Superlattice of spin vortices has been proposed in an earlier article as an alternative to the stripe interpretation of spin modulations in 1/8-doped lanthanum cuprates. The present article addresses several additional characteristics of the spin vortex lattice, namely: (i) the nature of extended charge states; (ii) the position of neutron spin peaks as a function of doping; and (iii) the absence of higher order spin harmonics. All these characteristics afford straightforward connection to the experimental results produced by angle-resolved photoemission spectroscopy, resistivity measurements, and neutron scattering.
We investigate the dimensionality of inhomogeneous spin modulation patterns in the cuprate family of high-temperature superconductors with particular focus on 1/8-doped lanthanum cuprates. We compare one-dimensional stripe modulation pattern with two-dimensional checkerboard of spin vortices in the context of nuclear quadrupole resonance(NQR) and muon spin rotation(muSR) experiments. In addition, we also consider the third pattern, a two-dimensional superposition of spin spirals. Overall, we have found that none of the above patterns leads to a consistent interpretation of the two types of exp…
It is proposed, that a two-dimensional magnetic superstructure closely related to the one mentioned recently by Christensen et al. [cond-mat/0608204] constitutes a viable interpretation of the four-fold splitting of the magnetic (π, π) peak in lanthanum cuprates. (This splitting is usually interpreted as the evidence for stripes.) The superstructure in question has the topology of the square crystal of magnetic vortices with approximate periodicity (4a x 4a). This vortex crystal exhibits no magnetic antiphase lines. It is shown that such a superstructure is magnetically stable in the approxima…
The doping, temperature and energy dependence of the dynamical spin structure factors of the underdoped lanthanum cuprates in the normal state is studied within the t-J model using the fermion-spin transformation technique. Incommensurate peaks are found at $[(1\pmδ)π,π]$, $[π,(1\pmδ)π]$ at relatively low temperatures with $δ$ linearly increasing with doping at the beginning and then saturating at higher dopings. These peaks broaden and weaken in amplitude with temperature and energy, in good agreement with experiments. The theory also predicts a rotation of these peaks by $π/4$ at even higher…
Suppression of superconductivity in favour of a striped phase, and its coincidence with a structural transition from a low-temperature orthorhombic (LTO) to a low-temperature tetragonal (LTT) phase, is a ubiquitous feature of hole-doped lanthanum cuprates. We study the effect of anisotropic strain on this transition using density-functional theory on both La$_2$CuO$_4$ and the recently-synthesised surrogate La$_2$MgO$_4$ to decouple electronic and structural effects. Strikingly, we find that compressive strain applied diagonally to the in-plane metal-oxygen bonds dramatically stabilises the LT…
Using Cu NQR in Eu-doped La_{2- x}Sr_xCuO_4 we show the evidence of the pinned stripe phase for moderate doping at 1.3K. The pinned fraction increases by one order of magnitude near hole doping x=1/8. The NQR lineshape reveals three inequivalent Cu positions: i) sites in the charged stripe; ii) nonmagnetic sites outside the stripes; iii) sites with a magnetic moment of 0.29 Bohr magnethon in the AF correlated regions. A dramatic change of the NQR signal for x > 0.18 correlating with the onset of bulk superconductivity corresponds to the depinning of the stripe phase. .
High Tc superconductors show a rich variety of phases associated with their charge degrees of freedom. Valence charges can give rise to charge ordering or acoustic plasmons in these layered cuprate superconductors. While charge ordering has been observed for both hole- and electron-doped cuprates, acoustic plasmons have only been found in electron-doped materials. Here, we use resonant inelastic X-ray scattering (RIXS) to observe the presence of acoustic plasmons in two families of hole-doped cuprate superconductors [La2-xSrxCuO4 (LSCO) and Bi2Sr1.6La0.4CuO6+d (Bi2201)], crucially completing t…
We report $^{139}$La nuclear magnetic resonance (NMR) measurements on La$_{2-x}$Sr$_x$CuO$_4$ ($0.07\leq x \leq 0.15$) and La$_{2-x}$Ba$_x$CuO$_4$ ($x=1/8$) single crystals, focusing on the spin freezing observed in 1/8-doped lanthanum cuprates. Charge stripe order seems to induce the inhomogeneous slowing down of spin fluctuations toward spin order and compete with superconductivity.
