We report on the loading and trapping of ultracold atoms in a one dimensional permanent magnetic lattice of period 10 micron produced on an atom chip. The grooved structure which generates the magnetic lattice potential is fabricated on a silicon substrate and coated with a perpendicularly magnetized multilayered TbGdFeCo/Cr film of effective thickness 960 nm. Ultracold atoms are evaporatively cooled in a Z-wire magnetic trap and then adiabatically transferred to the magnetic lattice potential by applying an appropriate bias field. Under our experimental conditions trap frequencies of up to 90 kHz in the magnetic lattice are measured and the atoms are trapped at a distance of less than 5 micron from the surface with a measured lifetime of about 450 ms. These results are important in the context of studies of quantum coherence of neutral atoms in periodic magnetic potentials on an atom chip.
We have realized a two dimensional permanent magnetic lattice of Ioffe-Pritchard microtraps for ultracold atoms. The lattice is formed by a single 300 nm magnetized layer of FePt, patterned using optical lithography. Our magnetic lattice consists of more than 15000 tightly confining microtraps with a density of 1250 traps/mm$^2$. Simple analytical approximations for the magnetic fields produced by the lattice are used to derive relevant trap parameters. We load ultracold atoms into at least 30 lattice sites at a distance of approximately 10 $μ$m from the film surface. The present result is an …
We propose and numerically study two permanent magnetic micro-structures for creating Ioffe-Pritchard microtraps. A bias magnetic field is used to vary the depth, trap frequencies and the minimum of each microtrap. After the Bose-Einstein condensation achievement, the bias magnetic field can be slowly removed to increase the trap barrier heights for more efficiently holding the Bose-Einstein condensates. Even without the external magnetic field, it is possible to hold ultracold atoms in the microtraps. These microtraps may also be useful for single atom experiments for quantum information proc…
We report on the origin of fragmentation of ultracold atoms observed on a permanent magnetic film atom chip. A novel technique is used to characterize small spatial variations of the magnetic field near the film surface using radio frequency spectroscopy of the trapped atoms. Direct observations indicate the fragmentation is due to a corrugation of the magnetic potential caused by long range inhomogeneity in the film magnetization. A model which takes into account two-dimensional variations of the film magnetization is consistent with the observations.
We report on the design, fabrication and characterization of magnetic nanostructures to create a lattice of magnetic traps with sub--micron period for trapping ultracold atoms. These magnetic nanostructures were fabricated by patterning a Co/Pd multilayered magnetic film grown on a silicon substrate using high precision e-beam lithography and reactive ion etching. The Co/Pd film was chosen for its small grain size and high remanent magnetization and coercivity. The fabricated structures are designed to magnetically trap $^{87}$Rb atoms above the surface of the magnetic film with 1D and 2D (tri…
We describe the fabrication and construction of a setup for creating lattices of magnetic microtraps for ultracold atoms on an atom chip. The lattice is defined by lithographic patterning of a permanent magnetic film. Patterned magnetic-film atom chips enable a large variety of trapping geometries over a wide range of length scales. We demonstrate an atom chip with a lattice constant of 10 $μ$m, suitable for experiments in quantum information science employing the interaction between atoms in highly-excited Rydberg energy levels. The active trapping region contains lattice regions with square …
The laser-excitation of Rydberg atoms in ultracold gases is often described assuming that the atomic motion is frozen during the excitation time. We show that this frozen gas approximation can break down for atoms that are held in optical lattices or microtraps. In particular, we show that the excitation dynamics is in general strongly affected by mechanical forces among the Rydberg atoms as well as the spread of the atomic wavepacket in the confining potential. This causes decoherence in the excitation dynamics - resulting in a dissipative blockade effect - that renders the Rydberg excitation…
Recently demonstrated superconducting atom-chips provide a platform for trapping atoms and coupling them to solid-state quantum systems. Controlling these devices requires a full understanding of the supercurrent distribution in the trapping structures. For type-II superconductors, this distribution is hysteretic in the critical state due to the partial penetration of the magnetic field in the thin superconducting film through pinned vortices. We report here an experimental observation of this memory effect. Our results are in good agreement with the redictions of the Bean model of the critica…
We report the realization of a robust magnetic transport scheme to bring 3x10^8 ultracold 87Rb atoms into a cryostat. The sequence starts with standard laser cooling and trapping of 87Rb atoms, transporting first horizontally and then vertically through the radiation shields into a cryostat by a series of normal- and superconducting magnetic coils. Loading the atoms in a superconducting microtrap paves the way for studying the interaction of ultracold atoms with superconducting surfaces and quantum devices requiring cryogenic temperatures.
