We study the quantum phase transitions of a model that describes the interconversion of interacting bosonic atoms and molecules. Using a classical analysis, we identify a threshold coupling line separating a molecular phase and a mixed phase. Through studies of the energy gap, von Neumann entanglement entropy, and fidelity, we give evidence that this line is associated to a boundary line in the ground-state phase diagram of the quantum system.
We study the scattering of a matter-wave from an interacting system of bosons in an optical lattice, focusing on the strong-interaction regime. Analytical expressions for the many-body scattering cross section are derived from a strong-coupling expansion and a site-decoupling mean-field approximation, and compared to numerically obtained exact results. In the thermodynamic limit, we find a non-vanishing inelastic cross section throughout the Mott insulating regime, which decays quadratically as a function of the boson-boson interaction.
We convert a strongly interacting ultracold Bose gas into a mixture of atoms and molecules by sweeping the interactions from resonant to weak. By analyzing the decay dynamics of the molecular gas, we show that in addition to Feshbach dimers it contains Efimov trimers. Typically around 8\% of the total atomic population is bound into trimers, identified by their density-independent lifetime of about 100~$μ$s. The lifetime of the Feshbach dimers shows a density dependence due to inelastic atom-dimer collisions, in agreement with theoretical calculations. We also vary the density of the gas acros…
We reveal the existence of polarizing quantum phases for the enantiomers of cold, interacting chiral molecules in an optical helicity lattice by means of an extended Bose-Hubbard model. These recently proposed lattices have sites with alternating helicity which exert a discriminatory force on chiral molecules with different handedness. In our study of the phase diagram we find that a strong dipolar repulsion between molecules results in the separation of left and right enantiomers.
We study the scattering of matter-waves from interacting bosons in a one-dimensional optical lattice, described by the Bose-Hubbard Hamiltonian. We derive analytically a formula for the inelastic cross section as a function of the atomic interaction in the lattice, employing Bogoliubov's formalism for small condensate depletion. A linear decay of the inelastic cross section for weak interaction, independent of number of particles, condensate depletion and system size, is found.
We compute the pair entanglement between two interacting bosons in a two dimensional (2D)isotropic harmonic trap. The interaction potential is modeled by a 2D regularized pseudo-potential. By analytically decomposing the wave function into the single particle basis, we show the dependency of the pair entanglement on the scattering length. Our results turn out to be in good agreements with earlier results using a quasi-2D geometry.
We study theoretically quantum dynamics of interacting bosons in artificial magnetic fields as engineered in recent ultracold atomic experiments, where quantum cyclotron orbital motion has been observed. With exact numerical simulations and perturbative analyses, we find that interactions induce damping in the cyclotron motion. The damping time is found to be dependent on interaction and tunneling strengths monotonically, while its dependence on magnetic flux is non-monotonic. Sufficiently strong interactions would render bosons dynamically localized inhibiting the cyclotron motion. The dampin…
We show that multichannel interactions significantly alter the phase diagram of ultracold bosonic molecules in an optical lattice. Most prominently, an unusual fluid region intervenes between the conventional superfluid and the Mott insulator. In it, number fluctuations remain but phase coherence is suppressed by a significant factor. This factor can be made arbitrarily large, at least in a two-site configuration. We calculate the phase diagram using complementary methods, including Gutzwiller mean-field and density matrix renormalization group (DMRG) calculations. Although we focus on bosonic…
This paper reviews recent advances in the study of strongly interacting systems of dipolar molecules. Heteronuclear molecules feature large and tunable electric dipole moments, which give rise to long-range and anisotropic dipole-dipole interactions. Ultracold samples of dipolar molecules with long-range interactions offer a unique platform for quantum simulations and the study of correlated many-body physics. We provide an introduction to the physics of dipolar quantum gases, both electric and magnetic, and summarize the multipronged efforts to bring dipolar molecules into the quantum regime.…
We report the creation of ultracold bosonic dipolar $^{23}\textrm{Na}^{39}\textrm{K}$ molecules in their absolute rovibrational ground state. Starting from weakly bound molecules immersed in an ultracold atomic mixture, we coherently transfer the dimers to the rovibrational ground state using an adiabatic Raman passage. We analyze the two-body decay in a pure molecular sample and in molecule-atom mixtures and find an unexpectedly low two-body decay coefficient for collisions between molecules and $^{39}\textrm{K}$ atoms in a selected hyperfine state. The preparation of bosonic $^{23}\textrm{Na…
We develop a diagrammatic scattering theory for interacting bosons in a three-dimensional, weakly disordered potential. We show how collisional energy transfer between the bosons induces the thermalization of the inelastic single-particle current which, after only few collision events, dominates over the elastic contribution described by the Gross-Pitaevskii ansatz.
