We expose an analysis of the magnetic field distribution in the Abrikosov lattice of high-kappa superconductors with d-wave pairing in the case where the critical field is mainly determined by the Pauli limit and the superfluid currents mainly come from the paramagnetic interaction of electron spins with the local magnetic field. The result found in frame of the generalized Clem variational approach is compatible with the recent observation that the form factor in CeCoIn_5 increases with increasing field and then decreases at the approach of H_c2. (A. D. Bianchi et al., Science vol. 319, 177 (2008)).
From small-angle neutron scattering studies of the flux line lattice (FLL) in CeCoIn5, with magnetic field applied parallel to the crystal c-axis, we obtain the field- and temperature-dependence of the FLL form factor, which is a measure of the spatial variation of the field in the mixed state. We extend our earlier work [A.D. Bianchi et al. 2008 Science 319, 177] to temperatures up to 1250 mK. Over the entire temperature range, paramagnetism in the flux line cores results in an increase of the form factor with field. Near H_c2 the form factor decreases again, and our results indicate that thi…
We present scanning tunneling spectroscopy measurements of the local quasiparticles' excitation spectra of CeCoIn$_5$ between 440mK and 3K in samples with a bulk $T_{\rm c}=2.25$K. The spectral shape of our low-temperature tunneling data, quite textbook nodal-gap conductance, allow us to confidently fit the spectra with a d-wave density of states considering also a shortening of quasiparticles' lifetime term $Γ$. The $Δ(0)$ value obtained from the fits yields a BCS ratio $2Δ/kT_{\rm c} =7.73$ suggesting that CeCoIn$_5$ is an unconventional superconductor in the strong coupling limit. The fits …
Very recently large Nernst effect and Seebeck effect were observed above the superconducting transition temperature 2.3K in a heavy fermion superconductor CeCoIn_5. We shall interpret this large Nernst effect in terms of unconventional density wave (UDW), which appears around T=18K. Also the temperature dependence of the Seebeck coefficient below T=18K is described in terms of UDW. Another hallmark for UDW is the angular dependent magnetoresistance, which should be readily accessible experimentally.
We present In NMR measurements in a novel thermodynamic phase of CeCoIn5 in high magnetic field, where exotic superconductivity coexists with the incommensurate spin-density wave order. We show that the NMR spectra in this phase provide direct evidence for the emergence of the spatially distributed normal quasiparticle regions. The quantitative analysis for the field evolution of the paramagnetic magnetization and newly-emerged low-energy quasiparticle density of states is consistent with the nodal plane formation, which is characterized by an order parameter in the Fulde-Ferrell-Larkin-Ovchin…
Field-angle dependent specific heat measurement has been done on the heavy-fermion superconductor CeCoIn5 down to ~ 0.29 K, in a magnetic field rotating in the tetragonal c-plane. A clear fourfold angular oscillation is observed in the specific heat with the minima (maxima) occurring along the [100] ([110]) directions. Oscillation persists down to low fields H << Hc2, thus directly proving the existence of gap nodes. The results indicate that the superconducting gap symmetry is most probably of dxy type.
Ultrasound velocity measurements of the unconventional superconductor CeCoIn_5 with extremely large Pauli paramagnetic susceptibility reveal an unusual structural transformation of the flux line lattice (FLL) in the vicinity of the upper critical field. The transition field coincides with that at which heat capacity measurements reveal a second order phase transition. The lowering of the sound velocity at the transition is consistent with the collapse of the FLL tilt modulus and a crossover to quasi two-dimensional FLL pinning. These results provide a strong evidence that the high field state …
Antiferromagnetic (AFM) (or spin-density wave) quantum critical fluctuation enhanced just below H_c2(0) have been often observed in d-wave superconductors with a strong Pauli paramagnetic depairing (PD) including CeCoIn_5. It is shown here that such a tendency of field-induced AFM ordering is a consequence of strong PD and should appear particularly in superconductors with a gap node along the AFM modulation. Two phenomena seen in CeCoIn_5, the anomalous vortex lattice form factor and the AFM order in the Fulde-Ferrell-Larkin-Ovchinnikov state, are explained based on this peculiar PD effect.
