We propose a procedure to fully reconstruct the time-dependent coefficients of convolutionless non-Markovian dissipative generators via a finite number of experimental measurements. By combining a tomography based approach with a proper data sampling, our proposal allows to relate the time-dependent coefficients governing the dissipative evolution of a quantum system to experimentally accessible quantities. The proposed scheme not only provides a way to retrieve full information about potentially unknown dissipative coefficients but also, most valuably, can be employed as a reliable consistency test for the approximations involved in the theoretical derivation of a given non-Markovian convolutionless master equation.
Stochastic Schr{ö}dinger equations for quantum trajectories offer an alternative and sometimes superior approach to the study of open quantum system dynamics. Here we show that recently established convolutionless non-Markovian stochastic Schr{ö}dinger equations may serve as a powerful tool for the derivation of convolutionless master equations for non-Markovian open quantum systems. The most interesting example is quantum Brownian motion (QBM) of a harmonic oscillator coupled to a heat bath of oscillators, one of the most-employed exactly soluble models of open system dynamics. We show explic…
The time-convolutionless (TCL) non-Markovian master equation was generally thought to break down at finite time due to its singularity and fail to produce the asymptotic behavior in strong coupling regime. However, in this paper, we show that the singularity is not an obstacle for validity of the TCL master equation. Further, we propose a multiscale perturbative method valid for solving the TCL master equation in strong coupling regime, though the ordinary perturbative method invalidates therein.
We consider a general open system dynamics and we provide a recursive method to derive the associated non-Markovian master equation in a perturbative series. The approach relies on a momenta expansion of the open system evolution. Unlike previous perturbative approaches of this kind, the method presented in this paper provides a recursive definition of each perturbative term. Furthermore, we give an intuitive diagrammatic description of each term of the series, which pro- vides an useful analytical tool to build them and to derive their structure in terms of commutators and anticommutators. We…
We consider the exact reduced dynamics of a two-level system coupled to a bosonic reservoir, further obtaining the exact time-convolutionless and Nakajima-Zwanzig non-Markovian equations of motion. The considered system includes the damped and undamped Jaynes-Cummings model. The result is obtained by exploiting an expression of quantum maps in terms of matrices and a simple relation between the time evolution map and time-convolutionless generator as well as Nakajima-Zwanzig memory kernel. This non-perturbative treatment shows that each operator contribution in Lindblad form appearing in the e…
Driven two-level system is a useful model to describe many quantum objects, particularly in quantum information processing. However, the exact master equation for such a system is barely explored. Making use of the Feynman-Vernon influence functional theory, we derive an exact non-Markovian master equation for the driven two-level system and show the lost feature in the perturbative treatment for this system. The perturbative treatment leads to the time-convolutionless (TCL) and the Nakajima-Zwanzig (NZ) master equations. So to this end, we derive the time-convolutionless (TCL) and the Nakajim…
The dynamics of atom lasers with a continuous output coupler based on two-photon Raman transitions is investigated. With the help of the time-convolutionless projection operator technique the quantum master equations for pulsed and continuous wave (cw) atom lasers are derived. In the case of the pulsed atom laser the power of the time-convolutionless projection operator technique is demonstrated through comparison with the exact solution. It is shown that in an intermediate coupling regime where the Born-Markov approximation fails the results of this algorithm agree with the exact solution. To…
Convolutionless and convolution master equations are the two mostly used physical descriptions of open quantum systems dynamics. We subject these equations to time deformations: local dilations and contractions of time scale. We prove that the convolutionless equation remains legitimate under any time deformation (results in a completely positive dynamical map) if and only if the original dynamics is completely positive divisible. Similarly, for a specific class of convolution master equations we show that uniform time dilations preserve positivity of the deformed map if the original map is po…
We study the analytically solvable Ising model of a single qubit system coupled to a spin bath. The purpose of this study is to analyze and elucidate the performance of Markovian and non-Markovian master equations describing the dynamics of the system qubit, in comparison to the exact solution. We find that the time-convolutionless master equation performs particularly well up to fourth order in the system-bath coupling constant, in comparison to the Nakajima-Zwanzig master equation. Markovian approaches fare poorly due to the infinite bath correlation time in this model. A recently proposed p…
We present a detailed microscopic derivation for a non-Markovian master equation for a driven two-state system interacting with a general structured reservoir. The master equation is derived using the time-convolutionless projection operator technique in the limit of weak coupling between the two-state quantum system and its environment. We briefly discuss the Markov approximation, the secular approximation and their validity.