We report the analysis of the magnetic fluctuations in the superconducing La_{2-x}Sr_xCuO_4 and the related lanthanum cuprates having the different symmetry of the low temperature structure. The NMR and ESR investigations revealed the dynamical coexistence of the superconductivity and the antiferromagnetic correlations in the large part of superconductivity region of the phase diagram. We show that for all compounds, independent on their low temperature symmetry and on their superconducting properties, the enhancement of the spin stiffness near 1/8 doping takes place.
Based on the time-dependent Gutzwiller approximation we study the possibility that the diagonal incommensurate spin scattering in strongly underdoped lanthanum cuprates originates from antiferromagnetic domain walls (stripes). Calculation of the dynamic spin response for stripes in the diagonal phase yields the characteristic hour glass dispersion with the crossing of low energy Goldstone and high-energy branches at a characteristic energy Ecross at the antiferromagnetic wave-vector Q_{AF}. The high energy part is close to the parent antiferromagnet. Our results suggest that inelastic neutron …
Using Cu NQR in Eu-doped La_(2-x)Sr_xCuO_4 we find the evidence of the pinned stripe phase at 1.3K for 0.08<x<0.18. The pinned fraction increases by one order of magnitude near hole doping x=1/8. The NQR lineshape reveals three inequivalent Cu positions. A dramatic change of the NQR signal for x > 0.18 correlating with the onset of bulk superconductivity corresponds to the depinning of the stripe phase.
We report detailed 17O, 139La, and 63Cu Nuclear Magnetic Resonance (NMR) and Nuclear Quadrupole Resonance (NQR) measurements in a stripe ordered La1.875Ba0.125CuO4 single crystal and in oriented powder samples of La1.8-xEu0.2SrxCuO4. We observe a partial wipeout of the 17O NMR intensity and a simultaneous drop of the 17O electric field gradient (EFG) at low temperatures where the spin stripe order sets in. In contrast, the 63Cu intensity is completely wiped out at the same temperature. The drop of the 17O quadrupole frequency is compatible with a charge stripe order. The 17O spin lattice relax…
By comparing experimental results obtained in the study of the electron transport and magnetic properties of samples of lightly strontium-substituted lanthanum cuprates and the results of a previously published numerical analysis in the reduced elastic scattering space (RPS) of the elastic scattering cross-section, we construct a phenomenological classical self-consistent strong-binding energy density profile in the superconducting $La_{2-x}Sr_xCuO_4$ cuprate. It is found that the imaginary part of the reduced phase scattering space can be zero, almost constant, or strongly self-consistent, de…
Recent theoretical and experimental studies of hydrogen-rich materials at megabar pressures (i.e., >100 GPa) have led to the discovery of very high-temperature superconductivity in these materials. Lanthanum superhydride LaH$_{10}$ has been of particular focus as the first material to exhibit a superconducting critical temperature (T$_c$) near room temperature. Experiments indicate that the use of ammonia borane as the hydrogen source can increase the conductivity onset temperatures of lanthanum superhydride to as high as 290 K. Here we examine the doping effects of B and N atoms on the superc…
The phase diagram for hole-doped cuprates is discussed. By examining some recent inelastic neutron scattering data obtained on hole-doped cuprates we conclude that the coherent gap in hole-doped cuprates has most likely the magnetic origin and scales with Tc, on average, as 2Delta/kTc = 5.4.
Within a model that supports stripe spin and charge order coexisting with a d$_{x^2-y^2}$-wave superconducting phase, we study the self-consistently obtained electronic structure and the associated transverse dynamical spin susceptibility. In the coexisting phase of superconducting and static stripe order, the resulting particle-hole continuum can strongly damp parts of the low-energy spin wave branches. This provides insight into recent inelastic neutron scattering data revealing the dispersion of the low-energy collective magnetic modes of lanthanum based cuprate superconductors.
Within the t-t'-J model, the charge asymmetry in superconductivity of hole- and electron-doped cuprates is studied based on the kinetic energy driven superconducting mechanism. It is shown that superconductivity appears over a narrow range of doping in electron-doped cuprates, and the superconducting transition temperature displays the same kind of the doping controlled behavior that is observed in the hole-doped case. However, the maximum achievable superconducting transition temperature in the optimal doping in electron-doped cuprates is much lower than that of the hole-doped case due to the…
The tunneling spectra of the electron-doped cuprate Pr_2-xCe_xCuO4 as a function of doping and temperature is reported. We find that the superconducting gap, delta, shows a BCS-like temperature dependence even for extremely low carrier concentrations (studied here for the first time). Moreover, delta follows the doping dependence of Tc, in strong contrast with tunneling studies of hole-doped cuprates. From our results we conclude that there is a single superconducting energy scale in the electron-doped cuprates.
