The superconducting state of SRO is widely believed to have chiral p-wave order that breaks time reversal symmetry. Such a state is expected to have a spontaneous magnetization, both at sample edges and at domain walls between regions of different chirality. Indeed, muon spin resonance experiments are interpreted as evidence of spontaneous magnetization due to domain walls or defects in the bulk. However, recent magnetic microscopy experiments place upper limits on the magentic fields at the sample edge and surface which are as much as two orders of magnitude smaller than the fields predicted theoretically for a somewhat idealized chiral p-wave superconductor. We investigate the effects on the spontaneous supercurrents and magnetization of rough and pair breaking surfaces for a range of parameters within a Ginzburg-Landau formalism. The effects of competing orders nucleated at the surface are also considered. We find the conditions under which the edge currents are significantly reduced while leaving the bulk domain wall currents intact, are quite limited. The implications for interpreting the existing body of experimental results on superconducting SRO within a chiral p-wave model are discussed.
It is widely believed that the perovskite Sr$_2$RuO$_4$ is an unconventional superconductor with broken time reversal symmetry. It has been predicted that superconductors with broken time reversal symmetry should have spontaneously generated supercurrents at edges and domain walls. We have done careful imaging of the magnetic fields above Sr$_2$RuO$_4$ single crystals using scanning Hall bar and SQUID microscopies, and see no evidence for such spontaneously generated supercurrents. We use the results from our magnetic imaging to place upper limits on the spontaneously generated supercurrents a…
We investigate superconducting phase transition in superconductor(S)/ferromagnet(F) bilayer with Rasba spin-orbit interaction at S/F interface. This spin-orbit coupling produces spontaneous supercurrents flowing inside the atomic-thickness region near the interface, which are compensated by the screening Meissner currents [S. Mironov and A. Buzdin, Phys. Rev. Lett \textbf{118}, 077001 (2017)]. In the case of thin superconducting film the emergence of the spontaneous surface currents causes the increase of the superconducting critical temperature and we calculate the actual value of the critica…
We present magnetization measurements of mesoscopic superconducting niobium loops containing a ferromagnetic (PdNi) pi-junction. The loops are prepared on top of the active area of a micro Hall-sensor based on high mobility GaAs/AlGaAs heterostructures. We observe asymmetric switching of the loop between different magnetization states when reversing the sweep direction of the magnetic field. This provides evidence for a spontaneous current induced by the intrinsic phase shift of the pi-junction. In addition, the presence of the spontaneous current near zero applied field is directly revealed b…
We study $d$-wave superconductivity in twisted bilayer graphene and reveal phenomena that arise due to the moiré superlattice. In the $d$-wave pairing, the relative motion (RM) of two electrons in a Cooper pair can have either $d+id$ or $d-id$ symmetry with opposite angular momenta. Due to the enlarged moiré superlattice, the center-of-mass motion (COMM) can also carry a finite angular momentum while preserving the moiré periodicity. By matching the total angular momentum, which has contributions from both the RM and the COMM, Cooper pairs with $d+id$ and $d-id$ RMs are intrinsically coupled i…
Recently, a theoretical study [Li {\it et al.},~npj Quantum Materials 6, 36 (2021)] investigated a model of a disordered $d$-wave superconductor, and reported local time-reversal symmetry breaking current loops for sufficiently high disorder levels. Since the pure $d$-wave superconducting state does not break time-reversal symmetry, it is surprising that such persistent currents arise purely from nonmagnetic disorder. Here we perform a detailed theoretical investigation of such disorder-induced orbital currents, and show that the occurrence of the currents can be traced to local extended $s$-w…
We report a coherence-length scale phenomenon related to how the high-Tc order parameter (OP) evolves under a directly-applied supercurrent. Scanning tunneling spectroscopy was performed on current-carrying YBa_2Cu_3O_7-delta thin-film strips at 4.2K. At current levels well below the theoretical depairing limit, the low-energy Andreev states are suppressed by the supercurrent, while the gap-like structures remain unchanged. We rule out the likelihood of various extrinsic effects, and propose instead a model based on phase fluctuations in the d-wave BTK formalism to explain the suppression. Our…
