Ultracold atoms loaded on optical lattices can provide unprecedented experimental systems for the quantum simulations and manipulations of many quantum phases. However, so far, how to detect these quantum phases effectively remains an outstanding challenge. Here, we show that the optical Bragg scattering of cold atoms loaded on optical lattices can be used to detect many quantum phases which include not only the conventional superfluid and Mott insulating phases, but also other important phases such as various kinds of density waves (CDW), valence bond solids (VBS), CDW supersolids and VBS supersolids.
We demonstrate Babinet's principle by the absorption of high intensity light from dense clouds of ultracold atoms. Images of the diffracted light are directly related to the spatial distribution of atoms. The advantages of employing Babinet's principle as an imaging technique are that it is easy to implement and the detected signal is large. We discuss the regimes of applicability of this technique as well as its limitations.
We have formulated and experimentally demonstrated an improved algorithm for design of arbitrary two-dimensional holographic traps for ultracold atoms. Our method builds on the best previously available algorithm, MRAF, and improves on it in two ways. First, it allows for creation of holographic atom traps with a well defined background potential. Second, we experimentally show that for creating trapping potentials free of fringing artifacts it is important to go beyond the Fourier approximation in modelling light propagation. To this end, we incorporate full Helmholtz propagation into our cal…
We propose a novel approach to site-resolved detection of a 2D gas of ultracold atoms in an optical lattice. A near resonant laser beam is coherently scattered by the atomic array and its interference pattern is holographically recorded by superimposing it with a reference laser beam on a CCD chip. Fourier transformation of the recorded intensity pattern reconstructs the atomic distribution in the lattice with single-site resolution. The holographic detection method requires only a few hundred scattered photons per atom in order to achieve a high reconstruction fidelity. Therefore, additional …
The quantum mechanical few-body problem at ultracold energies poses severe challenges to theoretical techniques, particularly when long-range interactions are present that decay only as a power-law potential. In this paper we review the techniques and progress in studies of universal few-body physics for ultracold atoms, particularly those related to long-range interactions.
Ultracold atoms in optical lattices are a powerful tool for quantum simulation, precise measurement, and quantum computation. A fundamental problem in applying this quantum system is how to manipulate the higher bands or orbitals in Bloch states effectively. Here we mainly review our methods for manipulating high orbital ultracold atoms in optical lattices with different configurations. Based on these methods, we construct the atom-orbital qubit under nonadiabatic holonomic quantum control and Ramsey interferometry with trapped motional quantum states. Then we review the observation of the nov…
Experimental studies with ultracold atoms have enabled major breakthroughs in understanding three-body physics, historically a fundamental yet challenging problem. This is because the interactions among ultracold atoms can be precisely varied using magnetically tunable scattering resonances known as Feshbach resonances. The collisions of ultracold atoms have been discovered to have many universal aspects near the unitarity limit. Away from this limit, many quantum states are expected to be active during a three-body collision, making the collisional observables practically unpredictable. Here …
Imaging ultracold atomic gases close to surfaces is an important tool for the detailed analysis of experiments carried out using atom chips. We describe the critical factors that need be considered, especially when the imaging beam is purposely reflected from the surface. In particular we present methods to measure the atom-surface distance, which is a prerequisite for magnetic field imaging and studies of atom surface-interactions.
The creation of ultracold molecules is currently limited to diatomic species. In this letter we present a theoretical description of the photoassociation of ultracold atoms and molecules to create ultracold excited triatomic molecules, thus being a novel example of light-assisted ultracold chemical reaction. The calculation of the photoassociation rate of ultracold Cs atoms with ultracold Cs$_2$ molecules in their rovibrational ground state is reported, based on the solution of the quantum dynamics involving the atom-molecule long-range interactions, and assuming a model potential for the shor…
We report on a far above saturation absorption imaging technique to investigate the characteristics of dense packets of ultracold atoms. The transparency of the cloud is controlled by the incident light intensity as a result of the non-linear response of the atoms to the probe beam. We detail our experimental procedure to calibrate the imaging system for reliable quantitative measurements, and demonstrate the use of this technique to extract the profile and its spatial extent of an optically thick atomic cloud.