Arrays of trapped atoms are the ideal starting point for developing registers comprising large numbers of physical qubits for storing and processing quantum information. One very promising approach involves neutral atom traps produced on microfabricated devices known as atom chips, as almost arbitrary trap configurations can be realised in a robust and compact package. Until now, however, atom chip experiments have focused on small systems incorporating single or only a few individual traps. Here we report experiments on a two-dimensional array of trapped ultracold atom clouds prepared using a…
This article reviews the development in our laboratory of magnetic lattices comprising periodic arrays of magnetic microtraps created by patterned magnetic films to trap periodic arrays of ultracold atoms. Recent achievements include the realisation of multiple Bose-Einstein condensates in a 10 micron-period one-dimensional magnetic lattice; the fabrication of sub-micron-period square and triangular magnetic lattice structures suitable for quantum tunnelling experiments; the trapping of ultracold atoms in a sub-micron-period triangular magnetic lattice; and a proposal to use long-range interac…
Two-dimensional arrays of optical micro-traps created by microoptical elements present a versatile and scalable architecture for neutral atom quantum information processing, quantum simulation, and the manipulation of ultra-cold quantum gases. In this article, we demonstrate advanced capabilities of this approach by introducing novel techniques and functionalities as well as the combined operation of previously separately implemented functions. We introduce piezo-actuator based transport of atom ensembles over distances of more than one trap separation, examine the capabilities of rapid atom t…
Heteronuclear alkali-metal dimers represent the class of molecules of choice for creating samples of ultracold molecules exhibiting an intrinsic large permanent electric dipole moment. Among them, the KCs molecule, with a permanent dipole moment of 1.92~Debye still remains to be observed in ultracold conditions. Based on spectroscopic studies available in the literature completed by accurate quantum chemistry calculations, we propose several optical coherent schemes to create ultracold bosonic and fermionic KCs molecules in their absolute rovibrational ground level, starting from a weakly boun…
We propose a scheme to realize a heavy Rydberg system (HRS), a bound pair of oppositely charged ions, from a gas of ultracold atoms. The intermediate step to achieve large internuclear separations is the creation of a unique class of ultra-long-range Rydberg molecules bound in a stairwell potential energy curve. Here, a ground-state atom is bound to a Rydberg atom in an oscillatory potential emerging due to attractive singlet $p$-wave electron scattering. The utility of our approach originates in the large electronic dipole transition element between the Rydberg- and the ionic molecule, while …
The properties of the electronic ground state of the polar and paramagnetic chromium--closed-shell-atom molecules have been investigated. State-of-the-art \textit{ab initio} techniques have been applied to compute the potential energy curves for the chromium--alkaline-earth-metal-atom, CrX (X = Be, Mg, Ca, Sr, Ba), and chromium--ytterbium, CrYb, molecules in the Born-Oppenheimer approximation for the $X^7Σ^+$ high-spin electronic ground state. The spin restricted open-shell coupled cluster method restricted to single, double, and noniterative triple excitations, RCCSD(T), was employed and the …
We study the effects of a static electric field on the photoassociation of a heteronuclear atom-pair into a polar molecule. The interaction of permanent dipole moment with a static electric field largely affects the ground state continuum wave function of the atom-pair at short separations where photoassociation transitions occur according to Franck-Condon principle. Electric field induced anisotropic interaction between two heteronuclear ground state atoms leads to scattering resonances at some specific electric fields. Near such resonances the amplitude of scattering wave function at short s…
We report on the implementation of a dynamically configurable, servomotor- controlled, permanent magnet Zeeman slower for quantum optics experiments with ultracold atoms and molecules. This atom slower allows for switching between magnetic field profiles that are designed for different atomic species. Additionally, through feedback on the atom trapping rate, we demonstrate that computer-controlled genetic optimization algorithms applied to the magnet positions can be used in situ to obtain field profiles that maximize the trapping rate for any given experimental conditions. The device is light…
We report the creation of ultracold bosonic $^{23}$Na$^{87}$Rb Feshbach molecules via magneto-association. By ramping the magnetic field across an interspecies Feshbach resonance, at least 4000 molecules can be produced out of the near degenerate ultracold mixture. Fast loss due to inelastic atom-molecule collisions is observed, which limits the pure molecule number, after residual atoms removal, to 1700. The pure molecule sample can live for 21.8(8) ms in the optical trap, long enough for future molecular spectroscopy studies toward coherently transferring to the singlet ro-vibrational ground…
We provide an introduction to the experimental physics of quantum gases. At the low densities of ultracold quantum gases, confinement can be understood from single-particle physics, and interactions can be understood from two-body physics. The structure of atoms provides resonances both in the optical domain and in the radio-frequency domain. Atomic structure data is given for the 27 atomic isotopes that had been brought to quantum degeneracy at the time this chapter was written. We discuss the motivations behind choosing among these species. We review how static and oscillatory fields are tre…