Employing a Keldysh-Eilenberger technique, we theoretically study the generation of a sponta- neous supercurrent and the appearance of the $ϕ$0 phase shift parallel to uniformly in-plane mag- netized superconducting interfaces made of the surface states of a three-dimensional topological insulator. We consider two weakly coupled uniformly magnetized superconducting surfaces where a macroscopic phase difference between the s-wave superconductors can be controlled externally. We find that, depending on the magnetization strength and orientation on each side, a spontaneous supercurrent due to the…
The interface properties of high-temperature cuprate superconductors have been of interest for many years, and play an essential role in Josephson junctions, superconducting cables, and microwave electronics. In particular, the maximum critical current achievable in high-Tc wires and tapes is well known to be limited by the presence of grain boundaries, regions of mismatch between crystallites with misoriented crystalline axes. In studies of single, artificially fabricated grain boundaries the striking observation has been made that the critical current Jc of a grain boundary junction depends …
The RCSJ model of resistively and capacitively shunted Josephson junctions is used to describe superconducting point contacts over a wide range of resistances up to the metallic -- tunneling transition. Their small dynamic capacitance of order $C = 0.1 $fF due to the point-contact geometry results in a huge plasma frequency. The critical current is then strongly suppressed and the contact resistance becomes finite because of quantum-mechanical zero-point fluctuations of the Josephson plasma and the rather large escape rate out of the zero-voltage state due to quantum tunneling. We test the pre…
Twin boundaries are generic crystalline defects in noncentrosymmetric crystal structures. We study theoretically twin boundaries in time-reversal symmetric noncentrosymmetric superconductors that admit parity-mixed Cooper pairing. Twin boundaries support spin currents as a consequence of this parity mixing. If the singlet and triplet components of the superconducting order parameter are of comparable magnitude, the superconducting state breaks spontaneously the bulk time-reversal symmetry locally near the twin boundary. By self-consistently evaluating the Bogoliubov-de-Gennes equations and the…
A nonmonotonic dependence of the critical Josephson supercurrent on the injection current through a normal metal/ferromagnet weak link from a single domain ferromagnetic strip has been observed experimentally in nanofabricated planar crosslike S-N/F-S Josephson structures. This behavior is explained by 0-pi and pi-0 transitions, which can be caused by the suppression and Zeeman splitting of the induced superconductivity due to interaction between N and F layers, and the injection of spin-polarized current into the weak link. A model considering both effects has been developed. It shows the qua…
We investigate transport properties of ballistic magnetic Josephson junctions and establish that suppression of supercurrent is an intrinsic property of the junctions, even in absence of disorder. By studying the role of ferromagnet thickness, magnetization, and crystal orientation we show how the supercurrent decays exponentially with thickness and identify two mechanisms responsible for the effect: (i) large exchange splitting may gap out minority or majority carriers leading to the suppression of Andreev reflection in the junction, (ii) loss of synchronization between different modes due to…
We demonstrate that superconducting aluminium nano-bridges can be driven into a state with complete suppression of the critical supercurrent via electrostatic gating. Probing both in- and out-of-plane magnetic field responses in the presence of electrostatic gating can unveil the mechanisms that primarily cause the superconducting electric field effects. Remarkably, we find that a magnetic field, independently of its orientation, has only a weak influence on the critical electric field that identifies the transition from the superconducting state to a phase with vanishing critical supercurrent…
The interplay of the electron exchange interaction and spin-orbit coupling results in spontaneous supercurrents near magnetic insulator islands, which are placed on the top of a two-dimensional (2D) superconductor, and whose magnetization is parallel to 2D electron gas. It is shown that in contrast to the well studied situation, where such an effect involves only topologically trivial spatial variations of the superconducting order parameter, one should take into account supercurrent vortices. The latter are spontaneously generated around the island's boundary of an arbitrary shape and result …
We analyze $s + is$ state proposed as a candidate superconducting state for strongly hole-doped Ba$_{1-x}$K$_x$Fe$_2$As$_2$. Such a state breaks time-reversal symmetry (TRS) but does not break any other discrete symmetry. We address the issue whether TRS breaking alone can generate spontaneous currents near impurity sites, which could be detected in, e.g., muSR experiments. We argue that there are no spontaneous currents if only TRS is broken. However, supercurrents do emerge if the system is put under external strain and C4 lattice rotation symmetry is externally broken.
