我们报告了一个新的四元硼碳化物PrRh $_{2}$ B $_{2}$ C，磁化强度，电阻率和比热研究的基础上的磁性和输运性质。该化合物形成LuNi $_{2}$ B $_{2}$ C型四元结构（空间群{ \it I4/mmm}），并且在低至0.5 K时不表现出磁有序或超导性。比热数据的晶体场分析表明，在该化合物的单重基态。索末菲系数$γ$ $\approx$ 250 mJ/mole K $^{2}$的高值以及单重基态表明PrRh $_{2}$ B $_{2}$ C中的重费米子行为是由传导电子与低位晶场激发的相互作用引起的。在压力高达23 kbar的情况下，没有观察到PrRh $_{2}$ B $_{2}$ C中的磁有序或超导性。
英文摘要：
We report magnetic and transport properties of a new quaternary borocarbide PrRh$_{2}$B$_{2}$C, based on magnetisation, resistivity and specific heat studies. This compound forms in LuNi$_{2}$B$_{2}$C-type tetragonal structure (space group {\it I4/mmm}) and does not exhibit magnetic ordering or superconductivity down to 0.5 K. The crystal field analysis of specific heat data suggests a singlet ground state in this compound. The high value of the Sommerfeld coefficient, $γ$ $\approx$ 250 mJ/mole K$^{2}$, together with a singlet ground state suggests that the heavy fermion behaviour in PrRh$_{2}$B$_{2}$C results from the interaction of the conduction electrons with the low lying crystal field excitations. No signature of magnetic ordering or superconductivity is observed in PrRh$_{2}$B$_{2}$C under the application of pressure up to 23 kbar.
Photoinduced dynamics in an excitonic insulator is studied theoretically by using a two-orbital Hubbard model on the square lattice where the excitonic phase in the ground state is characterized by the BCS-BEC crossover as a function of the interorbital Coulomb interaction. We consider the case where the order has a wave vector $Q=(0,0)$ and photoexcitation is introduced by a dipole transition. Within the mean-field approximation, we show that the excitonic order can be enhanced by the photoexcitation when the system is initially in the BEC regime of the excitonic phase, whereas it is reduced …
We study the dynamics of excitonic insulators coupled to phonons. Without phonon couplings, the linear response is given by the damped amplitude oscillations of the order parameter with frequency equal to the minimum band gap. A phonon coupling to the interband transfer integral induces two types of long-lived collective oscillations of the amplitude, one originating from the phonon dynamics and the other from the phase mode, which becomes massive. We show that even for small phonon coupling, a photo-induced enhancement of the exciton condensation and the gap can be realized. Using the Anderso…
The effects associated with exciton Bose condensate formation in strongly correlated spin crossover systems are considered within the effective Hamiltonian obtained from the two-orbital Hubbard-Kanamori model. The collective excitations spectrum at various points of the temperature-crystal field phase diagram is calculated. The role of the electron-phonon interaction is discussed. The exciton and magnetic order photoenhancement (induction) in strongly correlated spin crossover systems a new mechanism based on the cooperative effect of electron-phonon and interatomic exchange interactions and t…
Extraordinary Lifetime Enhancement of Coherent Phonon-Amplitude Modes in the Excitonic Insulator Phase of Ta2Pd3Te5
Technische Universität Dresden（德累斯顿工业大学）；Max Planck Institute for Chemical Physics of Solids（马克斯·普朗克固体化学物理研究所）；Korea Institute of Science and Technology（韩国科学技术院）；University of Cologne（科隆大学）
Recent advances in the study of nodal Weyl fermions (WFs), quasi-relativistic massless particles, constitute a novel realm of quantum many-body phenomena. The Coulomb interaction in such systems, having a zero density of states at the Fermi level, is of particular interest, since in contrast to conventional correlated metals, its long-ranged component is unscreened. Here, through nuclear-magnetic-resonance (NMR) measurements, we unveil the exotic spin correlations of two-dimensional WFs in an organic material, causing a divergent increase of the Korringa ratio by a factor of 1000 upon cooling,…
We investigate the condition for the photoinduced enhancement of an excitonic order in a two-orbital Hubbard model, which has been theoretically proposed in our previous work [Phys. Rev. B 97, 115105 (2018)], and analyze it from the viewpoint of the Rabi oscillation. Within the mean-field approximation, we simulate real-time dynamics of an excitonic insulator with a direct gap, where the pair condensation in the initial state is of BEC nature and the photoexcitation is introduced by electric dipole transitions. We first discuss that in the atomic limit our model is reduced to a two-level syste…
Pezzini et al. reported an unconventional mass enhancement in topological nodal line semimetal ZrSiS (Nat. Phys. 14, 178 (2018), whose origin remains puzzling. In this material, strong short-range interactions might induce excitonic particle-hole pairs. Here we study the renormalization of fermion velocities and find that the mass enhancement in ZrSiS can be well understood if we suppose that ZrSiS is close to the quantum critical point between semimetal and excitonic insulator. Near this quantum critical point, the fermion velocities are considerably reduced by excitonic quantum fluctuation, …
Two-dimensional Dirac fermions are subjected to two types of interactions, namely the long-range Coulomb interaction and the short-range on-site interaction. The former induces excitonic pairing if its strength $α$ is larger than some critical value $α_c$, whereas the latter drives an antiferromagnetic Mott transition when its strength $U$ exceeds a threshold $U_c$. Here, we study the impacts of the interplay of these two interactions on excitonic pairing with the Dyson-Schwinger equation approach. We find that the critical value $α_c$ is increased by weak short-range interaction. As $U$ incre…
