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arXiv 0907.5070cond-mat.str-el
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GaFeO_3的光磁电效应分析

Analysis of optical magnetoelectric effect in GaFeO_3

Jun-ichi Igarashi, Tatsuya Nagao

摘要:

研究了极性亚铁磁体GaFeO_3的光吸收谱。我们考虑了Fe原子上的E1、E2和M1过程。结果表明,在Fe原子的非中心对称环境中,由于4p和3d态的杂化,产生了E1-M1干涉过程,从而产生了对吸收谱的磁电效应.我们对由八面体氧原子和偏离中心的Fe原子组成的FeO_6团簇模型进行了光谱的微观计算,计算中考虑了合理的库仑相互作用和杂化作用。我们得到的磁电光谱,这取决于磁化的方向,作为光子能量的函数在光学区域1.0-2.5 eV,与实验一致。

英文摘要:

We study the optical absorption spectra in a polar ferrimagnet GaFeO_3. We consider the E1, E2 and M1 processes on Fe atoms. It is shown that the magnetoelectric effect on the absorption spectra arises from the E1-M1 interference process through the hybridization between the 4p and 3d states in the noncentrosymmetry environment of Fe atoms. We perform a microscopic calculation of the spectra on a cluster model of FeO_6 consisting of an octahedron of O atoms and an Fe atom displaced from the center with reasonable values for Coulomb interaction and hybridization. We obtain the magnetoelectric spectra, which depend on the direction of magnetization, as a function of photon energy in the optical region 1.0-2.5 eV, in agreement with the experiment.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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