We discuss our recent observation of an atom-dimer Efimov resonance in an ultracold mixture of Cs atoms and Cs_2 Feshbach molecules [Nature Phys. 5, 227 (2009)]. We review our experimental procedure and present additional data involving a non-universal g-wave dimer state, to contrast our previous results on the universal s-wave dimer. We resolve a seeming discrepancy when quantitatively comparing our experimental findings with theoretical results from effective field theory.
A powerful experimental technique to study Efimov physics at positive scattering lengths is demonstrated. We use the Feshbach dimers as a local reference for Efimov trimers by creating a coherent superposition of both states. Measurement of its coherent evolution provides information on the binding energy of the trimers with unprecedented precision and yields access to previously inaccessible parameters of the system such as the Efimov trimers' lifetime and the elastic processes between atoms and the constituents of the superposition state. We develop a comprehensive data analysis suitable for…
A universal dimer is subject to secondary collisions with atoms when formed in a cloud of ultracold atoms via three-body recombination. We show that in a collisionally opaque medium, the value of the scattering length that results in the maximum number of secondary collisions may not correspond to the Efimov resonance at the atom-dimer threshold and thus can not be automatically associated with it. This result explains a number of controversies in recent experimental results on universal three-body states and supports the emerging evidence for the significant finite range corrections to the fi…
The Efimov effect, with its ladder of weakly bound three-atomic molecules, poses intriguing questions in the theoretically controversial and experimentally demanding regime of merging of the first excited Efimov energy level with the atom-dimer continuum. Using an original experimental technique, where a coherent superposition state of diatomic and triatomic molecules is utilized, we investigate this regime and reveal a striking behavior: Instead of merging with the atom-dimer continuum the trimer energy level rebounds from it and becomes a deeper bound state again. In addition, instead of a t…
We report on the observation of triatomic Efimov resonances in an ultracold gas of cesium atoms. Exploiting the wide tunability of interactions resulting from three broad Feshbach resonances in the same spin channel, we measure magnetic-field dependent three-body recombination loss. The positions of the loss resonances yield corresponding values for the three-body parameter, which in universal few-body physics is required to describe three-body phenomena and in particular to fix the spectrum of Efimov states. Our observations show a robust universal behavior with a three-body parameter that st…
We report a thorough investigation of finite-temperature effects on three-body recombination near a triatomic Efimov resonance in an ultracold gas of cesium atoms. Our measurements cover a wide range from a near-ideal realization of the zero-temperature limit to a strongly temperature-dominated regime. The experimental results are analyzed within a recently introduced theoretical model based on a universal zero-range theory. The temperature-induced shift of the resonance reveals a contribution that points to an energy-dependence of the three-body parameter. We interpret this contribution in te…
The multichannel Efimov physics is investigated in ultracold heteronuclear admixtures of K and Rb atoms. We observe a shift in the scattering length where the first atom-dimer resonance appears in the $^{41}$K-$^{87}$Rb system relative to the position of the previously observed atom-dimer resonance in the $^{40}$K-$^{87}$Rb system. This shift is well explained by our calculations with a three-body model including the van der Waals interactions, and, more importantly, the multichannel spinor physics. With only minor difference in the atomic masses of the admixtures, the shift in the atom-dimer …
We study Efimov resonances via three-body loss in an ultracold two-component gas of fermionic $^6$Li and bosonic $^{133}$Cs atoms close to a Feshbach resonance at 843~G, extending results reported previously [Pires \textit{et al.}, Phys. Rev. Lett. 112, 250404 (2014)] to temperatures around 120~nK. The experimental scheme for reaching lower temperatures is based upon compensating the gravity-induced spatial separation of the mass-imbalanced gases with bichromatic optical dipole traps. We observe the first and second excited Li-Cs-Cs Efimov resonance in the magnetic field dependence of the thre…
