We propose a new light source based on having alkaline-earth atoms in an optical lattice collectively emit photons on an ultra-narrow clock transition into the mode of a high Q-resonator. The resultant optical radiation has an extremely narrow linewidth in the mHz range, even smaller than that of the clock transition itself due to collective effects. A power level of order $10^{-12}W$ is possible, sufficient for phase-locking a slave optical local oscillator. Realizing this light source has the potential to improve the stability of the best clocks by two orders of magnitude.
We propose a new type of superradiant laser based on a hot atomic beam traversing an optical cavity. We show that the theoretical minimum linewidth and maximum power are competitive with the best ultracoherent clock lasers. Also, our system operates naturally in continuous wave mode, which has been elusive for superradiant lasers so far. Unlike existing ultracoherent lasers, our design is simple and rugged. This makes it a candidate for the first widely accessible ultracoherent laser, as well as the first to realize sought-after applications of ultracoherent lasers in challenging environments.
We report on the development of a diode laser system - the `Faraday laser' - using an atomic Faraday filter as the frequency-selective element. In contrast to typical external-cavity diode laser systems which offer tunable output frequency but require additional control systems in order to achieve a stable output frequency, our system only lases at a single frequency, set by the peak transmission frequency of the internal atomic Farady filter. Our system has both short-term and long-term stability of less than 1~MHz, which is less than the natural linewidth of alkali-atomic D-lines, making sim…
We report the efficient generation of subnatural-linewidth (< 6 MHz, for Rb D1/D2 lines) biphotons from a Doppler-broadened (530 MHz) hot atomic vapor cell. We use on-resonance spontaneous four-wave mixing in a hot paraffin-coated 87Rb vapor cell at 63 C to produce time-frequency entangled photon pairs with controllable bandwidth (1.9 - 3.2 MHz) and coherence time (47 - 94 ns). Our backward phase-matching scheme with optical pumping is the key to minimize the generation of uncorrelated photons from resonance fluorescence. The result paves the way toward miniature narrowband biphoton source bas…
We utilized the all-copropagating scheme, which maintains the phase-match condition, in the spontaneous four-wave mixing (SFWM) process to generate biphotons from a hot atomic vapor. The scheme enables our biphotons not only to surpass those in the previous works of hot-atom SFWM, but also to compete with the biphotons that are generated by either the cold-atom SFWM or the cavity-assisted spontaneous parametric down conversion. The biphoton linewidth in this work is tunable for an order of magnitude. As we tuned the linewidth to 610 kHz, the maximum two-photon correlation function, $g_{s,as}^{…
Nuclear spins of noble gases feature extremely long coherence times but are inaccessible to optical photons. Here we realize a coherent interface between light and noble-gas spins that is mediated by alkali atoms. We demonstrate the optical excitation of the noble-gas spins and observe the coherent back-action on the light in the form of high-contrast two-photon spectra. We report on a record two-photon linewidth of 5$\pm$0.7 mHz (millihertz) above room-temperature, corresponding to a one-minute coherence time. This experiment provides a demonstration of coherent bi-directional coupling betwee…
Biphotons of narrow bandwidth and long temporal length play a crucial role in long-distance quantum communication (LDQC) and linear optical quantum computing (LOQC). However, generation of these photons usually requires atomic ensembles with high optical depth or spontaneous parametric down-conversion with sophisticated optical cavity. By manipulating the two-component biphoton wavefunction generated from a low-optical-depth (low-OD) atomic ensemble, we demonstrate biphotons with subnatural linewidth in the sub-MHz regime. The potential of shaping and manipulating the quantum wavepackets of th…
We studied the optical properties of a resonantly excited trivalent Er ensemble in Si accessed via in situ single photon detection. A novel approach which avoids nanofabrication on the sample is introduced, resulting in a highly efficient detection of 70 excitation frequencies, of which 63 resonances have not been observed in literature. The center frequencies and optical lifetimes of all resonances have been extracted, showing that 5% of the resonances are within 1 GHz of our electrically detected resonances and that the optical lifetimes range from 0.5 ms up to 1.5 ms. We observed inhomogene…
