The effects of a nearby two-level charge fluctuator on a double-dot two-spin qubit are studied theoretically. Assuming no direct tunneling between the charge fluctuator and the qubit quantum dots, the Coulomb couplings between the qubit orbital states and the fluctuator are calculated within the Hund-Mulliken framework to quadrupole-quadrupole order in a multipole expansion. We identify and quantify the coupling term that entangles the qubit to the fluctuator and analyze qubit decoherence effects that result from the decay of the fluctuator to its reservoir. Our results show that the charge environment can severely impact the performance of spin qubits, and indicate working points at which this decoherence channel is minimized. Our analysis also suggests that an ancillary double-dot can provide a convenient point for single-qubit operations and idle position, adding flexibility in the quantum control of the two-spin qubit.
1/f noise, the major source of dephasing in Josephson qubits, may be produced by an ensemble of two-level systems. Depending on the statistical properties of their distribution, the noise distribution can be Gaussian or non-Gaussian. The latter situation is realized, for instance, when the distribution of coupling strengths has a slowly decaying power-law tail. In this regime questions of self-averaging and sample-to-sample fluctuations become crucial. We study the dephasing process for a class of distribution functions and analyze the self-averaging properties of the results.
The efficiency of the future devices for quantum information processing is limited mostly by the finite decoherence rates of the qubits. Recently a substantial progress was achieved in enhancing the time, which a solid-state qubit demonstrates a coherent dynamics. This progress is based mostly on a successful isolation of the qubits from external decoherence sources. Under these conditions the material-inherent sources of noise start to play a crucial role. In most cases the noise that quantum device demonstrate has 1/f spectrum. This suggests that the environment that destroys the phase coher…
We investigate the decoherence of a qubit coupled to either a quantum two-level system (TLS) again coupled to an environment, or a classical fluctuator modeled by random telegraph noise. In order to do this we construct a model for the quantum TLS where we can adjust the temperature of its environment, and the decoherence rate independently. The model has a well-defined classical limit at any temperature and this corresponds to the appropriate random telegraph process, which is symmetric at high temperatures and becomes asymmetric at low temperatures. We find that the difference in the qubit d…
We study decoherence in a qubit with the distance between the two levels affected by random flips of bistable fluctuators. For the case of a single fluctuator we evaluate explicitly an exact expression for the phase-memory decay in the echo experiment with a resonant ac excitation. The echo signal as a function of time shows a sequence of plateaus. The position and the height of the plateaus can be used to extract the fluctuator switching rate γand its coupling strength v. At small times the logarithm of the echo signal is proportional to t^3. The plateaus disappear when the decoherence is ind…
The major contribution to decoherence of a double quantum dot or a Josephson junction charge qubit comes from the electrostatic coupling to fluctuating background charges hybridized with the conduction electrons in the reservoir. However, estimations according to previously developed theories show that finding a sufficient number of effective fluctuators in a realistic experimental layout is quite improbable. We show that this paradox is resolved by allowing for a short-range Coulomb interaction of the fluctuators with the electrons in the reservoir. This dramatically enhances both the number …
We report on long-term measurements of a highly coherent, non-tunable superconducting transmon qubit, revealing low-frequency burst noise in coherence times and qubit transition frequency. We achieve this through a simultaneous measurement of the qubit's relaxation and dephasing rate as well as its resonance frequency. The analysis of correlations between these parameters yields information about the microscopic origin of the intrinsic decoherence mechanisms in Josephson qubits. Our results are consistent with a small number of microscopic two-level systems located at the edges of the supercon…
By performing experiments with thin-film resonators of NbSi, we elucidate a decoherence mechanism at work in disordered superconductors. This decoherence is caused by charged Two Level Systems (TLS) which couple to the conduction electrons in the BCS ground state; it does not involve any out-of-equilibrium quasiparticles, vortices, etc. Standard theories of mesoscopic disordered conductors enable making predictions regarding this mechanism, notably that decoherence should increase as the superconductor cross section decreases. Given the omnipresence of charged TLS in solid-state systems, this …
Thermal-fluctuator driven decoherence of an oscillator resonantly coupled to a two-level system
School of Physics and Astronomy and Centre for the Mathematics and Theoretical Physics of Quantum Non-Equilibrium Systems, University of Nottingham（诺丁汉大学物理与天文学院及量子非平衡系统数学与理论物理中心）
We study dynamical decoupling of a qubit from non gaussian quantum noise due to discrete sources, as bistable fluctuators and 1/f noise. We obtain analytic and numerical results for generic operating point. For very large pulse frequency, where dynamic decoupling compensates decoherence, we found universal behavior. At intermediate frequencies noise can be compensated or enhanced, depending on the nature of the fluctuators and on the operating point. Our technique can be applied to a larger class of non-gaussian environments.