We report the observation of a dimer-dimer inelastic collision resonance for ultracold Feshbach molecules made of bosonic sodium and rubidium atoms. This resonance, which we attribute to the crossing of the dimer-dimer threshold with a heteronuclear tetramer state, manifests itself as a pronounced inelastic loss peak of dimers when the interspecies scattering length between the constituent atoms is tuned. Near this resonance, a strong modification of the temperature dependence of the dimer-dimer scattering is observed. Our result provides insight into the heteronuclear four-body system consist…
We report the experimental determination of the scattering parameters for a p-wave Feshbach resonance in a single component Fermi gas of 6Li atoms in the lowest spin state. The time scale of the cross-dimensional relaxation reflects the elastic scattering rate of the atoms, and scattering parameters are determined from the scattering rate as a function of magnetic field by taking into account the momentum distribution and inhomogeneous density profile of the atoms in a trap. Precise determination of the scattering parameters for a p-wave Feshbach resonance is an important step toward the reali…
Noise correlation analysis is a detection tool for spatial structures and spatial correlations in the in-trap density distribution of ultracold atoms. In this book chapter, we discuss the implementation, properties and limitations of the method applied to ensembles of ultracold atoms in optical lattices, and describe some instances where it has been applied.
Analytic expressions for the differential cross sections of ultracold atoms and molecules that scatter primarily due to dipolar interactions are derived within the first Born approximation, and are shown to agree with the partial wave expansion. These cross sections are applied to the problem of cross-dimensional rethermalization. Strikingly, the rate of rethermalization can vary by as much as a factor of two, depending on the orientation of polarization of the dipoles. Thus the anisotropic dipole-dipole interaction can have a profound effect even on the behavior of a nondegenerate ultracold g…
We investigate the occurence of Wigner-localization phenomena in bosonic dipolar ultracold few-body systems with Rashba-like spin-orbit coupling. We show that the latter strongly enhances the effects of the dipole-dipole interactions, allowing to reach the Wigner-localized regime for strengths of the dipole moment much smaller than those necessary in the spin-orbit-free case.
We propose and numerically study two permanent magnetic micro-structures for creating Ioffe-Pritchard microtraps. A bias magnetic field is used to vary the depth, trap frequencies and the minimum of each microtrap. After the Bose-Einstein condensation achievement, the bias magnetic field can be slowly removed to increase the trap barrier heights for more efficiently holding the Bose-Einstein condensates. Even without the external magnetic field, it is possible to hold ultracold atoms in the microtraps. These microtraps may also be useful for single atom experiments for quantum information proc…
A major goal of ultracold atomic physics is quantum simulation of spin Hamiltonians in optical lattices. Progress towards this goal requires the attainment of extremely low temperatures. Here we demonstrate a new cooling method which consists of applying a time-varying magnetic field gradient to a spin mixture of ultracold atoms. We have used this method to prepare isolated spin distributions at positive and negative spin temperatures of +/-50 picokelvin. The spin system can also be used to cool other degrees of freedom, and we have used this coupling to reduce the temperature of an apparently…
We describe how to realize magnetic and magneto-optical confinement of ultracold atoms in a torus with adjustable diameter and how an elliptical cloud of ultracold atoms can be adiabatically transformed to have a toroidal shape. An experiment with cold 87Rb atoms demonstrates the feasibility of shape transformations. These techniques can be used for atom interferometry and quantum computation.
Recently it has been shown that pairs of atoms can form metastable bonds due to non-conservative forces induced by dissipation [Lemeshko&Weimer, Nature Comm. 4, 2230 (2013)]. Here we study the dynamics of interaction-induced coherent population trapping - the process responsible for the formation of dissipatively bound molecules. We derive the effective dissipative potentials induced between ultracold atoms by laser light, and study the time evolution of the scattering states. We demonstrate that binding occurs on short timescales of ~10 microseconds, even if the initial kinetic energy of the …
This article reviews the development in our laboratory of magnetic lattices comprising periodic arrays of magnetic microtraps created by patterned magnetic films to trap periodic arrays of ultracold atoms. Recent achievements include the realisation of multiple Bose-Einstein condensates in a 10 micron-period one-dimensional magnetic lattice; the fabrication of sub-micron-period square and triangular magnetic lattice structures suitable for quantum tunnelling experiments; the trapping of ultracold atoms in a sub-micron-period triangular magnetic lattice; and a proposal to use long-range interac…
We review experimental and theoretical studies of coherent backscattering of near resonant radiation from an ultracold atomic gas in the weak localization regime. Recent accomplishments in high resolution spectroscopy of atomic ensembles based on the coherent backscattering process are discussed. We also propose several new experimental schemes for time-dependent spectroscopy as applied to multiple scattering in the regime of weak localization.