Quantum stochastic methods based on effective wave functions form a framework for investigating the generally non-Markovian dynamics of a quantum-mechanical system coupled to a bath. They promise to be computationally superior to the master-equation approach, which is numerically expensive for large dimensions of the Hilbert space. Here, we numerically investigate the suitability of a known stochastic Schrödinger equation that is local in time to give a description of thermal relaxation and energy transport. This stochastic Schrödinger equation can be solved with a moderate numerical cost, ind…
Recursive perturbation approach to time-convolutionless master equations: Explicit construction of generalized Lindblad generators for arbitrary open systems
Università degli Studi di Milano（米兰大学）；INFN, Sezione di Milano（意大利国家核物理研究所米兰分部）；University of Freiburg（弗赖堡大学）；Universität Siegen（锡根大学）；Universitat Autònoma de Barcelona（巴塞罗那自治大学）
We have studied the non-Markovianity of dichotomously driven spin-boson model in the strong coupling regime in both memory kernel and time convolutionless master equation formulations. A strong correlation between the decay time of the environmental correlation function and the non-zero non-Markovianity is found in the absence of the external noise. Stochastic driving is shown to create strong non-Markovianity when the dynamics of the system without driving is Markovian. Also, exact analytical expressions for the trace distance distinguishability and the non-Markovianity were obtained for the …
We derive a time-convolutionless master equation for the spin-boson model in the weak coupling limit. The temporarily negative decay rates in the master equation indicate short time memory effects in the dynamics which is explicitly revealed when the dynamics is studied using the non-Markovian jump description. The approach gives new insight into the memory effects influencing the spin dynamics and demonstrates, how for the spin-boson model the the co-operative action of different channels complicates the detection of memory effects in the dynamics.
The non-Markovian dynamics of a three-level quantum system coupled to a bosonic environment is a difficult problem due to the lack of an exact dynamic equation such as a master equation. We present for the first time an exact quantum trajectory approach to a dissipative three-level model. We have established a convolutionless stochastic Schrödinger equation called time-local quantum state diffusion (QSD) equation without any approximations, in particular, without Markov approximation. Our exact time-local QSD equation opens a new avenue for exploring quantum dynamics for a higher dimensional q…
It is shown that the operator sum representation for non-Markovian dynamics and the Lindblad master equation in Markovian limit can be derived from a formal solution to quantum Liouville equation for a qubit system in the presence of decoherence processes self-consistently. Our formulation is the first principle theory based on projection-operator formalism to obtain an exact reduced density operator in time-convolutionless form starting from the quantum Liouville equation for a noisy quantum computer. The advantage of our approach is that it is general enough to describe a realistic quantum c…
The interrelationship between the non-Markovian stochastic Schrödinger equations and the corresponding non-Markovian master equations is investigated in the finite temperature regimes. We show that the general finite temperature non-Markovian trajectories can be used to derive the corresponding non-Markovian master equations. A simple, yet important solvable example is the well-known damped harmonic oscillator model in which a harmonic oscillator is coupled to a finite temperature reservoir in the rotating wave approximation. The exact convolutionless master equation for the damped harmonic os…
The reduced dynamics of two interacting qubits coupled to two independent bosonic baths is investigated. The one-excitation dynamics is derived and compared with that based on the resolution of appropriate non-Markovian master equations. The Nakajima-Zwanzig and the time-convolutionless projection operator techniques are exploited to provide a description of the non-Markovian features of the dynamics of the two-qubits system. The validity of such approximate methods and their range of validity in correspondence to different choices of the parameters describing the system are brought to light.