An inhomogeneous magnetic exchange field at a superconductor/ferromagnet interface converts spin-singlet Cooper pairs to a spin-aligned (i.e. spin-polarized) triplet state. Although the decay envelope of such triplet pairs within ferromagnetic materials is well studied, little is known about their decay in non-magnetic metals and superconductors, and in particular in the presence of spin-orbit coupling (SOC). Here we investigate devices in which triplet supercurrents are injected into the s-wave superconductor Nb. In the normal state of Nb, triplet supercurrents decay over a distance of 5 nm, …
A major challenge to the chiral $p$-wave hypothesis for the pairing symmetry of the unconventional superconductor Sr$_2$RuO$_4$ is the null result of sensitive scanning magnetometry experiments designed to detect the expected spontaneous charge currents. Motivated by junction tunneling conductance measurements which indicate the quenching of superconductivity at the surfaces of even high-purity samples, we examine the spontaneous currents in a chiral $p$-wave superconductor near a normal metal / superconductor interface using the lattice Bogoliubov-de Gennes equations and Ginzburg-Landau theor…
We study the physical properties of an $s$-wave -- normal metal -- $d$-wave junction in terms of the Andreev bound states in the normal metal layer. The phase dependence of bound states with different orientations leads to superconducting states with broken time reversal symmetry for generic orientations of the $d$-wave superconductor crystal. The occurrence of such a state and the associated spontaneous supercurrent along the junction is analyzed in the framework of Ginzburg-Landau theory and by the solution of the Bogolyubov-de Gennes equations.
The distinctive quasiparticle distribution existing under nonequilibrium in a superconductor-insulator-normal metal-insulator-superconductor (SINIS) mesoscopic line is proposed as a novel tool to control the supercurrent intensity in a long Josephson weak link. We present a description of this system in the framework of the diffusive-limit quasiclassical Green-function theory and take into account the effects of inelastic scattering with arbitrary strength. Supercurrent enhancement and suppression, including a marked transition to a $π$-junction are striking features leading to a fully tunable…
The gauge symmetry of the Ginzburg-Landau theory for two-gap superconductors is analyzed in this letter. We argue that the existence of two different phases, associated with the two independent scalar Higgs fields, explicitly breaks the gauge symmetry of the Ginzburg-Landau hamiltonian, unless a new additional vector field is included. Furthermore, the interference term, or Josephson coupling, holding a direct dependence with the phase difference, also explicitly breaks down the gauge symmetry. We show that a solution for the problem is achieved by adding an additional kinetic coupling term be…
Materials with transition metals in triangular lattices are of great interest for their potential combination of strong correlation, exotic magnetism and electronic topology. Kagome nets are of particular importance since the discovery of geometrically frustrated magnetism and topological band structures in crystals like Herbertsmithite and Fe3Sn2, respectively. KV3Sb5 was discovered to be a layered topological metal with a Kagome net of vanadium. Here, we fabricated Josephson Junctions (JJ) of K1-xV3Sb5 and induced superconductivity over long junction lengths. Through magnetoresistance and cu…
We investigate several theoretical possibilities for the suppression in a c-axis magnetic field of the magnetic resonance recently observed in inelastic neutron scattering experiments on YBCO_{6.6}. We find that neither the Doppler shift of the quasiparticle states caused by supercurrents outside the vortex core, nor an assumed spatially uniform suppression of the coherence factors or spectral gap due to the applied field, can account for the observed effect. In contrast, suppressing the gap or the coherence factors in the vortex core to zero is consistent with the data. We demonstrate that an…
The distinctive quasiparticle distribution existing under nonequilibrium in a superconductor-insulator-normal metal-insulator-superconductor (SINIS) mesoscopic line is proposed as a novel tool to control the supercurrent intensity in a long Josephson weak link. We present a description of this system in the framework of the diffusive-limit quasiclassical Green-function theory and take into account the effects of inelastic scattering with arbitrary strength. Supercurrent enhancement and suppression, including a marked transition to a $π$-junction are striking features leading to a fully tunable…
