We establish a theoretical correspondence between spin-one antiferromagnetic spinor condensates in an external magnetic field and quantum rotor models in an external potential. We show that the rotor model provides a conceptually clear picture of the possible phases and dynamical regimes of the antiferromagnetic condensate. We also show that this mapping simplifies calculations of the condensate's spectrum and wavefunctions. We use the rotor mapping to describe the different dynamical regimes recently observed in $^{23}$Na condensates. We also suggest a way to experimentally observe quantum mechanical effects (collapse and revival) in spinor condensates.
In this work, we theoretically construct exact mappings of many-particle bosonic systems onto quantum rotor models. In particular, we analyze the rotor representation of spinor Bose-Einstein condensates. In a previous work it was shown that there is an exact mapping of a spin-one condensate of fixed particle number with quadratic Zeeman interaction onto a quantum rotor model. Since the rotor model has an unbounded spectrum from above, it has many more eigenstates than the original bosonic model. Here we show that for each subset of states with fixed spin F_z, the physical rotor eigenstates are…
We report on the observation of half-quantum vortices (HQVs) in the easy-plane polar phase of an antiferromagnetic spinor Bose-Einstein condensate. Using in situ magnetization-sensitive imaging, we observe that pairs of HQVs with opposite core magnetization are generated when singly charged quantum vortices are injected into the condensate. The dynamics of HQV pair formation is characterized by measuring the temporal evolutions of the pair separation distance and the core magnetization, which reveals the short-range nature of the repulsive interactions between the HQVs. We find that spin fluct…
We experimentally demonstrate that spin dynamics and the phase diagram of spinor condensates can be conveniently tuned by a two-dimensional optical lattice. Spin population oscillations and a lattice-tuned separatrix in phase space are observed in every lattice where a substantial superfluid fraction exists. In a sufficiently deep lattice, we observe a phase transition from a longitudinal polar phase to a broken-axisymmetry phase in steady states of lattice-confined spinor condensates. The steady states are found to depend sigmoidally on the lattice depth and exponentially on the magnetic fiel…
We have experimentally observed the emergence of spontaneous antiferromagnetic spatial order in a sodium spinor Bose-Einstein condensate that was quenched through a magnetic phase transition. For negative values of the quadratic Zeeman shift, a gas initially prepared in the F = 1, mF = 0 state collapsed into a dynamically evolving superposition of all 3 spin projections, mF = 0, +/-1. The quench gave rise to rich, nonequilibrium behavior where both nematic and magnetic spin waves were generated. We characterized the spatiotemporal evolution through two particle correlations between atoms in ea…
We present the creation and time evolution of two-dimensional Skyrmion excitations in an antiferromagnetic spinor Bose-Einstein condensate. Using a spin rotation method, the Skyrmion spin textures were imprinted on a sodium condensate in a polar phase, where the two-dimensional Skyrmion is topologically protected. The Skyrmion was observed to be stable on a short time scale of a few tens of ms but to have dynamical instability to deform its shape and eventually decay to a uniform spin texture. The deformed spin textures reveal that the decay dynamics involves breaking the polar phase inside th…
We have experimentally investigated the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition at zero quadratic Zeeman shift $q$. The rate of instability shows good agreement with predictions based upon solutions to the Bogoliubov de-Gennes equations. A key feature of this work was removal of magnetic field inhomogeneities, resulting in a steep change in behavior near the transition point. The quadratic Zeeman shift at the transition point was resolved to 250 milliHertz uncertainty, equivalent to an energy resolutio…
Large spin systems can exhibit unconventional types of magnetic ordering different from the ferromagnetic or Néel-like antiferromagnetic order commonly found in spin 1/2 systems. Spin-nematic phases, for instance, do not break time-reversal invariance and their magnetic order parameter is characterized by a second rank tensor with the symmetry of an ellipsoid. Here we show direct experimental evidence for spin-nematic ordering in a spin-1 Bose-Einstein condensate of sodium atoms with antiferromagnetic interactions. In a mean field description this order is enforced by locking the relative phas…
We investigate the phase transition dynamics of a quasi-2D antiferromagnetic spin-1 Bose-Einstein condensate from the easy-axis polar phase to the easy-plane polar phase, which is initiated by suddenly changing the sign of the quadratic Zeeman energy $q$. We observe the emergence and decay of spin turbulence and the formation of half-quantum vortices (HQVs) in the quenched condensate. The characteristic time and length scales of the turbulence generation dynamics are proportional to $|q|^{-1/2}$ as inherited from the dynamic instability of the initial state. In the evolution of the spin turbul…
We study the emergence of hysteresis during the process of quantum phase transition from an antiferromagnetic to a phase-separated state in a spin-1 Bose Einstein condensate of ultracold atoms. We explicitly demonstrate the appearance of a hysteresis loop with various quench times showing that it is rate-independent for large magnetizations only. In other cases scaling of the hysteresis loop area is observed, which we explain by using the Kibble-Zurek theory in the limit of small magnetization. The effect of an external harmonic trapping potential is also discussed.