Electronic structure and the shape of the Fermi surface are known to be of fundamental importance for the superconducting instability in real materials. We demonstrate that such an instability may be explored by static Cooper pair susceptibility renormalized by pairing interaction and present an efficient method of its evaluation using Wannier orbitals derived from ab initio calculation. As an example, this approach is used to search for an unconventional superconducting phase of the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) type in a heavy-fermion compound CeCoIn$_5$ and an iron-based supercond…
Beside the spin density wave (SDW) order inside the superconducting phase in $\mathrm{CeCoIn_5}$ at high magnetic fields, recent neutron scattering measurements have found Bragg peaks in $5\%$ Nd doped $\mathrm{CeCoIn_5}$ at low fields. The intensity of Bragg peaks in low fields is suppressed by increasing field. Based on the phenomenological and microscopic modeling, we show that for the Pauli limited $d$-wave superconductors in the vicinity of SDW instability relevant for $\mathrm{CeCoIn_5}$, magnetic impurities locally induce droplets of SDW order. Because of the strong anisotropy in the mo…
We demonstrate that the electronic bandstructure extracted from quasi-particle interference spectroscopy [Nat. Phys. 9, 468 (2013)] and the theoretically computed form of the superconducting gaps [Proc. Nat. Acad. Sci. 111, 11663 (2014)] can be used to understand the $dI/dV$ lineshape measured in the normal and superconducting state of CeCoIn$_5$ [Nat. Phys. 9, 474 92103)]. In particular, the $dI/dV$ lineshape, and the spatial structure of defect-induced impurity states, reflects the existence of multiple superconducting gaps of $d_{x^2-y^2}$-symmetry. These results strongly support a recently…
Unconventional superconductivity and magnetism are intertwined on a microscopic level in a wide class of materials, including high-$T_c$ cuprates, iron pnictides, and heavy-fermion compounds. A new approach to this most fundamental and hotly debated subject focuses on the role of interactions between superconducting electrons and bosonic fluctuations at the interface between adjacent layers in heterostructures. A recent state-of-the-art molecular-beam-epitaxy technique has enabled us to fabricate superlattices consisting of different heavy-fermion compounds with atomic thickness. These Kondo s…
Using the quasiclassical theory, we analyze the vortex structure of strong-paramagnetic superconductors.There, induced paramagnetic moments are accumulated exclusively around the vortex core. We quantitatively evaluate the significant paramagnetic effect in the H-dependence of various quantities, such as low temperature specific heat, Knight shift, magnetization and the flux line lattice (FLL) form factor. The anomalous H-dependence of the FLL form factor observed by the small angle neutron scattering in CeCoIn_5 is attributable to the large paramagnetic contribution.
It is theoretically shown that, in the four-fold symmetric d-wave superconducting phase, a paramagnetic pair-breaking (PPB) enhanced sufficiently by increasing the applied magnetic field induces not only the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) superconducting state but also an incommensurate antiferromagnetic (AFM) order with Q-vector parallel to a gap node. This AFM ordering tends to occur only below H_{c2} at low temperatures, i.e., in the presence of a nonvanishing superconducting energy gap $Δ$ rather than in the normal phase. Through a detailed study on the resulting AFM order and its…
Superconductivity and fractionalized magnetic excitations in CeCoIn5
Oak Ridge National Laboratory（橡树岭国家实验室）；The University of Tennessee, Knoxville（田纳西大学诺克斯维尔分校）；Harvard University（哈佛大学）；Max Planck Institute for Solid State Research（马克斯·普朗克固体研究所）；Neutron Scattering Division, Oak Ridge National Laboratory（橡树岭国家实验室中子散射部）；Department of Physics, Brookhaven National Laboratory（布鲁海文国家实验室物理系）；University of Edinburgh（爱丁堡大学）；Center for Computational Quantum Physics, Flatiron Institute（平顿研究所计算量子物理中心）；Quantum Condensed Matter Division and Shull-Wollan Center, Oak Ridge National Laboratory（橡树岭国家实验室量子凝聚态物质部和舒尔-沃兰中心）
We theoretically study the effect of a nonmagnetic impurity in heavy fermion superconductor CeCoIn$_{5}$ within a realistic band model and the T-matrix approximation approach. By considering two known possible pairing symmetry candidates $d_{x^{2}-y^{2}}$ and $d_{xy}$, we find that although both total density of states exhibit a similar V-shaped gaplike feature, only the $d_{x^{2}-y^{2}}$-wave pairing symmetry gives rise to robust intragap impurity resonance states reflected by the resonance peaks near the Fermi energy in the local density of states. These features can be readily probed by sca…
We theoretically study effects of surface roughness on the magnetic response of small unconventional superconductors by solving the Eilenberger equation for the quassiclassical Green function and the Maxwell equation for the vector potential simultaneously and self-consistently. The paramagnetic phase of spin-singlet $d$-wave superconducting disks is drastically suppressed by the surface roughness, whereas that of spin-triplet $p$-wave disks is robust even in the presence of the roughness. Such difference derives from the orbital symmetry of paramagnetic odd-frequency Cooper pairs appearing at…
The evolution of the magnetic excitation spectrum of the unconventional superconductor CeCoIn$_{5}$ was studied by inelastic neutron scattering as a function of magnetic field applied in the [1, -1, 0] direction. The spin resonance characteristic of the superconducting states was observed up to about $H_{c2}$/2 : it is still centered at (1/2, 1/2, 1/2) when the magnetic field increases while its characteristic energy decreases and its lineshape substantially broadens.
