We employ Monte Carlo simulations to investigate the two-time density autocorrelation function for the two-dimensional Coulomb glass. We find that the nonequilibrium relaxation properties of this highly correlated disordered system can be described by a full aging scaling ansatz. The scaling exponents are non-universal, and depend on temperature and charge density.
We discuss the relaxation dynamics of a simple structural glass which has been quenched below its glass transition temperature. We demonstrate that time correlation functions show strong aging effects and investigate in what way the fluctuation dissipation theorem is violated.
This is a Reply to the Comment of Muessel and Rieger cond-mat/9804063 to out paper on ``Aging Effects in a Lennerd-Jones Glass''. We show that the scaling function proposed by Muessel and Rieger does not lead to a satisfactory scaling of our aging data.
We present a detailed study of the scaling behavior of correlations functions and AC susceptibility relaxations in the aging regime in three dimensional spin glasses. The agreement between simulations and experiments is excellent confirming the validity of the full aging scenario with logarithmic corrections which manifests as weak sub-aging effects.
In a recent letter [PRL 78 (1997) 4581] Kob and Barrat reported results of their molecular dynamics simulation of the non-equilibrium dynamics of a binary Lennard-Jones glass. They propose an aging scenario in this system that is close to a t/t_w scaling behavior. In this comment we present new results and show that a different aging scenario, known under the name activated dynamics scaling [i.e. log((t+t_w)/tau)/log(t_w/tau)], describes the aging regime of this kind of glassy systems much better.
We extend the standard droplet scaling theory for isothermal aging in spin glasses assuming that the effective stiffness constant of droplets as large as extended defects is vanishingly small. A novel dynamical order parameter and the associated dynamical susceptibility emerge. Breaking of the fluctuation dissipation theorem takes place at the dynamical order parameter well below the equilibrium Edwards-Anderson order parameter at which the time translational invariance is strongly broken. The scenario is examined numerically in a 4 dimensional EA Ising spin glass model.
We employ Monte Carlo simulations to study the relaxation properties of the two-dimensional Coulomb glass in disordered semiconductors and the three-dimensional Bose glass in type-II superconductors in the presence of extended linear defects. We investigate the effects of adding non-zero random on-site energies from different distributions on the properties of the correlation-induced Coulomb gap in the density of states (DOS) and on the non-equilibrium aging kinetics highlighted by the density autocorrelation functions. We also probe the sensitivity of the system's equilibrium and non-equilibr…
We study the non-equilibrium aging behavior of the gauge glass model in three dimensions at the critical temperature. We perform Monte Carlo simulations with a Metropolis update, and correlation and response functions are calculated for different waiting times. We obtain a multiplicative aging scaling of the correlation and response functions, calculating the aging exponent $b$ and the nonequilibrium autocorrelation decay exponent $λ_c/z_c$. We also analyze the fluctuation-dissipation relationship at the critical temperature, obtaining the critical fluctuation-dissipation ratio $X_\infty$. By …
Using molecular dynamics simulations we study the out of equilibrium dynamic correlations in a model glass-forming liquid. The system is quenched from a high temperature to a temperature below its glass transition temperature and the decay of the two-time intermediate scattering function C(t_w,t+t_w) is monitored for several values of the waiting time t_w after the quench. We find that C(t_w,t+t_w) shows a strong dependence on the waiting time, i.e. aging, depends on the temperature before the quench and, similar to the case of spin glasses, can be scaled onto a master curve.
We review the field of the glass transition, glassy dynamics and aging from a statistical mechanics perspective. We give a brief introduction to the subject and explain the main phenomenology encountered in glassy systems, with a particular emphasis on spatially heterogeneous dynamics. We review the main theoretical approaches currently available to account for these glassy phenomena, including recent developments regarding mean-field theory of liquids and glasses, novel computational tools, and connections to the jamming transition. Finally, the physics of aging and off-equilibrium dynamics e…
The deviations from full or pure aging behavior, i.e. perfect $t/t_w$ scaling of the correlation and response functions of aging glassy systems, are not well understood theoretically. Recent experiments of Rodriguez et al. (Phys. Rev. Lett. 91, 037203 (2003)) have shown that full aging applies to the thermoremanent magnetization in the limit of infinite cooling rate during the initial quench. In numerical models, instantaneous thermal quenches can be--and usually are--applied. This has motivated the present numerical investigations of the aging behavior of Edwards-Anderson Ising spin glass mod…
We study the aging dynamics in a model for dense simple liquids, in which particles interact through a hard-core repulsion complemented by a short-ranged attractive potential, of the kind found in colloidal suspensions. In this system, at large packing fractions, kinetically arrested disordered states can be created both on cooling (attractive glass) and on heating (repulsive glass). The possibility of having two distinct glasses, at the same packing fraction, with two different dynamics offers the unique possibility of comparing -- within the same model -- the differences in aging dynamics. W…
We consider a simple model of a structural glass, represented by a lattice gas with kinetic constraints in contact with a particle reservoir. Quench below the glass transition is represented by the jump of the chemical potential above a threshold. After a quench, the density approaches the critical density-where the diffusion coefficient of the particles vanishes-following a power law in time. In this regime, the two-time self-correlation functions exhibit aging. The behavior of the model can be understood in terms of simple mean-field arguments.