We have analytically solved one-dimensional interacting two-component bosonic gases with spin-orbit (SO) coupling by the Bethe-ansatz method. Through a gauge transformation, the effect of SO coupling is incorporated into a spin-dependent twisted boundary condition. Our result shows that the SO coupling can influence the eigenenergy in a periodical pattern. The interplay between interaction and SO coupling may induce the energy level crossing for the ground state, which leads to a transition from the ferromagnetic to antiferromagnetic state.
We theoretically and numerically investigate the generation of fractional-charge vortex dipoles in spinor condensates with non-zero magnetization. We find that in the antiferromagnetic phase of spin-1 and spin-2 and the cyclic phase of spin-2 condensate with non-zero magnetization coupling of the density (phonon) and a spin-excitation mode results in two critical speeds for vortex-antivortex pair creation in the condensate. As a result, a Gaussian obstacle potential moving across the antiferromagnetic spin-1 or spin-2 and cyclic spin-2 spinor condensates with non-zero magnetization can lead to…
We study the effects of an on-site disorder potential in a gas of spinor (spin-1) ultracold atoms loaded in an optical lattice corresponding to both ferromagnetic and antiferromagnetic spin dependent interactions. Starting with a disordered spinor Bose-Hubbard model (SBHM) on a two dimensional square lattice, we observe the appearance of a Bose glass phase using the fraction of the lattice sites having finite superfluid order parameter and non integer local densities as an indicator. A precise distinction between three different types of phases namely, superfluid (SF), Mott insulator (MI) and …
We have experimentally observed the dynamics of an antiferromagnetic sodium Bose-Einstein condensate (BEC) quenched through a quantum phase transition. Using an off-resonant microwave field coupling the F = 1 and F = 2 atomic hyperfine levels, we rapidly switched the quadratic energy shift q from positive to negative values. At q = 0 the system undergoes a transition from a polar to antiferromagnetic phase. We measured the dynamical evolution of the population in the F = 1, m_F = 0 state in the vicinity of this transition point and observed a mixed state of all 3 hyperfine components for q < 0…
We investigate, both experimentally and theoretically, the quench dynamics of antiferromagnetic spinor Bose-Einstein condensates in the vicinity of a zero temperature quantum phase transition at zero quadratic Zeeman shift q. Both the rate of instability and the associated finite wavevector of the unstable modes - show good agreement with predictions based upon numerical solutions to the Bogoliubov de-Gennes equations. A key feature of this work is inclusion of magnetic field inhomogeneities that smooth the phase transition. Once these were removed, we observed a dramatic sharpening of the tra…
We present experimental observations of coherent spin-population oscillations in a cold thermal, Bose gas of spin-1 sodium-23 atoms. The population oscillations in a multi-spatial-mode thermal gas have the same behavior as those observed in a single-spatial-mode antiferromagnetic spinor Bose Einstein condensate. We demonstrate this by showing that the two situations are described by the same dynamical equations, with a factor of two change in the spin-dependent interaction coefficient, which results from the change to particles with distinguishable momentum states in the thermal gas. We compar…
We consider an antiferromagnetic Bose-Einstein condensate in a traverse magnetic field with a fixed macroscopic magnetization. The system exhibits two different critical behaviors corresponding to transitions from polar to broken-axisymmetry and from antiferromagnetic to broken-axisymmetry phases depending on the value of magnetization. We exploit both types of system criticality as a resource in the precise estimation of control parameter value. We quantify the achievable precision by the quantum Fisher information. We demonstrate supersensitivity and show that the precision scales with the n…
We theoretically study counterflow instability and turbulence in a spin-1 spinor Bose--Einstein condensate by the Gross--Pitaevskii equation and the Bogoliubov--de Gennes equation. Our study considers (i) the dynamics induced by the counterflow of two components with different magnetic quantum numbers, which leads to turbulence with spin degrees of freedom, and (ii) the properties of the turbulence. For (i), the behavior of the condensate induced by the counterflow strongly depends on whether the spin-dependent interaction is ferromagnetic or antiferromagnetic, leading to different behaviors f…
We show that metastable phases of an antiferromagnetic spin-1 condensate in a simple model with pure contact interactions can exhibit a rotonlike minimum in the excitation spectrum. The introduction of magnetic field gives rise to the instability of roton modes, which can lead to spontaneous emergence of regular periodic, polygonal, polyhedral or crystalline patterns, as shown in numerical simulations within the truncated Wigner approximation. An explanation of the occurrence of rotonlike instability is given based on the energy and spin conservation laws.