Ultracold molecules offer remarkable opportunities to study chemical reactions at nearly zero temperature. Although significant progresses have been achieved in exploring ultracold bimolecular reactions, the investigations are usually limited to measurements of the overall loss rates of the reactants. Detection of the reaction products will shed new light on understanding the reaction mechanism and provide a unique opportunity to study the state-to-state reaction dynamics. Here we report on the direct observation of an exoergic atom-exchange reaction in an ultracold atom-dimer mixture. Both th…
A combined experimental and theoretical investigation of time- and alignment-dependent propagation of light in an ultracold atomic gas of atomic $^{85}$Rb is reported. Coherences among the scattering amplitudes for light scattering off excited hyperfine levels produce strong variations of the light polarization in the vicinity of atomic resonance. Measurements are in excellent agreement with Monte-Carlo simulations of the multiple scattering process.
We present a general model allowing "quantum simulation" of one-dimensional Dirac models with 2- and 4-component spinors using ultracold atoms in driven 1D tilted optical latices. The resulting Dirac physics is illustrated by one of its well-known manifestations, Zitterbewegung. This general model can be extended and applied with great flexibility to more complex situations.
We show theoretically that ultracold hydrogen atoms have very favorable properties for sympathetic cooling of molecules to microkelvin temperatures. We calculate the potential energy surfaces for spin-polarized interactions of H atoms with the prototype molecules NH(triplet-Sigma-) and OH(doublet-Pi) and show that they are shallow (50 to 80 cm-1) and only weakly anisotropic. We carry out quantum collision calculations on H+NH and H+OH and show that the ratio of elastic to inelastic cross sections is high enough to allow sympathetic cooling from temperatures well over 1 K for NH and around 250 …
Charge exchange collisions between ultracold fermionic 6Li atoms and 40Ca+ ions are observed in the mK temperature range. The reaction product of the charge exchange collision is identified via mass spectrometry during which the motion of the ions is excited parametrically. The cross-sections of the charge exchange collisions between 6Li atoms in the ground state and 40Ca+ ions in the ground and metastable excited states are determined. Investigation of the inelastic collision characteristics in the atom-ion mixture is an important step toward ultracold chemistry based on ultracold atoms and i…
We present a scheme to embed molecular anions in a gas of ultracold rubidium atoms as a route towards the preparation of cold molecular ions by collisional cooling with ultracold atoms. Associative detachment as an important loss process in collisions between OH- molecules and rubidium atoms is studied. The density distribution of trapped negative ions in the multipole radiofrequency trap is measured by photodetachment tomography, which allows us to derive absolute rate coefficients for the process. We define a regime where translational and internal cooling of molecular ions embedded into the…
We have realized a hybrid optomechanical system by coupling ultracold atoms to a micromechanical membrane. The atoms are trapped in an optical lattice, which is formed by retro-reflection of a laser beam from the membrane surface. In this setup, the lattice laser light mediates an optomechanical coupling between membrane vibrations and atomic center-of-mass motion. We observe both the effect of the membrane vibrations onto the atoms as well as the backaction of the atomic motion onto the membrane. By coupling the membrane to laser-cooled atoms, we engineer the dissipation rate of the membrane.…
We study collisions of para-H$_2$ with five rare gas atomic species (He, Ne, Ar, Kr and Xe) over the range from 1 K to 1 $μ$ K and evaluate the feasibility of sympathetic cooling H$_2$ with ultracold ground state rare gas atoms co-trapped within a deep optical trap. Collision cross-sections over this large temperature range show that all of these species could be used to cool H$_2$ to ultracold temperatures and that argon and helium are the most promising species for future experiments.
