We investigate theoretically the combination of first-order quadrupole-quadrupole and second-order dipole-dipole effects on the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom. As the electrostatic energy is comparable to the dimer rotational structure, we develop a general description of the long-range interactions which allows for couplings between the dimer rotational levels. The resulting adiabatic potential energy curves, which exhibit avoided crossings, cannot be expanded on the usual $1/R^{n}$ series. We study in details the breakdown of this approximation in the particular case Cs$_{2}+$Cs. Our results are found promising in the prospect of accomplishing the photoassociation of ultracold trimers.
The formation of ultracold molecules via stimulated emission followed by a radiative deexcitation cascade in the presence of a static electric field is investigated. By analyzing the corresponding cross sections, we demonstrate the possibility to populate the lowest rotational excitations via photoassociation. The modification of the radiative cascade due to the electric field leads to narrow rotational state distributions in the vibrational ground state. External fields might therefore represent an additional valuable tool towards the ultimate goal of quantum state preparation of molecules.
The different resonant regimes that can be achieved by using a magnetic Feshbach resonance are analyzed with a separable two-channel model. Emphasis is put on the case of narrow resonances in a region of intermediate detuning where a shallow dimer exists and an approximate law including the background scattering length for the three-body recombination rate is derived.
We measure chemical reactions between a single trapped $^{174}$Yb$^+$ ion immersed in an ultracold bath of $^6$Li atoms containing trace amounts of Li$_2$ dimers. This produces LiYb$^+$ molecular ions that we detect via mass spectrometry. We explain the reaction rates by modelling the dimer density as a function of the magnetic field and obtain excellent agreement when we assume the reaction to follow the Langevin rate. Our results present a novel approach towards the creation of cold molecular ions and point to the exploration of ultracold chemistry in ion molecule collisions. What is more, w…
We discuss our recent observation of an atom-dimer Efimov resonance in an ultracold mixture of Cs atoms and Cs_2 Feshbach molecules [Nature Phys. 5, 227 (2009)]. We review our experimental procedure and present additional data involving a non-universal g-wave dimer state, to contrast our previous results on the universal s-wave dimer. We resolve a seeming discrepancy when quantitatively comparing our experimental findings with theoretical results from effective field theory.
We solve the three-body problem of an ultracold Fermi gas with parabolic confinement length $a_\perp$ and 3D scattering length $a$. On the two-body level, there is a Feshbach-type resonance at $a_\perp/a\approx 1.46$, and a dimer state for arbitrary $a_\perp/a$. The three-body problem is shown to be universal, an d described by the atom-dimer scattering length $a_{ad}$ and a range parameter $b_{ad}$. In the dimer limit $a_\perp/a\gg 1$, we find a repulsive zero-range atom-dimer interaction. For $a_\perp/a\ll -1$, however, the potential has long range, with $a_{ad}>0$ and $b_{ad}\gg a_{ad}$. Th…
We report on the observation of an elementary exchange process in an optically trapped ultracold sample of atoms and Feshbach molecules. We can magnetically control the energetic nature of the process and tune it from endoergic to exoergic, enabling the observation of a pronounced threshold behavior. In contrast to relaxation to more deeply bound molecular states, the exchange process does not lead to trap loss. We find excellent agreement between our experimental observations and calculations based on the solutions of three-body Schrödinger equation in the adiabatic hyperspherical representat…
The optical nondestructive method for in situ detection of the bound states of ultracold polar molecules is developed. It promises a minimally destructive measurement scheme up to a physically exciting quantum non-demolition (QND) level. The detection of molecular complexes beyond simple pairs of quantum particles (dimers, known, e.g., from the BEC-BCS theory) is suggested, including three-body (trimers) and four-body (tertramers) complexes trapped by one-dimensional tubes. The intensity of scattered light is sensitive to the molecule number fluctuations beyond the mean-density approximation. …
We sudy the creation of nonlocal states with ultracold atoms trapped in an optical lattice. We show that these states violate Bell inequality by measuring one- and two-body correlations. Our scheme only requires beam splitting operations and global phase shifts, and can be realized within the current technology, employing single-site addressing. This proposal paves the way to study multipartite nonlocality and entanglement in ultracold atomic systems.
We use a right unitary decomposition to study an ultracold two-level atom interacting with a quantum field. We show that such a right unitary approach simplifies the numerical evolution for arbitrary position-dependent atom-field couplings. In particular, we provide a closed form, analytic time evolution operator for atom-field couplings with quadratic dependence on the position of the atom.