Ultracold atomic gases have developed into prime systems for experimental studies of Efimov three-body physics and related few-body phenomena, which occur in the universal regime of resonant interactions. In the last few years, many important breakthroughs have been achieved, confirming basic predictions of universal few-body theory and deepening our understanding of such systems. We review the basic ideas along with the fast experimental developments of the field, focussing on ultracold cesium gases as a well-investigated model system. Triatomic Efimov resonances, atom-dimer Efimov resonances…
We observed an enhanced atom-dimer relaxation due to the existence of Efimov states in a three-component mixture of 6Li atoms. We measured the magnetic-field dependence of the atom-dimer loss coefficient in the mixture of atoms in state |1> and dimers formed in states |2> and |3>, and found two peaks corresponding to the degeneracy points of the |23> dimer energy level and energy levels of Efimov trimers. We found that the locations of these peaks disagree with universal theory predictions, in a way that cannot be explained by non-universal two-body properties. We constructed theoretical model…
We study the universality of the three-body parameters for systems relevant for ultracold quantum gases with positive $s$-wave two-body scattering lengths. Our results account for finite-range effects and their universality is tested by changing the number of deeply bound diatomic states supported by our interaction model. We find that the physics controlling the values of the three-body parameters associated with the ground and excited Efimov states is constrained by a variational principle and can be strongly affected by $d$-wave interactions that prevent both trimer states from merging into…
We study the interspecies scattering properties of ultracold Li-Cs mixtures in their two energetically lowest spin channels in the magnetic field range between 800 G and 1000 G. Close to two broad Feshbach resonances we create weakly bound LiCs dimers by radio-frequency association and measure the dependence of the binding energy on the external magnetic field strength. Based on the binding energies and complementary atom loss spectroscopy of three other Li-Cs s-wave Feshbach resonances we construct precise molecular singlet and triplet electronic ground state potentials using a coupled-channe…
An Efimov trimer near the atom-dimer threshold can increase the atom loss rate in ultracold trapped atoms through the {\it avalanche mechanism} proposed by Zaccanti et al. A 3-body recombination event creates an energetic atom and dimer, whose subsequent elastic collisions produce additional atoms with sufficient energy to escape from the trapping potential. We use Monte Carlo methods to calculate the average number of atoms lost and the average heat generated by recombination events in both a Bose-Einstein condensate and a thermal gas. We take into account the energy-dependence of the cross s…
Bosonic dimer-dimer scattering is studied near the unitary limit using momentum-space equations for the four-particle transition operators. The impact of the Efimov effect on the dimer-dimer scattering observables is explored and a number of universal relations is established with high accuracy. The rate for the creation of Efimov trimers via dimer-dimer collisions is calculated.
Lithium-6 atoms in the three lowest hyperfine states display universal properties when the S-wave scattering length between each pair of states is large. Recent experiments reported four pronounced features arising from Efimov physics in the atom-dimer relaxation rate, namely two resonances and two local minima. We use the universal effective field theory to calculate the atom-dimer relaxation rate at zero temperature. Our results describe the four features qualitatively and imply there is a hidden local minimum. In the vicinity of the resonance at 685 G, we perform a finite temperature calcul…
We study the two-body and three-body bound states in ultracold atomic mixtures with one of the atoms subjected to an isotropic spin-orbit (SO) coupling. We consider a system of two identical fermions interacting with one SO coupled atom. It is found that there can exist two types of three-body bound states, Efimov trimers and universal trimers. The Efimov trimers are energetically less favored by the SO coupling, which will finally merge into the atom-dimer threshold as increasing the SO coupling strength. Nevertheless, these trimers exhibit a new kind of discrete scaling law incorporating the…
We report on the measurement of four-body recombination rate coefficients in an atomic gas. Our results obtained with an ultracold sample of cesium atoms at negative scattering lengths show a resonant enhancement of losses and provide strong evidence for the existence of a pair of four-body states, which is strictly connected to Efimov trimers via universal relations. Our findings confirm recent theoretical predictions and demonstrate the enrichment of the Efimov scenario when a fourth particle is added to the generic three-body problem.
