We have studied the zero and low-temperature behavior of anisotropic alternating antiferromagnetic-ferromagnetic Heisenberg spin-1/2 chains in a transverse magnetic field. Using the analytical spinless fermion approach, the thermodynamic behavior of the model has been studied. We have introduced a new order parameter to distinguish the gapless Luttinger liquid phase from the other gapped phases. The exact diagonalization Lanczos results are also used to compare with the spinless fermion ones. We have found a double peak structure in the specific heat curves for the region between the two quantum critical points. Using the numerical full diagonalization results, the existence of the double peak structure is confirmed.
A recently derived general formula and older numerical results are combined to deduce the behavior of the transverse correlation exponent for the spin-1 Heisenberg antiferromagnetic chain in an applied magnetic field: eta = 1/2 - (2.0)m +O(m^2), where m is the magnetization per site. A comparison with the O(3) non-linear sigma-model is also made.
We study a phase diagram for the sliding Luttinger liquid (SLL) of coupled one-dimensional quantum wires packed in a two-dimensional array in the absence of a magnetic field. We analyze whether nearest-neighbor inter-wire interactions, stabilize the SLL phase. We construct an analogue of a Su-Schriefer-Heeger (SSH) model (allowing alternating couplings between wires). Calculating the scaling dimensions of the two most relevant perturbations, charge-density wave, and superconducting inter-wire couplings, but excluding the inter-wire single-particle hybridization, we find a finite stability regi…
We determine the phase diagram of copper nitrate Cu(NO$_3$)$_2\cdot$2.5D$_2$O in the context of quantum phase transitions and novel states of matter. We establish this compound as an ideal candidate to study quasi-1D Luttinger liquids, 3D Bose-Einstein-Condensation of triplons, and the crossover between 1D and 3D physics. Magnetocaloric effect, magnetization, and neutron scattering data provide clear evidence for transitions into a Luttinger liquid regime and a 3D long-range ordered phase as function of field and temperature. Theoretical simulations of this model material allow us to fully est…
Using micromechanical force magnetometry, we have measured the magnetization of the strong-leg spin-1/2 ladder compound (C$_7$H$_{10}$N)$_2$CuBr$_2$ at temperatures down to 45 mK. Low-temperature magnetic susceptibility as a function of field exhibits a maximum near the critical field H_c at which the magnon gap vanishes, as expected for a gapped one-dimensional antiferromagnet. Above H_c a clear minimum appears in the magnetization as a function of temperature as predicted by theory. In this field region, the susceptibility in conjunction with our specific heat data yields the Wilson ratio R_…
We investigate the properties of the Heisenberg S=1 chain with bilinear and biquadratic interactions in a magnetic field using the Density Matrix Renormalization Group, Bethe ansatz and field theoretical considerations. In a large region of the parameter space, we identify a magnetized ferroquadrupolar Luttinger liquid consisting of a quasi-condensate of bound magnon pairs. This liquid undergoes a continuous pair unbinding transition to a more conventional Luttinger liquid region obtained by polarizing the system above the Haldane gap region. This pair unbinding transition is shown to be in th…
Magnetization curves of the ferrimagnetic mixed spin-(1/2,S) Heisenberg chains are calculated with the help of density-matrix renormalization group method for several quantum spin numbers S=1, 3/2, 2 and 5/2. It is shown that the ferrimagnetic mixed spin-(1/2,S) Heisenberg chains exhibit irrespective of the spin value S exactly one intermediate magnetization plateau, which can be identified with the gapped Lieb-Mattis ferrimagnetic ground state. The magnetization plateau due to the Lieb-Mattis ferrimagnetism breaks down at a quantum phase transition towards the Luttinger spin liquid, which is …
We use bosonization and renormalization group methods to determine the ground state phase diagram of a one-dimensional frustrated Kondo-Heisenberg system consisting of a one-dimensional spin-1/2 Luttinger liquid coupled by a Kondo exchange interaction $J_K$ to a frustrated quantum antiferromagnetic Heisenberg chain, with a nearest-neighbor exchange coupling $J_1$ and a next-nearest-neighbor (frustrating) exchange interaction $J_2$. We analyze the interplay of quantum frustration in the antiferromagnetic chain with the Kondo exchange coupling $J_K$ with the Luttinger liquid. We discuss the stru…
We discuss the transition strength between the disordered ground state and the basic low-lying triplet excitation for the Heisenberg chain with alternating exchange based on series expansions in the interdimer interaction up to tenth order. We demonstrate that the wave vector dependence of the simple dimer approximation is strongly modified in higher orders.