Today's best atomic clocks are limited by frequency noise on the lasers used to interrogate the atoms. A proposed solution to this problem is to create a superradiant laser using an optical clock transition as its gain medium. This laser would act as an active atomic clock, and would be highly immune to the fluctuations in reference cavity length that limit today's best lasers. Here, we demonstrate and characterize superradiant emission from the mHz linewidth clock transition in an ensemble of laser-cooled $^{87}$Sr atoms trapped within a high-finesse optical cavity. We measure a collective en…
Near transform-limited single photon sources are required for perfect photon indistinguishability in quantum networks. Having such sources in nanodiamonds is particularly important since it can enable engineering hybrid quantum photonic systems. In this letter, we report the generation of optically stable, nearly transform-limited single silicon vacancy emitters in nanodiamonds. Lines as narrow as 325 MHz are reported, which is comparable to the lifetime limited linewidth. Moreover, the emitters exhibit minimal spectrum diffusion and absolute photostability, even if pumped well above saturatio…
We have obtained a low optical inhomogeneous linewidth of 25 MHz in the stoichiometric rare earth crystal EuCl3 .6H2 O by isotopically purifying the crystal in 35 Cl. With this linewidth, an important limit for stoichiometric rare earth crystals is surpassed: the hyperfine structure of 153Eu is spectrally resolved, allowing the whole population of 153Eu3+ ions to be prepared in the same hyperfine state using hole burning techniques. This material also has a very high optical density and can have long coherence times when deuterated. This combination of properties offers new prospects for quant…
Single photon emitters with narrow linewidths are highly sought after for applications in quantum information processing and quantum communications. In this letter, we report on a bright, highly polarized near infrared single photon emitter embedded in diamond nanocrystals with a narrow, sub GHz optical linewidths at 10K. The observed zero phonon line at ~ 780 nm is optically stable under low power resonant excitation and blue shifts as the excitation power increases. Our results highlight the prospect for using new near infrared color centers in nanodiamonds for quantum applications.
A Broadband Squeezed Light Source for Table-Top Interferometry
Cardiff University（卡迪夫大学）；Max Planck Institute for Gravitational Physics (Albert Einstein Institute)（马克斯·普朗克引力物理研究所（阿尔伯特·爱因斯坦研究所））；Leibniz Universität Hannover（汉诺威莱布尼茨大学）
We report on the all-optical detection of Rydberg states in a effusive atomic beam of strontium atoms using electromagnetically induced transparency (EIT). Using narrow-linewidth CW lasers we obtain an EIT linewidth of 5 MHz. To illustrate the high spectroscopic resolution offered by this method, we have measured isotope shifts of the 5s18d ^1D_2 and 5s19s ^1S_0 Rydberg states. This technique could be applied to high-resolution, non-destructive measurements of ultra-cold Rydberg gases and plasmas.
We propose to build a bad cavity laser using forbidden transitions in large ensembles of cold ions that form a Coulomb crystal in a linear Paul trap. This laser might realize an active optical frequency standard able to serve as a local oscillator in next-generation optical clock schemes. In passive optical clocks, large ensembles of ions appear less promising, as they suffer from inhomogeneous broadening due to quadrupole interactions and micromotion-relates shifts. In bad cavity lasers however, the radiating dipoles can synchronize and generate stable and narrow-linewidth radiation. Furtherm…
We investigate the effects of a novel approach to diamond nanofabrication and nitrogen vacancy (NV) center formation on the optical linewidth of the NV zero-phonon line (ZPL). In this post-implantation method, nitrogen is implanted after all fabrication processes have been completed. We examine three post-implanted samples, one implanted with $^{14}$N and two with $^{15}$N isotopes. We perform photoluminescence excitation (PLE) spectroscopy to assess optical linewidths and optically detected magnetic resonance (ODMR) measurements to isotopically classify the NV centers. From this, we find that…