We used microwave radiation to evaporatively cool a mixture of of 133Cs and 87Rb atoms in a magnetic trap. A mixture composed of an equal number (around 10^4) of Rb and Cs atoms in their doubly polarized states at ultracold temperatures was prepared. We also used microwaves to selectively evaporate atoms in different Zeeman states.
Utilizing single-photon photoassociation, we have achieved ultracold rubidium molecules with a high number density that provides a new efficient approach toward molecular quantum degeneracy. A new detection mechanism for ultracold molecule utilizing the inelastic atom-molecule collision is demonstrated. The resonant coupling effect on the formation of the ${\rm X^1Σ^+_g}$ ground state ${\rm ^{85}Rb_2}$ allows for a sufficient number of more deeply bound ultracold molecules, which induced an additional trap loss and heating of the co-existing atoms owing to the inelastic atom-molecule collision…
A quantum simulator based on ultracold optically trapped atoms for simulating the physics of atoms and molecules in ultrashort intense laser fields is introduced. The slowing down by about 13 orders of magnitude allows to watch in slow motion the tunneling and recollision processes that form the heart of attosecond science. The extreme flexibility of the simulator promises a deeper understanding of strong-field physics, especially for many-body systems beyond the reach of classical computers. The quantum simulator can experimentally straightforwardly be realized and is shown to recover the ion…
A theoretical approach is described for an exact numerical treatment of a pair of ultracold atoms interacting via a central potential that are trapped in a finite three-dimensional optical lattice. The coupling of center-of-mass and relative-motion coordinates is treated using an exact diagonalization (configuration-interaction) approach. The orthorhombic symmetry of an optical lattice with three different but orthogonal lattice vectors is explicitly considered as is the Fermionic or Bosonic symmetry in the case of indistinguishable particles.
We describe a hybrid vacuum system in which a single ion or a well defined small number of trapped ions (in our case Ba$^+$ or Rb$^+$) can be immersed into a cloud of ultracold neutral atoms (in our case Rb). This apparatus allows for the study of collisions and interactions between atoms and ions in the ultracold regime. Our setup is a combination of a Bose-Einstein condensation (BEC) apparatus and a linear Paul trap. The main design feature of the apparatus is to first separate the production locations for the ion and the ultracold atoms and then to bring the two species together. This schem…
Mixtures of ultracold quantum gases are at the heart of high-precision quantum tests of the weak equivalence principle, where extremely low expansion rates have to be reached with matter-wave lensing techniques. We propose to simplify this challenging atom-source preparation by employing magic laser wavelengths for the optical lensing potentials which guarantee that all atomic species follow identical trajectories and experience common expansion dynamics. In this way, the relative shape of the mixture is conserved during the entire evolution while cutting in half the number of required lensing…
We investigate an attractive force caused by light induced dipole-dipole interactions in freely expanding ultracold 87Rb atoms. This collective, light-triggered effect results in a self-confining potential with interesting features: it exhibits nonlocal properties, is attractive for both red and blue-detuned light fields and induces a remarkably strong force that depends on the gradient of the atomic density. The experimental data are discussed in the framework of a theoretical model based on a local-field approach for the light scattered by the atomic cloud.
We report the realization of a robust magnetic transport scheme to bring 3x10^8 ultracold 87Rb atoms into a cryostat. The sequence starts with standard laser cooling and trapping of 87Rb atoms, transporting first horizontally and then vertically through the radiation shields into a cryostat by a series of normal- and superconducting magnetic coils. Loading the atoms in a superconducting microtrap paves the way for studying the interaction of ultracold atoms with superconducting surfaces and quantum devices requiring cryogenic temperatures.
We show how impurity atoms can measure moments of ultracold atomic gas densities, using the example of bosons in a one-dimensional lattice. This builds on a body of work regarding the probing of systems by measuring the dephasing of an immersed qubit. We show this dephasing is captured by a function resembling characteristic functions of probability theory, of which the derivatives at short times reveal moments of the system operator to which the qubit couples. For a qubit formed by an impurity atom, in a system of ultracold atoms, this operator can be the density of the system at the location…
This review describes the production of atomic strontium samples at ultra-low temperature and at high phase-space density, and their possible use for physical studies and applications. We describe the process of loading a magneto-optical trap from an atomic beam and preparing the sample for high precision measurements. Particular emphasis is given to the applications of ultracold Sr samples, spanning from optical frequency metrology to force sensing at micrometer scale.