We apply reservoir engineering to construct a thermal environment with controllable temperature in an ultracold atomic Rydberg system. A Boltzmann distribution of the system's eigenstates is produced by optically driving a small environment of ultracold atoms, which is coupled to a photonic continuum through spontaneous emission. This technique provides a useful tool for quantum simulation of dynamics coupled to a thermal environment. Additionally, we demonstrate that pure eigenstates, such as Bell states, can be prepared in the Rydberg atomic system using this method.
We experimentally demonstrate optical spectroscopy of magnetically trapped atoms on an atom chip. High resolution optical spectra of individual trapped clouds are recorded within a few hundred milliseconds. Detection sensitivities close to the single atom level are obtained by photoionization of the excited atoms and subsequent ion detection with a channel electron multiplier. Temperature and decay rates of the trapped atomic cloud can be monitored in real time for several seconds with only little detection losses. The spectrometer can be used for investigations of ultracold atomic mixtures an…
We investigate the presence of Feshbach resonances in ultracold alkali-dialkali reactive collisions. Quantum scattering calculations are performed on a new Na_3 quartet potential energy surface. An analysis of scattering features is performed through a systematic variation of the nonadditive three-body interaction potential. Our results should provide useful information for interpreting future atom-molecule collision experiments.
We present a complete theoretical description of atomic storage states in the multimode framework by including spatial coherence in atomic collective operators and atomic storage states. We show that atomic storage states are Dicke states with the maximum cooperation number. In some limits, a set of multimode atomic storage states has been established in correspondence with multimode Fock states of the electromagnetic field. This gives better understanding of both the quantum and coherent information of optical field can be preserved and recovered in ultracold medium. In this treatment, we dis…
We theoretically explore photoassociation by Adiabatic Passage of two colliding cold ^{85}Rb atoms in an atomic trap to form an ultracold Rb_2 molecule. We consider the incoherent thermal nature of the scattering process in a trap and show that coherent manipulations of the atomic ensemble, such as adiabatic passage, are feasible if performed within the coherence time window dictated by the temperature, which is relatively long for cold atoms. We show that a sequence of ~2*10^7 pulses of moderate intensities, each lasting ~750 ns, can photoassociate a large fraction of the atomic ensemble at t…
Long-range bound states of the excited heteronuclear 3He*--4He* system that dissociate to either 3He(1s2s 3S_1) + 4He(1s2p 3P_j) or 3He(1s2p 3P_j) + 4He(1s2s 3S_1), where j=0, 1, 2, are investigated using both single-channel and multichannel calculations in order to analyse the effects of Coriolis and non-adiabatic couplings. The multichannel calculations predict two groups of resonances above the lowest asymptotic energy. One of these groups dissociates to an atomic pair with the 2p excitation on the fermionic atom and the other dissociates to two asymptotes which correspond to the 2p excitat…
We study the effect of quantum motion in a Mach-Zehnder interferometer where ultracold, two-level atoms cross a $π/2 $-$π$-$π/2$ configuration of separated, laser illuminated regions. Explicit and exact expressions are obtained for transmission amplitudes of monochromatic, incident atomic waves using recurrence relations which take into account all possible paths: the direct ones usually considered in the simple semiclassical treatment, but including quantum motion corrections, and the paths in which the atoms are repeatedly reflected at the fields.
We present the experimental implementation of a new trap for cold atoms proposed by O. Zobay and B. M. Garraway. It relies on adiabatic potentials for atoms dressed by a rf field in an inhomogeneous magnetic field. This trap is well suited to confine atoms tightly along one direction to produce a two-dimensional atomic gas. We transferred ultracold atoms into this trap, starting either from thermal samples or Bose--Einstein condensates. In the latter case, technical noise during the loading stage caused heating and prevented us from observing 2D BECs.