Campbell penetration depth in a single crystal of heavy fermion superconductor CeCoIn$_5$
Ames National Laboratory（艾姆斯国家实验室）；Iowa State University（爱荷华州立大学）；Missouri University of Science and Technology（密苏里科技大学）；Brookhaven National Laboratory（布鲁克海文国家实验室）；Shanghai Advanced Research in Physical Sciences (SHARPS)（上海物理科学研究院）；Vinca Institute of Nuclear Sciences, University of Belgrade（贝尔格莱德大学温卡核科学研究所）
The Bardeen-Cooper-Schrieffer mechanism for superconductivity is a triumph of the theory of many-body systems. Implicit in its formulation is the existence of long-lived (quasi)particles, originating from the electronic building blocks of the materials, which interact to form Cooper pairs that move coherently in lock-step. The challenge of unconventional superconductors is that it is not only unclear what the nature of the interactions are, but whether the familiar quasi-particles that form a superconducting condensate even exist. In this work, we reveal, by the study of applied magnetic field…
It is shown by detailed inelastic neutron scattering experiments that the gapped collective magnetic excitation of the unconventional superconductor CeCoIn$_{5}$, the spin resonance mode, is incommensurate and that the corresponding fluctuations are of Ising nature. The incommensurate peak position of these fluctuations corresponds to the propagation vector of the adjacent field induced static magnetic ordered phase, the so-called Q-phase. Furthermore, the direction of the magnetic moment fluctuations is also the direction of the ordered magnetic moments of the Q-phase. Hence the resonance mod…
Effects of the paramagnetic depairing on structural transitions between vortex lattices of a quasi two dimensional d-wave superconductor are examined. It is found that, in systems with Maki parameter $α_{\rm M}$ of order unity, a square lattice induced by a d-wave pairing is destabilized with {\it increasing} fields, and that a reentrant rhombic lattice occurs in higher fields. Further, a weak Fermi surface anisotropy competitive with the pairing symmetry induces another structural transition near $H_{c2}$. These results are consistent with the structure changes of the vortex lattice in CeCoIn…
The high field phase diagram and magnetic properties of CeCoIn_5 below H_c2(0) are examined from the picture regarding the high field and low temperature (HFLT) phase as a possible Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) vortex lattice. Crucial roles of antiferromagnetic (AFM) fluctuations enhanced close to H_c2(0) are stressed. The FFLO vortex lattice with a longitudinal modulation parallel to the field is stabilized compared with those with lateral modulations as a consequence of the presence of AFM fluctuations. Further, an unusual field-induced enhancement of the flux distribution is argue…
Motivated by recent thermal conductivity measurements in the superconductor CeCoIn5, we theoretically examine a possible staggered spin-triplet superconducting order to be induced by the coupled spin-density-wave (SDW) and d-wave superconducting (SC) orders in the high field and low temperature (HFLT) SC phase peculiar to this material with strong paramagnetic pair-breaking (PPB). It is shown that one type of the $π$-triplet order is consistent with the thermal conductivity data and can naturally be incorporated in the picture that the Q-phase is a consequence of the strong PPB effect inducing…