We study the effect of charge and spin noise on singlet-triplet qubits in Si quantum dots. We set up a theoretical framework aimed at enabling experiment to efficiently identify the most deleterious defects, and complement it with the knowledge of defects gained in decades of industrial and academic work. We relate the dephasing rates $Γ_ϕ$ due to various classes of defects to experimentally measurable parameters such as charge dipole moment, spin dipole moment and fluctuator switching times. We find that charge fluctuators are more efficient in causing dephasing than spin fluctuators.
We propose and study a model of dephasing due to an environment of bistable fluctuators. We apply our analysis to decoherence of Josephson Qubits, induced by background charges present in the substrate, which are also responsible for the 1/f noise. The discrete nature of the environment leads to a number of new features which are mostly pronounced for slowly moving charges. Far away from degeneracy this model for the dephasing is solved exactly.
We study a pair of quantum dot exciton qubits interacting with a number of fluctuating charges that can induce a Stark shift of both exciton transition energies. We do this by solving the optical master equation using a numerical transfer matrix method. We find that the collective influence of the charge environment on the dots can be detected by measuring the correlation between the photons emitted when each dot is driven independently. Qubits in a common charge environment display photon bunching, if both dots are driven on resonance or if the driving laser detunings have the same sense for …
We consider quantum decoherence in solid-state systems by studying the transverse dynamics of a single qubit interacting with a fermionic bath and driven by external pulses. Our interest is in investigating the extent to which the lost coherence can be restored by the application of external pulses to the qubit. We show that the qubit evolution under various pulse sequences can be mapped onto Keldysh path integrals. This approach allows a simple diagrammatic treatment of different bath excitation processes contributing to qubit decoherence. We apply this theory to the evolution of the qubit co…
We study the dynamics of dephasing in a quantum two-level system by modeling both 1/f and high-frequency noise by random telegraph processes. Our approach is based on a so-called spin-fluctuator model in which a noisy environment is modeled by a large number of fluctuators. In the continuous limit we obtain an effective random process (ERP) that is described by a distribution function of the fluctuators. In a simplified model, we reduce the ERP to the two (slow and fast) ensembles of fluctuators. Using this model, we study decoherence in a superconducting flux qubit and we compare our theoreti…
With the growing efforts in isolating solid-state qubits from external decoherence sources, the material-inherent sources of noise start to play crucial role. One representative example is electron traps in the device material or substrate. Electrons can tunnel or hop between a charged and an empty trap, or between a trap and a gate electrode. A single trap typically produces telegraph noise and can hence be modeled as a bistable fluctuator. Since the distribution of hopping rates is exponentially broad, many traps produce flicker-noise with spectrum close to 1/f. Here we develop a theory of d…
We investigate heavy-hole spin relaxation and decoherence in quantum dots in perpendicular magnetic fields. We show that at low temperatures the spin decoherence time is two times longer than the spin relaxation time. We find that the spin relaxation time for heavy holes can be comparable to or even longer than that for electrons in strongly two-dimensional quantum dots. We discuss the difference in the magnetic-field dependence of the spin relaxation rate due to Rashba or Dresselhaus spin-orbit coupling for systems with positive (i.e., GaAs quantum dots) or negative (i.e., InAs quantum dots) …
In this article we review our work on the dynamics and decoherence of electron and hole spins in single and double quantum dots. The first part, on electron spins, focuses on decoherence induced via the hyperfine interaction while the second part covers decoherence and relaxation of heavy-hole spins due to spin-orbit interaction as well as the manipulation of heavy-hole spin using electric dipole spin resonance.