Elucidating similarities and differences between quantum-optics biphoton interference phenomena and the quantum physics of quasi-one-dimensional double-well optically-trapped ultracold neutral bosonic or fermionic atoms, we show that the analog of the optical biphoton joint-coincidence spectral correlations, studied with massless non-interacting biphotons emanating from EPR-Bell-Bohm single-occupancy sources, corresponds to a distinct contribution in the total second-order momentum correlations of the massive, interacting, and time-evolving ultracold atoms. This single-occupancy contribution c…
In this article we address the general approach for calculating dynamical dipole polarizabilities of small quantum systems, based on a sum-over-states formula involving in principle the entire energy spectrum of the system. We complement this method by a few-parameter model involving a limited number of effective transitions, allowing for a compact and accurate representation of both the isotropic and anisotropic components of the polarizability. We apply the method to the series of ten heteronuclear molecules composed of two of ($^7$Li,$^{23}$Na,$^{39}$K,$^{87}$Rb,$^{133}$Cs) alkali-metal ato…
We study the three-body problem for both fermionic and bosonic cold atom gases in a parabolic transverse trap of lengthscale $a_\perp$. For this quasi-one-dimensional (1D) problem, there is a two-body bound state (dimer) for any sign of the 3D scattering length $a$, and a confinement-induced scattering resonance. The fermionic three-body problem is universal and characterized by two atom-dimer scattering lengths, $a_{ad}$ and $b_{ad}$. In the tightly bound `dimer limit', $a_\perp/a\to\infty$, we find $b_{ad}=0$, and $a_{ad}$ is linked to the 3D atom-dimer scattering length. In the weakly bound…
We report efficient all-optical creation of an ultracold gas of alkaline-earth-metal dimers, $^{88}\rm{Sr}_2$, in their absolute ground state. Starting with weakly bound singlet molecules formed by narrow-line photoassociation in an optical lattice, followed by stimulated Raman adiabatic passage (STIRAP) via a singlet-dominant channel in the $(1)0_u^+$ excited potential, we prepare pure samples of more than 5500 molecules in $X^1Σ_g^+(v=0,J=0)$. We observe two-body collisional loss rates close to the universal limit for both the least bound and most bound vibrational states in $X^1Σ_g^+$. We d…
Few-body correlations emerging in two-dimensional harmonically trapped mixtures, are comprehensively investigated. The presence of the trap leads to the formation of atom-dimer and trap states, in addition to trimers. The Tan's contacts of these eigenstates are studied for varying interspecies scattering lengths and mass ratio, while corresponding analytical insights are provided within the adiabatic hyperspherical formalism. The two- and three-body correlations of trimer states are substantially enhanced compared to the other eigenstates. The two-body contact of the atom-dimer and trap states…
We investigate theoretically the long-range electrostatic interactions between a ground-state homonuclear alkali-metal dimer and an excited alkali-metal atom taking into account its fine-structure. The interaction involves the combination of first-order quadrupole-quadrupole and second-order dipole-dipole effects. Depending on the considered species, the atomic spin-orbit may be comparable to the atom-molecule electrostatic energy and to the dimer rotational structure. Here we extend our general description in the framework of the second-order degenerate perturbation theory [M. Lepers and O. D…
A measurement technique is described which has the potential to map the atomic site occupancies of ultracold atoms in a short-period three-dimensional optical lattice. The method uses accordion and pinning lattices, together with polarization gradient cooling and fluorescence detection, to measure the positions of individual atoms within the sample in three dimensions at a resolution of around half the atomic resonant wavelength. The method measures the site occupancy, rather than the parity of the site occupancy, of atoms in the lattice. It is expected that such measurements hold significant …
We report the realization of a robust magnetic transport scheme to bring 3x10^8 ultracold 87Rb atoms into a cryostat. The sequence starts with standard laser cooling and trapping of 87Rb atoms, transporting first horizontally and then vertically through the radiation shields into a cryostat by a series of normal- and superconducting magnetic coils. Loading the atoms in a superconducting microtrap paves the way for studying the interaction of ultracold atoms with superconducting surfaces and quantum devices requiring cryogenic temperatures.
We report on the controlled insertion of individual Cs atoms into an ultracold Rb gas at about 400 nK. This requires to combine the techniques necessary for cooling, trapping and manipulating single laser cooled atoms around the Doppler temperature with an experiment to produce ultracold degenerate quantum gases. In our approach, both systems are prepared in separated traps and then combined. Our results pave the way for coherent interaction between a quantum gas and a single or few neutral atoms of another species.
The recent advances in single atom detection and manipulation in experiments with ultracold quantum gases are reviewed. The discussion starts with the basic principles of trapping, cooling and detecting single ions and atoms. The realization of single atom detection in ultracold quantum gases is presented in detail and the employed methods, which are based on light scattering, electron scattering, field ionization and direct neutral particle detection are discussed. The microscopic coherent manipulation of single atoms in a quantum gas is also covered. Various examples are given in order to hi…
We propose an experimentally viable setup for the realization of one-dimensional ultracold atom gases in a nanoscale magnetic waveguide formed by two doubly-clamped suspended carbon nanotubes. All common decoherence and atom loss mechanisms are shown to be small. We discuss general consequences of a non-parabolic confinement potential, in particular novel two-body shape resonances, which could be observed in this trap.