We show that the stray field generated by isolated magnetic skyrmions can be used to trap ultracold atoms. Specially, ring-shaped and double-well trapping potentials for ultracold atoms can be created by combining the field from two isolated skyrmions. The geometry size, potential barrier, trapping frequency and Majorana loss rate of these magnetic traps can be tuned by the external magnetic field or device configuration. The results here could be useful to develop atomtronics devices by manipulating the magnetic skyrmions with modern spintronics techniques.
Elastic scattering resonances occurring in ultracold collisions of either bosonic or fermionic polar molecules are investigated. The Born-Oppenheimer adiabatic representation of the two-bodydynamics provides both a qualitative classification scheme and a quantitative WKB quantization condition that predicts several sequences of resonant states. It is found that the near-threshold energy dependence of ultracold collision cross sections varies significantly with the particle exchange symmetry, with bosonic systems showing much smoother energy variations than their fermionic counterparts. Resonan…
We investigate magnetically tunable Feshbach resonances between ultracold europium atoms and between europium and alkali-metal atoms using multichannel quantum scattering calculations. For ultracold gases of europium atoms both homonuclear $^{153}$Eu+$^{153}$Eu and heteronuclear $^{151}$Eu+$^{153}$Eu systems are studied. Calculations for mixtures of europium and alkali-metal atoms are carried out for prototype systems of $^{153}$Eu+$^{87}$Rb and $^{153}$Eu+$^7$Li. We analyze the prospects for the control of scattering properties, observation of quantum chaotic behavior, and magnetoassociation …
A modified static exchange model is introduced, it could be useful to control the elastic s-wave scattering length in studying cold-atomic interaction. The theory includes the long-range van der Waals interaction in addition to short-range exchange force. The model is applied on Ps-H system to study the Feshbach resonances e.g. the s-wave elastic phase shifts and the corresponding cross sections at ultracold energies. These are compared with the data obtained using the static exchange model. A very interesting features are observed when we vary the interatomic separation i.e. the strength of d…
We explore how the extraordinary properties of Rydberg atoms can be employed to impact the motion of ultracold ground state atoms. Specifically, we use an off-resonant two-photon laser dressing to map features of the Rydberg states on ground state atoms. It is demonstrated that the interplay between the spatially varying quantization axis of the considered Ioffe-Pritchard field and the fixed polarizations of the laser transitions provides the possibility of substantially manipulating the ground state trapping potential.
We discuss the properties of ultracold Rydberg atoms in a Ioffe-Pritchard magnetic field configuration. The derived two-body Hamiltonian unveils how the large size of Rydberg atoms affects their coupling to the inhomogeneous magnetic field. The properties of the compound electronic and center of mass quantum states are thoroughly analyzed. We find very tight confinement of the center of mass motion in two dimensions to be achievable while barely changing the electronic structure compared to the field free case. This paves the way for generating a one-dimensional ultracold quantum Rydberg gas.
Cold Rydberg atoms exposed to strong magnetic fields possess unique properties which open the pathway for an intriguing many-body dynamics taking place in Rydberg gases consisting of either matter or anti-matter systems. We review both the foundations and recent developments of the field in the cold and ultracold regime where trapping and cooling of Rydberg atoms have become possible. Exotic states of moving Rydberg atoms such as giant dipole states are discussed in detail, including their formation mechanisms in a strongly magnetized cold plasma. Inhomogeneous field configurations influence t…
We study three-body recombination in an optically trapped ultracold gas of cesium atoms with precise magnetic control of the s-wave scattering length a. At large positive values of a, we measure the dependence of the rate coefficient on a and confirm the theoretically predicted scaling proportional to a^4. Evidence of recombination heating indicates the formation of very weakly bound molecules in the last bound energy level.
We estimate the radiative quenching rate of the $^{40}$Ca - $^{174}$Yb$^{+}$ molecular ion and find that it under-estimates the value reported in recent experiments by about 5 orders of magnitude. We comment on possible explanations for this large discrepancy.