We report an experimental realization of a narrow-band polarization-entangled photon source with a linewidth of 9.6 MHz through cavity-enhanced spontaneous parametric down-conversion. This linewidth is comparable to the typical linewidth of atomic ensemble based quantum memories. Single-mode output is realized by setting a reasonable cavity length difference between different polarizations, using of temperature controlled etalons and actively stabilizing the cavity. The entangled property is characterized with quantum state tomography, giving a fidelity of 94% between our state and a maximally…
We perform hole burning with a low drift stabilized laser within the zero phonon line of the 4f-5d transition in Ce$^{3+}$:Y$_2$SiO$_5$ at 2K. The narrowest spectral holes appear for small applied magnetic fields and are $6\pm4$ MHz wide (FWHM). This puts an upper bound on the homogeneous linewidth of the transition to $3\pm2$ MHz, which is close to lifetime limited. The spin level relaxation time is measured to $72\pm21$ ms with a magnetic field of 10 mT. A slow permanent hole burning mechanism is observed. If the excitation frequency is not changed the fluorescence intensity is reduced by mo…
We report on a fast, bandwidth-tunable single-photon source based on an epitaxial GaAs quantum dot. Exploiting spontaneous spin-flip Raman transitions, single photons at $780\,$nm are generated on-demand with tailored temporal profiles of durations exceeding the intrinsic quantum dot lifetime by up to three orders of magnitude. Second-order correlation measurements show a low multi-photon emission probability ($g^{2}(0)\sim\,0.10-0.15$) at a generation rate up to $10\,$MHz. We observe Raman photons with linewidths as low as $200\,$MHz, narrow compared to the $1.1\,$GHz linewidth measured in re…
We investigate the potential for optical quantum technologies of Pr3+:Y2O3 in the form of monodisperse spherical nanoparticles. We measured optical inhomogeneous lines of 27 GHz, and optical homogeneous linewidths of 108 kHz and 315 kHz in particles of 400 nm and 150 nm average diameters respectively for the 1D2(0)--> 3H4(0) transition at 1.4 K. Furthermore, ground state and 1D2 excited state hyperfine structures in Y2O3 are here for the first time determined by spectral hole burning and modeled by complete Hamiltonian calculations. Ground-state spin transitions have energies of 5.99 MHz and 1…
We present a new method for determining the intrinsic natural linewidth or lifetime of exceptionally long-lived optical excited states. Such transitions are key to the performance of state-of-the-art atomic clocks, have potential applications in searches for fundamental physics and gravitational wave detectors, as well as novel quantum many-body phenomena. With longer lifetime optical transitions, sensitivity is increased, but so far it has proved challenging to determine the natural lifetime of many of these long lived optical excited states because standard population decay detection techniq…
We report results important for the creation of a best-of-both-worlds quantum hybrid system consisting of a solid-state source of single photons and an atomic ensemble as quantum memory. We generate single photons from a GaAs quantum dot (QD) frequency-matched to the Rb D2-transitions and then use the Rb transitions to analyze spectrally the quantum dot photons. We demonstrate lifetime-limited QD linewidths (1.48 GHz) with both resonant and non-resonant excitation. The QD resonance fluorescence in the low power regime is dominated by Rayleigh scattering, a route to match quantum dot and Rb ato…
We report the experimental realization of an optical trap that localizes single Cs atoms ~215 nm from surface of a dielectric nanofiber. By operating at magic wavelengths for pairs of counter-propagating red- and blue-detuned trapping beams, differential scalar light shifts are eliminated, and vector shifts are suppressed by ~250. We thereby measure an absorption linewidth Γ/2π= 5.7 \pm 0.1 MHz for the Cs 6S1/2,F=4 - 6P3/2,F'=5 transition, where Γ/2π= 5.2 MHz in free space. Optical depth d~66 is observed, corresponding to an optical depth per atom d_1~0.08. These advances provide an important …
We demonstrate a tunable, narrow-band filter based on optical-pumping-induced circular dichroism in rubidium vapor. The filter achieves a peak transmission of 14.6%, a linewidth of 80 MHz, and an out-of-band extinction >35 dB. The transmission peak can be tuned within the range of the Doppler linewidth of the D1 line of atomic rubidium at 795 nm. While other atomic filters work at frequencies far from absorption, the presented technique provides light resonant with atomic media, useful for atom-photon interaction experiments. The technique could readily be extended to other alkali atoms.