Local spins coupled to superconductors give rise to several emerging phenomena directly linked to the competition between Cooper pair formation and magnetic exchange. These effects are generally scrutinized using a spectroscopic approach which relies on detecting the in-gap bound modes arising from Cooper pair breaking, the so-called Yu-Shiba-Rusinov (YSR) states. However, the impact of local magnetic impurities on the superconducting order parameter remains largely unexplored. Here, we use scanning Josephson spectroscopy to directly visualize the effect of magnetic perturbations on Cooper pai…
We propose a method to distinguish between trivial and topological, Majorana, zero-energy states in both short and long superconductor-normal-superconductor junctions based on Rashba nanowires using phase-biased equilibrium transport measurements. In particular, we show how the sawtooth profile of the supercurrent, due to the Majorana oscillation suppression in the topological phase for sufficiently long superconductor regions, leads to a strong signal in its zero-frequency susceptibility for a phase difference of $ϕ=π$. This signal is notably insensitive to the chemical potential in the norma…
Optical conductivity of a dirty current-carrying superconductor
L. D. Landau Institute for Theoretical Physics（列夫·朗道理论物理研究所）；Laboratory for Condensed Matter Physics, HSE University（高等经济学院凝聚态物理实验室）；Moscow Institute of Physics and Technology（莫斯科物理技术学院）
The internal chirality of Cooper pairs is shown to modify strongly the response of a superconductor to the local heating by a laser beam. The suppression of the chiral order parameter inside the hot spot appears to induce the supercurrents flowing around the spot region. The chirality affects also the sequential stage of thermal quench developing according to the Kibble-Zurek scenario: besides the generation of vortex-antivortex pairs the quench facilitates the formation of superconducting domains with different chirality. These fingerprints of the chiral superconducting state can be probed by…
The Higgs mode in superconductors is a scalar mode without electric or magnetic dipole moment. Thus, it is commonly believed that its excitation is restricted to a nonlinear two-photon Raman process. However, recent efforts have shown that a linear excitation in the presence of a supercurrent is possible, resulting in a new resonant enhancement at $Ω=2Δ$ with the driving light frequency $Ω$ and the energy of the Higgs mode $2Δ$. This is in contrast to the usual $2Ω= 2Δ$ resonance condition found in nonlinear third-harmonic generation experiments. In this communication, we show that such a line…
We propose a superconducting instability where microscopic supercurrent loops form spontaneously within a unit cell at the superconducting transition temperature with only uniform, onsite and intra-orbital singlet pairing. As a result of the circulating currents time-reversal symmetry is spontaneously broken in the superconducting state. Using Ginzburg-Landau theory, we describe in detail how these currents emerge in a toy model. We discuss the crystallographic symmetry requirements to realize such a state and show that they are met by the Re6X (X=Zr, Hf, Ti) family of time-reversal symmetry b…
We extend the standard effective model of d-wave superconductivity of a single band tight-binding Hamiltonian with nearest-neighbor attraction to include finite range periodically modulated pair-hopping. The pair-hopping is characterized by a fixed wave number $\pmb{\mathcal{Q}}=\mathcal{Q}\hat{x}$ breaking lattice rotational symmetry. Within self-consistent BCS theory we study the general variational state consisting of two incommensurate singlet pair amplitudes $Δ_{{\bf Q}_1}$ and $Δ_{{\bf Q}_2}$ and find two types of near degenerate ground states; of the Larkin-Ovchnnikov (LO) or pair-densi…
We study the superconducting pairing symmetry in twisted bilayer graphene by solving the Bogoliubov-de Gennes equation for all electrons in moiré supercells. With increasing the pairing potential, the system evolves from the mixed nontopological $d+id$ and $p+ip$ phase to the $s+p+d$ phase via the first-order phase transition. In the time-reversal symmetry breaking $d+id$ and $p+ip$ phase, vortex and antivortex lattices accompanying spontaneous supercurrent are induced by the twist. The superconducting order parameter is nonuniform in the moiré unit cell. Nevertheless, the superconducting gap …
