Light scattering in inhomogeneous media induces wavefront distortions which pose an inherent limitation in many optical applications. Examples range from microscopy and nanosurgery to astronomy. In recent years, ongoing efforts have made the correction of spatial distortions possible by wavefront shaping techniques. However, when ultrashort pulses are employed scattering induces temporal distortions which hinder their use in nonlinear processes such as in multiphoton microscopy and quantum control experiments. Here we show that correction of both spatial and temporal distortions can be attained by manipulating only the spatial degrees of freedom of the incident wavefront. Moreover, by optimizing a nonlinear signal the refocused pulse can be shorter than the input pulse. We demonstrate focusing of 100fs pulses through a 1mm thick brain tissue, and 1000-fold enhancement of a localized two-photon fluorescence signal. Our results open up new possibilities for optical manipulation and nonlinear imaging in scattering media.
We report generation of ultrashort UV pulses by soliton self-compression in kagomé-style hollow-core photonic crystal fiber filled with ambient air. Pump pulses with energy 2.6 uJ and duration 54 fs at 400 nm were compressed temporally by a factor of 5, to a duration of ~11 fs. The experimental results are supported by numerical simulations, showing that both Raman and Kerr effects play a role in the compression dynamics. The convenience of using ambient air, and the absence of glass windows that would distort the compressed pulses, makes the setup highly attractive as the basis of an efficien…
Using numerical simulations, we study propagation of ultrashort light pulses in an inhomogeneously broadened two-level medium. There are two main issues in our study. The first one concerns the transient process of self-induced transparency soliton formation, in particular, the compression of the pulse which seems to be more effective in the case of homogeneous broadening. The second question deals with the collisions of counter-propagating solitons. It is shown that the level of inhomogeneous broadening has a substantial effect on the elasticity of such collisions.
We demonstrate generation of 7.6 fs near-UV pulses centered at 400 nm via 8-fold soliton-effect self-compression in an Ar-filled hollow-core kagomé-style photonic crystal fiber with ultrathin core walls. Analytical calculations of the effective compression length and soliton order permit adjustment of the experimental parameters, and numerical modelling of the nonlinear pulse dynamics in the fiber accurately predict the spectro-temporal profiles of the self-compressed pulses. After compensation of phase distortion introduced by the optical elements along the beam path from the fiber to the dia…
This is a summary directed to PhD students of the research work conducted on the problem of the production of "light bullets", or multidimensional wave packets that propagate without distortion in unbounded, homogeneous, nonlinear media, and on the actual nature of the self-localized light wave packets spontaneously generated in self-focusing experiments with ultrashort pulses.
Different optical nanostructures containing both loss and gain components attract ever-increasing attention as novel advanced materials and building blocks for a variety of nanophotonic and plasmonic applications. Unique tunable optical signatures of the so-called active metamaterials support their utilizing for sensing, imaging, and signal processing on micro- and nanoscales. However, this tunability requires flexible control over the metamaterials parameters, which could be provided by involving a set of nonlinear interactions. In this paper, we propose a method of governing ultrashort pulse…
Transparent materials do not absorb light but have profound influence on the phase evolution of transmitted radiation. One consequence is chromatic dispersion, i.e., light of different frequencies travels at different velocities, causing ultrashort laser pulses to elongate in time while propagating. Here we experimentally demonstrate ultrathin nanostructured coatings that resolve this challenge: we tailor the dispersion of silicon nanopillar arrays such that they temporally reshape pulses upon transmission using slow light effects and act as ultrashort laser pulse compressors. The coatings ind…
Supercontinuum (SC) generation based on ultrashort pulse compression constitutes one of the most promising technologies towards an ultra-wide bandwidth, high-brightness and spatially coherent light sources for applications such as spectroscopy and microscopy. Here, multi-octave SC generation in a gas-filled hollow-core antiresonant fiber (HC-ARF) is reported spanning from 200 nm in the deep ultraviolet (DUV) to 4000 nm in the mid-infrared (mid-IR). A measured average output power of 5 mW was obtained by pumping at the center wavelength of the first anti-resonance transmission window (2460 nm) …
We propose a novel method based on the so-called shortcut to adiabatic passage techniques to achieve fast compression of temporal solitons in a nonlinear waveguide. We demonstrate that soliton compression could be achieved, in principle, at an arbitrarily small distance by inverse engineering the pulse width and the nonlinearity of the medium. The proposed scheme could possibly be exploited for various short-distance communication protocols and may be even in nonlinear guided wave-optics devices and generation of ultrashort soliton pulses.