In this paper we develop a quantum optical method to detect the axion-nucleon interaction. We ultilize a levitated optomechanical system consisting of a silica nanosphere and an optical cavity here. We translate the trapping positions of the nanosphere, resulting the shift of its resonance frequency, which can be determined from measuring the resulting resonance shift in the transmission spectrum. Furthermore, The frequency shift can be related to the additional forces due to two-axion exchange via substraction. Based on noise ananlysis, estimation and calculation, we set the stringent prospec…
Surface passivation for narrowing optical linewidth of silicon T centers in nanophotonic devices
Institute for Research in Electronics and Applied Physics, University of Maryland（马里兰大学电子与应用物理研究所）；Joint Quantum Institute, University of Maryland（马里兰大学联合量子研究所）；Department of Electrical and Computer Engineering, University of Maryland（马里兰大学电气与计算机工程系）；Ulsan National Institute of Science and Technology（蔚山科学技术院）；Department of Physics, University of Maryland（马里兰大学物理系）
We report on pulsed-laser induced generation of nitrogen-vacancy (NV) centers in diamond facilitated by a solid-immersion lens (SIL). The SIL enables laser writing at energies as low as 5.8 nJ per pulse and allows vacancies to be formed close to a diamond surface without inducing surface graphitization. We operate in the previously unexplored regime where lattice vacancies are created following tunneling breakdown rather than multiphoton ionization. We present three samples in which NV-center arrays were laser-written at distances between ~1 $μ$m and 40 $μ$m from a diamond surface, all present…
Cavity optoelectromechanical regenerative amplification is demonstrated. An optical cavity enhances mechanical transduction, allowing sensitive measurement even for heavy oscillators. A 27.3 MHz mechanical mode of a microtoroid was linewidth narrowed to 6.6\pm1.4 mHz, 30 times smaller than previously achieved with radiation pressure driving in such a system. These results may have applications in areas such as ultrasensitive optomechanical mass spectroscopy.
Single photons of subnatural linewidth and high spectral brightness are necessary for efficient light-matter interaction at the single photon level, which lies at the heart of many quantum photonic technologies. Here we demonstrate a bright source of single photons with subnatural linewidth, controllable waveforms, and a high spectral brightness of $3.67 \times 10^5$ s$^{-1}$mW$^{-1}$MHz$^{-1}$. The interaction between the single photons and atoms is demonstrated by the controlled absorption of the single photons in an atomic vapor. Our work has potential applications in quantum information te…
We report the generation of biphotons, with a temporal full width at the half maximum (FWHM) of 13.4$\pm$0.3 $μ$s and a spectral FWHM of 50$\pm$1 kHz, via the process of spontaneous four-wave mixing. The temporal width is the longest, and the spectral linewidth is the narrowest up to date. This is also the first biphoton result that obtains a linewidth below 100 kHz, reaching a new milestone. The very long biphoton wave packet has a signal-to-background ratio of 3.4, which violates the Cauchy-Schwarz inequality for classical light by 4.8 folds. Furthermore, we demonstrated a highly-tunable-lin…
Integrating solid-state quantum emitters with photonic circuits is essential for realizing large-scale quantum photonic processors. Negatively charged tin-vacancy (SnV$^-$) centers in diamond have emerged as promising candidates for quantum emitters because of their excellent optical and spin properties including narrow-linewidth emission and long spin coherence times. SnV$^-$ centers need to be incorporated in optical waveguides for efficient on-chip routing of the photons they generate. However, such integration has yet to be realized. In this Letter, we demonstrate the coupling of SnV$^-$ c…
Context: Some stellar objects exhibit very narrow spectral lines in the visible range additional to their blackbody radiation. Natural lasing has been suggested as a mechanism to explain narrow lines in Wolf-Rayet stars. However, the spectral resolution of conventional astronomical spectrographs is still about two orders of magnitude too low to test this hypothesis. Aims: We want to resolve the linewidth of narrow spectral emissions in starlight. Methods: A combination of spectral filtering with single-photon-level temporal correlation measurements breaks the resolution limit of wavelength-dis…