Using the Lanczos method we determine the phase diagram of the 2-leg AF-Heisenberg ladder with alternating dimerization. It consists of a resonating valence bond phase and a dimer phase separated by a critical line. Our results are in good agreement with previous conjectures obtained with the non linear sigma model.
We study variable-rate linear quenches in the anisotropic Heisenberg (XXZ) chain, starting at the XX point. This is equivalent to switching on a nearest neighbour interaction for hard-core bosons or an interaction quench for free fermions. The physical observables we investigate are: the energy pumped into the system during the quench, the spin-flip correlation function, and the bipartite fluctuations of the z component of the spin in a box. We find excellent agreement between exact numerics (infinite system time-evolving block decimation, iTEBD) and analytical results from bosonization, as a …
We develop a low-temperature expansion for the finite temperature dynamical structure factor of the spin half Heisenberg chain with alternating nearest neighbour exchange in the limit of strong alternation of the exchange constants. We determine both the broadening of the low lying triplet lines and the contribution of the thermally activated intraband scattering.
We calculate dynamical structure factors of the S=1 bond-alternating Heisenberg chain with a single-ion anisotropy in transverse magnetic fields, using a continued fraction method based on the Lanczos algorithm. In the Haldane-gap phase and the dimer phase, dynamical structure factors show characteristic field dependence. Possible interpretations are discussed. The numerical results are in qualitative agreement with recent results for inelastic neutron-scattering experiments on the S=1 bond-alternating Heisenberg-chain compound $\rm{Ni(C_{9}D_{24}N_{4})(NO_{2})ClO_{4}}$ and the S=1 Haldane-gap…
We study the energy transport between two interacting spin chains which are initially separated, held at different temperatures and subsequently put in contact. We consider the spin-1/2 XXZ model in the gapless regime and exploit its integrability properties to formulate an analytical Ansatz for the non-equilibrium steady state even at temperatures where the low-energy Luttinger liquid description is not accurate. We apply our method to compute the steady energy current and benchmark it both with the known low-energy limit and at higher temperatures with numerical simulations. We find an excel…
An alternative triplet-wave expansion formalism for dimerized spin systems is presented, a modification of the 'bond operator' formalism of Sachdev and Bhatt. Projection operators are used to confine the system to the physical subspace, rather than constraint equations. The method is illustrated for the case of the alternating Heisenberg chain, and comparisons are made with the results of dimer series expansions and exact diagonalization. Some discussion is included of the phenomenon of 'quasiparticle breakdown', as it applies to the two-triplon bound states in this model.
The magnetic behaviors of a spin-1/2 alternating Heisenberg antiferromagnetic chain in a staggered transverse magnetic field is studied by means of the density-matrix renormalization group method and Jordan-Wigner transformation. Quantum phase transitions of different types are observed in the S=1 Neel and XY-like gapless phases, which result from the competitions between the staggered transverse field and magnetic orders induced by anisotropy and alternating interactions. The results are compared with the mean-field and some exactly resolved results.