Point-contact spectroscopy was performed on single crystals of the heavy-fermion superconductor CeCoIn_5 between 150 mK and 2.5 K. A pulsed measurement technique ensured minimal Joule heating over a wide voltage range. The spectra show Andreev-reflection characteristics with multiple structures which depend on junction impedance. Spectral analysis using the generalized Blonder-Tinkham-Klapwijk formalism for d-wave pairing revealed two coexisting order parameter components, with amplitudes Delta_1 = 0.95 +/- 0.15 meV and Delta_2 = 2.4 +/- 0.3 meV, which evolve differently with temperature. Our …
We calculate the wave-vector dependent electronic spin susceptibility $χ_{αβ}(\mathbf q, \mathbf H_0)$ of a d-wave superconductor in uniform magnetic field $\mathbf{H}_0$ with Pauli pair-breaking. We find that the transverse component of the susceptibility tensor can be greater than its normal state value; the longitudinal component also slightly increases but in a very limited range of $q$s. We identify several wave vectors $\{\mathbf q_\perp,\mathbf q_\parallel\}$, that correspond to the maxima of either $χ_\perp$ or $χ_\parallel$. We compare our results with available data on the high-field…
Although the diamagnetism is of the essence in the superconducting phenomena, small enough topological (or unconventional) superconductors are paramagnetic. By solving the quasiclassical Eilenberger equation and the Maxwell equation self-consistently in two-dimensional disks, we theoretically study the response of small superconductors to weak magnetic field. Because of the topologically nontrivial character of the wave function, the unconventional superconductor hosts the zero-energy surface Andreev bound states which always accompany the odd-frequency Cooper pairs. The paramagnetic property …
We show that the recently observed spin resonance modes in heavy-fermion superconductors CeCoIn$_5$ and CeCu$_2$Si$_2$ are magnetic excitons originating from superconducting quasiparticles. The wave vector ${\bf Q}$ of the resonance state leads to a powerful criterion for the symmetry and node positions of the unconventional gap function. The detailed analysis of the superconducting feedback on magnetic excitations reveals that the symmetry of the superconducting gap corresponds to a singlet $d_{x^2-y^2}$ state symmetry in both compounds. In particular this resolves the long-standing ambiguity…
We present small angle neutron scattering studies of the vortex lattice (VL) in CeCoIn5 with magnetic fields applied parallel (H) to the antinodal [100] and nodal [110] directions. For H || [100], a single VL orientation is observed, while a 90 degree reorientation transition is found for H || [110]. For both field orientations and VL configurations we find a distorted hexagonal VL with an anisotropy, Gamma = 2.0 +/- 0.05. The VL form factor shows strong Pauli paramagnetic effects similar to what have previously been reported for H || [001]. At high fields, above which the upper critical field…
Effects of Pauli paramagnetism on thermodynamic quantities in a vortex state, such as the specific heat $C$ and magnetization $M$, are studied using the quasiclassical Eilenberger formalism. We demonstrate that with an increase of paramagnetic depairing effect, the sigh of the curvature of the field dependence of $C$ changes from negative to positive, and that the Maki parameter $κ_2$ becomes an increasing function of temperature. Our results provide a natural explanation for the unusual field dependence of $C$ seen in CeCoIn$_5$ in terms of the paramagnetic effect.