We propose a procedure based on symplectic tomography for reconstructing the unknown parameters of a convolutionless non-Markovian Gaussian noisy evolution. Whenever the time-dependent master equation coefficients are given as a function of some unknown time-independent parameters, we show that these parameters can be reconstructed by means of a finite number of tomograms. Two different approaches towards reconstruction, integral and differential, are presented and applied to a benchmark model made of a harmonic oscillator coupled to a bosonic bath. For this model the number of tomograms neede…
The dynamics evolutions of discord and entanglement of two atoms in two independent Lorentzian reservoirs at zero or finite temperature have been investigated by using the time-convolutionless master-equation method. Our results show that, when both the non-Markovian effect and the detuning are present simultaneously, due to the memory and feedback effect of the non-Markovian reservoirs, the discord and the entanglement can be effectively protected even at nonzero temperature by increasing the non-Markovian effect and the detuning. The discord and the entanglement have different robustness for…
We utilize the novel non-Markovian quantum jump (NMQJ) approach to stochastically simulate exciton dynamics derived from a time-convolutionless master equation. For relevant parameters and time scales, the time-dependent, oscillatory decoherence rates can have negative regions, a signature of non-Markovian behavior and of the revival of coherences. This can lead to non-Markovian population beatings for a dimer system at room temperature. We show that strong exciton-phonon coupling to low frequency modes can considerably modify transport properties. We observe increased exciton transport, which…
We propose a systematic scheme to engineer quantum states of a quantum system governed by a time-convolutionless non-Markovian master equation. According to the idea of reverse engineering, the general algebraic equation to determine the control parameters, such as coherent and incoherent control fields, is presented. Without artificially engineering the time-dependent decay rates and retaining the environment-induced Lamb shifts, the quantum state can still be transferred into the target state in a finite period of time along an arbitrary designed trajectory strictly in Hilbert space. As an a…
We apply the time-convolutionless (TCL) projection operator technique to the model of a central spin which is coupled to a spin bath via nonuniform Heisenberg interaction. The second-order results of the TCL method for the coherences and populations of the central spin are determined analytically and compared with numerical simulations of the full von Neumann equation of the total system. The TCL approach is found to yield an excellent approximation in the strong field regime for the description of both the short-time dynamics and the long time behavior.
Exact master equations describing the decay of a two-state system into a structured reservoir are constructed. Employing the exact solution for the model we determine analytical expressions for the memory kernel of the Nakajima-Zwanzig master equation and for the generator of the corresponding time-convolutionless master equation. This approach allows a detailed investigation and comparison of the convergence behavior of the corresponding perturbation expansions. Moreover, we find that the structure of widely used phenomenological master equations with memory kernel may be incompatible with a …
The quantum entropic uncertainty relation and entanglement witness in the two-atom system coupling with the non-Markovian environments are studied by the time-convolutionless master-equation approach. The influence of non-Markovian effect and detuning on the lower bound of the quantum entropic uncertainty relation and entanglement witness is discussed in detail. The results show that, only if the two non-Markovian reservoirs are identical, increasing detuning and non-Markovian effect can reduce the lower bound of the entropic uncertainty relation, lengthen the time region during which the enta…
We show that two, non interacting 2-level systems, immersed in a common bath, can become mutually entangled when evolving according to a Markovian, completely positive reduced dynamics.