We observe evidence of first-order superfluid to Mott-insulator quantum phase transitions in a lattice-confined antiferromagnetic spinor Bose-Einstein condensate. The observed signatures include hysteresis effect and significant heatings across the phase transitions. The nature of the phase transitions is found to strongly depend on the ratio of the quadratic Zeeman energy to the spin-dependent interaction. Our observations are qualitatively understood by the mean field theory, and in addition suggest tuning the quadratic Zeeman energy is a new approach to realize superfluid to Mott-insulator …
We have studied the interaction between multiple, competing spatial modes that are excited by a quantum quench of an antiferromagnetic spinor Bose-Einstein condensate. We observed Hanbury Brown-Twiss correlations and associated super-Poissonian noise in the mode populations. The decay of these correlations was consistent with experimentally observed spin domain patterns. Data were compared with a real-space Bogoliubov theory as well as numerical solution of the coupled Gross-Pitaevskii equations that were seeded by quantum noise via the truncated Wigner approximation. The spatial modes that we…
We present an experimental study on the interaction and dynamics of half-quantum vortices (HQVs) in an antiferromagnetic spinor Bose-Einstein condensate. By exploiting the orbit motion of a vortex dipole in a trapped condensate, we perform a collision experiment of two HQV pairs, and observe that the scattering motions of the HQVs is consistent with the short-range vortex interaction that arises from nonsingular magnetized vortex cores. We also investigate the relaxation dynamics of turbulent condensates containing many HQVs, and demonstrate that spin wave excitations are generated by the coll…
Three-dimensional (3D) strongly correlated many-body systems, especially their dynamics across quantum phase transitions, are prohibitively difficult to be numerically simulated. We experimentally demonstrate that such complex many-body dynamics can be efficiently studied in a 3D spinor Bose-Hubbard model quantum simulator, consisting of antiferromagnetic spinor Bose-Einstein condensates confined in cubic optical lattices. We find novel dynamics and scaling effects beyond the scope of existing theories at superfluid-insulator quantum phase transitions and highlight spin populations as a new ob…
We study the instability of a moving spinor Bose-Einstein condensate when the speed of flow reaches the critical velocity. This we identify on the basis of Landau's criterion, i.e. the velocity above which some elementary excitation energy becomes negative. We show that the first-to-become unstable excitations are spin-carrying quasiparticles. We also discuss the temperature dependence of the critical velocity in a more advanced mean-field approximation.