We review recent studies on spin decoherence of electrons and holes in quasi-two-dimensional quantum dots, as well as electron-spin relaxation in nanowire quantum dots. The spins of confined electrons and holes are considered major candidates for the realization of quantum information storage and processing devices, provided that sufficently long coherence and relaxation times can be achieved. The results presented here indicate that this prerequisite might be realized in both electron and hole quantum dots, taking one large step towards quantum computation with spin qubits.
In double quantum dots, the exchange interaction between two electron spins renormalizes the excitation energy of pair-flips in the nuclear spin bath, which in turn modifies the non-Markovian bath dynamics. As the energy renormalization varies with the Overhauser field mismatch between the quantum dots, the electron singlet-triplet decoherence resulting from the bath dynamics depends on sampling of nuclear spin states from an ensemble, leading to the transition from exponential decoherence in single-sample dynamics to power-law decay under ensemble averaging. In contrast, the decoherence of a …
We discuss various methods of all-optical spin control in semiconductor quantum dots. We present different ways of rotating a single confined electron spin by optical coupling to a trion state. We also discuss a method for controlling the polarization of a confined exciton via a two-photon transition. Finally, we analyze the effect of phonon-induced decoherence on the fidelity of these optical spin control protocols.
We study the collective interaction of excitons in closely spaced artificial molecules and arrays of nearly identical quantum dots with the electromagnetic modes. We discuss how collective fluorescence builds up in the presence of a small mismatch of the transition energy. We show that a superradiant state of a single exciton in a molecule of two dots with realistic energy mismatch undergoes a two-rate decay. We analyze also the stability of subdecoherent states for non-identical systems.
The effects resulting due to dressing of an exciton with phonons are analysed as the source of unavoidable decoherence of orbital degrees of freedom in quantum dots. The dressing with longitudinal optical phonons results in energetic shift of order of a few meV even of the ground state of exciton in a state-of-the-art InAs/GaAs dot and the mediating role of longitudinal acoustical phonons is essential in this process. The characteristic time needed for dressing of the exciton with optical phonons is of a picosecond order. That time can be regarded as the lowest limit for decoherence for optica…
This Chapter contains a review of the recent results, both experimental and theoretical, related to optical control of carriers confined in semiconductor quantum dots. The physics of Rabi oscillations of exciton and biexciton occupations, as well as time-domain interference experiments are discussed. Next, the impact of carrier--phonon interaction in a semiconductor structure is described and modern methods of theoretical description of the carrier--phonon kinetics and of the resulting dephasing are presented.
We investigate in detail, using both analytical and numerical tools, the decoherence of electron spins in quantum dots (QDs) coupled to a bath of nuclear spins in magnetic fields or with various initial bath polarizations, focusing on the longitudinal relaxation in low and moderate field/polarization regimes. An increase of the initial polarization of nuclear spin bath has the same effect on the decoherence process as an increase of the external magnetic field, namely, the decoherence dynamics changes from smooth decay to damped oscillations. This change can be observed experimentally for a si…
We theoretically consider charge transport through two quantum dots coupled in series. The corresponding full counting statistics for noninteracting electrons is investigated in the limits of sequential and coherent tunneling by means of a master equation approach and a density matrix formalism, respectively. We clearly demonstrate the effect of quantum coherence on the zero-frequency cumulants of the transport process, focusing on noise and skewness. Moreover, we establish the continuous transition from the coherent to the incoherent tunneling limit in all cumulants of the transport process a…
Combining scattering matrix theory with non-linear $σ$-model and Keldysh technique we develop a unified theoretical approach enabling one to non-perturbatively study the effect of electron-electron interactions on weak localization and Aharonov-Bohm oscillations in arbitrary arrays of quantum dots. Our model embraces (i) weakly disordered conductors (ii) strongly disordered conductors and (iii) metallic quantum dots. In all these cases at $T \to 0$ the electron decoherence time is found to saturate to a finite value determined by the universal formula which agrees quantitatively with numerous …
We used resonant laser spectroscopy of multiple confocal InGaAs quantum dots to spatially locate charge fluctuators in the surrounding semiconductor matrix. By mapping out the resonance condition between a narrow-band laser and the neutral exciton transitions of individual dots in a field effect device, we identified spectral discontinuities as arising from charging and discharging events that take place within the volume adjacent to the quantum dots. Our analysis suggests that residual carbon dopants are a major source of charge-fluctuating traps in quantum dot heterostructures.
