We investigate by direct numerical simulations the flow that rising bubbles cause in an originally quiescent fluid. We employ the Eulerian-Lagrangian method with two-way coupling and periodic boundary conditions. In order to be able to treat up to 288000 bubbles, the following approximations and simplifications had to be introduced: (i) The bubbles were treated as point-particles, thus (ii) disregarding the near-field interactions among them, and (iii) effective force models for the lift and the drag forces were used. In particular, the lift coefficient was assumed to be 1/2, independent of the bubble Reynolds number and the local flow field. The results suggest that large scale motions are generated, owing to an inverse energy cascade from the small to the large scales. However, as the Taylor-Reynolds number is only in the range of 1, the corresponding scaling of the energy spectrum with an exponent of -5/3 cannot develop over a pronounced range. In the long term, the property of local energy transfer, characteristic of real turbulence, is lost and the input of energy equals the viscous dissipation at all scales. Due to the lack of strong vortices the bubbles spread rather uniformly in the flow. The mechanism for uniform spreading is as follows: Rising bubbles induce a velocity field behind them that acts on the following bubbles. Owing to the shear, those bubbles experience a lift force which make them spread to the left or right, thus preventing the formation of vertical bubble clusters and therefore of efficient forcing. Indeed, when the lift is artifically put to zero in the simulations, the flow is forced much more efficiently and a more pronounced energy accumulates at large scales is achieved.
We calculate the shape and the velocity of a bubble rising in an infinitely large and closed Hele-Shaw cell using Park and Homsy's boundary condition which accounts for the change of the three dimensional structure in the perimeter zone. We first formulate the problem in the form of a variational problem, and discuss the shape change assuming that the bubble takes elliptic shape. We calculate the shape and the velocity of the bubble as a function of the bubble size, gap distance and the inclination angle of the cell. We show that the bubble is flattened as it rises. This result is in agreement…
Shapes and paths of an air bubble rising inside a liquid are investigated experimentally. About three hundred experiments are conducted in order to generate a phase plot in the Galilei and Eotvos numbers plane, which separates distinct regimes in terms of bubble behaviour. A wide range of the Galilei and Eotvos numbers are obtained by using aqueous glycerol solutions of different concentrations as the surrounding fluid, and by varying the bubble size. The dynamics is investigated in terms of shapes, topological changes and trajectories of the bubbles. Direct numerical simulations are conducted…
We present accurate measurements of the relative motion and deformation of two large bubbles released consecutively in a quiescent liquid confined in a thin-gap cell. Though the second bubble injected is smaller, we observed that in all cases it accelerates and catches up with the leading bubble. This acceleration is related to the wake of the leading bubble which also induces significant changes in the width and curvature of the trailing bubble. On the contrary, the velocity of the leading bubble is unaltered during the whole interaction and coalescence process. Shape adaptation of the two bu…
We investigate the clustering morphology of a swarm of freely rising deformable bubbles. A three-dimensional Voronoï analysis enables us to quantitatively distinguish between two typical clustering configurations: preferential clustering and a grid-like structure. The bubble data is obtained from direct numerical simulations (DNS) using the front-tracking method. It is found that the bubble deformation, represented by the aspect ratio χ, plays a significant role in determining which type of clustering is realized: Nearly spherical bubbles with χ<~ 1.015 form a grid-like structure, while more d…
When a stationary bubble and a stationary droplet immersed in a liquid pool are brought in contact with each other, they form a bubble-droplet aggregate. Its equilibrium morphology and stability largely depend on the combination of different components' surface tensions, known as spreading factor. In this study, we look at the interaction between a rising bubble and a stationary droplet to better understand the dynamics of coalescence and rising as well as morphological changes for the bubble-droplet aggregate. A systematic study is conducted on the interaction processes with various bubble si…
Rising bubbles draw surface patterns: a numerical study
School of Engineering Science, University of Chinese Academy of Sciences（中国科学院大学工程科学学院）；Department of Energy and Power Engineering, Tsinghua University（清华大学能源与动力工程系）；State Key Laboratory of Nonlinear Mechanics, IMECH & UCAS（中国科学院力学研究所非线性力学国家重点实验室）
Detailed understanding of two-phase gas liquid flows is imperative for developing efficient multi-phase reactors through precise control of mixing and reaction kinetics. The bubble column is a good apparatus for elementary studies of such flows. In the current study experiments are conducted to assess the effect of liquid viscosity on flow dynamics inside a bubble column. Corn oil and water are used as the continuous media, and air was the dispersed media. The objective of this effort is to use the results for a qualitative validation of the numerical simulations.