The dispersion relation of ultracold atoms in variably shaped optical lattices can be tuned to resemble that of a relativistic particle, i.e. be linear instead of the usual nonrelativistic quadratic dispersion relation of a free atom. Cold atoms in such a lattice can be used to carry out quantum simulations of relativistic wave equation predictions. We begin this article by describing a Raman technique that allows to selectively load atoms into a desired Bloch band of the lattice near a band crossing. Subsequently, we review two recent experiments with quasirelativistic rubidium atoms in a bic…
The creation of ultracold molecules is currently limited to diatomic species. In this letter we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of ultracold Cs atoms with ultracold Cs$_2$ molecules in their rovibrational ground state is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions, and assuming a model potential for the shor…
Typical sources of ultracold atoms operate with a considerable delay between the delivery of ensembles due to sequential trapping and cooling schemes. Therefore, alternative schemes for the continuous generation of ultracold atoms are highly desirable. Here, we demonstrate the continuous loading of a magnetic trap from a quasi-continuous atom beam. We achieve a steady state with $3.8 \times 10^7$ magnetically trapped atoms and a temperature of $102 μ$K. The ensemble is protected from laser light sources, a requirement for its application for metrological tasks or sympathetic cooling. The conti…
We derive an analytical expression for the scattering amplitude of two ultracold atoms of arbitrary spin and with general spin-orbit (SO) coupling, on the basis of our recent work (Phys. Rev. A \textbf{86}, 053608 (2012)). As an application, we demonstrate that SO coupling can induce scattering resonance in the case with finite scattering length. The same approach can be applied to calculate the two-body bound state of SO-coupled ultracold atoms. For the ultracold spin-1/2 fermi gases in three- or two- dimensional systems with SO coupling, we also obtain the renormalization relation of effecti…
We introduce a general method for designing tailored lattices of magnetic microtraps for ultracold atoms, on the basis of patterned permanently magnetized films. A fast numerical algorithm is used to automatically generate patterns which provide optimal atom confinement while respecting desired lattice symmetries and trap parameters. The algorithm can produce finite and infinite lattices of any plane symmetry; we focus specifically on square and triangular lattices which are of interest to future experiments. Typical trap parameters are discussed as well as the impact of realistic imperfection…
We report the trapping of ultracold neutral $ \text{Rb}$ atoms and $ \text{Ba}^+ $ ions in a common optical potential in absence of any radiofrequency (RF) fields. We prepare $ \text{Ba}^+ $ at $ 370 ~ μK $ and demonstrate efficient sympathetic cooling by $100 ~ μK $ after one collision. Our approach is currently limited by the $ \text{Rb}$ density and related three-body losses, but it overcomes the fundamental limitation in RF traps set by RF-driven, micromotion-induced heating. It is applicable to a wide range of ion-atom species, and may enable novel ultracold chemistry experiments and comp…
Noise correlation analysis is a detection tool for spatial structures and spatial correlations in the in-trap density distribution of ultracold atoms. In this book chapter, we discuss the implementation, properties and limitations of the method applied to ensembles of ultracold atoms in optical lattices, and describe some instances where it has been applied.
A universal dimer is subject to secondary collisions with atoms when formed in a cloud of ultracold atoms via three-body recombination. We show that in a collisionally opaque medium, the value of the scattering length that results in the maximum number of secondary collisions may not correspond to the Efimov resonance at the atom-dimer threshold and thus can not be automatically associated with it. This result explains a number of controversies in recent experimental results on universal three-body states and supports the emerging evidence for the significant finite range corrections to the fi…
Heteronuclear alkali-metal dimers represent the class of molecules of choice for creating samples of ultracold molecules exhibiting an intrinsic large permanent electric dipole moment. Among them, the KCs molecule, with a permanent dipole moment of 1.92~Debye still remains to be observed in ultracold conditions. Based on spectroscopic studies available in the literature completed by accurate quantum chemistry calculations, we propose several optical coherent schemes to create ultracold bosonic and fermionic KCs molecules in their absolute rovibrational ground level, starting from a weakly boun…
We study cavity optomechanics of a mixture of ultracold atoms with tunable nonlinear collisions. We show that atomic collisions provide linear couplings between fictitious condensate oscillators, leading to possibilities of achieving a globally coupled quantum optomechanical network with an integrated atom chip. Potential applications range from simulating collective nonequilibrium dynamics in fields well past physics to probing unique properties of quantum mixtures.