Using a recently proposed perturbative numerical renormalization-group algorithm, we explore the connection between quantum criticality and the emergence of Luttinger liquid physics in $t-J$ chains coupled by frustrated interactions. This study is built on an earlier finding that at the maximally frustrated point, the ground state of weakly-coupled Heisenberg chains is disordered, the transverse exchanges being irrelevant. This result is extended here to transverse couplings up to $J_{\perp}=0.6$, and we argue that it may also be valid at the isotropic point. A finite size analysis of coupled …
We study a lattice realization of a Luttinger liquid interacting with a bath of quantum spins in terms of an antiferromagnetic S=1/2 Heisenberg chain, where each spin is also coupled to a σ=1/2 Kondo spin degree of freedom. This model describes the low-energy spin dynamics in quasi one dimensional materials, where the electronic spins of the magnetic ions interact with those of impurities, nuclei and possibly other spin species present in their environment. For large ferromagnetic and antiferromagnetic Kondo interaction J' there are two phases corresponding to an effective spin-1 Heisenberg ch…
Using the recently developed transfer-matrix renormalization group method, we have studied the thermodynamic properties of two-leg antiferromagnetic ladders in the magnetic field. Based on different behavior of magnetization, we found disordered spin liquid, Luttinger liquid, spin-polarized phases and a classical regime depending on magnetic field and temperature. Our calculations in Luttinger liquid regime suggest that both the divergence of the NMR relaxation rate and the anomalous specific heat behavior observed on Cu$_2$(C$_5$H$_{12}$N$_2$)$_2$Cl$_4$}are due to quasi-one-dimensional effect…
The promotion of collinear classical spin configurations as well as the enhanced tendency towards nearest-neighbor clustering of the quantum spins are typical features of the frustrating isotropic three-body exchange interactions in Heisenberg spin systems. Based on numerical density-matrix renormalization group calculations, we demonstrate that these extra interactions in the Heisenberg chain constructed from alternating S=3/2 and sigma=1/2 site spins can generate numerous specific quantum spin states, including some partially-polarized ferrimagnetic states as well as a doubly-degenerate non-…
We study the finite temperature, low energy, long wave-length spectrum of the dynamic structure factor of the spin-$1/2$ antiferromagnetic Heisenberg chain in the presence of exchange anisotropy and external magnetic fields. Using imaginary-time quantum Monte-Carlo we extract parameters, relevant to characterize a {\it renormalized} Luttinger liquid. For small momentum our results are consistent with a change from propagating spinon density waves to spin diffusion, described by a finite-frequency spin-current relaxation rate. Results for this relaxation rate as well as other Luttinger liquid p…
Dynamical structure factors of the S=1 bond-alternating spin chains in the dimer phase are calculated at finite temperature, using the pair dynamical correlated-effective-field approximation. At T=0, the delta-function-type peak of the one-magnon mode appears. When temperature is increased, such a sharp peak is broadened and the additional weak peak caused by the excitation from the triplet state to the quintet state emerges in the higher energy region. The results are discussed in comparison with those obtained by the exact diagonalization method.
We investigate the ground-state properties of the spin-half $J_1{-}J_2$ Heisenberg chain with a next-nearest-neighbor spin-Peierls dimerization using conformal field theory and Lanczos exact diagonalizations. In agreement with the results of a recent bosonization analysis by Sarkar and Sen, we find that for small frustration ($J_2/J_1$) the system is in a Luttinger spin-fluid phase, with gapless excitations, and a finite spin-wave velocity. In the regime of strong frustration the ground state is spontaneously dimerized and the bond alternation reduces the triplet gap, leading to a slight enhan…
We present a study of the spin-1/2 Heisenberg chain with alternating ferro- and antiferromagnetic exchange, focusing on the role of the exchange couplings to cover both, dimer and Haldane limit. Employing a complementary combination of perturbation theory and quantum Monte Carlo simulation, we report results for the magnetic susceptibility as well as the dynamic structure factor over a wide range of coupling constants and for different temperatures to extract the spin gap. For a small ferromagnetic coupling, we find good agreement between perturbation theory and quantum Monte Carlo. For arbitr…