Series of experiments on turbulent bubbly channel flows observed bubble clusters near the wall which can change large-scale flow structures. To gain insights into clustering mechanisms, we study the interaction of a pair of spherical bubbles rising in a vertical channel through combined experiments and modeling. Experimental imaging identifies that pairwise bubbles of 1.0 mm diameter take two preferred configurations depending on their mutual distance: side-by-side positions for a short distance ($S<5$) and nearly inline, oblique positions for a long distance ($S>5$), where $S$ is the mutual d…
This work describes an experimental investigation on the mixing induced by a swarm of high Reynolds number air bubbles rising through a nearly homogeneous and isotropic turbulent flow. The gas volume fraction $α$ and the velocity fluctuations $u'_0$ of the carrier flow before bubble injection are varied, respectively, in the ranges $0\leq α\leq 0.93\%$ and 2.3 cm/s $\leq u'_0 \leq 5.5$ cm/s, resulting in a variation of the bubblance parameter $b$ in the range [0, 1.3] ($b = \frac{V_r^2 α}{{u'}_0^2}$, where $V_r$ is the relative rising velocity). Mixing in the horizontal direction can be modell…
Deformation-induced lateral migration of a bubble slowly rising near a vertical plane wall in a stagnant liquid is numerically and theoretically investigated. In particular, our focus is set on a situation with a small clearance $c$ between the bubble interface and the wall. Motivated by the fact that experimentally measured migration velocity (Takemura et al. (2002, J. Fluid Mech. {\bf 461}, 277)) is higher than the velocity estimated by the available analytical solution (Magnaudet et al. (2003, J. Fluid Mech. {\bf 476}, 115)) using the Faxén mirror image technique for $κ(=a/(a+c))\ll 1$ (her…
Deformation-induced lateral migration of a bubble slowly rising near a vertical plane wall in a stagnant liquid is numerically and theoretically investigated. In particular, our focus is set on a situation with a short clearance $c$ between the bubble interface and the wall. Motivated by the fact that numerically and experimentally measured migration velocities are considerably higher than the velocity estimated by the available analytical solution using the Faxén mirror image technique for $a/(a+c)\ll 1$ (here $a$ is the bubble radius), when the clearance parameter $\varepsilon(= c/a)$ is com…
This paper presents novel insights about the influence of soluble surfactants on bubble flows obtained by Direct Numerical Simulation (DNS). Surfactants are amphiphilic compounds which accumulate at fluid interfaces and significantly modify the respective interfacial properties, influencing also the overall dynamics of the flow. With the aid of DNS local quantities like the surfactant distribution on the bubble surface can be accessed for a better understanding of the physical phenomena occurring close to the interface. The core part of the physical model consists in the description of the sur…
This work reports an experimental characterisation of the flow properties in a homogeneous bubble swarm rising at high-Reynolds-numbers within a homogeneous and isotropic turbulent flow. Both the gas volume fraction α and the velocity fluctuations of the carrier flow before bubble injection are varied, respectively, in the ranges 0% < alpha < 0.93% and 2.3 cm/s < urms < 5.5 cm/s. The so-called bubblance parameter is used to compare the ratio of the kinetic energy generated by the bubbles to the one produced by the incident turbulence, and is varied from 0 to 1.3. Conditional measurements of th…
In this article, we present experimental and numerical techniques to investigate the transfer, transport, and reaction of a chemical species in the vicinity of rising bubbles. In the experiment, single oxygen bubbles of diameter d b = 0.55 . . . 0.85 mm are released into a measurement cell filled with tap water. The oxygen dissolves and reacts with sulfite to sulfate. Laser-induced fluorescence is used to visualize the oxygen concentration in the bubble wake from which the global mass transfer coefficient can be calculated. The ruthenium-based fluorescent dye seems to be surface active, such t…
This study aims to investigate the behavior of multicomponent fluid flows consisting of Newtonian and non-Newtonian components, especially terminal velocity of a rising bubble in a power-law fluid. A recent lattice Boltzmann (LB) model is extended using power-law scheme to be able to simulate both Newtonian and non-Newtonian fluid flows at high density and viscosity ratios. Also, a variable mobility is introduced in this study to minimize the unphysical error around small bubbles in the domain. A three-component fluid flow system is examined using a constant and variable mobility. It is shown …
The buoyancy-driven dynamics of a pair of gas bubbles released in line is investigated numerically, focusing on highly inertial conditions under which isolated bubbles follow non-straight paths. In an early stage, the second bubble always drifts out of the wake of the leading one. Then, depending on the ratios of the buoyancy, viscous and capillary forces which define the Galilei ($Ga$) and Bond ($Bo$) numbers of the system, five distinct regimes specific to such conditions are identified, in which the two bubbles may rise independently or continue to interact and possibly collide in the end. …