The appearance of spin-density-wave (SDW) magnetic order in the low-temperature and high-field corner of the superconducting phase diagram of CeCoIn$_5$ is unique among unconventional superconductors. The nature of this magnetic $Q$ phase is a matter of current debate. Here, we present the thermal conductivity of CeCoIn$_5$ in a rotating magnetic field, which reveals the presence of an additional order inside the $Q$ phase that is intimately intertwined with the superconducting $d$-wave and SDW orders. A discontinuous change of the thermal conductivity within the $Q$ phase, when the magnetic f…
We analyse the magnetic structure of the antiferromagnetic order induced in Pauli limited d-wave superconductors by Zeeman coupling to magnetic field. We determine the phase diagram in the H-T plane, and find that the magnetic phase, which is stabilized at low temperatures and just below the upper critical field, can have two realizations depending primarily on the shape of the underlying Fermi surface. The double-Q magnetic ordering may persist over the entire coexistence range. Alternatively, there may exist a weak first order transition from a double-Q structure at lower fields to a single-…
We have performed de Haas-van Alphen (dHvA) measurements of the heavy-fermion superconductor CeCoIn$_5$ down to 2 mK above the upper critical field. We find that the dHvA amplitudes show an anomalous suppression, concomitantly with a shift of the dHvA frequency, below the transition temperature $T_{\rm n}=20$ mK. We suggest that the change is owing to magnetic breakdown caused by a field-induced antiferromagnetic (AFM) state emerging below $T_{\rm n}$, revealing the origin of the field-induced quantum critical point (QCP) in CeCoIn$_5$. The field dependence of $T_{\rm n}$ is found to be very w…
In the tetragonal heavy fermion system CeCoIn5 the unconventional superconducting state is probed by means of muon spin rotation. The pressure dependence (0-1 GPa) of the basal-plane magnetic penetration depth (λ_a), the penetration depth anisotropy (γ=λ_c/λ_a) and the temperature dependence of 1/λ_i^2 (i=a,c) were studied in single crystals. A strong decrease of λ_a with pressure was observed, while γand λ_i^2(0)/λ_i^2(T) are pressure independent. A linear relationship between 1/λ_a^2(270 mK) and Tc was also found. The large decrease of λ_a with pressure is the signature of an increase of the…
To study the mutual interaction between unconventional superconductivity and magnetic order through an interface, we fabricate Kondo superlattices consisting of alternating layers of heavy-fermion superconductor CeCoIn$_5$ and antiferromagnetic (AFM) heavy-fermion metal CeIn$_3$. The strength of the AFM fluctuations is tuned by applying hydrostatic pressure to CeCoIn$_5(m)$/CeIn$_3(n)$ superlattices with $m$ and $n$ unit-cell-thick layers of CeCoIn$_5$ and CeIn$_3$, respectively. Superconductivity in CeCoIn$_5$ and AFM order in CeIn$_3$ coexist in spatially separated layers. At ambient pressur…
Recent experiments on high-temperature superconductors show paramagnetic behavior localized at grain boundaries (GB). This paramagnetism can be attributed to the presence unconventional d-wave induced $π$-junctions. By modeling the GB as an array of $π$ and conventional Josephson junction we determine the conditions of the occurrence of the paramagnetic behavior.
Effects of the strong Pauli-paramagnetic pair-breaking (PPB) on the vortex lattice in d-wave superconductors are theoretically studied by putting emphasis on consequences of the PPB-induced antiferromagnetic (AFM) ordering in the spatial modulation in the vortex lattice. It is shown that the PPB-induced AFM fluctuation in the superconducting state leads to an enhancement of the vortex lattice form factor which is a measure of spatial variations of the internal magnetic field and that the enhancement becomes more remarkable as an AFM instability is approached. It is also demonstrated that the P…
Employing the elemental sensitivity of x-ray absorption spectroscopy (XAS) and x-ray magnetic circular dichroism (XMCD), we study the valence and magnetic order in the heavy fermion superconductor CeCoIn$_5$. We probe spin population of the f-electrons in Ce and d-electrons in Co as a function of temperature (down to 0.1 K) and magnetic field (up to 6 T). From the XAS we find a pronounced contribution of Ce$^{4+}$ component at low temperature and a clear temperature dependence of the Ce valence below 5 K, suggesting enhanced valence fluctuations, an indication for the presence of a nearby quan…
The Ce compounds CeCoIn$_5$ and CeRhIn$_5$ are ideal model systems to study the competition of antiferromagnetism (AF) and superconductivity (SC). Here we discuss the pressure--temperature and magnetic field phase diagrams of both compounds. In CeRhIn$_5$ the interesting observation is that in zero magnetic field a coexistence AF+SC phase exist inside the AF phase below the critical pressure $p_{\rm c}^\star \approx 2$ GPa. Above $p_{\rm c}^\star$ AF is suppressed in zero field but can be re-induced by applying a magnetic field. The collapse of AF under pressure coincides with the abrupt chang…
Diamagnetically coupled magnetic field can be used as a probe of nodal positions in unconventional superconductors. The heat capacity depends on the angle $ϕ_0$ between the magnetic field and the nodal directions. We show that the anisotropy $C(ϕ_0)$ persists even in systems with strong paramagnetic coupling to the electrons's spins.
