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arXiv 1010.6014cond-mat.mes-hall
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在顺序和共隧穿区中通过单分子磁体输运的自旋效应

Spin effects in transport through single-molecule magnets in the sequential and cotunneling regimes

Maciej Misiorny, Ireneusz Weymann, Jozef Barnas

摘要:

我们分析了通过弱耦合到外部铁磁引线的单分子磁体的稳态自旋相关输运。使用实时图形技术,我们计算的顺序和cotunneling贡献的电流,隧道磁电阻和Fano因子在线性和非线性响应制度。我们发现,共隧穿效应主要是可见的封锁制度,并导致隧道磁阻(TMR)的增强以上的Julliere值,这是伴随着超泊松散粒噪声由于聚束的非弹性共隧穿过程通过不同的虚拟自旋状态的分子。还考虑了外部磁场的影响以及LUMO能级和分子自旋之间交换相互作用的类型和强度的作用。当交换耦合是铁磁的,我们发现一个增强的TMR,而在反铁磁耦合的情况下,我们预测一个大的负TMR效应。

英文摘要:

We analyze the stationary spin-dependent transport through a single-molecule magnet weakly coupled to external ferromagnetic leads. Using the real-time diagrammatic technique, we calculate the sequential and cotunneling contributions to current, tunnel magnetoresistance and Fano factor in both linear and nonlinear response regimes. We show that the effects of cotunneling are predominantly visible in the blockade regime and lead to enhancement of tunnel magnetoresistance (TMR) above the Julliere value, which is accompanied with super-Poissonian shot noise due to bunching of inelastic cotunneling processes through different virtual spin states of the molecule. The effects of external magnetic field and the role of type and strength of exchange interaction between the LUMO level and the molecule's spin are also considered. When the exchange coupling is ferromagnetic, we find an enhanced TMR, while in the case of antiferromagnetic coupling we predict a large negative TMR effect.

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