We investigate the critical dynamics of spin superflow in an easy-plane antiferromagnetic spinor Bose-Einstein condensate. Spin-dipole oscillations are induced in a trapped condensate by applying a linear magnetic field gradient and we observe that the damping rate increases rapidly as the field gradient increases above a certain critical value. The onset of dissipation is found to be associated with the generation of dark-bright solitons due to the modulation instability of the counterflow of two spin components. Spin turbulence emerges as the solitons decay because of their snake instability…
We derive exact static as well as moving solitonic solutions to the one-dimensional spin-orbit-coupled F=1 Bose-Einstein condensates. The static polar soliton is shown to be the ground state by the imaginary-time evolution method. It shows a helical modulation of the order parameter due to the spin-orbit coupling. In particular, the moving soliton exhibits a periodic oscillation among the particle numbers of the hyperfine states. We further explore the temporal evolution of the static polar soliton and find that the spin-polarization exhibits dynamical oscillations. This disappearance and re-e…
We report the observation of spin domain walls bounded by half-quantum vortices (HQVs) in a spin-1 Bose-Einstein condensate with antiferromagnetic interactions. A spinor condensate is initially prepared in the easy-plane polar phase, and then, suddenly quenched into the easy-axis polar phase. Domain walls are created via the spontaneous $\mathbb{Z}_2$ symmetry breaking in the phase transition and the walls dynamically split into composite defects due to snake instability. The end points of the defects are identified as HQVs for the polar order parameter and the mass supercurrent in their proxi…
We investigate the early-time dynamics of a quasi-two-dimensional spin-1 antiferromagnetic Bose-Einstein condensate after a sudden quench from the easy-plane to the easy-axis polar phase. The post-quench dynamics shows a crossover behavior as the quench strength $\tilde{q}$ is increased, where $\tilde{q}$ is defined as the ratio of the initial excitation energy per particle to the characteristic spin interaction energy. For a weak quench of $\tilde{q}<1$, long-wavelength spin excitations are dominantly generated, leading to the formation of irregular spin domains. With increasing $\tilde{q}$, …
We theoretically and numerically study spin turbulence (ST) with small spin magnitude in spin-1 spinor Bose-Einstein condensates by using the spin-1 spinor Gross-Pitaevskii (GP)equations. This kind of ST is realized in two cases: (i) with antiferromagnetic interaction and (ii) with ferromagnetic interaction under a static magnetic field. The ST with small spin magnitude can exhibit two characteristic power laws in the spectrum of the spin-dependent interaction energy: -1 and -7/3 power laws in the low- and high-wave-number regions, respectively. These power laws are derived from a Kolmogorov-t…
We experimentally study spin dynamics in a sodium antiferromagnetic spinor condensate with off-resonant microwave pulses. In contrast to a magnetic field, a microwave dressing field enables us to explore rich spin dynamics under the influence of a negative net quadratic Zeeman shift $q_{\rm net}$. We find an experimental signature to determine the sign of $q_{\rm net}$, and observe harmonic spin population oscillations at every $q_{\rm net}$ except near each separatrix in phase space where spin oscillation period diverges. In the negative and positive $q_{\rm net}$ regions, we also observe a r…
Spinor Bose-Einstein condensates under external magnetic fields exhibit well-characterized spin domains of its ground state due to spin-dependent interactions. At low temperatures, collision-induced spin-mixing instabilities may promote the condensate to dwell into metastable states occurring near the phase boundaries. In this work, we study theoretically the metastable spin-phase diagram of a spin-1 antiferromagnetic Bose-Einstein condensate at zero and finite temperatures. The approach makes use of Hartree-Fock theory and exploits the symmetry of the Hamiltonian and of the order parameters y…
We introduce a Floquet spinor Bose-Einstein condensate induced by a periodically driven quadratic Zeeman coupling whose frequency is larger than any other energy scales. By examining a spin-1 system available in ultracold atomic gases, we demonstrate that such an external driving field has great effect on the condensate through emergence of a unique spin-exchange interaction. We uncover that the ferromagnetic condensate has several unconventional stationary states and thus exhibits rich continuous phase transitions. On the other hand, the antiferromagnetic condensate is found to possess a nont…
We investigate the stability of a hard-axis polar state in a spin-1 antiferromagnetic Bose-Einstein condensate under a magnetic field gradient, where the easy-plane spin anisotropy is controlled by a negative quadratic Zeeman energy $q<0$. In a uniform magnetic field, the axial polar state is dynamically unstable and relaxes into the planar polar ground state. However, under a field gradient $B'$, the excited spin state becomes metastable down to a certain threshold $q_{th}$ and as $q$ decreases below $q_{th}$, its intrinsic dynamical instability is rapidly recalled. The incipient spin excitat…
We theoretically study the stationary-state vortex lattice configurations of rotating spin-orbit- and coherently-coupled spin-1 Bose-Einstein condensates trapped in quasi-two-dimensional harmonic potentials. The combined effects of rotation, spin-orbit and coherent couplings are analyzed systematically from the single-particle perspective. Through the single-particle Hamiltonian, which is exactly solvable for one-dimensional coupling, under specific coupling and rotation strengths, we illustrate that a boson in these rotating spin-orbit- and coherently-coupled condensates are subjected to effe…
We consider a spin-1/2 Bose-Einstein condensate prepared initially in a single spin projection. The two channels of excitations existing in such a system (namely density and spin waves) are discussed and we show how pure spin waves can be excited in the presence of local magnetic defects. We analyze the role played by spin excitations on the Landau superfluidity criterion and demonstrate the absence of absolute superfluidity for the antiferromagnetic condensate. In the ferromagnetic case, we identify two critical velocities for the breakdown of superfluidity.