We convert a strongly interacting ultracold Bose gas into a mixture of atoms and molecules by sweeping the interactions from resonant to weak. By analyzing the decay dynamics of the molecular gas, we show that in addition to Feshbach dimers it contains Efimov trimers. Typically around 8\% of the total atomic population is bound into trimers, identified by their density-independent lifetime of about 100~$μ$s. The lifetime of the Feshbach dimers shows a density dependence due to inelastic atom-dimer collisions, in agreement with theoretical calculations. We also vary the density of the gas acros…
We develop an experimental technique for rf-association of Efimov trimers from three-atoms continuum. We apply it to probe the lowest accessible Efimov energy level in bosonic lithium in the region where strong deviations from the universal behavior are expected, and provide quantitative study of this effect. Position of the Efimov resonance at the atom-dimer threshold, measured with a different experimental technique, concurs with the rf-association results.
The mass-imbalanced three-body recombination process that forms a shallow dimer is shown to possess a rich Efimov-Stückelberg landscape, with corresponding spectra that differ fundamentally from the homonuclear case. A semi-analytical treatment of the three-body recombination predicts an unusual spectra with intertwined resonance peaks and minima, and yields in-depth insight into the behavior of the corresponding Efimov spectra. In particular, the patterns of the Efimov-Stückelberg landscape are shown to depend inherently on the degree of diabaticity of the three-body collisions, which strongl…
Recent measurements of Efimov resonances in a number of ultracold atom species have revealed an unexpected universality, in which three-body scattering properties are determined by the van der Waals length of the two-body interaction potential. To investigate whether this universality extends to heteronuclear mixtures, we measure loss rate coefficients in an ultracold trapped gas of $^{40}$K and $^{87}$Rb atoms. We find an Efimov-like resonance in the rate of inelastic collisions between $^{40}$K$^{87}$Rb Feshbach molecules and $^{87}$Rb atoms. However, we do not observe any Efimov-related res…
Using the framework of effective field theory, we present a detailed study of the Efimov effect in higher partial waves for systems of two identical particles and a third distinguishable particle. Depending on the total angular momentum $L$, the two identical particles must be bosons or fermions. We derive analytical expressions for the elastic and inelastic atom-dimer scattering cross sections as well as the atom-dimer relaxation rate at the dimer breakup threshold. For the experimentally most relevant case of P-waves, we numerically calculate the atom-dimer scattering cross sections and rela…
We study Efimov physics for three identical bosons interacting via a pairwise square-well potential, analyze the validity of the separable approximation as a function of the interaction strength, and investigate what is needed to improve this approximation. We find separable approximations to be accurate for potentials with just one (nearly) bound dimer state. For potentials with more bound or almost bound dimer states, these states need to be included for an accurate determination of the Efimov spectrum and the corresponding three-body observables. We also show that a separable approximation …
We use an effective-field-theory framework to analyze the Efimov effect in heteronuclear three-body systems consisting of two species of atoms with a large interspecies scattering length. In the leading-order description of this theory, various three-body observables in heteronuclear mixtures can be universally parameterized by one three-body parameter. We present the next-to-leading corrections, which include the effects of the finite interspecies effective range and the finite intraspecies scattering length, to various three-body observables. We show that only one additional three-body param…
Ultracold atomic gases have recently become a driving force in few-body physics due to the observation of the Efimov effect. While initially observed in equal mass systems, one expects even richer few-body physics in the heteronuclear case. In previous experiments with ultracold mixtures of potassium and rubidium, an unexpected non-universal behavior of Efimov resonances was observed. In contrast, we measure the scattering length dependent three-body recombination coefficient in ultracold heteronuclear mixtures of $^{39}\mathrm{K}$-\87Rb and $^{41}\mathrm{K}$-\87Rb and do not observe any signa…
We report the observation of a three-body recombination resonance in an ultracold gas of cesium atoms at a very large negative value of the $s$-wave scattering length. The resonance is identified as the second triatomic Efimov resonance, which corresponds to the situation where the first excited Efimov state appears at the threshold of three free atoms. This observation, together with a finite-temperature analysis and the known first resonance, allows the most accurate demonstration to date of the discrete scaling behavior at the heart of Efimov physics. For the system of three identical boson…
Ultracold gases of three distinguishable particles with large scattering lengths are expected to show rich few-body physics related to the Efimov effect. We have created three different mixtures of ultracold 6Li atoms and weakly bound 6Li2 dimers consisting of atoms in three different hyperfine states and studied their inelastic decay via atom-dimer collisions. We have found resonant enhancement of the decay due to the crossing of Efimov-like trimer states with the atom-dimer continuum in one mixture as well as minima of the decay in another mixture, which we interpret as a suppression of exch…