We develop a theory of the coexistence of superconductivity (SC) and antiferromagnetism (AFM) in CeCoIn5. We show that in Pauli-limited nodal superconductors the nesting of the quasi-particle pockets induced by Zeeman pair-breaking leads to incommensurate AFM with the moment normal to the field. We compute the phase diagram and find a first order transition to the normal state at low temperatures, absence of normal state AFM, and coexistence of SC and AFM at high fields, in agreement with experiments. We also predict the existence of a new double-Q magnetic phase.
Based on a theoretical argument and Monte Carlo simulations of a Ginzburg-Landau model derived microscopically, it is argued that, in type-II superconductors where {\it both} the paramagnetic {\it and} orbital depairings are important, a strong first-order transition (FOT) at $H_{c2}$ expected in the mean field (MF) approximation never occurs in real systems and changes due to the fluctuation into a crossover. The present result explains why a {\it nearly} discontinuous crossover at $H_{c2}$ with {\it no} intrinsic hysteresis is observed only in a clean superconducting material with a singlet …
We investigate the vortex state with Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) modulations suggested for a high field phase of CeCoIn_5. On the basis of the quasiclassical Eilenberger theory, we calculate the three dimensional structure of pair potentials, internal magnetic fields, paramagnetic moments, and electronic states, for the s-wave and the d-wave pairings comparatively. The π-phase shift of the pair potential at the FFLO nodal plane or at the vortex core induces sharp peak states in the local density of states, and enhances the local paramagnetic moment. We also discuss the NMR spectrum…
The interplay between magnetism and superconductivity has been a central issue in unconventional superconductors. While the dynamic magnetism could be the source of electron pairing, the static magnetism is generally believed to compete with superconductivity. In this sense, the observation of Q phase, the coupled spin-density wave order and superconductivity, in the heavy-fermion superconductor CeCoIn5 is very puzzling. Whether this Q phase origins from the novel Fulde-Ferrel-Larkin-Ovchinnikov state is under hot debate. Here we report the resistivity and thermal conductivity study of a newly…
We theoretically investigate k-space structures of $d_{x^2-y^2}$-wave superconducting (SC) and spin-density-wave (SDW) orders in their coexistent phase induced by a paramagnetic pair-breaking (PPB) effect in relation to the high field and low temperature (HFLT) SC phase in CeCoIn$_5$. It is shown that, in k-space, the SDW order develops near the gap nodes where the SC order is suppressed by PPB, and the nesting condition for the SDW ordering is satisfied. By comparing the results in the $d_{x^2-y^2}$-wave SC model and those in an artificial model with no sign change of the gap function in k-sp…
Resolving the high-field superconducting phase (HFSP), often called as the Q-phase, and the antiferromagnetic or spin-density-wave (SDW) order appearing in the phase remains a crucial issue on the superconductor CeCoIn$_5$. It is shown that a switching of the SDW domain due to a tiny change of the magnetic field direction in HFSP, reported and interpreted as an evidence of the presence of a $π$-triplet pairing inducing the SDW order [S. Gerber et al., Nature Physics 10, 126 (2014)], can be explained with no triplet pairing component if the $d$-wave superconducting order in HFSP includes the Fu…
We theoretically investigate the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state by using the microscopic quasi-classical Eilenberger equation. The Pauli paramagnetic effects and the orbital depairing effects due to vortices are treated in an equal footing for three dimensional spherical Fermi surface model and $s$-wave pairing. The field evolution of the LO state is studied in detail, such as the $H$-$T$ phase diagram, spatial structures of the order parameter, the paramagnetic moment, and the internal filed. Field-dependences of various thermodynamic quantities: the paramagnetic moment, entrop…
Local electronic effects in the vicinity of an impurity provide pivotal insight into the origin of unconventional superconductivity, especially when the materials are located on the edge of magnetic instability. In high-temperature cuprate superconductors, a strong suppression of superconductivity and appearance of low-energy bound states are clearly observed near nonmagnetic impurities. However, whether these features are common to other strongly correlated superconductors has not been established experimentally. Here, we report the {$in$} {$situ$} scanning tunneling microscopy observation of…