We study ground states and elementary excitations of a system of bosonic atoms and diatomic Feshbach molecules trapped in a one-dimensional optical lattice using exact diagonalization and variational Monte Carlo methods. We primarily study the case of an average filling of one boson per site. In agreement with bosonization theory, we show that the ground state of the system in the thermodynamic limit corresponds to the Pfaffian-like state when the system is tuned towards the superfluid-to-Mott insulator quantum phase transition. Our study clarifies the possibility of the creation of exotic Pfa…
The quantum kicked rotor is well-known to display dynamical localization in the non-interacting limit. In the interacting case, while the mean-field (Gross-Pitaevskii) approximation displays a destruction of dynamical localization, its fate remains debated beyond mean-field. Here we study the kicked Lieb-Liniger model in the few-body limit. We show that for any interaction strength, two kicked interacting bosons always dynamically localize, in the sense that the energy of the system saturates at long time. However, contrary to the non-interacting limit, the momentum distribution $Π(k)$ of the …
We demonstrate a generally applicable technique for mixing two-species quantum degenerate bosonic samples in the presence of an optical lattice, and we employ it to produce low-entropy samples of ultracold 87Rb133Cs Feshbach molecules with a lattice filling fraction exceeding 30%. Starting from two spatially separated Bose-Einstein condensates of Rb and Cs atoms, Rb-Cs atom pairs are efficiently produced by using the superfluid-to-Mott insulator quantum phase transition twice, first for the Cs sample, then for the Rb sample, after nulling the Rb-Cs interaction at a Feshbach resonance's zero cr…
We investigate the properties of two interacting ultracold polar molecules described as distinguishable quantum rigid rotors, trapped in a one-dimensional harmonic potential. The molecules interact via a multichannel two-body contact potential, incorporating the short-range anisotropy of intermolecular interactions including dipole-dipole interaction. The impact of external electric and magnetic fields resulting in Stark and Zeeman shifts of molecular rovibrational states is also investigated. Energy spectra and eigenstates are calculated by means of the exact diagonalization. The importance a…
We consider a simple quantum model of atom-molecule conversion where bosonic atoms can combine into diatomic molecules and vice versa. The many-particle system can be expressed in terms of the generators a deformed $SU(2)$ algebra, and the mean-field dynamics takes place on a deformed version of the Bloch sphere, a teardrop shaped surface with a cusp singularity. We analyse the mean-field and many-particle correspondence, which shows typical features of quantum-classical correspondence. We demonstrate that semiclassical methods can be employed to recover full many-particle features from the me…
The study of topological effects in physics is a hot area, and only recently researchers were able to address the important issues of topological properties of interacting quantum systems. But it is still a great challenge to describe multi-particle and interaction effects. Here, we introduce multi-particle Wannier states for interacting systems with co-translational symmetry. We reveal how the shift of multi-particle Wannier state relates to the multi-particle Chern number, and study the two-boson Thouless pumping in an interacting Rice-Mele model. In addition to the bound-state Thouless pump…
We present a mathematically rigorous analysis of the superfluid properties of a Bose-Einstein condensate in the many-body ground state of a one-dimensional model of interacting bosons in a random potential.
A theoretical study of interacting bosons in a periodic optical lattice is presented. Instead of the commonly used tight-binding approach (applicable near the Mott insulating regime of the phase diagram), the present work starts from the exact single-particle states of bosons in a cubic optical lattice, satisfying the Mathieu equation, an approach that can be particularly useful at large boson fillings. The effects of short-range interactions are incorporated using a self-consistent Hartree-Fock approximation, and predictions for experimental observables such as the superfluid transition tempe…
We show that tunneling and localization properties of interacting ultracold atoms in an optical lattice can be controlled by adiabatically turning on a fast oscillatory force even in the presence of disorder. Our calculations are based on the exact solution of the time-dependent Schroedinger equation, using the Floquet formalism. Implications of our findings for larger systems and the possibility of controlling the phase diagram of disordered-interacting bosonic systems are discussed.
We review the infrared behavior of interacting bosons at zero temperature. After a brief discussion of the Bogoliubov approximation and the breakdown of perturbation theory due to infrared divergences, we show how the non-perturbative renormalization group enables to obtain the exact infrared behavior of the correlation functions.