An efficient technique to produce a periodic sequence of ultrashort pulses of recoilless gamma-radiation via its transmission through the optically thick vibrating resonant absorber was demonstrated recently [Nature, 508, 80 (2014)]. In this work we extend the theoretical analysis to the case of a set of multiple absorbers. We consider an analytical model describing the control of spectral content of a frequency modulated gamma-radiation by selective correction of amplitudes and initial phases of some spectral components, using, respectively, the resonant absorption or dispersion of nuclei. On…
Random resonant media being one of the possible realizations of disordered metamaterials open a room of opportunities for achieving new fundamental effects and designing advanced nanophotonic devices. Strongly nonlinear optical properties of such media attract ever increasing attention nowadays from both theoretical and experimental points of view. Hereinafter we consider the case of the photonic-crystal-like structure with a randomly varying light-matter coupling provided by the random density of quantum particles. Using numerical solution of the Maxwell-Bloch equations, we study the effects …
We identify a novel regime of soliton-plasma interactions in which high-intensity ultrashort pulses of intermediate soliton order undergo coherent plasma-induced fission. Experimental results obtained in gas-filled hollow-core photonic crystal fibers are supported by rigorous numerical simulations. The cumulative blueshift of higher-order input solitons with ionizing intensities results in pulse splitting before the ultimate self-compression point, leading to the generation of robust pulse pairs with PHz bandwidths. The novel dynamics closes the gap between plasma-induced adiabatic soliton com…
Soliton self-compression is demonstrated during the propagation of high spatial modes in hollow core fibers in the near-infrared spectral region, taking advantage of their negative dispersion response. We have found that there is always an optimum spatial mode to observe this phenomenon, compressing the pulses down to the single-cycle regime without needing any external compression device and with a consequent increase in the output peak power. Our result is relevant for any ultrashort laser application in which few- or single-cycle pulses are crucial.
The critical power of self-focusing in the air for ultrashort UV laser pulses stretched due to dispersion from 90 up to 730 fs was experimentally measured. It was shown that the pulse duration enhancement due to its propagation in condensed media within above mentioned time-range leads to almost linear decrease of self-focusing critical power. It was also observed that when the pulse peak power exceeds the critical one, the maximum of linear plasma distribution along the UV laser filament does not shifted in the direction opposite to the laser pulse propagation as in the case of IR laser filam…
Multimode optical fibers has emerged as the platform that will bridge the gap between nonlinear optics in bulk media and in single-mode fibers. However, the understanding of the transition between these two research fields still remains incomplete despite numerous investigations of intermodal nonlinear phenomena and spatiotemporal coupling. Some of the striking phenomena observed in bulk media with ultrashort and ultra-intense pulses (i.e., conical emission, harmonic generation and light bullets) require a deeper insight to be possibly unveiled in multimode fibers. Here we generalize the conce…
We report a method to characterize the propagation of an ultrashort pulse of light through a multiple scattering medium by measuring its time-resolved transmission matrix. This method is based on the use of a spatial light modulator together with a coherent time-gated detection of the transmitted speckle field. Using this matrix, we demonstrate the focusing of the scattered pulse at any arbitrary position in space and time after the medium. Our approach opens new perspectives for both fundamental studies and applications in imaging and coherent control in disordered media.
Few-cycle lasers are essential for many research areas such as attosecond physics that promises to address fundamental questions in science and technology. Therefore, further advancements are connected to significant progress in the underlying laser technology. Here, two-stage nonlinear compression of a 660 W femtosecond fiber laser system is utilized to achieve unprecedented average power levels of energetic ultrashort or even few-cycle laser pulses. In a first compression step 408 W, 320 uJ, 30fs pulses are achieved, which can be further compressed to 216 W, 170 uJ, 6.3 fs pulses in a second…
Several matrix approaches were developed to control light propagation through multiple scattering media under illumination of ultrashort pulses of light. These matrices can be recorded either with spectral or temporal resolution. Thanks to wavefront shaping, temporal and spatial refocusing have been demonstrated. In this work, we study how these different methods can be exploited to enhance a two-photon excitation fluorescence process. We first compare the different techniques on micrometer-size isolated fluorescent beads. We then demonstrate point-scanning imaging of such fluorescent microbea…