This article reviews the development in our laboratory of magnetic lattices comprising periodic arrays of magnetic microtraps created by patterned magnetic films to trap periodic arrays of ultracold atoms. Recent achievements include the realisation of multiple Bose-Einstein condensates in a 10 micron-period one-dimensional magnetic lattice; the fabrication of sub-micron-period square and triangular magnetic lattice structures suitable for quantum tunnelling experiments; the trapping of ultracold atoms in a sub-micron-period triangular magnetic lattice; and a proposal to use long-range interac…
Confining ultracold gases in cavities creates a paradigm of quantum trapping potentials. We show that this allows to bridge models with global collective and short-range interactions as novel quantum phases possess properties of both. Some phases appear solely due to quantum light-matter correlations. Due to global, but spatially structured, interaction, the competition between quantum matter and light waves leads to multimode structures even in single-mode cavities, including delocalized dimers of matter-field coherences (bonds), beyond density orders as supersolids and density waves.
The universal aspects of atom-dimer elastic collisions are investigated within the framework of Faddeev equations. The two-body interactions between the neutral atoms are approximated by the separable potential approach. Our analysis considers a pure van der Waals potential tail as well as soft-core van der Waals interactions permitting us in this manner to address the universally general features of atom-dimer resonant spectra. In particular, we show that the atom-dimer resonances are solely associated with the {\it excited} Efimov states. Furthermore, the positions of the corresponding reson…
We present a general model allowing "quantum simulation" of one-dimensional Dirac models with 2- and 4-component spinors using ultracold atoms in driven 1D tilted optical latices. The resulting Dirac physics is illustrated by one of its well-known manifestations, Zitterbewegung. This general model can be extended and applied with great flexibility to more complex situations.
We discuss the possibility to create hybrid quantum systems that combine ultracold atoms with graphene membranes. We investigate a setup in which a cold atom cloud is placed close to a free-standing sheet of graphene at distances on the order of a few hundred nanometers. The atoms then couple to the graphene membrane via Casimir-Polder forces. Temporal changes in the atomic state of the atomic cloud changes the Casimir-Polder interaction, thereby leading to the creation of a backaction force in the graphene sheet. This setup provides a controllable way to engineer ripples in a graphene sheet.
With radiofrequency fields one can control ultracold atoms in magnetic traps. These fields couple the atomic spin states, and are used in evaporative cooling which can lead to Bose-Einstein condensation in the atom cloud. Also, they can be used in controlled release of the condensate from the trap, thus providing output couplers for atom lasers. In this paper we show that the time-dependent multistate models for these processes have exact solutions which are polynomials of the solutions of the corresponding two-state models. This allows simple, in many cases analytic descriptions for the time-…
Superconducting atom chips have very significant advantages in realizing trapping structures for ultracold atoms compared to conventional atom chips. We extend these advantages further by developing the ability to dynamically tailor the superconducting trap architecture. Heating the chosen parts of a superconducting film by transferring optical images onto its surface we are able to modify the current density distribution and create desired trapping potentials. This method enables us to change the shape and structure of magnetic traps, enabling versatile applications in atomtronics.
We suggest a method to simulate lattice compact Quantum Electrodynamics (cQED) using ultracold atoms in optical lattices, which includes dynamical Dirac fermions in 2+1 dimensions. This allows to test dynamical effects of confinement as well as 2d flux loops deformations and breaking, and to observe Wilson-loop area-law.
The dynamics of two traps with ultracold atoms and connected by Josephson type coupling, is shown to exhibit a transition from dispersive dynamics to localized coherent oscillations. This transition is controlled by coupling strength and energy offset between the traps. The dynamics is also shown to be exactly that of a Heisenberg chain with a linear magnetic field. Possible applications for ``quantum-state engineering'' are discussed.
We show how impurity atoms can measure moments of ultracold atomic gas densities, using the example of bosons in a one-dimensional lattice. This builds on a body of work regarding the probing of systems by measuring the dephasing of an immersed qubit. We show this dephasing is captured by a function resembling characteristic functions of probability theory, of which the derivatives at short times reveal moments of the system operator to which the qubit couples. For a qubit formed by an impurity atom, in a system of ultracold atoms, this operator can be the density of the system at the location…