We have analyzed our recently-measured three-body loss rate coefficient for a Bose-Einstein condensate of spin-polarized metastable triplet 4He atoms in terms of Efimov physics. The large value of the scattering length for these atoms, which provides access to the Efimov regime, arises from a nearby potential resonance. We find the loss coefficient to be consistent with the three-body parameter (3BP) found in alkali-metal experiments, where Feshbach resonances are used to tune the interaction. This provides new evidence for a universal 3BP, the first outside the group of alkali-metal elements.…
In view of recent experiments in ultracold atomic systems, the photoassociation of Efimov trimers, composed of three identical bosons, is studied utilizing the multipole expansion. We study both the normal hierarchy case, where one-body current is dominant, and the strong hierarchy case, relevant for photoassociation in ultracold atoms, where two-body current is dominant. For identical particles in the normal hierarchy case, the leading contribution comes from the r^2 s-mode operator and from the quadrupole d-mode operator. The s-mode reaction is found to be dominant at low temperature, while …
We report on the observation of an elementary exchange process in an optically trapped ultracold sample of atoms and Feshbach molecules. We can magnetically control the energetic nature of the process and tune it from endoergic to exoergic, enabling the observation of a pronounced threshold behavior. In contrast to relaxation to more deeply bound molecular states, the exchange process does not lead to trap loss. We find excellent agreement between our experimental observations and calculations based on the solutions of three-body Schrödinger equation in the adiabatic hyperspherical representat…
Ultracold atomic gases are an important testing ground for understanding few-body physics. In particular, these systems enable a detailed study of the Efimov effect. We use ultracold $^{39}\mathrm{K}$ to investigate the temperature dependence of an Efimov resonance. The shape and position of the observed resonance are analyzed by employing an empirical fit, and universal finite-temperature zero-range theory. Both procedures suggest that the resonance position shifts towards lower absolute scattering lengths when approaching the zero-temperature limit. We extrapolate this shift to obtain an est…
We consider three-body recombination into deep dimers in a mass-imbalanced two-component atomic gas. We use an optical model where a phenomenological imaginary potential is added to the lowest adiabatic hyper-spherical potential. The consequent imaginary part of the energy eigenvalue corresponds to the decay rate or recombination probability of the three-body system. The method is formulated in details and the relevant qualitative features are discussed as functions of scattering lengths and masses. We use zero-range model in analyses of recent recombination data. The dominating scattering len…
A new narrow 3-atom loss resonance associated with an Efimov trimer crossing the 3-atom threshold has recently been discovered in a many-body system of ultracold 6Li atoms in the three lowest hyperfine spin states at a magnetic field near 895 G. O'Hara and coworkers have used measurements of the 3-body recombination rate in this region to determine the complex 3-body parameter associated with Efimov physics. Using this parameter as the input, we calculate the universal predictions for the spectrum of Efimov states and for the 3-body recombination rate in the universal region above 600 G where …
We report the observation of a dimer-dimer inelastic collision resonance for ultracold Feshbach molecules made of bosonic sodium and rubidium atoms. This resonance, which we attribute to the crossing of the dimer-dimer threshold with a heteronuclear tetramer state, manifests itself as a pronounced inelastic loss peak of dimers when the interspecies scattering length between the constituent atoms is tuned. Near this resonance, a strong modification of the temperature dependence of the dimer-dimer scattering is observed. Our result provides insight into the heteronuclear four-body system consist…
We investigate theoretically and experimentally the heteronuclear Efimov scenario for a three-body system that consists of two bosons and one distinguishable particle with positive intraspecies scattering lengths. The three-body parameter at the three-body scattering threshold and the scaling factor between consecutive Efimov resonances are found to be controlled by the scattering length between the two bosons, approximately independent of short-range physics. We observe two excited-state Efimov resonances in the three-body recombination spectra of an ultracold mixture of fermionic $^6 $Li and…
In this paper we discuss the recent discovery of the universality of the three-body parameter (3BP) from Efimov physics. This new result was identified by recent experimental observations in ultracold quantum gases where the value of the s-wave scattering length, $a=a_-$, at which the first Efimov resonance is created was found to be nearly the same for a range of atomic species --- if scaled as $a_-/r_{\rm vdW}$, where $r_{\rm vdW}$ is the van der Waals length. Here, we discuss some of the physical principles related to these observations that emerge from solving the three-body problem with v…
We use exact four-boson scattering equations in the momentum-space framework to study the universal properties of shallow Efimov tetramers and their dependence on the two-boson scattering length. We demonstrate that, in contrast to previous predictions, the shallow tetramer in a particular experimentally unexplored regime is not an unstable bound state but an inelastic virtual state. This leads to a resonant behaviour of the atom-trimer scattering length and thereby to a resonant enhancement of the trimer relaxation in ultracold atom-trimer mixtures.