The ground state phase diagram of the alternating spin-1/2 chains with anisotropic ferromagnetic coupling under the influence of a symmetry breaking transverse magnetic field is studied. We have used the exact diagonalization technique. In the limit where the antiferromagnetic coupling is dominant, we have identified two Ising-type quantum phase transitions. We have calculated two critical fields $h_{c_{1}}$ and $h_{c_{2}}$, corresponding to the transition between different magnetic phases of the system. It is found that the intermediate state ($h_{c_{1}}<h<h_{c_{2}}$) is gapful, describing th…
We have measured the specific heat of an S=1/2 antiferromagnetic alternating Heisenberg chain pentafulorophenyl nitronyl nitroxide under magnetic fields up to H>H_C2. This compound has the field-induced magnetic ordered (FIMO) phase between H_C1 and H_C2. Characteristic behaviors are observed depending on the magnetic field up to above H_C2 outside of the H-T boundary for the FIMO. Temperature and field dependence of the specific heat are qualitatively in good agreement with the theoretical calculation on an S=1/2 two-leg ladder. [Wang et al. Phys. Rev. Lett 84 5399 (2000)] This agreement sugg…
Ground state properties, dispersion relations and scaling behaviour of spin gap of a bond alternating spin-$\frac{1}{2}$ anisotropic Heisenberg chain have been studied where the exchange interactions on alternate bonds are ferromagnetic (FM) and antiferromagnetic (AFM) in two separate cases. The resulting models separately represent nearest neighbour (NN) AFM-AFM and AFM-FM bond alternating chains. Ground state energy has been estimated analytically by using both bond operator and Jordan-Wigner representations and numerically by using exact diagonalization. Dispersion relations, spin gap and s…
We study the XXZ Heisenberg model in a staggered magnetic field using the HOTRG tensor renormalization method. Built into the tensor representation of the XXZ model is the U(1) symmetry, which is systematically maintained at each renormalization step. We determine the phase diagram of the model from the low lying spectrum, and from the finite size dependence of the spectrum we extract scaling dimensions, which are compared to predictions of low energy field theory.
We study different phases of the one-dimensional bond-alternating spin-$1/2$ Heisenberg model by using the symmetry fractionalization mechanism. We employ the infinite matrix-product state representation of the ground state (through the infinite-size density matrix renormalization group algorithm) to obtain inequivalent projective representations of the (unbroken) symmetry groups of the model, which are used to identify the different phases. We find that the model exhibits trivial as well as symmetry-protected topological phases. The symmetry-protected topological phases are Haldane phases on …
We present results for the dynamic structure factor of the S=1/2 bond alternating Heisenberg chain over a large range of frequencies and temperatures. Data are obtained from a numerical evaluation of thermal averages based on the calculation of all eigenvalues and eigenfunctions for chains of up to 20 spins. Interpretation is guided by the exact temperature dependence in the noninteracting dimer limit which remains qualitatively valid up to an interdimer exchange $λ\approx 0.5$. The temperature induced central peak around zero frequency is clearly identified and aspects of the crossover to spi…
We present a 14N nuclear magnetic resonance study of a single crystal of CuBr4(C5H12N)2 (BPCB) consisting of weakly coupled spin-1/2 Heisenberg antiferromagnetic ladders. Treating ladders in the gapless phase as Luttinger liquids, we are able to fully account for (i) the magnetic field dependence of the nuclear spin-lattice relaxation rate 1/T_1 at 250 mK and for (ii) the phase transition to a 3D ordered phase occuring below 110 mK due to weak interladder exchange coupling. BPCB is thus an excellent model system where the possibility to control Luttinger liquid parameters in a continuous manne…
We obtain the phase diagram in the parameter space $(J'/J, γ)$ and an accurate estimate of the critical line separating the different phases. We show several measuments of the magnetization, dimerization, nearest neighbours correlation, and density of energy in the different zones of the phase diagram, as well as a measurement of the string order parameter proposed as the non vanishing phase order parameter characterizing Haldane phases. All these results will be compared in the limit $J'/J\gg 1$ with the behaviour of the $\textbf{S}=1$ Bond Alternated Heisenberg Chain (BAHC). The analysis of …