Strongly underdoped RuSr_1.9La_0.1GdCu_2O_8 has been comprehensively studied by dc magnetization, microwave measurements, magnetoresistivity and Hall resistivity in fields up to 9 T and temperatures down to 1.75 K. Electron doping by La reduces the hole concentration in the CuO2 planes and completely suppresses superconductivity. Microwave absorption, dc resistivity and ordinary Hall effect data indicate that the carrier concentration is reduced and a semiconductor-like temperature dependence is observed. Two magnetic ordering transitions are observed. The ruthenium sublattice orders antiferro…
The symmetries of the order parameter (OP) responsible for pairing and the OP responsible for phase coherence in hole-doped cuprates are discussed. We analyze angle-resolved tunneling, ARPES, Raman scattering and torque measurements performed on hole-doped cuprates. We conclude that, most likely, the OP responsible for phase coherence has the d-wave symmetry whereas the OP responsible for pairing has an anisotropic s-wave symmetry.
We study a model for low doped cuprates where holes aggregate into oriented stripe segments which have a vortex and an antivortex fixed to the extremes. We argue that due to the interaction between segments a state with macroscopic polarization is stabilized, which we call a ferronematic. This state can be characterized as a charge nematic which, due to the net polarization, breaks inversion symmetry and also exhibits an incommensurate spin modulation. Our calculation can reproduce the doping dependent spin structure factor of lanthanum cuprates in excellent agreement with experiment and allow…
Stripe fluctuations in La2NiO4.17 have been studied by 139La NMR using the field and temperature dependence of the linewidth and relaxation rates. In the formation process of the stripes the NMR line intensity is maximal below 230K, starts to diminish around 140K, disappears around 50K and recovers at 4K. These results are shown to be consistent with, but completely complementary to neutron measurements, and to be generic for oxygen doped nickelates and underdoped cuprates.
Within the t-t'-J model, the electron spectrum and quasiparticle dispersion in doped bilayer cuprates in the normal state are discussed by considering the bilayer interaction. It is shown that the bilayer interaction splits the electron spectrum of doped bilayer cuprates into the bonding and antibonding components around the $(π,0)$ point. The differentiation between the bonding and antibonding components is essential, which leads to two main flat bands around the $(π,0)$ point below the Fermi energy. In analogy to the doped single layer cuprates, the lowest energy states in doped bilayer cupr…
Within the t-t'-J model, the asymmetry of the electron spectrum and quasiparticle dispersion in hole-doped and electron-doped cuprates is discussed. It is shown that the quasiparticle dispersions of both hole-doped and electron-doped cuprates exhibit the flat band around the (π,0) point below the Fermi energy. The lowest energy states are located at the (π/2,π/2) point for the hole doping, while they appear at the (π,0) point in the electron-doped case due to the electron-hole asymmetry. Our results also show that the unusual behavior of the electron spectrum and quasiparticle dispersion is in…
We investigate the formation of charge domain walls in an electron-doped extended Hubbard model for the superconducting cuprates. Within an unrestricted Hartree-Fock approach, extended by the introduction of slave-bosons to obtain a more proper treatment of strong correlations, we demonstrate the occurrence of stripes in the (1,1) and (1,-1) directions having one doped electron per stripe site. The different filling, direction and width of these electron-doped stripes with respect to those obtained in the hole-doped systems have interesting observable consequences, which are discussed.
There is a clear discrepancy among the energy-gap values for different 90 K cuprates, inferred from tunneling measurements. By using the phase diagram for hole-doped cuprates we show that tunneling measurements performed on 90 K cuprates, simply, detect two different energy gaps: the pairing gap and the coherent gap, which are identical in conventional superconductors. We find that there are two reasons why tunneling measurements show in one cuprate exclusively the coherent gap while, in another cuprate, they show the pairing gap: (i) the number of CuO2 planes per unit cell in the cuprate, and…
We report neutron scattering studies on single crystals of the electron-doped (n-type) superconducting cuprate Nd2-xCexCuO4 (x=0.15) with Tc = 18 K and 25 K. Unlike the hole-doped (p-type) superconducting cuprates where incommensurate magnetic fluctuations commonly exist, the n-type cuprate shows commensurate magnetic fluctuations at the tetragonal (1/2 1/2 0) reciprocal points both in the superconducting and in the normal state. A spin gap opens up when the n-type cuprate becomes superconducting, as in the optimally doped p-type La2-xSrxCuO4. The gap energy, however, increases gradually up to…
We calculate the normal state Nernst signal in the cuprates resulting from a reconstruction of the Fermi surface due to spin density wave order. An order parameter consistent with the reconstruction of the Fermi surface detected in electron-doped materials is shown to sharply enhance the Nernst signal close to optimal doping. Within a semiclassical treatment, the obtained magnitude and position of the enhanced Nernst signal agrees with Nernst measurements in electron-doped cuprates.