The reduced dynamics of a central spin coupled to a bath of N spin-1/2 particles arranged in a spin star configuration is investigated. The exact time evolution of the reduced density operator is derived, and an analytical solution is obtained in the limit of an infinite number of bath spins, where the model shows complete relaxation and partial decoherence. It is demonstrated that the dynamics of the central spin cannot be treated within the Born-Markov approximation. The Nakajima-Zwanzig and the time-convolutionless projection operator technique are applied to the spin star system. The perfo…
We explore the behavior in time of the energy exchange between a system of interest and its environment, together with its relationship to the non-Markovianity of the system dynamics. In order to evaluate the energy exchange we rely on the full counting statistics formalism, which we use to evaluate the first moment of its probability distribution. We focus in particular on the energy backflow from environment to system, to which we associate a suitable condition and quantifier, which enables us to draw a connection with a recently introduced notion of non-Markovianity based on information bac…
Sixth-order time-convolutionless master equation and beyond: Late-time resummations, two types of divergences, and the limits of validity
Duke University（杜克大学）；University of California, Berkeley（加州大学伯克利分校）；University of Central Florida（中佛罗里达大学）；Northwestern University（西北大学）；Georgia Institute of Technology（佐治亚理工学院）
A generalization of the stochastic wave function method to quantum master equations which are not in Lindblad form is developed. The proposed stochastic unravelling is based on a description of the reduced system in a doubled Hilbert space and it is shown, that this method is capable of simulating quantum master equations with negative transition rates. Non-Markovian effects in the reduced systems dynamics can be treated within this approach by employing the time-convolutionless projection operator technique. This ansatz yields a systematic perturbative expansion of the reduced systems dynamic…
The so-called Maryland model is a linear version of the quantum kicked rotor; it exhibits Anderson localization in momentum space. By turning the kicks into a Markovian stochastic process, the dynamics becomes a dissipative quantum process described by a discrete family of completely positive maps that allows to explicitly study the relation between divisibility of the maps and the degree of memory of the process.
We provide the exact analytic solution of the stochastic Schrödinger equation describing an harmonic oscillator interacting with a non-Markovian and dissipative environment. This result represents an arrival point in the study of non-Markovian dynamics via stochastic differential equations. It is also one of the few exactly solvable models, for infinite dimensional systems. We compute the Green's function; in the case of a free particle, and with an exponentially correlated noise, we discuss the evolution of Gaussian wave functions.
In this paper, the exact dynamics of open quantum systems in the presence of initial system-reservoir correlations is investigated for a photonic cavity system coupled to a general non-Markovian reservoir. The exact time-convolutionless master equation incorporating with initial system-reservoir correlations is obtained. The non-Markovian dynamics of the reservoir and the effects of the initial correlations are embedded into the time-dependent coefficients in the master equation. We show that the effects induced by the initial correlations play an important role in the non-Markovian dynamics o…
We investigate the non-Markovian quantum dynamics of a hybrid open system consisting of one qubit and one qutrit by employing a stochastic Schrödinger equation to generate diffusive quantum trajectories. We have established an exact quantum state diffusion (QSD) equation for the dissipative qubit-qutrit system coupled to a bosonic heat bath at zero temperature. As an important application, the non-Markovian QSD equation is employed to simulate the entanglement decay and generation measured by negativity. Finally, some steady state properties of the hybrid system are also discussed.
We study a stochastic Schroedinger equation that generates a family of Gaussian dynamical maps in one dimension permitting a detailed exam of two different definitions of non-Markovianity: one related to the explicit dependence of the generator on the starting time, the other to the non-divisibility of the time-evolution maps. The model shows instances where one has non-Markovianity in both senses and cases when one has Markovianity in the second sense but not in the first one.