Using the Algebraic Bethe Ansatz in conjunction with a simple Monte Carlo sampling technique, we study the problem of the decoherence of a central spin coupled to a nuclear spin bath. We describe in detail the full crossover from strong to weak external magnetic field field, a limit where a large non-decaying coherence factor is found. This feature is explained by Bose-Einstein-condensate-like physics which also allows us to argue that the corresponding zero frequency peak would not be broadened by statistical or ensemble averaging.
We analyse various phonon-assisted mechanisms which contribute to the decoherence of excitonic qubits in quantum dot systems coupled by the Förster-type transfer process. We show the significant loss of coherence accompanied by dissipation due to charge carrier oscillations between qubit states by using a model of one-phonon assisted Förster-type transfer process. We obtain explicit expressions for the relaxation and dephasing times for excitonic qubits interacting with acoustic phonons via both deformation potential and piezoelectric coupling. We compare the decoherence times of the GaAs/AlGa…
Destructive interference of single-electron tunneling between three quantum dots can trap an electron in a coherent superposition of charge on two of the dots. Coupling to external charges causes decoherence of this superposition, and in the presence of a large bias voltage each decoherence event transfers a certain number of electrons through the device. We calculate the counting statistics of the transferred charges, finding a crossover from sub-Poissonian to super-Poissonian statistics with increasing ratio of tunnel and decoherence rates.
We investigate electron charge decoherence in a laterally-coupled single-electron semiconductor double quantum dot through electron-phonon interaction. We analytically and numerically evaluate the relaxation and dephasing rates due to electron coupling to both acoustic and optical phonons, and explore the system parameter space in terms of interdot distance, strength of single-dot confinement, and inter-dot coupling strength. Our numerical results show that the electron scattering rates are strongly dependent on the strength of the electron confinement and the size of the system. In addition, …
Coupled quantum dots are an example of the ubiquitous quantum double potential well. In a typical transport experiment, each quantum dot is also coupled to a continuum of states. Our approach takes this into account by using a Green's function formalism to solve the full system. The time-dependent solution is then explored in different limiting cases. In general, a combination of coherent and incoherent behavior is observed. In the case that the coupling of each dot to the macroscopic world is equal, however, the time evolution is purely coherent.
We present experiments on the dynamics of a two-state parametric fluctuator in a superconducting flux qubit. In spectroscopic measurements, the fluctuator manifests itself as a doublet line. When the qubit is excited in resonance with one of the two doublet lines, the correlation of readout results exhibits an exponential time decay which provides a measure of the fluctuator transition rate. The rate increases with temperature in the interval 40 to 158 mK. Based on the magnitude of the transition rate and the doublet line splitting we conclude that the fluctuation is induced by quasiparticle t…
We review our recent contributions to two topics that have become of interest in the field of open, dissipative quantum systems: non-Gaussian noise and decoherence in fermionic systems. Decoherence by non-Gaussian noise, i.e. by an environment that cannot be approximated as a bath of harmonic oscillators, is important in nanostructures (e.g. qubits) where there might be strong coupling to a small number of fluctuators. We first revisit the pedagogical example of dephasing by classical telegraph noise. Then we address two models where the quantum nature of the noise becomes essential: "quantum …
A tunable microwave scattering device is presented which allows the controlled variation of Fano line shape parameters in transmission through quantum billiards. We observe a non-monotonic evolution of resonance parameters that is explained in terms of interacting resonances. The dissipation of radiation in the cavity walls leads to decoherence and thus to a modification of the Fano profile. We show that the imaginary part of the complex Fano q-parameter allows to determine the absorption constant of the cavity. Our theoretical results demonstrate further that the two decohering mechanisms, de…
