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用于缩小纳米光子器件中硅T中心光学线宽的表面钝化

Surface passivation for narrowing optical linewidth of silicon T centers in nanophotonic devices

Fariba Islam, Chang-Min Lee, Kyu-Young Kim, Sorah Fischer, Purbita Purkayastha, Amirehsan Alizadehherfati, Edo Waks

arXiv 2608.09904首次发表:更新:

AI 中文总结

本研究采用原子层沉积Al₂O₃钝化硅表面,最多将纳米光子器件中硅T中心的光学线宽降低57%,为产生不可区分光子提供了CMOS兼容的路径。

AI 中文摘要

硅T中心是固态平台中极具潜力的自旋-光子接口,适用于兼容电信的可扩展量子信息技术。纳米光子学中T中心面临的主要挑战是光谱扩散,即来自表面和体电荷态的局部电场环境波动会加宽光学跃迁,降低光子不可区分性。因此,直接抑制光谱扩散的策略对改进基于T中心的量子光子器件至关重要。本研究采用原子层沉积的Al₂O₃钝化硅表面,实现了T中心光学线宽的系统性窄化。在所有测量中,Al₂O₃钝化使T中心发射线宽最多降低57%。互补的带隙以上照明和光谱烧孔测量表明,剩余线宽包含由相邻电荷陷阱导致的显著光谱扩散分量,同时为均匀线宽设定了约75 MHz的上限。本研究提供了一条与CMOS兼容的路径,可用于从硅T中心产生不可区分的光子,以应用于可扩展量子光子学。

英文摘要

Silicon T centers are promising spin-photon interfaces in solid-state platforms for telecom-compatible, scalable quantum information technologies. A major challenge for T centers in nanophotonics is spectral diffusion, where fluctuations in the local electric-field environment from surface and bulk charge states broaden the optical transition and reduce photon indistinguishability. Strategies that directly suppress spectral diffusion are therefore critical for improving T-center-based quantum photonic devices. Here, we use atomic-layer-deposited Al2O3 to passivate the silicon surface and demonstrate a systematic narrowing of T center optical linewidths. Across our measurements, Al2O3 passivation reduces the T center emission linewidth by up to 57%. Complementary above-bandgap illumination and spectral hole burning measurements show that the remaining linewidth contains a significant spectral-diffusion component caused by adjacent charge traps, while placing an upper bound of approximately 75 MHz on the homogeneous linewidth. This work provides a CMOS-compatible path toward generating indistinguishable photons from silicon T centers for scalable quantum photonic applications.

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