Simulating the detailed movement of a rising bubble can be challenging, especially when it comes to bubble path instabilities. Free rising ellipsoidal bubbles not only move in straight lines but can describe sinusoidal, zigzag or spiraling paths. The common Euler Euler (EE) simulation techniques can no longer resolve the actual movement patterns and Direct Numerical Simulations (DNS) tend to be very costly when simulating a larger number of bubbles. A solution based on the Euler Lagrange (EL) approach is presented, where the bubbles show oscillating shape and/or instable paths while computatio…
An extended volume of fluid method is developed for two-phase direct numerical simulations of systems with one viscoelastic and one Newtonian phase. A complete set of governing equations is derived by conditional volume-averaging of the local instantaneous bulk equations and interface jump conditions. The homogeneous mixture model is applied for the closure of the volume-averaged equations. An additional interfacial stress term arises in this volume-averaged formulation which requires special treatment in the finite-volume discretization on a general unstructured mesh. A novel numerical scheme…
The buoyancy-driven motion of two identical gas bubbles released in line in a liquid at rest is examined with the help of highly resolved simulations, focusing on moderately inertial regimes in which the path of an isolated bubble is vertical. Assuming first an axisymmetric evolution, equilibrium configurations of the bubble pair are determined as a function of the buoyancy-to-viscous and buoyancy-to-capillary force ratios which define the Galilei ($Ga$) and Bond ($Bo$) numbers of the system, respectively. The three-dimensional solutions reveal that this axisymmetric equilibrium is actually ne…
Influence of a vertical-wall leading edge on bouncing and escape bubble rising regimes
Universidad de Extremadura（埃斯特雷马杜拉大学）；Instituto de Computación Científica Avanzada (ICCAEx), Universidad de Extremadura（埃斯特雷马杜拉大学先进科学计算研究所）；Universidad de Jaén（哈恩大学）
Bubbly flows are present in various industrial processes including metallurgical processes in which gas bubbles are injected at the bottom of bulk liquid metal to stir the liquid metal and homogenize the metal. Understanding the motion of such bubbles is essential, as it has been shown that bubble flotation can remove inclusions. In this work, we have numerically studied three-dimensional dynamics of a pair of inline Argon bubbles rising in molten steel under the influence of a transverse magnetic field. We have explored the effects of two transverse magnetic field strengths (Bx = 0 and 0.2 T)…
In this paper, we have studied the three-dimensional dynamics of two equally sized air bubbles rising in a shear-thinning fluid. We have used the combined level set and volume of fluid (CLSVOF) method to track interface, maintain mass balance and estimate the interface curvature. Additionally, we have incorporated a Sharp Surface Force Method (SSF) for surface tension forces. This method significantly suppressed the spurious velocities commonly observed with the conventional volume of fluid method and the Continuum Surface Force (CSF). The algorithm is implemented in an in-house code called CU…
The results of the flow structure visualization experiments conducted on the surface of a single bubble streamlined by uniform flow are presented. It is shown that, at certain critical values for bubble size, flow velocity, and contamination level, the axial symmetry of the surface flow loses its stability in a threshold manner, and the first instability mode in the form of two vortices appears. Below the threshold, the stationary flow on the bubble surface is impossible. The experimental results indicate that the assumption about the axial symmetry of the motion on the bubble surface containi…
A three-field local projection stabilized finite element method is developed for computations of a 3D-axisymmetric buoyancy driven bubble rising in a liquid column in which either the bubble or the liquid column can be viscoelastic. The two-phase flow is described by the time-dependent incompressible Navier--Stokes equations, whereas the viscoelasticity is modeled by the Giesekus constitutive equation in a time-dependent domain. The arbitrary Lagrangian Eulerian~(ALE) formulation with finite elements is used to solve the governing equations in the time-dependent domain. The interface-resolved …
Detailed water kinematics are important for understanding atmosphere-ice-ocean energy transfer processes in the Arctic. There are few in situ observations of 2D velocity fields in the marginal ice zone. Particle tracking velocimetry and particle image velocimetry are well known laboratory techniques for measuring 2D velocity fields, but they usually rely on fragile equipment and pollutive plastic tracers. Therefore, in order to bring these methods to the field, we have developed a new system which combines a compact open-source remotely operated vehicle as an imaging device, and air bubbles as…