We study the dynamics of an electron spin in a graphene quantum dot, which is interacting with a bath of less than ten nuclear spins via the anisotropic hyperfine interaction. Due to substantial progress in the fabrication of graphene quantum dots, the consideration of such a small number of nuclear spins is experimentally relevant. This choice allows us to use exact diagonalization to calculate the longtime average of the electron spin as well as its decoherence time. We investigate the dependence of spin observables on the initial states of nuclear spins and on the position of nuclear spins …
We study the decoherence of a single electron spin in an isolated quantum dot induced by hyperfine interaction with nuclei for times smaller than the nuclear spin relaxation time. The decay is caused by the spatial variation of the electron envelope wave function within the dot, leading to a non-uniform hyperfine coupling. We evaluate the spin correlation function with and without magnetic fields and find that the decay of the spin precession amplitude is not exponential but rather power (inverse logarithm) law-like. For fully polarized nuclei we find an exact solution and show that the preces…
We propose to use optical detection of magnetic resonance (ODMR) to measure the decoherence time T_{2} of a single electron spin in a semiconductor quantum dot. The electron is in one of the spin 1/2 states and a circularly polarized laser can only create an optical excitation for one of the electron spin states due to Pauli blocking. An applied electron spin resonance (ESR) field leads to Rabi spin flips and thus to a modulation of the photoluminescence or, alternatively, of the photocurrent. This allows one to measure the ESR linewidth and the coherent Rabi oscillations, from which the elect…
Recent experiments on Josephson junction qubits have suggested the existence in the tunnel barrier of bistable two level fluctuators that are responsible for decoherence and 1/f critical current noise. In this article we treat these two-level systems as fictitious spins and investigate their influence quantum mechanically with both analytical and numerical means. We find that the Rabi oscillations of the qubit exhibit multiple stages of decay. New approaches are established to characterize different decoherence times and to allow for easier feature extraction from experimental data. The Rabi o…
Solid state quantum bits are a promising candidate for the realization of a scalable quantum computer, however, they are usually strongly limited by decoherence. We consider a double quantum dot charge qubit, whose basis states are defined by the position of an additional electron in the system of two laterally coupled quantum dots. The coupling of these two states can be controlled externally by a quantum point contact between the two dots. We discuss the decoherence through coupling to the electronic leads due to cotunneling processes. We focus on a simple Gedanken experiment, where the syst…
We theoretically consider the effect of strain on the spin dynamics of a single heavy-hole (HH) confined to a self-assembled quantum dot and interacting with the surrounding nuclei via hyperfine interaction. Confinement and strain hybridize the HH states, which show an exponential decay for a narrowed nuclear spin bath. For different strain configurations within the dot, the dependence of the spin decoherence time $T_2$ on external parameters is shifted and the non-monotonic dependence of the peak is altered. Application of external strain yields considerable shifts in the dependence of $T_2$ …
With the growing efforts in isolating solid-state qubits from external decoherence sources, the origins of noise inherent to the material start to play a relevant role. One representative example are charged impurities in the device material or substrate, which typically produce telegraph noise and can hence be modelled as bistable fluctuators. In order to demonstrate the possibility of the active suppression of the disturbance from a {\em single} fluctuator, we theoretically implement an elementary bang-bang control protocol. We numerically simulate the random walk of the qubit state on the B…
We analytically calculate the nuclear-spin interactions of a single electron confined to a carbon nanotube or graphene quantum dot. While the conduction-band states in graphene are p-type, the accordant states in a carbon nanotube are sp-hybridized due to curvature. This leads to an interesting interplay between isotropic and anisotropic hyperfine interactions. By using only analytical methods, we are able to show how the interaction strength depends on important physical parameters, such as curvature and isotope abundances. We show that for the investigated carbon structures, the 13C hyperfin…
We demonstrate full suppression of dephasing tied to deformation potential coupling of confined electrons to longitunidal acoustic (LA) phonons in optical control experiments on large semiconductor quantum dots (QDs) with emission compatible with the low-dispersion telecommunications band at 1.3~$μ$m. By exploiting the sensitivity of the electron-phonon spectral density to the size and shape of the QD, we demonstrate a four-fold reduction in the threshold pulse area required to enter the decoupled regime for exciton inversion using adiabatic rapid passage (ARP). Our calculations of the quantum…