For the time being isotropic three-body exchange interactions are scarcely explored and mostly used as a tool for constructing various exactly solvable one-dimensional models, although, generally speaking, such competing terms in generic Heisenberg spin systems can be expected to support specific quantum effects and phases. The Heisenberg chain constructed from alternating S=1 and sigma=1/2 site spins defines a realistic prototype model admitting extra three-body exchange terms. Based on numerical density-matrix renormalization group (DMRG) and exact diagonalization (ED) calculations, we demon…
The ground state phase diagrams and thermodynamic properties of a spin-1 bond-alternating Heisenberg antiferromagnetic chain with a single-ion anisotropy in longitudinal and transverse magnetic fields are investigated jointly by means of the infinite time evolving block decimation, the linearized tensor renormalization group and the density matrix renormalization group methods. It is found that in the magnetic field-bond alternating ratio plane six phases such as singlet dimer, Haldane, two Tomonaga-Luttinger liquid, 1/2 magnetization plateau and spin polarized phases are identified in a longi…
We present NMR measurements of a strong-leg spin-1/2 Heisenberg antiferromagnetic ladder compound (C7H10N)2CuBr4 under magnetic fields up to 15 T in the temperature range from 1.2 K down to 50 mK. From the splitting of NMR lines we determine the phase boundary and the order parameter of the low-temperature (3-dimensional) long-range-ordered phase. In the Tomonaga-Luttinger regime above the ordered phase, NMR relaxation reflects characteristic power-law decay of spin correlation functions as 1/T1 T^(1/2K-1), which allows us to determine the interaction parameter K as a function of field. We fin…
The fidelity and entanglement entropy in an antiferromagnetic-ferromagnetic alternating Heisenberg chain are investigated by using the method of density-matrix renormalization-group. The effect of anisotropy on fidelity and entanglement entropy are investigated. The relations between fidelity, entanglement entropy and quantum phase transition are analyzed. It is found that the quantum phase transition point can be well characterized by both the ground-state entropy and fidelity for large system.
The effect of the canting of local anisotropy axes on the ground-state phase diagram and magnetization of a ferrimagnetic chain with regularly alternating Ising and Heisenberg spins is exactly examined in an arbitrarily oriented magnetic field. It is shown that individual contributions of Ising and Heisenberg spins to the total magnetization basically depend on the spatial orientation of the magnetic field and the canting angle between two different local anisotropy axes of the Ising spins.
A series of symmetry-protected topological(SPT) and trivial spin-gap phases in the spin-1/2 ferromagnetic--antiferromagnetic alternating Heisenberg chain with alternating next-nearest-neighbour interaction are investigated using two kinds of entanglement spectra defined by different divisions of the whole chain. In the case one of the next-nearest-neighbor interaction vanishes, the model reduces to the $Δ$-chain in which a series of spin-gap phases are found in J. Phys. Soc. Jpn. 77, 044707 (2008). From the degeneracy of the entanglement spectra, these phases are identified as the SPT and triv…
By using the coupled cluster method, the numerical exact diagonalization method, and the numerical density matrix renormalization group method, we investigated the properties of the one-dimensional Heisenberg chain with alternating antiferromagnetic and ferromagnetic next nearest neighbor interactions. In the classical limit, the ground state is in the collinear Neel state if a<1/2, while for a>1/2, there is an noncollinear canted state. For the quantum case, we found that, although the classical Neel state is absent, the canted state exists if the frustration parameter a exceeds a critical po…
Inelastic neutron scattering is employed to study transverse spin correlations of a Heisenberg $S=1/2$ chain compound in a magnetic field of 7.5 T. The target compound is the antiferromagnetic Heisenberg $S=1/2$ chain material 2(1,4-Dioxane)$\cdot$2(H$_2$O)$\cdot$CuCl$_2$, or CuDCl for short. The validity and the limitations of the scaling relation for the transverse dynamic structure factor are tested, discussed and compared to the Tomonaga-Luttinger spin liquid theory and to Bethe-ansatz results for the Heisenberg model.