We present a microscopic approach to the calculations of thermal conductivity in unconventional superconductors for a wide range of temperatures and magnetic fields. Our work employs the non-equilibrium Keldysh formulation of the quasiclassical theory. We solve the transport equations using a variation of the Brandt-Pesch-Tewordt (BPT) method, that accounts for the quasiparticle scattering on vortices. We focus on the dependence of the thermal conductivity on the direction of the field with the respect to the nodes of the order parameter, and discuss it in the context of experiments aiming to …
The field-induced antiferromagnetic (AFM) ordering in the $d_{x^2-y^2}$-paired superconducting phase, which has been recently found in the weak-coupling approach as a basic mechanism due to the Pauli paramagnetic pair-breaking (PPB) in relation to the high-field behaviors in CeCoIn_5, is studied in the strong-coupling approach taking account of the electron correlation. Applying the fluctuation-exchange (FLEX) approximation to the two-dimensional Hubbard model including the Zeeman term, it is shown that the PPB-induced AFM ordering in the superconducting (SC) phase and the first order SC trans…
Unconventional density waves (UDW) are one of the ground states in metallic crystalline solids and have been speculated already in 1968. However, more focused studies on UDW started only recently, perhaps after the identification of the low temperature phase in alpha-(BEDT-TTF)_2KHg(SCN)_4 as unconventional charge density wave (UCDW) in 2002. More recently, the metallic phase of Bechgaard salts (TMTSF)_2X with X=PF_6 and ReO_4 under both pressure and magnetic field appears to be unconventional spin density wave (USDW). The pseudogap regime of high T_c superconductors LSCO, YBCO, Bi2212 and the…
Vortex tilt response in Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) vortex lattice is theoretically examined as a probe reflecting the spatial structure of this state. In the FFLO state with nodal planes perpendicular to the magnetic field in a quasi 2D material under a parallel field, the tilt modulus E_{2} {\it of the nodal planes} decreases as the paramagnetic effect is effectively enhanced, and this reduction of E_{2} in turn reduces the vortex tilt modulus. This reduction of vortex tilt modulus, more remarkable in more anisotropic systems, accompanying the FFLO transition may be an origin of …
The review of recent developments in the unconventional superconductivity theory is given. In the fist part I consider the physical origin of the Kerr rotation polarization of light reflected from the surface of superconducting $Sr_2RuO_4$. Then the comparison of magneto-optical responses in superconductors with orbital and spin spontaneous magnetization is presented. The latter result is applied to the estimation of the magneto-optical properties of neutral superfluids with spontaneous magnetization. The second part is devoted to the natural optical activity or gyrotropy properties of noncent…
We develop a fully microscopic theory for the calculations of the angle-dependent properties of unconventional superconductors under a rotated magnetic field. We employ the quasiclassical Eilenberger equations, and use a variation of the Brandt-Pesch-Tewordt (BPT) method to obtain a closed form solution for the Green's function. The equations are solved self-consistently for quasi-two-dimensional $d_{x^2-y^2}$ ($d_{xy}$) superconductors with the field rotated in the basal plane. The solution is used to determine the density of states and the specific heat. We find that applying the field along…
We derive the generalized Ginzburg-Landau free energy functional for conventional and unconventional singlet superconductors in the presence of paramagnetic, orbital and impurity effects. Within the mean field theory, we determine the criterion for appearence of the non uniform (Fulde-Ferrell-Larkin-Ovchinnikov) superconducting state, with vortex lattice structure and additional modulation along the magnetic field. We also discuss the possible change of the order of transition from normal to superconducting state. We find that the superconducting phase diagram is very sensitive to geometrical …
Measurements of the current-voltage characteristics were performed on Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals with doping level $0.044 \leq x \leq 0.1$. An unconventional increase in the flux-flow resistivity $ρ_{\rm ff}$ with decreasing magnetic field was observed across this doping range. Such an abnormal field dependence of flux-flow resistivity is in contrast with the linear field dependence of $ρ_{\rm ff}$ in conventional type-II superconductors, but is similar to the behavior recently observed in the heavy-fermion superconductor CeCoIn$_5$. A significantly enhanced $ρ_{\rm ff}$ wa…