The different resonant regimes that can be achieved by using a magnetic Feshbach resonance are analyzed with a separable two-channel model. Emphasis is put on the case of narrow resonances in a region of intermediate detuning where a shallow dimer exists and an approximate law including the background scattering length for the three-body recombination rate is derived.
We provide an exact solution of the Efimov spectrum in ultracold gases within the standard two-channel model for Feshbach resonances. It is shown that the finite range in the Feshbach coupling makes the introduction of an adjustable three-body parameter obsolete. The solution explains the empirical relation between the scattering length a_- where the first Efimov state appears at the atom threshold and the van der Waals length l_vdw for open channel dominated resonances. There is a continuous crossover to the closed channel dominated limit, where the scale in the energy level diagram as a func…
We experimentally and theoretically study the effect of the intraspecies scattering length onto the heteronuclear Efimov scenario, following up on our earlier observation of Efimov resonances in an ultracold Cs-Li mixture for negative [Pires et al., Phys. Rev. Lett. 112, 250404 (2014)] and positive Cs-Cs scattering length [Ulmanis et al., Phys. Rev. Lett. 117, 153201 (2016)]. Three theoretical models of increasing complexity are employed to quantify its influence on the scaling factor and the three-body parameter: a simple Born-Oppenheimer picture, a zero-range theory, and a spinless van der W…
We measure the critical scattering length for the appearance of the first three-body bound state, or Efimov three-body parameter, at seven different Feshbach resonances in ultracold 39K atoms. We study both intermediate and narrow resonances, where the three-body spectrum is expected to be determined by the non-universal coupling of two scattering channels. We observe instead approximately the same universal relation of the three-body parameter with the two-body van der Waals radius already found for broader resonances, which can be modeled with a single channel. This unexpected observation su…
We study three-atom inelastic scattering in ultracold \textsuperscript{39}K near a Feshbach resonance of intermediate coupling strength. The non-universal character of such resonance leads to an abnormally large Efimov absolute length scale and a relatively small effective range $r_e$, allowing the features of the \textsuperscript{39}K Efimov spectrum to be better isolated from the short-range physics. Meticulous characterization of and correction for finite temperature effects ensure high accuracy on the measurements of these features at large-magnitude scattering lengths. For a single Feshba…
Unstable four-boson states having an approximate dimer-atom-atom structure are studied using momentum-space integral equations for the four-particle transition operators. For a given Efimov trimer the universal properties of the lowest associated tetramer are determined. The impact of this tetramer on the atom-trimer and dimer-dimer collisions is analyzed. The reliability of the three-body dimer-atom-atom model is studied.