We study the quantum properties of Rydberg atoms in a magnetic Ioffe-Pritchard trap which is superimposed by a homogeneous electric field. Trapped Rydberg atoms can be created in long-lived electronic states exhibiting a permanent electric dipole moment of several hundred Debye. The resulting dipole-dipole interaction in conjunction with the radial confinement is demonstrated to give rise to an effectively one-dimensional ultracold Rydberg gas with a macroscopic interparticle distance. We derive analytical expressions for the electric dipole moment and the critical linear density of Rydberg at…
We present a time-independent quantum formalism to describe the dynamics of molecules with permanent electric dipole moments in a two-dimensional confined geometry such as a one-dimensional optical lattice, in the presence of an electric field. Bose/Fermi statistics and selection rules play a crucial role in the dynamics. As examples, we compare the dynamics of confined fermionic and bosonic polar KRb molecules under different confinements and electric fields. We show how chemical reactions can be suppressed, either by a "statistical suppression" which applies for fermions at small electric fi…
Progress in ultracold experiments with polar molecules requires a clear understanding of their interactions and reactivity at ultra-low collisional energies. Two important theoretical steps in this process are the characterization of interaction potentials between molecules and the modeling of reactive scattering mechanism. Here, we report on the {\it abinitio} calculation of isotropic and anisotropic van der Waals interaction potentials for polar KRb and RbCs colliding with each other or with ultracold atoms. Based on these potentials and two short-range scattering parameters we then develop …
We investigate the formation of weakly bound, electronically excited, heteronuclear 6Li40K* molecules by single-photon photoassociation in a magneto-optical trap. We performed trap loss spectroscopy within a range of 325 GHz below the Li(2S_(1/2))+K(4P_(3/2)) and Li(2S_(1/2))+K(4P_(1/2)) asymptotic states and observed more than 60 resonances, which we identify as rovibrational levels of 7 of 8 attractive long-range molecular potentials. The long-range dispersion coefficients and rotational constants are derived. We find large molecule formation rates of up to ~3.5x10^7s^(-1), which are shown t…
The Ca$^+$, Sr$^+$, Ba$^+$, and Yb$^+$ ions immersed in an ultracold gas of the Cr atoms are proposed as experimentally feasible heteronuclear systems in which ion-atom interactions at ultralow temperatures can be controlled with magnetically tunable Feshbach resonances without charge transfer and radiative losses. \textit{Ab initio} techniques are applied to investigate electronic-ground-state properties of the (CaCr)$^+$, (SrCr)$^+$, (BaCr)$^+$, and (YbCr)$^+$ molecular ions. The potential energy curves, permanent electric dipole moments, and static electric dipole polarizabilities are compu…
Experiments with cold ion-atom mixtures have recently opened the way for the production and application of ultracold molecular ions. Here, in a comparative study, we theoretically investigate ground and several excited electronic states and prospects for the formation of molecular ions composed of a calcium ion and an alkali-metal atom: CaAlk$^{+}$ (Alk=Li, Na, K, Rb, Cs). We use a quantum chemistry approach based on non-empirical pseudopotential, operatorial core-valence correlation, large Gaussian basis sets, and full configuration interaction method for valence electrons. Adiabatic potentia…
Ultracold YbAg molecules have been recently proposed as promising candidates for electron electric dipole moment searches [Verma, Jayich, and Vutha, Phys. Rev. Lett. 125, 153201 (2020)]. Here, we calculate potential energy curves, permanent electric dipole and quadrupole moments, and static electric dipole polarizabilities for the YbCu, YbAg, and YbAu molecules in their ground electronic states. We use the coupled cluster method restricted to single, double, and noniterative triple excitations with large Gaussian basis sets, while the scalar relativistic effects are included within the small-c…
We consider collisional properties of polyatomic aromatic hydrocarbon molecules immersed into ultracold atomic gases and investigate intermolecular interactions of exemplary benzene, naphthalene, and azulene with alkali-metal (Li, Na, K, Rb, Cs) and alkaline-earth-metal (Mg, Ca, Sr, Ba) atoms. We apply the state-of-the-art \textit{ab initio} techniques to compute the potential energy surfaces (PESs). We use the coupled cluster method restricted to single, double, and noniterative triple excitations to reproduce the correlation energy and the small-core energy-consistent pseudopotentials to mod…
Alkaline-earth-like transition-metal atoms such as Zn and Cd are promising candidates for precision measurements and quantum many-body physics experiments. Here, we theoretically investigate the properties of diatomic molecules containing these closed-shell atoms. We calculate potential energy curves, permanent electric dipole moments, and spectroscopic constants for molecules consisting of either a Zn or Cd atom interacting with an alkali-metal (Li, Na, K, Rb, Cs, Fr) or alkaline-earth-metal (Be, Mg, Ca, Sr, Ba, Ra) atom. We use the ab initio electronic structure coupled cluster method with s…
Spin models are the prime example of simplified manybody Hamiltonians used to model complex, real-world strongly correlated materials. However, despite their simplified character, their dynamics often cannot be simulated exactly on classical computers as soon as the number of particles exceeds a few tens. For this reason, the quantum simulation of spin Hamiltonians using the tools of atomic and molecular physics has become very active over the last years, using ultracold atoms or molecules in optical lattices, or trapped ions. All of these approaches have their own assets, but also limitations…
We have designed and realized magnetic trapping geometries for ultracold atoms based on permanent magnetic films. Magnetic chip based experiments give a high level of control over trap barriers and geometric boundaries in a compact experimental setup. These structures can be used to study quantum spin physics in a wide range of energies and length scales. By introducing defects into a triangular lattice, kagome and hexagonal lattice structures can be created. Rectangular lattices and (quasi-)one-dimensional structures such as ladders and diamond chain trapping potentials have also been created…