A generalized version of the nonequilibrium linear Glauber model with $q$ states in $d$ dimensions is introduced and analyzed. The model is fully symmetric, its dynamics being invariant under all permutations of the $q$ states. Exact expressions for the two-time autocorrelation and response functions on a $d$-dimensional lattice are obtained. In the stationary regime, the fluctuation-dissipation theorem holds, while in the transient the aging is observed with the fluctuation-dissipation ratio leading to the value predicted for the linear Glauber model.
We study the non-equilibrium dynamics of the spherical p-spin models in the scaling regime near the plateau and derive the corresponding scaling functions for the correlators. Our main result is that the matching between different time regimes fixes the aging function in the aging regime to $h(t)=\exp(t^{1-μ})$. The exponent $μ$ is related to the one giving the length of the plateau. Interestingly $1-μ$ is quickly very small when one goes away from the dynamic transition temperature in the glassy phase. This gives new light on the interpretation of experiments and simulations where simple agin…
We numerically study the non-equilibrium dynamics of the three dimensional Heisenberg Edwards-Anderson spin glass following a sudden quench to its low temperature phase. The subsequent aging behavior of the system is analyzed in detail, and the scaling behavior of various space-time correlation functions is investigated for both spin and chiral degrees of freedom. We carefully compare our results with those obtained from simulations of the more studied Ising version of the model, and with experiments on real spin glasses in which the spins have vectorial character. Finally, the present dynamic…
Using Monte Carlo simulations, we have studied the relaxation of energy of the three-dimensional Ising spin-glass model in aging process. Our finite-size-scaling analysis on the isothermal energy decay after the quench suggests strongly that the energy relaxes by coarsening of domain walls in agreement with the droplet theory. We have also evaluated relaxation times required for spin configurations in small systems, which are regarded as isolated droplets, to flip globally. The results support the fundamental assumption of the droplet theory that coarsening of domain walls, in case of spin gla…
We show that the dynamical behavior of the 3D Ising spin glass with Gaussian couplings is not compatible with a droplet dynamics. We show that this is implied from the data of reference cond-mat/9904143, that, when analyzed in an accurate way, give multiple evidences of this fact. Our study is based on the analysis of the overlap-overlap correlation function, at different values of the separation r and of the time t.
We measure the fluctuations of the position of a silica bead trapped by an optical tweezers during the aging of a Laponite suspension. We find that the effective temperature is equal to the bath temperature.
Aging phenomena of short-range Ising spin glass models have been investigated using Monte Carlo simulations. It is found that in the low-temperature spin-glass phase the mean domain size exhibits a crossover from a power-law growth associated with the critical fluctuation at the transition temperature to slower growth inherent in the low-temperature phase. The temperature dependence of the growth law of the domain size can be almost explained by this crossover. We also find that the spin-autocorrelation function in the quasi-equilibrium regime follows the expected scaling behavior from the dro…
Motivated by the mean field prediction of a Gardner phase transition between a "normal glass" and a "marginally stable glass", we investigate the off-equilibrium dynamics of three-dimensional polydisperse hard spheres, used as a model for colloidal or granular glasses. Deep inside the glass phase, we find that a sharp crossover pressure $P_{\rm G}$ separates two distinct dynamical regimes. For pressure $P < P_{\rm G}$, the glass behaves as a normal solid, displaying fast dynamics that quickly equilibrates within the glass free energy basin. For $P>P_{\rm G}$, instead, the dynamics becomes stro…
Using RG we investigate the non-equilibrium relaxation of the (Cardy-Ostlund) 2D random Sine-Gordon model, which describes pinned arrays of lines. Its statics exhibits a marginal ($θ=0$) glass phase for $T<T_g$ described by a line of fixed points. We obtain the universal scaling functions for two-time dynamical response and correlations near $T_g$ for various initial conditions, as well as the autocorrelation exponent. The fluctuation dissipation ratio is found to be non-trivial and continuously dependent on $T$.