Many fundamental one-dimensional lattice models such as the Heisenberg or the Hubbard model are integrable. For these microscopic models, parameters in the Luttinger liquid theory can often be fixed and parameter-free results at low energies for many physical quantities such as dynamical correlation functions obtained where exact results are still out of reach. Quantum integrable models thus provide an important testing ground for low-energy Luttinger liquid physics. They are, furthermore, also very interesting in their own right and show, for example, peculiar transport and thermalization pro…
The topological classification of a series of frustration-induced spin-gap phases in the spin-1/2 ferromagnetic--antiferromagnetic alternating Heisenberg chain with next-nearest-neighbour interaction reported in J. Phys. Soc. Jpn. 82, 064703 (2013) is confirmed using two kinds of entanglement spectra defined by different divisions of the whole chain. For the numerical calculation, the iDMRG method is used. The results are consistent with the valence bond solid picture proposed in the previous paper.
Magnetic excitations in the strong-leg quantum spin ladder compound (C$_7$H$_{10}$N)$_2$CuBr$_4$ (known as DIMPY) in the field-induced Tomonaga-Luttinger spin liquid phase are studied by means of high-field electron spin resonance (ESR) spectroscopy. The presence of a gapped ESR mode with unusual non-linear frequency-field dependence is revealed experimentally. Using a combination of analytic and exact diagonalization methods, we compute the dynamical structure factor and identify this mode with longitudinal excitations in the antisymmetric channel. We argue that these excitations constitute a…
Antiferromagnetic Heisenberg spin chains in a sufficiently strong magnetic field are Luttinger liquids, whose parameters depend on the actual magnetization of the chain. Here we present precise numerical estimates of the Luttinger liquid dressed charge $Z$, which determines the critical exponents, by calculating the magnetization and quadrupole operator profiles for $S=1/2$ and S=1 chains using the density matrix renormalization group method. Critical amplitudes and the scattering length at the chain ends are also determined. Although both systems are Luttinger liquids the characteristic param…
Motivated by a novel bimetallic chain compound in which alternating magnetic centers are ferromagnetically coupled, we investigate thermodynamic properties of one-dimensional spin-$(S,s)$ Heisenberg ferromagnets both numerically and analytically. On the one hand, quantum Monte Carlo calculations illuminate the overall thermal behavior. The specific heat may exhibit a double-peaked structure at intermediate temperatures for $S\agt 3s$ in general. On the other hand, a modified spin-wave theory precisely describes the low-temperature properties. Expanding the specific heat and the magnetic suscep…
We make a matrix-product variational approach to spin-1/2 ferromagnetic-antiferromagnetic bond-alternating chains with anisotropy on their ferromagnetic bonds, especially under the open boundary condition. The rich phase diagram containing the Haldane, large-D, and two types of Neel phases is well reproduced with only two variational parameters. The on-bond anisotropy has a significant effect on the ferromagnetic coupling between neighboring spins and induces novel edge states peculiar to spin-1/2 chains.
We study the one-dimensional extended Hubbard model with alternating size of the hopping integrals using the density-matrix renormalization group method. We calculate the spin gap, the Tomonaga-Luttinger parameter, and the charge-density-wave order parameter for various dimerizations, interaction strengths, and band fillings. At half band-filling the spin and charge excitations are gapped but these gaps disappear for infinitesimal hole doping. At quarter filling, the Umklapp scattering in the half-filled lower Peierls band generates a gap for the charge excitations but the gapless spin excitat…
We successfully synthesized the zinc-verdazyl complex [Zn(hfac)$_2$]$\cdot$($o$-Py-V) [hfac = 1,1,1,5,5,5-hexafluoroacetylacetonate; $o$-Py-V = 3-(2-pyridyl)-1,5-diphenylverdazyl], which is an ideal model compound with an $S$ = 1/2 ferromagnetic-antiferromagnetic alternating Heisenberg chain (F-AF AHC). $Ab$ $initio$ molecular orbital (MO) calculations indicate that two dominant interactions $J_{\rm{F}}$ and $J_{\rm{AF}}$ form the $S=1/2$ F-AF AHC in this compound. The magnetic susceptibility and magnetic specific heat of the compound exhibit thermally activated behavior below approximately 1 …
The low temperature magnetization process of the ferromagnetic-antiferromagnetic Heisenberg chain is studied using the interacting boson approximation. In the low field regime and near the saturation field, the spin wave excitations are approximated by the $δ$ function boson gas for which the Bethe ansatz solution is available. The finite temperature properties are calculated by solving the integral equation numerically. The comparison is made with Monte Carlo calculation and the limit of the applicability of the present approximation is discussed.