Quantum coherence and non-Markovianity of an atom in dissipative cavity under weak measurement are investigated in this work. We find that, the quantum coherence obviously depends on the atomic initial state, the strength of the weak measurement and its reversal, the atom-cavity coupling constant and the non-Markovian effecct. The more obvious the weak measurement effect is, the better the protection of coherence is. The quantum coherence is preserved more efficiently for lager the atom-cavity coupling. The stronger the non-Markovian effect, the more slowly the coherence reduces. This is, the …
We investigate the optimal control problem for non-Markovian open, dissipative quantum system. Optimal control using Pontryagin maximum principle is specifically derived. The influences of Ohmic reservoir with Lorentz-Drude regularization are numerically studied in a two-level system under the following three conditions: ω_0\llω_c, ω_0\approxω_c or ω_0\ggω_c, where ω_0 is the characteristic frequency of the quantum system of interest, and ω_c the cut-off frequency of Ohmic reservoir. The optimal control process shows its remarkable influences on the decoherence dynamics. The temperature is a k…
We evaluate exactly the non-Markovian effect on the decoherence dynamics of a qubit interacting with a dissipative vacuum reservoir and find that the coherence of the qubit can be partially trapped in the steady state when the memory effect of the reservoir is considered. Our analysis shows that it is the formation of a bound state between the qubit and its reservoir that results in this residual coherence in the steady state under the non-Markovian dynamics. A physical condition for the decoherence suppression is given explicitly. Our results suggest a potential way to decoherence control by …
The dynamics of quantum Fisher information (QFI) of the phase parameter in a driven two-state system is studied within the framework of non-Markovian dissipative process. The influences of memory effects, classical driving and detunings on the parameter-estimation precision are demonstrated by exactly solving the Hamiltonian under rotating-wave approximation. In sharp contrast with the results obtained in the presence of Markovian dissipation, we find that classical driving can drastically enhance the QFI, namely, the precision of parameter estimation in the non-Markovian regime. Moreover, the…
The time-convolutionless (TCL) projection operator technique allows a systematic analysis of the non-Markovian quantum dynamics of open systems. We introduce a class of projection superoperators which project the states of the total system onto certain correlated system-environment states. It is shown that the application of the TCL technique to this class of correlated superoperators enables the non-perturbative treatment of the dynamics of system-environment models for which the standard approach fails in any finite order of the coupling strength. We demonstrate further that the correlated s…
An approach based on a non-Markovian time-convolutionless polaron master equation is used to probe the quantum dynamics of a chromophore-qubit in a super-Ohmic bath. Utilizing a measure of non-Markovianity based on dynamical fixed points, we study the effects of the environment temperature and the coupling strength on the non-Markovian behavior of the chromophore in a super-Ohmic bath. It is found that an increase in the temperature results in a reduction in the backflow information from the environment to the chromophore, and therefore, a suppression of non-Markovianity. In the weak coupling …
By use of the two measures presented recently, the indivisibility and the backflow of information, we study the non-Markovianity of the dynamics for a two-level system interacting with a zero-temperature structured environment without using rotating wave approximation (RWA). In the limit of weak coupling between the system and the reservoir, and by expanding the time-convolutionless (TCL) generator to the forth order with respect to the coupling strength, the time-local non-Markovian master equation for the reduced state of the system is derived. Under the secular approximation, the exact anal…
We investigate the geometric phase of a two-level atom (qubit) coupled to a bosonic reservoir with Lorentzian spectral density, and find that for the non-Markovian dynamics in which rotating-wave approximation (RWA) is performed, geometric phase has a $π$-phase jump at the nodal point. However, the exact result without RWA given by hierarchy equation of motion method shows that there is no such a phase jump or nodal structure in geometric phase. Thus our results demonstrate that the counter-rotating terms significantly contribute to the geometric phase in multi-mode Hamiltonian under certain c…
We give the map representing the evolution of a qubit under the action of non-dissipative random external fields. From this map we construct the corresponding master equation that in turn allows us to phenomenologically introduce population damping of the qubit system. We then compare, in this system, the time-regions when non-Markovianity is present on the basis of different criteria both for the non-dissipative and dissipative case. We show that the adopted criteria agree both in the non-dissipative case and in the presence of population damping.