A sufficiently strong long-range Coulomb interaction can induce excitonic pairing in gapless Dirac semimetals, which generates a finite gap and drives semimetal-insulator quantum phase transition. This phenomenon is in close analogy to dynamical chiral symmetry breaking in high energy physics. In most realistic Dirac semimetals, including suspended graphene, Coulomb interaction is too weak to open an excitonic gap. The Coulomb interaction plays a more important role at low energies in a two-dimensional semi-Dirac semimetal, in which the fermion spectrum is linear in one component of momenta an…
Motivated by the remarkable discovery of superconductivity in elemental Bismuth, we study its normal state in detail using a combination of tight-binding (TB) and-structural supplemented by dynamical mean-field theory (DMFT). We show that a two-fluid model composed of preformed and dynamically fluctuating excitons coupled to a tiny number of carriers provides a unified rationalization of a range of ill-understood normal state spectral and transport data. Based on these, we propose that resonant scattering involving a very low density of renormalized carriers and the excitonic liquid drives log…
Effects of the spin-orbit coupling (SOC) and magnetic field on excitonic insulating (EI) states are investigated. We introduce the two-orbital Hubbard model with the crystalline field splitting, which is a minimal model for discussing the exciton condensation in strongly correlated electron systems, and analyze its effective Hamiltonian in the strong correlation limit by using the mean-field theory. In the absence of the SOC and magnetic field, the ground state changes from the nonmagnetic band-insulating state to the EI state by increasing the Hund coupling. In an applied magnetic field, the …
The electron-electron Coulomb interaction in Dirac-Weyl semimetals harbours a novel paradigm of correlation effects that hybridizes diverse realms of solid-state physics with their relativistic counterpart. Driving spontaneous mass acquisition, the excitonic condensate of strongly-interacting massless Dirac fermions is one such example whose exact nature remains debated. Here, by focussing on the two-dimensional tilted Dirac cones in the organic salt $α$-(BEDT-TTF)$_2$I$_3$, we show that the excitonic instability is controlled by a small chemicalpotential shift and an in-plane magnetic field. …
Dominant Excitonic Superconductivity in a Three-component Hubbard Chain
School of Physics, Sun Yat-Sen University（中山大学物理学院）；School of Science, Great Bay University（大湾区大学理学院）；School of Physics, University of Science and Technology of China（中国科学技术大学物理学院）
We study the conditions for spontaneously generating an excitonic mass gap due to Coulomb interactions between anisotropic Dirac fermions in uniaxially strained graphene. The mass gap equation is realized as a self-consistent solution for the self-energy within the Hartree-Fock mean-field and static random phase approximations. It depends not only on momentum, due to the long-range nature of the interaction, but also on the velocity anisotropy caused by the presence of uniaxial strain. We solve the nonlinear integral equation self-consistently by performing large scale numerical calculations o…
The new Kondo material YbIr$_3$Si$_7$, similar to other Kondo insulators, has been reported to exhibit charge-neutral fermionic excitations through measurements of specific heat and thermal conductivity at low temperatures. We performed $^{29}$Si-NMR on YbIr$_3$Si$_7$ to investigate the magnetic response of charge-neutral fermions from a microscopic perspective. In low magnetic fields parallel to the $c$ axis, a single NMR peak in the paramagnetic state splits into three peaks below $T_{\rm N}$. In contrast, only a slight shift of the single NMR peak was observed in high magnetic fields. This …
The strongly enhanced magnetic excitations near the quantum critical point of Cr$_{1-x}$V$_x$ and why strong exchange enhancement need not imply heavy fermion behavior
非弹性中子散射揭示了近反铁磁金属Cr $_{0.95}$ V $_{0.05}$中能量高达0.4eV的强自旋涨落。磁响应很好地描述了一个修改的Millis-Monien-Pines函数。从低能量响应，我们推导出一个大的交换增强，超过一个数量级以上的低温电子热容$γT$的相应增强。对一些磁关联金属，证明了$γ$与波矢平均自旋弛豫速率的倒数$Γ_{\text{ave}}$之间的标度关系
Enhancement of Superconducting Transition Temperature due to the strong Antiferromagnetic Spin Fluctuations in Non-centrosymmetric Heavy-fermion Superconductor CeIrSi3 :A 29Si-NMR Study under Pressure
We investigate a spin-$\frac{1}{2}$ fermion chain minimally coupled to a $\mathbb{Z}_2$ gauge field. In the sector of the gauge generator $\hat G_j =-1$, the model reduces to the Hubbard model with repulsive onsite interaction coupled to a $\mathbb{Z}_2$ gauge field. We uncover how electric fields affect low-energy excitations by both analytical and numerical methods. In the half-filling case, despite electric fields, the system is still a Mott insulator, just like the Hubbard model. For hole-doped systems, holes are confined under nonzero electric fields, resulting in a hole-pair bound state.…
Particle-hole symmetry breaking in the fractional quantum Hall effect has recently been studied both theoretically and experimentally with most works focusing on non-Abelian states in the second electronic Landau level. In this work, we theoretically investigate particle-hole symmetry breaking of incompressible fractional quantum Hall states in the lowest Landau level under the influence of the realistic effect of a finite magnetic field strength. A finite magnetic field induces Landau level and sub-band mixing which are known to break particle-hole symmetry at the level of the Hamiltonian. We…
The ZrSiS family of compounds hosts various exotic quantum phenomena due to the presence of both topological nonsymmorphic Dirac fermions and nodal-line fermions. In this material family, the LnSbTe (Ln= lanthanide) compounds are particularly interesting owing to the intrinsic magnetism from magnetic Ln which leads to new properties and quantum states. In this work, the authors focus on the previously unexplored compound SmSbTe. The studies reveal a rare combination of a few functional properties in this material, including antiferromagnetism with possible magnetic frustration, electron correl…