We investigate the condensate wave function and elementary excitations of strongly interacting bosonic polar molecules in a harmonic trap, treating the scattering amplitude beyond the standard first Born approximation (FBA). By using an appropriate trial wave function in the variational method, effects of the leading order correction beyond the FBA have been investigated and shown to be significantly enhanced when the system is close to the phase boundary of collapse. How such leading order effect of going beyond the FBA can be observed in a realistic experiment is also discussed.
Motivated by recent advance in orbitally tuned Feshbach resonance experiments, we analyze the ground-state phase diagram and related low-energy excitation spectra of a d-wave interacting Bose gas. A two-channel model with d-wave symmetric interactions and background s-wave interactions is adopted to characterize the gas. The ground state is found to show three interesting phases: atomic, molecular, and atomic-molecular superfluidity. Remarkably differently from what was previously known in the p-wave case, the atomic superfluid is found to be momentum-independent in the present d-wave case. Bo…
We study the properties of dilute bosons immersed in a single component Fermi sea across a broad boson-fermion Feshbach resonance. The stability of the mixture requires that the bare interaction between bosons exceeds a critical value, which is a universal function of the boson-fermion scattering length, and exhibits a maximum in the unitary region. We calculate the quantum depletion, momentum distribution and the boson contact parameter across the resonance. The transition from condensate to molecular Fermi gas is also discussed.
A weakly interacting Bose gas on a simple cubic lattice is considered. We prove the existence of the standard or zero-mode Bose condensation at sufficiently low temperature. This result is valid for sufficiently small interaction potential and small values of chemical potential. Our method exploits infrared bound for the suitable two-point Bogolyubov's inner product. We do not use the reflection positivity or some expansion methods.
We theoretically investigate the magnetic properties and nonequilibrium dynamics of two interacting ultracold polar and paramagnetic molecules in a one-dimensional harmonic trap in external electric and magnetic fields. The molecules interact via a multichannel two-body contact potential, incorporating the short-range anisotropy of intermolecular interactions. We show that various magnetization states arise from the interplay of the molecular interactions, electronic spins, dipole moments, rotational structures, external fields, and spin-rotation coupling. The rich magnetization diagrams depen…
We study persistent currents for interacting one-dimensional bosons on a tight ring trap, subjected to a rotating barrier potential, which induces an artificial U(1) gauge field. We show that, at intermediate interactions, the persistent current response is maximal, due to a subtle interplay of effects due to the barrier, the interaction and quantum fluctuations. These results are relevant for ongoing experiments with ultracold atomic gases on mesoscopic rings.
We investigate quantum phase transitions occurring in a system of strongly interacting ultracold bosons in a 1D optical lattice. After discussing the commensurate-incommensurate transition, we focus on the phases appearing at incommensurate filling. We find a rich phase diagram, with superfluid, supersolid and solid (kink-lattice) phases. Supersolids generally appear in theoretical studies of systems with long-range interactions; our results break this paradigm and show that they may also emerge in models including only short-range (contact) interactions, provided that quantum fluctuations are…
We spectroscopically investigate a pathway for the conversion of $^{23}\textrm{Na}^{39}\textrm{K}$ Feshbach molecules into rovibronic ground state molecules via STImulated Raman Adiabatic Passage (STIRAP). Using photoassociation spectroscopy from the diatomic scattering threshold in the $a^3Σ^+$ potential, we locate the resonantly mixed electronically excited intermediate states $|B^1Π, v=8\rangle$ and $|c^3Σ^+, v=30\rangle$ which, due to their singlet-triplet admixture, serve as an ideal bridge between predominantly $a^3Σ^+$ Feshbach molecules and pure $X^1Σ^+$ ground state molecules. We inve…
Superpositions of rotational states in polar molecules induce strong, long-range dipolar interactions. Here we extend the rotational coherence by nearly one order of magnitude to 8.7(6) ms in a dilute gas of polar $^{23}$Na$^{40}$K molecules in an optical trap. We demonstrate spin-decoupled magic trapping, which cancels first-order and reduces second-order differential light shifts. The latter is achieved with a dc electric field that decouples nuclear spin, rotation and trapping light field. We observe density-dependent coherence times, which can be explained by dipolar interactions in the bu…
We study the ground-state physics of a single-component Haldane model on a hexagonal two-leg ladder geometry with a particular focus on strongly interacting bosonic particles. We concentrate our analysis on the regime of less than one particle per unit-cell. As a main result, we observe several Meissner-like and vortex-fluid phases both for a superfluid as well as a Mott-insulating background. Furthermore, we show that for strongly interacting bosonic particles an unconventional vortex-lattice phase emerges, which is stable even in the regime of hardcore bosons. We discuss the mechanism for it…
We probe photo-induced loss for chemically stable bosonic $^{23}$Na$^{87}$Rb and $^{23}$Na$^{39}$K molecules in chopped optical dipole traps where the molecules spend a significant time in the dark. We expect the effective two-body decay to be largely suppressed in chopped traps due to the small expected complex lifetimes of about $13μ$s and $6μ$s for $^{23}$Na$^{87}$Rb and $^{23}$Na$^{39}$K respectively. However, instead we do observe near-universal loss even at the lowest chopping frequencies we can probe. Our data thus either suggest a so far unknown loss mechanism or a drastic underestimat…
The success of Gross--Pitevskii and Bogoliubov theories in the description of large systems of interacting bosons led to a substantial effort into rigorously deriving these effective theories. In this work we shall review the related existing literature in the context of dynamics of large bosonic systems.