Broadband mid-infrared (MIR) molecular spectroscopy demands a bright and broadband light source in the molecular fingerprint region. To this end, intra-pulse difference frequency generation (IDFG) has shown excellent properties among various techniques. However, previous IDFG systems have mainly used unconventional long-wavelength 2-$μ$m ultrashort pulsed lasers. A few systems have been demonstrated with 1-$μ$m lasers, but they use bulky 100-W-class high-power Yb thin-disk lasers. In this work, we demonstrate a simple and robust approach of 1-$μ$m-pumped broadband IDFG with a conventional mode…
In most applications of ultrashort pulse lasers, temporal compressors are used to achieve a desired pulse duration in a target or sample, and precise temporal characterization is important. The dispersion-scan (d-scan) pulse characterization technique usually involves using glass wedges to impart variable, well-defined amounts of dispersion to the pulses, while measuring the spectrum of a nonlinear signal produced by those pulses. This works very well for broadband few-cycle pulses, but longer, narrower bandwidth pulses are much more difficult to measure this way. Here we demonstrate the conce…
Controlling the wave function of free electrons is important to improve the spatial resolution of electron microscopes, the efficiency of electron interaction with sample modes of interest, and our ability to probe ultrafast materials dynamics at the nanoscale. In this context, attosecond electron compression has been recently demonstrated through interaction with the near fields created by scattering of ultrashort laser pulses at nanostructures followed by free electron propagation. Here, we show that control over electron pulse shaping, compression, and statistics can be improved by replacin…
An optical kink is a shock-wave-like field structure which can appear in a resonant two-level medium as a result of the nonlinear process of self-steepening. We numerically simulate this process using an adiabatically switching waveform as an input and confirm the self-similarity of resulting kinks. The analysis is also applicable to a more general waveform with a decaying trailing edge which we call a kinklike pulse. We study in detail collisions of kinks with other kinks and ultrashort pulses and demonstrate the possibility to control kink speed by changing the parameters of counterpropagati…
External driving of passive, nonlinear optical resonators has emerged over the past decade as a novel route for the generation of ultrashort optical pulses and corresponding broadband frequency combs. Whilst the pulse formation dynamics in such systems differ dramatically from those manifesting themselves in conventional mode-locked lasers, the demarcation between the two traditionally distinct paradigms has recently begun to blur, with demonstrations of hybrid systems incorporating both external driving and active media shown to offer specific advantages. Here we explore a new pathway for ult…
We propose an all-optical, three-dimensional electron pulse compression scheme in which Hermite-Gaussian optical modes are used to fashion a three-dimensional optical trap in the electron pulse's rest frame. We show that the correct choices of optical incidence angles are necessary for optimal compression. We obtain analytical expressions for the net impulse imparted by Hermite-Gaussian free-space modes of arbitrary order. Although we focus on electrons, our theory applies to any charged particle and any particle with non-zero polarizability in the Rayleigh regime. We verify our theory numeric…
The complex temporal behavior of an ultrashort pulse of light propagating through a multiply scattering medium can be characterized experimentally through a time-gated transmission matrix. Using a spatial light modulator, we demonstrate here, that injecting singular vectors of this matrix allows us to optimally control energy deposition at any controllable delay time. Our approach provides insights into fundamental aspects of multi-spectral light scattering and could find applications in imaging or coherent control.
Advances in the amplification and manipulation of ultrashort laser pulses has led to revolutions in several areas. Examples include chirped pulse amplification for generating high peak-power lasers, power-scalable amplification techniques, pulse shaping via modulation of spatially-dispersed laser pulses, and efficient frequency-mixing in quasi-phase-matched nonlinear crystals to access new spectral regions. In this work, we introduce and demonstrate a new platform for nonlinear optics which has the potential to combine all of these separate functionalities (pulse amplification, frequency trans…
Shortcuts to adiabaticity for rapid soliton compression in nonlocal media
Shanghai University（上海大学）；University of the Basque Country UPV/EHU（巴斯克大学）；Quantum Advanced Research Center (QuARC), CSIC（CSIC量子先进研究中心）；Instituto de Ciencia de Materiales de Madrid (ICMM), CSIC（CSIC马德里材料科学研究所）
The Free-Electron Laser (FEL) FLASH offers the worldwide still unique capability to study ultrafast processes with high-flux, high-repetition rate XUV and soft X-ray pulses. The vast majority of experiments at FLASH are of pump-probe type. Many of them rely on optical ultrafast lasers. Here, a novel FEL facility laser is reported which combines high average power output from Yb:YAG amplifiers with spectral broadening in a Herriott-type multi-pass cell and subsequent pulse compression to sub-100 fs durations. Compared to other facility lasers employing optical parametric amplification, the new …
Université Bourgogne Europe, CNRS（勃艮第欧洲大学）；University of Calabria（卡拉布里亚大学）；University of Limoges, CNRS（利摩日大学）；Niccolò Cusano University（尼古拉·库萨诺大学）；Sapienza Universit‘a di Roma（罗马第一大学）