We propose a scheme to probe quantum coherence in the state of a nano-cantilever based on its magnetic coupling (mediated by a magnetic tip) with a spinor Bose Einstein condensate (BEC). By mapping the BEC into a rotor, its coupling with the cantilever results in a gyroscopic motion whose properties depend on the state of the cantilever: the dynamics of one of the components of the rotor angular momentum turns out to be strictly related to the presence of quantum coherence in the state of the cantilever. We also suggest a detection scheme relying on Faraday rotation, which produces only a very…
We consider a phase transition from antiferromagnetic to phase separated ground state in a spin-1 Bose-Einstein condensate of ultracold atoms. We demonstrate the occurrence of two scaling laws, for the number of spin fluctuations just after the phase transition, and for the number of spin domains in the final, stable configuration. Only the first scaling can be explained by the standard Kibble-Żurek mechanism. We explain the occurrence of two scaling laws by a model including post-selection of spin domains due to the conservation of condensate magnetization.
We study the effect of an external harmonic trapping potential on an outcome of the non-adiabatic quantum phase transition from an antiferromagnetic to a phase-separated state in a spin-1 atomic condensate. Previously, we demonstrated that the dynamics of an untrapped system exhibits double universality with two different scaling laws appearing due to conservation of magnetization. We show that in the presence of a trap double universality persists. However, the corresponding scaling exponents are strongly modified by transfer of local magnetization across the system. The values of these expon…
One of the excitements generated by the cold atom systems is the possibility to realize, and explore, varied topological phases stemming from multi-component nature of the condensate. Popular examples are the antiferromagnetic (AFM) and the ferromagnetic (FM) phases in the three-component atomic condensate with effective spin-1, to which different topological manifolds can be assigned. It follows, from consideration of homotopy, that different sorts of topological defects will be stable in each manifold. For instance, Skyrmionic texture is believed to be a stable topological object in two-dime…
We show that strongly interacting multicomponent gases in one dimension realize an effective spin chain, offering an alternative simple scenario for the study of one-dimensional quantum magnetism in cold gases in the absence of an optical lattice. The spin-chain model allows for an intuitive understanding of recent experiments and for a simple calculation of relevant observables. We analyze the adiabatic preparation of antiferromagnetic and ferromagnetic ground states, and show that many-body spin states may be efficiently probed in tunneling experiments. The spin-chain model is valid for more…
Heat generated as a result of the breakdown of an adiabatic process is one of the central concepts of thermodynamics. In isolated systems, the heat can be defined as an energy increase due to transitions between distinct energy levels. Across a second-order quantum phase transition (QPT), the heat is predicted theoretically to exhibit a power-law scaling, but it is a significant challenge for an experimental observation. In addition, it remains elusive whether a power-law scaling of heat can exist for a first-order QPT. Here we experimentally observe a power-law scaling of heat in a spinor con…
We analyze sound waves (phonons, Bogoliubov excitations) propagating on continuous wave (cw) solutions of repulsive $F=1$ spinor Bose-Einstein condensates (BECs), such as $^{23}$Na (which is antiferromagnetic or polar) and $^{87}$Rb (which is ferromagnetic). Zeeman splitting by a uniform magnetic field is included. All cw solutions to ferromagnetic BECs with vanishing $M_F=0$ particle density and non-zero components in both $M_F=\pm 1$ fields are subject to modulational instability (MI). MI increases with increasing particle density. MI also increases with differences in the components' wavenu…
The static properties, i.e., existence and stability, as well as the quench-induced dynamics of vortex-bright type excitations in two-dimensional harmonically confined spin-1 Bose-Einstein condensates are investigated. Linearly stable vortex-bright-vortex and bright-vortex-bright solutions arise in both antiferromagnetic and ferromagnetic spinor gases upon quadratic Zeeman energy shift variations. Their deformations across the relevant transitions are exposed and discussed in detail evincing also that emergent instabilities can lead to pattern formation. Spatial elongations, precessional motio…
The Kibble-Zurek mechanism provides a unified theory to describe the universal scaling laws in the dynamics when a system is driven through a second-order quantum phase transition. However, for first-order quantum phase transitions, the Kibble-Zurek mechanism is usually not applicable. Here, we experimentally demonstrate and theoretically analyze a power-law scaling in the dynamics of a spin-1 condensate across a first-order quantum phase transition when a system is slowly driven from a polar phase to an antiferromagnetic phase. We show that this power-law scaling can be described by a general…
We investigate the cavity optomechanical properties of an antiferromagnetic Bose-Einstein con- densate, where the role of the mechanical element is played by spin-wave excitations. We show how this system can be described by a single rotor that can be prepared deep in the quantum regime under realizable experimental conditions. This system provides a bottom-up realization of dispersive rotational optomechanics, and opens the door to the direct observation of quantum spin fluctuations.