Single defect centers in layered hexagonal boron nitride (hBN) are promising candidates as single photon sources for quantum optics and nanophotonics applications. However, until today spectral instability hinders many applications. Here, we perform resonant excitation measurements and observe Fourier-Transform limited (FL) linewidths down to $\approx 50$ MHz. We investigate optical properties of more than 600 quantum emitters (QE) in hBN. The QEs exhibit narrow zero-phonon lines (ZPL) distributed over a spectral range from 580 nm to 800 nm and with dipole-like emission with high polarization …
The mechanisms responsible for ultraviolet to mid-infrared light generation in sodium vapours two-photon excited with continuous-wave sub-100 mW power resonant laser radiation are elucidated from orbital angular momentum transfer of the applied light to the generated fields. The measured 9.5 MHz-wide spectral linewidth of the light at 819.7 nm generated by four-wave mixing, sets an upper limit to the linewidth of two fields resulting from amplified spontaneous emission at 2338 nm and 9093 nm on population inverted transitions. Understanding details of this new-field generation is central to ap…
Atomic and atom-like defects in the solid-state are widely explored for quantum computers, networks and sensors. Rare earth ions are an attractive class of atomic defects that feature narrow spin and optical transitions that are isolated from the host crystal, allowing incorporation into a wide range of materials. However, the realization of long electronic spin coherence times is hampered by magnetic noise from abundant nuclear spins in the most widely studied host crystals. Here, we demonstrate that Er$^{3+}$ ions can be introduced via ion implantation into TiO$_2$, a host crystal that has n…
We use the strong intrinsic non-linearity of a microwave superconducting qubit with a 4 GHz transition frequency to directly detect and control the energy of a micro-mechanical oscillator vibrating at 25 MHz. The qubit and the oscillator are coupled electrostatically at a rate of approximately $2π\times$22 MHz. In this far off-resonant regime, the qubit frequency is shifted by 0.52 MHz per oscillator phonon, or about 14 % of the 3.7 MHz qubit linewidth. The qubit behaves as a vibrational energy detector and from its lineshape we extract the phonon number distribution of the oscillator. We mani…
We demonstrate an ultrabright narrow-band two-photon source at the 1.5 -μm telecom wavelength for long-distance quantum communication. By utilizing a bow-tie cavity, we obtain a cavity enhancement factor of $4.06\times 10^4$. Our measurement of the second-order correlation function $G^{(2)} (τ)$ reveals that the linewidth of $2.4$ MHz has been hitherto unachieved in the 1.5 -μm telecom band. This two-photon source is useful for obtaining a high absorption probability close to unity by quantum memories set inside quantum repeater nodes. Furthermore, to the best of our knowledge, the observed sp…
We report the generation of squeezed vacuum states of light at 1550 nm with a broadband quantum noise reduction of up to 4.8 dB ranging from 5 MHz to 1.2 GHz sideband frequency. We used a custom-designed 2.6 mm long biconvex periodically-poled potassium titanyl phosphate (PPKTP) crystal. It featured reflectively coated end surfaces, 2.26 GHz of linewidth and generated the squeezing via optical parametric amplification. Two homodyne detectors with different quantum efficiencies and bandwidths were used to characterize the non-classical noise suppression. We measured squeezing values of up to 4.…
The nitrogen-vacancy center (NV) in diamond, with its exceptional spin coherence and convenience in optical spin initialization and readout, is increasingly used both as a quantum sensor and as a building block for quantum networks. Employing photonic structures for maximizing the photon collection efficiency in these applications typically leads to broadened optical linewidths for the emitters, which are commonly created via nitrogen ion implantation. With studies showing that only native nitrogen atoms contribute to optically coherent NVs, a natural conclusion is to either avoid implantation…
We created dense ensembles of negatively charged nitrogen-vacancy (NV-) centers in diamond by neutron and electron irradiation for applications in hybrid quantum systems and magnetometry. We characterize fluorescence intensity, optical and coherence properties of the resulting defects by confocal microscopy, UV/Vis and FTIR spectroscopy, optically detected magnetic resonance and small angle X-ray scattering. We find the highest densities of NV- at neutron fluences on the order of 10^17 cm^-2 and electron doses of 10^18 cm^-2, with spin resonance linewidths of 6 MHz. Lower electron energies inc…