The critical behavior of the gauge-glass and the XY spin-glass models in three dimensions is studied by analyzing their nonequilibrium aging dynamics. A new numerical method, which relies on the calculation of the two-time correlation and integrated response functions, is used to determine both the critical temperature and the nonequilibrium scaling exponents, both for spin and chiral degrees of freedom. First, the ferromagnetic XY model is studied to validate this nonequilibirum aging method (NAM), since for this nondisordered system we can compare with known results obtained with standard eq…
By using extensive Molecular Dynamics simulations, we have determined the violation of the fluctuation-dissipation theorem in a Lennard-Jones liquid quenched to low temperatures. For this we have calculated $X(C)$, the ratio between a one particle time-correlation function $C$ and the associated response function. Our results are best fitted by assuming that $X(C)$ is a discontinuous, piecewise constant function. This is similar to what is found in spin systems with one step replica symmetry breaking. This strengthen the conjecture of a similarity between the phase space structure of structura…
Pinning particles at random in supercooled liquids is a promising route to make substantial progress on the glass transition problem. Here we develop a mean-field theory by studying the equilibrium and non-equilibrium dynamics of the spherical p-spin model in presence of a fraction c of pinned spins. Our study shows the existence of two dynamic critical lines: one corresponding to usual Mode Coupling transitions and the other one to dynamic spinodal transitions. Quenches in the portion of the c - T phase diagram delimited by those two lines leads to aging. By extending our results to finite di…
We construct the equations for the growth kinetics of an aging structural glass within mode-coupling theory through a non-stationary variant of the 3-density correlator defined in Phys. Rev. Lett. {\bf 97}, 195701 (2006). We solve a schematic form of the resulting equations to obtain the coarsening of the dynamic heterogeneity, characterized via the 3-point correlator $χ_3(t,t_w)$, as a function of waiting time $t_w$. For a quench into the glass, we find that $χ_3$ attains a peak value $\sim t_w^{0.5}$ at $t -t_w \sim t_w^{0.8}$, providing a theoretical basis for the numerical observations of …
In this paper we present a short survey on the concept of effective temperature, on its onset as a glass former vitrifies, on the various definitions in literature and their limits of applicability. An exactly solvable model glass is employed to compare effective temperatures among them and to set a criterion for the occurrence of a universal extra temperature in the framework of a "two temperature thermodynamics" for off-equilibrium aging systems. It will be shown that aging in glass formers is not a sufficient requirement. As an instance, memory effects typical of glasses are not compatible …
Aging in kinetics of three different phase transitions, viz., magnetic, binary solid and single component fluid, have been studied via Monte Carlo and molecular dynamics simulations in three space dimensions with the objective of identifying the effects of order-parameter conservation and hydrodynamics. We observe that the relevant autocorrelations exhibit power-law decay in ferromagnet and binary solid but with different exponents. At early time fluid autocorrelation function nicely follows that of binary solid, the order parameter being conserved for both of them, as opposed to a ferromagnet…
We provide a direct experimental test of the Stokes-Einstein relation as a special case of the fluctuation-dissipation theorem (FDT) in an aging colloidal glass. The use of combined active and passive microrheology allows us to independently measure both the correlation and response functions in this non-equilibrium situation. Contrary to previous reports, we find no deviations from the FDT over several decades in frequency (1 Hz-10 kHz) and for all aging times. In addition, we find two distinct viscoelastic contributions in the aging glass, including a nearly elastic response at low frequenci…
Via Monte Carlo simulations we study nonequilibrium dynamics in the nearest-neighbor Ising model, following quenches to points inside the ordered region of the phase diagram. With the broad objective of quantifying the nonequilibrium universality classes corresponding to spatially correlated and uncorrelated initial configurations, in this paper we present results for the decay of the order-parameter autocorrelation function for quenches from the critical point. This autocorrelation is an important probe for the aging dynamics in far-from-equilibrium systems and typically exhibits power-law sc…
Recent experiments and simulations have revealed glassy features in the cytoplasm, living tissues as well as dense assemblies of self propelled colloids. This leads to a fundamental question: how do these non-equilibrium (active) amorphous materials differ from conventional passive glasses, created either by lowering temperature or by increasing density? To address this we investigate the aging behaviour after a quench to an almost arrested state of a model active glass former, a Kob-Andersen glass in two dimensions. Each constituent particle is driven by a constant propulsion force whose dire…
We show numerically that a three-dimensional model for structural glass displays aging, rejuvenation and memory effects when submitted to a temperature cycle. These effects indicate that the free energy landscape of structural glasses may possess the complex hierarchical structure that characterize materials such as spin and polymer glasses. We use the theoretical concept of marginal stability to interpret our results, and explain in which physical conditions a complex aging dynamics can emerge in dense supercooled liquids, paving the way for future experimental studies of complex aging dynami…