Mean-field phase diagrams of spinor bosons in an optical cavity
Szkoła Doktorska Nauk Ścisłych i Przyrodniczych, Uniwersytet Jagielloński（雅盖隆大学自然科学博士学院）；Instytut Fizyki Teoretycznej, Wydział Fizyki, Astronomii i Informatyki Stosowanej, Uniwersytet Jagielloński（雅盖隆大学应用物理、天文学和计算机科学系理论物理研究所）；Mark Kac Complex Systems Research Center, Jagiellonian University in Kraków（克拉科夫雅盖隆大学马克·卡克复杂系统研究中心）
We present the phase diagram, the underlying stability and magnetic properties as well as the dynamics of nonlinear solitary wave excitations arising in the distinct phases of a harmonically confined spinor $F=1$ Bose-Einstein condensate. Particularly, it is found that nonlinear excitations in the form of dark-dark-bright solitons exist in the antiferromagnetic and in the easy-axis phase of a spinor gas, being generally unstable in the former while possessing stability intervals in the latter phase. Dark-bright-bright solitons can be realized in the polar and the easy-plane phases as unstable …
Strongly interacting one-dimensional quantum systems often behave in a manner that is distinctly different from their higher-dimensional counterparts. When a particle attempts to move in a one-dimensional environment it will unavoidably have to interact and 'push' other particles in order to execute a pattern of motion, irrespective of whether the particles are fermions or bosons. A present frontier in both theory and experiment are mixed systems of different species and/or particles with multiple internal degrees of freedom. Here we consider trapped two-component bosons with short-range inter…
We propose to probe the quantum ground state of a spin-1 Bose-Einstein condensate with the transmission spectra of an optical cavity. By choosing a circularly polarized cavity mode with an appropriate frequency, we can realize coupling between the cavity mode and the magnetization of the condensate. The cavity transmission spectra then contain information of the magnetization statistics of the condensate and thus can be used to distinguish the ferromagnetic and antiferromagnetic quantum ground states. This technique may also be useful for continuous observation of the spin dynamics of a spinor…
Motivated by a recent experiment in an antiferromagnetic spin-1 Bose-Einstein condensate of ${}^{23} \textrm{Na}$ atoms, we study the energetical stability of a singly quantum vortex injected into the center of a quasi-two-dimensional gas with zero total spin against dissocation into a pair of half-quantum vortices. We find that the critical dissociation point of this confinement-deconfinement type phase transition can be expressed in terms of the ratio of density-density ($c_0$) and spin-spin ($c_2$) coupling constants. The transition of bound to unbound vortices, in particular, sensitively d…
Vector solitons are a type of solitary, or non-spreading wavepacket occurring in a nonlinear medium comprised of multiple components. As such, a variety of synthetic systems can be constructed to explore their properties, from nonlinear optics to ultracold atoms, and even in human-scale metamaterials. In quantum systems such as photons or Bose-Einstein condensates (BECs), such vector nonlinearities offer a window into complex many-body dynamics, and offer possibilities for quantum communication and information processing. BECs have a rich panoply of internal hyperfine levels, or spin component…