The discrete Efimov scaling behavior, well-known in the low-energy spectrum of three-body bound systems for large scattering lengths (unitary limit), is identified in the energy dependence of atom-molecule elastic cross-section in mass imbalanced systems. That happens in the collision of a heavy atom with mass $m_H$ with a weakly-bound dimer formed by the heavy atom and a lighter one with mass $m_L \ll m_H$. Approaching the heavy-light unitary limit the $s-$wave elastic cross-section $σ$ will present a sequence of zeros/minima at collision energies following closely the Efimov geometrical law.…
In 1970 V. Efimov predicted a puzzling quantum-mechanical effect that is still of great interest today. He found that three particles subjected to a resonant pairwise interaction can join into an infinite number of loosely bound states even though each particle pair cannot bind. Interestingly, the properties of these aggregates, such as the peculiar geometric scaling of their energy spectrum, are universal, i.e. independent of the microscopic details of their components. Despite an extensive search in many different physical systems, including atoms, molecules and nuclei, the characteristic sp…
We observe two consecutive heteronuclear Efimov resonances in an ultracold Li-Cs mixture by measuring three-body loss coefficients as a function of magnetic field near a Feshbach resonance. The first resonance is detected at a scattering length of $a_-^{(1)}=-320(10)~a_0$ corresponding to $\sim 7 $ ($\sim 3$) times the Li-Cs (Cs-Cs) van der Waals range. The second resonance appears at $5.8(1.0) a_-^{(1)}$ close to the unitarity-limited regime at the sample temperature of 450 nK. Indication of a third resonance is found in the atom loss spectra. The scaling of the resonance positions is close t…
The universal aspects of atom-dimer elastic collisions are investigated within the framework of Faddeev equations. The two-body interactions between the neutral atoms are approximated by the separable potential approach. Our analysis considers a pure van der Waals potential tail as well as soft-core van der Waals interactions permitting us in this manner to address the universally general features of atom-dimer resonant spectra. In particular, we show that the atom-dimer resonances are solely associated with the {\it excited} Efimov states. Furthermore, the positions of the corresponding reson…
Under certain circumstances, three or more interacting particles may form bound states. While the general few-body problem is not analytically solvable, the so-called Efimov trimers appear for a system of three particles with resonant two-body interactions. The binding energies of these trimers are predicted to be universally connected to each other, independent of the microscopic details of the interaction. By exploiting a Feshbach resonance to widely tune the interactions between trapped ultracold lithium atoms, we find evidence for two universally connected Efimov trimers and their associat…
We study the collisional properties of an ultracold mixture of cesium atoms and dimers close to a Feshbach resonance near 550G in the regime of positive $s$-wave scattering lengths. We observe an atom-dimer loss resonance that is related to Efimov's scenario of trimer states. The resonance is found at a value of the scattering length that is different from a previous observation at low magnetic fields. This indicates non-universal behavior of the Efimov spectrum for positive scattering lengths. We compare our observations with predictions from effective field theory and with a recent model bas…
While Efimov physics in ultracold atoms is usually modeled with an isolated Feshbach resonance many real world resonances appear in close vicinity to each other and are therefore overlapping. Here we derive a realistic model based on the mutual coupling of an open channel and two closed molecular channels while neglecting short-range physics as permitted by the narrow character of the considered resonances. The model is applied to three distinct scenarios with experimental relevance. We show that the effect of overlapping resonances is manifested most strikingly at a narrow resonance in whose …
We explore the properties of weakly bound bosonic states in the strongly interacting regime. Combining a correlated-Gaussian (CG) basis set expansion with a complex scaling method, we extract the energies and structural properties of bosonic cluster states with $N\le6$ for different two-body potentials. The identification of five- and six-body resonances attached to an excited Efimov trimer provides strong support to the premise of Efimov universality in bosonic systems. Our study also reveals a rich structure of bosonic cluster states. Besides the lowest cluster states which behave as bosonic…
The Efimov effect is the only experimentally realized universal phenomenon that exhibits the renormalization-group limit cycle with the three-body parameter parametrizing a family of universality classes. Recent experiments in ultracold atoms have unexpectedly revealed that the three-body parameter itself is universal when measured in units of an effective range. By performing an exact functional renormalization-group analysis with various finite-range interaction potentials, we demonstrate that the onset of the renormalization-group flow into the limit cycle is universal, regardless of short-…
We show that isotope-exchange reactions between ground-state alkali-metal, alkaline-earth-metal, and lanthanide heteronuclear dimers consisting of two isotopes of the same atom are exothermic with an energy change in the range of 1-8000$\,$MHz thus resulting in cold or ultracold products. For these chemical reactions there are only one rovibrational and at most several hyperfine possible product states. The number and energetics of open and closed reactive channels can be controlled by the laser and magnetic fields. We suggest a laser-induced isotope- and state-selective Stark shift control to…