Quantum phase transitions (QPTs) and the ground-state phase diagram of the spin-1/2 Heisenberg-Ising alternating chain (HIAC) with uniform Dzyaloshinskii-Moriya (DM) interaction are investigated by a matrix-product-state (MPS) method. By calculating the odd- and even-string order parameters, we recognize two kinds of Haldane phases, i.e., the odd- and even-Haldane phases. Furthermore, doubly degenerate entanglement spectra on odd and even bonds are observed in odd- and even-Haldane phases, respectively. A rich phase diagram including four different phases, i.e., an antiferromagnetic (AF), AF s…
The magnetization process of the $S=1$ antiferromagnetic chain with the single-ion anisotropy $D$ and the biquadratic interaction is investigated using the numerical diagonalization. Both interactions stabilize the 2-magnon Tomonaga-Luttinger liquid (TLL) phase in the magnetization process. Based on several excitation gaps calculated by the numerical diagonalization, some phase diagrams of the magnetization process are presented. These phase diagrams reveal that the spin nematic dominant TLL phase appears at higher magnetizations for sufficiently large negative $D$.
A comprehensive comparison between the magnetic field- and temperature-dependent low frequency spin dynamics in the antiferromagnetic spin-1/2 Heisenberg chain (AFHC) system copper pyrazine dinitrate, probed via the 13C-nuclear magnetic resonance (NMR) relaxation rate 1/T1, and the field theoretical approach in the Luttinger liquid (LL) regime has been performed. We have found a very good agreement between the experiment and theory in the investigated temperature and field range. Our results demonstrate how strongly the quantum critical point affects the spin dynamics of Heisenberg spin chain …
We study the nearest neighboring spin-1/2 Kitaev-Heisenberg-Gamma ($KJΓ$) model on the honeycomb lattice in the parameter region of ferromagnetic (FM) Kitaev and antiferromagnetic (AFM) Heisenberg couplings relevant for honeycomb iridates, using a coupled-chain analysis. Starting from the gapless Luttinger liquid phase of a decoupled $KJΓ$ chain, the inter-chain interactions in the two-dimensional model is treated within a self-consistent mean field approach based on the Luttinger liquid theory. In the FM Gamma region, our analysis recovers the reported 120$^\circ$ magnetic order, previously o…
The spin-1/2 ferromagnetic-antiferromagnetic alternating Heisenberg chain with ferromagnetic next-nearest-neighbour (NNN) interaction is investigated. The ground state is the Haldane phase for weak NNN interaction, and is the ferromagnetic phase for weak antiferromagnetic interaction. We find a series of topologically distinct spin-gap phases with various magnitudes of edge spins for strong NNN interaction. The phase boundaries between these phases are determined on the basis of the DMRG calculation with additional spins that compensate the edge spins. It is found that each of the exact soluti…
Specific heat experiments on single crystals of the S=1 quasi-one-dimensional bond-alternating antiferromagnet Ni(C_9H_24N_4)(NO_2)ClO_4, alias NTENP, have been performed in magnetic fields applied both parallel and perpendicular to the spin chains. We have found for the parallel field configuration that the magnetic specific heat (C_mag) is proportional to temperature (T) above a critical field H_c, at which the energy gap vanishes, in a temperature region above that of the long-range ordered state. The ratio C_mag/T increases as the magnetic field approaches H_c from above. The data are in g…
The mixture of bond-alternating and uniform S=1/2 antiferromagnetic Heisenberg chains is investigated by the density matrix renormalization group method. The ground state magnetization curve is calculated and the exchange parameters are determined by fitting to the experimentally measured magnetization curve of \CuCl$_{2x}$Br$_{2(1-x)}$($γ$-pic)$_2$. The low field behavior of the magnetization curve and low temperature behavior of the magnetic susceptibility are found to be sensitive to whether the bond-alternation pattern (parity) is fixed all over the sample or randomly distributed. The both…