We report a molecular dynamics simulation study of the properties of the potential energy landscape sampled by a system of water molecules during the process of generating a glass by cooling, and during the process of regenerating the equilibrium liquid by heating the glass. We study the dependence of these processes on the cooling/heating rates as well as on the role of aging (the time elapsed in the glass state). We compare the properties of the potential energy landscape sampled during these processes with the corresponding properties sampled in the liquid equilibrium state to elucidate und…
We present a direct experimental measurement of an effective temperature in a colloidal glass of Laponite, using a micrometric bead as a thermometer. The nonequilibrium fluctuation-dissipation relation, in the particular form of a modified Einstein relation, is investigated with diffusion and mobility measurements of the bead embedded in the glass. We observe an unusual non-monotonic behavior of the effective temperature : starting from the bath temperature, it is found to increase up to a maximum value, and then decreases back, as the system ages. We show that the observed deviation from the …
The relaxation dynamics of many disordered systems, such as structural glasses, proteins, granular materials or spin glasses, is not completely frozen even at very low temperatures. This residual motion leads to a change of the properties of the material, a process commonly called aging. Despite recent advances in the theoretical description of such aging processes, the microscopic mechanisms leading to the aging dynamics are still a matter of dispute. In this Letter we investigate the aging dynamics of a simple glass former by means of molecular dynamics computer simulation. Using the concept…
Linear response functions of aging systems are routinely interpreted using the scaling variable $t_{\rm obs}/t_{\rm w}^μ$,where $t_{\rm w}$ is the time at which the field conjugated to the response is turned on or off, and where $t_{\rm obs}$ is the `observation' time elapsed from the field change. The response curve obtained for different values of $t_w$ are usually collapsed using values of $μ$ slightly below one, a scaling behavior generally known as \emph{sub-aging}. Recent spin glass Thermoremanent Magnetization experiments have shown that the value of $μ$ is strongly affected by the form…
We introduce a simple two-dimensional spin model with short-range interactions which shows glassy behavior despite a Hamiltonian which is completely homogeneous and possesses no randomness. We solve exactly for both the static partition function of the model and the distribution of energy barriers, giving us the equilibration time-scales at low temperature. Simulations of instantaneous quenches and of annealing of the model are in good agreement with the analytic calculations. We also measure the two-time spin correlation as a function of waiting time, and show that the model has aging behavio…
We go over our finding that the dynamics at the noise-perturbed edge of chaos in logistic maps is comparable to that observed in supercooled liquids close to vitrification. That is, the three major features of glassy dynamics in structural glass formers, two-step relaxation, aging, and a relationship between relaxation time and configurational entropy, are displayed by orbits with vanishing Lyapunov exponent. The known properties in control-parameter space of the noise-induced bifurcation gap play a central role in determining the characteristics of dynamical relaxation at the chaos threshold.…
Colloidal dispersions of Laponite platelets are known to age slowly from viscous sols to colloidal glasses. We follow this aging process by monitoring the diffusion of probe particles embedded in the sample via dynamic light scattering. Our results show that the time-dependent diffusion of the probe particles scales with their size. This implies that the fluctuation-dissipation theorem can be generalized for this out-of-equilibrium system by replacing the bath temperature with an effective temperature. Simultaneous dynamic rheological measurements reveal that this effective temperature increas…
Molecular dynamics computer simulations of a binary Lennard-Jones glass under shear are presented. The mechanical response of glassy states having different thermal histories is investigated by imposing a wide range of external shear rates, at different temperatures. The stress-strain relations exhibit an overshoot at a strain of around 0.1, marking the yielding of the glass sample and the onset of plastic flow. The amplitude of the overshoot shows a logarithmic behavior with respect to a dimensionless variable, given by the age of the sample times the shear rate. Dynamical heterogeneities hav…
We present evidence in favor of the possibility of treating an out-of-equilibrium supercooled simple liquid as a system in quasi-equilibrium. Two different temperatures, one controlled by the external bath and one internally selected by the system characterize the quasi-equilibrium state. The value of the internal temperature is explicitly calculated within the inherent structure thermodynamic formalism. We find that the internal temperature controls the relation between the response to an external perturbation and the long-time decay of fluctuations in the liquid.
We consider time-dependent Lifshitz-type solutions in type IIB supergravity. The solutions describe a time evolution from Lifshitz spacetimes to AdS spaces. We argue the holographic relation of them to aging phenomena in condensed matter physics. The solutions have no time-translation invariance and possess the dynamical scaling symmetry with z_c=2. In addition, the time evolution corresponds to slow (nonexponential) dynamics from nonequilibrium states to the equilibrium. We also discuss a mechanism of quantum quench to generate nonequilibrium states.