Superconductors separated by a thin tunneling barrier exhibit the Josephson effect that allows charge transport at zero voltage, typically with no phase shift between the superconductors in the lowest energy state. Recently, Josephson junctions with ground state phase shifts of pi proposed by theory three decades ago have been demonstrated. In superconducting loops, pi-junctions cause spontaneous circulation of persistent currents in zero magnetic field, analogous to spin-1/2 systems. Here we image the spontaneous zero-field currents in superconducting networks of temperature-controlled pi-jun…
We perform a microscopic study on the redistribution of electric charge near the surface of a model $d$-wave superconductor cut along the [110] direction, with a Fermi surface appropriate for cuprate superconductors, using the augmented quasiclassical equations. We identify two possible mechanisms for the redistribution of charged particles different from the well-known magnetic Hall effect, namely; the pair potential gradient (PPG) force due to surface effects on the pair potential and the pressure difference between the normal and superconducting regions arising from the slope of the density…
We present a study of strain modulation effects on electronic structures of a two-dimensional single-band chiral p-wave superconductor within the BCS mean-field scheme. We employ a lattice model and numerically solve the corresponding Bogolyubov-de Gennes equations. Assuming that strain modulation only modifies hopping amplitudes, we observe the emergence of local spontaneous supercurrents that are attributed to the non-trivial band topology of the system. We also report that strain modulation could induce the formation of topologically distinct domains within a single system, which is capture…
We report the observation of a weak spontaneous magnetic field appearing at the transition temperature of $\rm YBa_2Cu_3O_{7-δ}$ into the superconducting state. The effect is observed in 14 out of 15 epitaxial films grown on different substrates and by two distinct techniques. The average magnetic field sensed by the SQUID magnetometer is of the order of 10$^{-5}$ G. The effect indicates a breaking of both parity and time reversal symmetries in the superconductor. We consider two different interpretations: (i) The condensate carries an intrinsic magnetic moment. At T=0, this moment is between …
We demonstrate that films of unconventional (d-wave) superconductor at temperatures $T\lesssim 0.43 T_c$ can exhibit unusual superconducting phases. The new ground states beside the broken gauge and the point group symmetries can spontaneously break (i) continuous translational symmetry and form periodic order parameter structures in the plane of the film, or (ii) time-reversal symmetry and develop supercurrent flowing along the film. These states are result of the strong transverse inhomogeniety present in films with thickness of several coherence lengths. We show a natural similarity between…
We theoretically study spin and charge currents through finite-size two-dimensional $s$-wave superconductor/uniform ferromagnet/s-wave superconductor (SFS) junctions with intrinsic spin-orbit interactions (ISOIs) using a quasiclassical approach. Considering experimentally realistic parameters, we demonstrate that the combination of spontaneously broken time-reversal symmetry and lack of inversion symmetry can result in spontaneously accumulated spin currents at the edges of finite-size two-dimensional magnetic SF hybrids. Due to the spontaneous edge spin accumulation, the corners of the F wire…
We analyze theoretically the influence of domain walls (DWs) on the DC Josephson current in magnetic superconducting S$_{m}$/Fl/F/Fl/S$_{m}$ junctions. The Josephson junction consists of two "magnetic" superconductors S$_{m}$ (superconducting film covered by a thin ferromagnetic layer), spin filters Fl and a ferromagnetic layer F with or without DW (DWs). The spin filters Fl allow electrons to pass with one specific spin orientation, such that the Josephson coupling is governed by a fully polarized long-range triplet component. In the absence of DW(s), the Josephson and spin currents are nonze…
We discuss the ground state properties of the system composed of a normal metal sandwiched between ferromagnet and superconductor within a tight binding Hubbard model. We have solved the spin-polarized Hartree-Fock-Gorkov equations together with the Maxwell's equation (Ampere's law) and found a proximity induced Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) state in this system. Here we show that the inclusion of the normal metal layer in between those subsystems does not necessarily lead to the suppression of the FFLO phase. Moreover, we have found that depending on the thickness of the normal meta…
