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arXiv 0902.4564cond-mat.str-elcond-mat.other
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反铁磁分子轮中的量子相位干涉和Neel矢量隧穿

Quantum Phase Interference and Neel-Vector Tunneling in Antiferromagnetic Molecular Wheels

O. Waldmann, T. C. Stamatatos, G. Christou, H. U. Güdel, I. Sheikin, H. Mutka

摘要:

本文用磁矩、磁化强度和中子非弹性散射谱研究了18个交换耦合Fe(III)离子的反铁磁分子轮Fe_(18)。综合数据表明,Fe 18的低温磁性是非常准确地描述了尼尔矢量隧道(NVT)的情况下,由半经典理论展开。此外,作为所施加的场的函数的磁转矩表现出振荡,该振荡反映了由于量子相位干涉而导致的NVT隧道中的振荡与场分裂。

英文摘要:

The antiferromagnetic molecular wheel Fe18 of eighteen exchange-coupled Fe(III) ions has been studied by measurements of the magnetic torque, the magnetization, and the inelastic neutron scattering spectra. The combined data show that the low-temperature magnetism of Fe18 is very accurately described by the Neel-vector tunneling (NVT) scenario, as unfolded by semiclassical theory. In addition, the magnetic torque as a function of applied field exhibits oscillations that reflect the oscillations in the NVT tunnel splitting with field due to quantum phase interference.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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