Quantum metrology utilizes quantum effects to reach higher precision measurements of physical quantities compared with their classical counterparts. However the ubiquitous decoherence obstructs its application. Recently, non-Markovian effects are shown to be effective in performing quantum optical metrology under locally dissipative environments\cite{PhysRevLett.123.040402}. However, the mechanism is still rather hazy. Here, we uncover the reason why forming a bound state can protect the quantumness against a dissipative ambient via the quantum Fisher information of entangled coherent states. …
Based on tensor network realizations of path integrals reducing exponential memory scaling to polynomial efficiency and a Liouville space implementation of a time-discrete quantum memory, we investigate a quantum system simultaneously exposed to two structured reservoirs. For this purpose, we employ a numerically exact quasi-2D tensor network combining both diagonal and off-diagonal system-reservoir interactions with a twofold memory for continuous and discrete retardation effects. As a possible example, we study the non-Markovian dynamical interplay between discrete photonic feedback and stru…
We investigate the dynamical information exchange between a two-state system and its environment which is measured by von Neumann entropy. It is found that in the underdamping regime, the entropy dynamics exhibits an extremely non-Markovian oscillation-hump feature, in which oscillations manifest quantum coherence and a hump of envelop demonstrates temporal memory of bath. It indicates that the process of entropy exchange is bidirectional. When the coupling strength increases a certain threshold, the hump along with ripple disappears, which is indicative of the coherent-incoherent dynamical cr…
The dynamics of an open quantum system is usually studied by performing a weak-coupling and weak-correlation expansion in the system-bath interaction. For systems exhibiting strong couplings and highly non-Markovian behavior this approach is not justified. We apply a recently proposed correlated projection superoperator technique to the model of a central spin coupled to a spin bath via full Heisenberg interaction. Analytical solutions to both the Nakajima-Zwanzig and the time-convolutionless master equation are determined and compared with the results of the exact solution. The correlated pro…
We study the geometric phase of a two-level atom coupled to an environment with Lorentzian spectral density. The non-Markovian effect on the geometric phase is explored analytically and numerically. In the weak coupling limit the lowest-order correction to the geometric phase is derived analytically and the general case is calculated numerically. It is found that the correction to the geometric phase is significantly large if the spectral width is small and in this case the non-Markovian dynamics has a significant impact to the geometric phase. When the spectral width increases, the correction…
Non-Markovian master equations describe general open quantum systems when no approximation is made. We provide the exact closed master equation for the class of Gaussian, completely positive, trace preserving, non-Markovian dynamics. This very general result allows to investigate a vast variety of physical systems. We show that the master equation for non-Markovian quantum Brownian motion is a particular case of our general result. Furthermore, we derive the master equation unraveled by a non-Markovian, dissipative stochastic Schrödinger equation, paving the way for the analysis of dissipative…
We explore the dynamics of $N$ coupled atoms to a generic bosonic reservoir under specific system symmetries. In the regime of multiple atoms coupled to a single reservoir with identical couplings, we identify remarkable effects, notably that the initial configuration of the atomic excited state amplitudes strongly impacts the dynamics of the system and can even fully sever the system from its environment. Additionally, we find that steady state amplitudes of the excited states become independent of the choice of the reservoir. The framework introduced is applied to a structured photonic reser…
It has been found that Markovian quantum dissipative processes, described by the Lindblad equation, may have attractive steady-state manifolds, in which dissipation and decoherence can play a positive role to quantum information processing. In this article, we show that such attractive steady-state manifolds with the same positive features as in Markovian dissipative processes can exist in the non-Markovian dissipative processes. Our finding indicates that the dissipation-assisted schemes implemented in the Markovian systems can be directly generalized to the non-Markovian systems.
The time evolution of low energy spin states of a single molecular magnet in a local electric field is investigated. The decoherence of the driven single molecular magnet weakly coupled to a thermal bosonic environment is analyzed by the second-order time-convolutionless non-Markovian master equation. If the characteristic time of the system is much smaller than the correlation time of the environment, the analytical expression of the reduced density matrix of the system is obtained. The non-Markovian dynamics of the spin states at low temperatures is induced by the memory effects in the decay…