In this thesis I find an analytic expression for the conductance of a single electron transistor in the regime when temperature, level spacing, and charging energy of an island are all of the same order. I also study the correction to the spacing between Coulomb blockade peaks due to finite dot-lead tunnel couplings. I find analytic expressions for both correction to the spacing averaged over mesoscopic fluctuations and the rms of the correction fluctuations. In the second part of the thesis I discuss the feasibility of quantum dot based spin- and charge-qubits. Firstly, I study the effect of …
We study the evolution of a quantum dot controlled by a frequency-swept (chirped), linearly polarized laser pulse in the presence of carrier-phonon coupling. The final occupation of the exciton state is limited both due to phonon-induced transitions between the adiabatic spectral branches and because of phonon-assisted transitions to the biexciton state. When the biexciton shift is large enough, the quantum dot can be modeled as a two-level system, which corresponds to excitation with circularly polarized light. For this case, we compare different methods of simulations: (i) a time convolution…
The interplay between interference effects and electron-electron interactions in electron transport through an interacting double quantum dot system is investigated using a hierarchical quantum master equation approach which becomes exact if carried to infinite order and converges well if the temperature is not too low. Decoherence due to electron-electron interactions is found to give rise to pronounced negative differential resistance, enhanced broadening of structures in current-voltage characteristics and an inversion of the electronic population. Dependence on gate voltage is shown to be …
We investigate the spin relaxation and decoherence in a single-electron graphene quantum dot with Rashba and intrinsic spin-orbit interactions. We derive an effective spin-phonon Hamiltonian via the Schrieffer-Wolff transformation in order to calculate the spin relaxation time T_1 and decoherence time T_2 within the framework of the Bloch-Redfield theory. In this model, the emergence of a non-monotonic dependence of T_1 on the external magnetic field is attributed to the Rashba spin-orbit coupling-induced anticrossing of opposite spin states. A rapid decrease of T_1 occurs when the spin and or…
We investigate theoretically acoustic phonon induced decoherence in quantum dots. We calculate the dephasing of fundamental (interband or intraband) optical transitions due to real and virtual transitions with higher energy levels. Up to two acoustic phonon processes (absorption and/or emission) are taken into account simultaneously in a non-perturbative manner. An analytic expression of acoustic phonon induced broadening is given as a function of the electron-phonon matrix elements and is physically interpreted. The theory is applied to the dephasing of intersublevel transitions in self-assem…
We analyze how decoherence appears in the I-V characteristics of a voltage-biased single-Cooper-pair transistor. Especially the effect on resonant single or several Cooper-pair tunneling is studied. We consider both a symmetric and an asymmetric transistor. As a decoherence source we use a small resistive impedance (Re[Z(w)]<<R_Q=h/4e^2) in series with the transistor, which provides both thermal and quantum fluctuations of the voltage. Additional decoherence sources are quasiparticle tunneling across the Josephson junctions and quantum f-noise caused by spurious charge fluctuators nearby the i…
We uncover two microscopic physical settings with significant pure spin decoherence. First, for quantum dots (QD) electrostatically confined in two-dimensional hole gas, decoherence comes from qubit spin-orbit (SO) coupling to phonons, whose decay due to free charge carriers in contacts is described by Ohmic weighted phonon spectral function. We derive significant SO interactions affecting holes with origin and symmetry distinct from that of conventionally considered Dresselhaus and Rashba terms. In the second setting of electron or hole QDs coupled to a linear chain of atoms, decoherence is d…
Decoherence in nearly-isolated GaAs quantum dots is investigated using the change in average Coulomb blockade peak height upon breaking time-reversal symmetry. The normalized change in average peak height approaches the predicted universal value of 1/4 at temperatures well below the single-particle level spacing, but is greatly suppressed for temperature greater than the level spacing, suggesting that inelastic scattering or other dephasing mechanisms dominate in this regime.