We develop a new method that allows us to map models of interacting fermions onto bosonic models describing collective excitations in an arbitrary dimension. This mapping becomes exact in the thermodynamic continuous time limit. The boson models can be written either in the form of a model of non-interacting bosons in a fluctuating auxiliary field or in the form of a superfield theory of interacting bosons. We show how one can study the latter version using perturbation theory. Using the developed diagrammatic technique we compared the first two orders of perturbation theory with the correspon…
We theoretically investigate the properties of highly polar diatomic molecules containing $^2S$-state transition-metal atoms. We calculate potential energy curves, permanent electric dipole moments, spectroscopic constants, and leading long-range dispersion-interaction coefficients for molecules consisting of either a Cu or Ag atom interacting with an alkali-metal (Li, Na, K, Rb, Cs, Fr) or alkaline-earth-metal (Be, Mg, Ca, Sr, Ba, Ra) atom. We use ab initio electronic structure methods, such as the coupled cluster and configuration interaction ones, with large Gaussian basis sets and small-co…
An understanding of the possible ways in which interactions can produce fundamentally new emergent many-body states is a central problem of condensed matter physics. We ask if a Fermi sea can arise in a system of bosons subject to contact interaction. Based on exact diagonalization studies and variational wave functions, we predict that such a state is likely to occur when a system of two-component bosons in two dimensions, interacting via a species independent contact interaction, is exposed to a synthetic magnetic field of strength that corresponds to a filling factor of unity. The fermions …
Interacting bosons generically form a superfluid state. In the presence of disorder it can get converted into a compressible Bose glass state. Here we study such transition in one dimension at moderate interaction using bosonization and renormalization group techniques. We derive the two-loop scaling equations and discuss the phase diagram. We find that the correlation functions at the transition are characterized by universal exponents in a finite region around the fixed point.
We provide an account of the static and dynamic properties of hard-core bosons in a one-dimensional lattice subject to a multi-chromatic quasiperiodic potential for which the single-particle spectrum has mobility edges. We use the mapping from strongly interacting bosons to weakly interacting fermions, and provide exact numerical results for hard-core bosons in and out of equilibrium. In equilibrium, we find that the system behaves like a quasi-condensate (insulator) depending on whether the Fermi surface of the corresponding fermionic system lies in a spectral region where the single-particle…
Understanding the behavior of molecules interacting with superfluid helium represents a formidable challenge and, in general, requires approaches relying on large-scale numerical simulations. Here we demonstrate that experimental data collected over the last 20 years provide evidence that molecules immersed in superfluid helium form recently-predicted angulon quasiparticles [Phys. Rev. Lett. 114, 203001 (2015)]. Most importantly, casting the many-body problem in terms of angulons amounts to a drastic simplification and yields effective molecular moments of inertia as straightforward analytic s…
We investigate the low energy excitation spectrum of a Bose gas with weak, long range repulsive interactions. In particular, we prove that the Bogoliubov spectrum of elementary excitations with linear dispersion relation for small momentum becomes exact in the mean-field limit.
We consider a system of $N$ bosons in the mean-field scaling regime for a class of interactions including the repulsive Coulomb potential. We derive an asymptotic expansion of the low-energy eigenstates and the corresponding energies, which provides corrections to Bogoliubov theory to any order in $1/N$.
We investigate the low-energy excitation spectrum of a Bose gas confined in a trap, with weak long-range repulsive interactions. In particular, we prove that the spectrum can be described in terms of the eigenvalues of an effective one-particle operator, as predicted by the Bogoliubov approximation.