Taking advantage of the known analytic expression of the eigenfunctions and eigenenergies of the Morse Hamiltonian, explicit expressions are found for the scattering length $a$ and the effective range $r_e$ which determine the s-wave scattering of ultracold atoms. The effects on $a$ and $r_e$ of considering the radial coordinate in the interval $[0,\infty)$ or in the extended region $(-\infty, \infty)$ are studied in detail.
Three-body recombination of identical, spin-polarized fermionic atoms in the ultracold limit is investigated. The mechanisms for recombination are described in terms of the ``scattering volume'' $V_p$ in the framework of the adiabatic hyperspherical representation. We have calculated numerically the recombination rate $K_3$ as a function of $V_p$ and have found that $K_3$ scales as $|V_p|^{8/3}$ for small $|V_p|$. A comparison with experimental data is also presented.
We consider the prospect of using ultracold hydrogen atoms for sympathetic cooling of fluorine atoms to microkelvin temperatures. We carry out quantum-mechanical calculations on collisions between cold F and H atoms in magnetically trappable states and show that the ratio of elastic to inelastic cross sections remains high across a wide range of temperatures and magnetic fields. For F atoms initially in the spin-stretched state ($^2$P$_{3/2}$, $f=m_f=+2$), sympathetic cooling appears likely to succeed from starting temperatures around 1 K or even higher. This occurs because inelastic collision…
We report on the loading and trapping of ultracold atoms in a one dimensional permanent magnetic lattice of period 10 micron produced on an atom chip. The grooved structure which generates the magnetic lattice potential is fabricated on a silicon substrate and coated with a perpendicularly magnetized multilayered TbGdFeCo/Cr film of effective thickness 960 nm. Ultracold atoms are evaporatively cooled in a Z-wire magnetic trap and then adiabatically transferred to the magnetic lattice potential by applying an appropriate bias field. Under our experimental conditions trap frequencies of up to 90…
We discuss the properties of Rydberg atoms in a magnetic Ioffe-Pritchard trap being commonly used in ultracold atomic physics experiments. The Hamiltonian is derived and it is demonstrated how tight traps alter the coupling of the atom to the magnetic field. We solve the underlying Schroedinger equation of the system within a given n-manifold and show that for a sufficiently large Ioffe field strength the 2n^2-dimensional system of coupled Schroedinger equations decays into several decoupled multicomponent equations governing the center of mass motion. An analysis of the fully quantized center…
We demonstrate how to realize an optical clock with neutral atoms that is competitive to the currently best single ion optical clocks in accuracy and superior in stability. Using ultracold atoms in a Ca optical frequency standard we show how to reduce the relative uncertainty to below 1E-15. We observed atom interferences for stabilization of the laser to the clock transition with a visibility of 0.36, which is 70 % of the ultimate limit achievable with atoms at rest. A novel scheme was applied to detect these atom interferences with the prospect to reach the quantum projection noise limit at …
Collisions between tightly confined atoms can lead to ionization and hence to loss of atoms from the trap. We develop second-order perturbation theory for a tensorial perturbation of a spherically symmetric system and the theory is then applied to processes mediated by the spin-dipole interaction. Redistribution and loss mechanisms are studied for the case of spin-polarized metastable helium atoms and results obtained for the five lowest s states in the trap and trapping frequencies ranging from 1 kHz to 10 MHz.
We demonstrated that final states of ultracold scattering between atom and molecule can be selectively produced using dynamic magnetic fields of multiple frequencies. The mechanism of the dynamic magnetic field control is based on a generalized quantum Zeno effect for the selected scattering channels. In particular, we use an atom-molecule spin flip scattering to show that the transition to the selected final spin projection of the molecule in the inelastic scattering can be suppressed by dynamic modulation of coupling between the Floquet engineered initial and final states.
In the laser excitation of ultracold atoms to Rydberg states, we observe a dramatic suppression caused by van der Waals interactions. This behavior is interpreted as a local excitation blockade: Rydberg atoms strongly inhibit excitation of their neighbors. We measure suppression, relative to isolated atom excitation, by up to a factor of 6.4. The dependence of this suppression on both laser irradiance and atomic density are in good agreement with a mean-field model. These results are an important step towards using ultracold Rydberg atoms in quantum information processing.
