组成多样性的影响有限。
CO is commonly used as a tracer of the total gas mass in both the interstellar medium and in protoplanetary disks. Recently there has been much debate about the utility of CO as a mass tracer in disks. Observations of CO in protoplanetary disks reveal a range of CO abundances, with measurements of low CO to dust mass ratios in numerous systems. One possibility is that carbon is removed from CO via chemistry. However, the full range of physical conditions conducive to this chemical reprocessing is not well understood. We perform a systematic survey of the time dependent chemistry in protoplanet…
We present an integrated thermal-chemical model for the atmosphere of the inner region of a protoplanetary disk that includes irradiation by both far ultraviolet (FUV) and X-ray radiation. We focus on how the photodissociation of water and OH affects the abundances of these and related species and how it contributes to the heating of the atmosphere. The dust in the atmosphere plays several important roles, primarily as the site of H$_2$ formation and by absorbing the FUV. Large amounts of water can be synthesized within the inner 4 AU of a disk around a typical classical T~Tauri star. OH is fo…
The gas dynamics of protoplanetary disks (PPDs) is largely controlled by non-ideal magnetohydrodynamic (MHD) effects including Ohmic resistivity, the Hall effect and ambipolar diffusion. Among these the role of the Hall effect is the least explored and most poorly understood. We have included all three non-ideal MHD effects in a self-consistent manner to investigate the role of the Hall effect on PPD gas dynamics using local shearing-box simulations. In this first paper, we focus on the inner region of PPDs, where previous studies excluding the Hall effect have revealed that the inner disk up …
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