The collision of a rising bubble with a superhydrophilic horizontal surface is studied numerically using the Cahn-Hilliard diffuse-interface method. For the studied systems, the Bond number, $Bo=ρR^2 g/σ$, varies between 0.25 to 1.5, and the Galileo number, $Ga=ρ(R^3 g)^{1/2}/μ$, changes between 8.5 to 50. We assume that the viscosity and density of the bubble are negligible compared to the surrounding medium. We show that our computations reproduce experimentally observed dynamics for the collision of a bubble with a solid surface. Furthermore, for the studied range of parameters, the bubble-…
3D-Particle Tracking (3D-PTV) and Phase Sensitive Constant Temperature Anemometry in pseudo-turbulence--i.e., flow solely driven by rising bubbles-- were performed to investigate bubble clustering and to obtain the mean bubble rise velocity, distributions of bubble velocities, and energy spectra at dilute gas concentrations ($α\leq2.2$%). To characterize the clustering the pair correlation function $G(r,θ)$ was calculated. The deformable bubbles with equivalent bubble diameter $d_b=4-5$ mm were found to cluster within a radial distance of a few bubble radii with a preferred vertical orientatio…
We use experiments to explore the effect of surfactants on bubble-induced turbulence (BIT) at different scales, considering how the bubbles affect the flow kinetic energy, anisotropy and extreme events. To this end, high-resolution Particle Shadow Velocimetry measurements are carried out in a bubble column in which the flow is generated by bubble swarms rising in water for two different bubble diameters ($3$ mm $\&$ $4$ mm) and moderate gas volume fractions ($0.5\%\sim1.3\%$). To contaminate the flow, different amounts of 1-Pentanol were added to the flow, leading to different bubble shapes an…
The bubble size distribution below a breaking wave is of paramount interest when quantifying mass exchanges between the atmosphere and oceans. Mass fluxes at the interface are driven by bubbles that are small compared to the Hinze scale $d_h$, the critical size below which bubbles are stable, even though individually these are negligible in volume. Combining experimental and numerical approaches, we report a power law scaling 3/2 of the diameter of small bubble size distribution, for sufficiently large separation of scales between the injection size and the Hinze scale. From an analysis of ind…
Bubbles play an important role in the transport of chemicals and nutrients in many natural and industrial flows. Their dispersion is crucial to understand the mixing processes in these flows. Here we report on the dispersion of millimetric air bubbles in a homogeneous and isotropic turbulent flow with Reynolds number $\text{Re}_λ$ from $110$ to $310$. We find that the mean squared displacement (MSD) of the bubbles far exceeds that of fluid tracers in turbulence. The MSD shows two regimes. At short times, it grows ballistically ($\propto τ^2$), while at larger times, it approaches the diffusive…
We present experimental results for spherical particles rising and settling in a still fluid. Imposing a well-controlled center of mass offset enables us to vary the rotational dynamics selectively by introducing an intrinsic rotational timescale to the problem. Results are highly sensitive even to small degrees of offset, rendering this a practically relevant parameter by itself. We further find that for a certain ratio of the rotational to a vortex shedding timescale (capturing a Froude-type similarity) a resonance phenomenon sets in. Even though this is a rotational effect in origin, it als…
Taylor bubbles are a feature of the slug flow regime in gas-liquid flows in vertical pipes. Their dynamics exhibits a number of transitions such as symmetry-breaking in the bubble shape and wake when rising in downward-flowing and stagnant liquids, respectively, as well as breakup in sufficiently turbulent environments. Motivated by the need to examine the stability of a Taylor bubble in liquids, a systematic numerical study of a steadily-moving Taylor bubble in stagnant and flowing liquids is carried out, characterised by a dimensionless inverse viscosity ($Nf$), and Eötvös ($Eo$), and Froude…
Enhancing the efficiency of water electrolysis, which can be severely impacted by the nucleation and growth of bubbles, is key in the energy transition. In this combined experimental and numerical study, in-situ bubble evolution and dissolution processes are imaged and compared to numerical simulations employing the immersed boundary method. We find that it is crucial to include solutal driven natural convection in order to represent the experimentally observed bubble behaviour even though such effects have commonly been neglected in modelling efforts so far. We reveal how the convective patte…
Understanding the dynamics of liquid films that make up bubbles is of practical and fundamental importance. Practically, this understanding is crucial for tuning bubble stability, while fundamentally, thin films are an excellent platform to study 2D flows. Here we study the spatiotemporal film thickness dynamics of bubbles subjected to evaporation driven Marangoni flows. Initially, we demonstrate how bubble stability can be dramatically tuned with the help of evaporation driven flows. Subsequently, we reveal that the spatial symmetry of thickness profiles evolves non-monotonically with the vol…