Based on the unrestricted Gutzwiller approximation we study the possibility that the diagonal incommensurate spin scattering in the spin glass phase of lanthanum cuprates originates from stripe formation. Similar to the metallic phase two types of diagonal stripe structures appear to be stable: (a) site-centered textures which have one hole per site along the stripe and (b) ferromagnetic stair-case structures which are the diagonal equivalent to bond-centered stripes in the metallic phase and which on average have a filling of 3/4 holes per stripe site. We give a detailed analysis of the stabi…
A new electron-doped superconductor Li_x_Sr_2_CuO_2_Br_2_ with x = 0.15 has successfully been synthesized by an electrochemical Li-intercalation technique. The magnetic susceptibility shows superconductivity of bulk with the superconducting transition temperature Tc = 8 K. This compound is the first electron-doped superconducting cuprate with the K_2_NiF_4_ structure.
We present experimental data obtained by different techniques. Some of them are not easy to explain by any theoretical model presented in the literature. However, a MCS model of the superconductivity in hole-doped cuprates, proposed in our previous work, is capable to explain them. Thus, we present an evidence in favor of the MCS model.
Within the kinetic energy driven superconducting mechanism, the effect of the pressure on superconductivity in doped two-leg ladder cuprates is studied. It is shown that the superconducting transition temperature in doped two-leg ladder cuprate superconductors increases with increasing pressure in the underpressure regime, and reaches a maximum in the optimal pressure, then decreases in the overpressure regime. This domed shape of the pressure dependence of the superconducting transition temperature is similar to that of the pressure dependence of the longitudinal part of the superconducting g…
Within the framework of the kinetic energy driven d-wave superconductivity, the electronic structure of the electron doped cuprate superconductors is studied. It is shown that although there is an electron-hole asymmetry in the phase diagram, the electronic structure of the electron-doped cuprates in the superconducting-state is similar to that in the hole-doped case. With increasing the electron doping, the spectral weight in the $(π,0)$ point increases, while the position of the superconducting quasiparticle peak is shifted towards the Fermi energy. In analogy to the hole-doped case, the sup…
Using as a model the Hubbard Hamiltonian we determine various basic properties of electron-doped cuprate superconductors like ${Nd}_{2-x}{Ce}_{x}{CuO}_{4}$ and ${Pr}_{2-x}{Ce}_{x}{CuO}_{4}$ for a spin-fluctuation-induced pairing mechanism. Most importantly we find a narrow range of superconductivity and like for hole-doped cuprates $d_{x^{2}-y^{2}}$ - symmetry for the superconducting order parameter. The superconducting transition temperatures $T_{c}(x)$ for various electron doping concentrations $x$ are calculated to be much smaller than for hole-doped cuprates due to the different Fermi surf…
Within the t-J ladder model, superconductivity with a modified d-wave symmetry in doped two-leg ladder cuprates is investigated based on the kinetic energy driven superconducting mechanism. It is shown that the spin-liquid ground-state at the half-filling evolves into the superconducting ground-state upon doping. In analogy to the doping dependence of the superconducting transition temperature in the planar cuprate superconductors, the superconducting transition temperature in doped two-leg ladder cuprates increases with increasing doping in the underdoped regime, and reaches a maximum in the …
The doping and temperature dependent conductivity of electron-doped cuprates is analysed. The variation of kinetic energy with doping is shown to imply that the materials are approximately as strongly correlated as the hole-doped materials. The optical spectrum is fit to a quasiparticle scattering model; while the model fits the optical data well, gross inconsistencies with photoemission data are found, implying the presence of a large, strongly doping dependent Landau parameter.
Inelastic Neutron Scattering (INS) data in LSCO, YBCO and Bi2212 are discussed. In the literature, the INS spectra remain far from being comprehensively understood. We show that local (Q-integrated) susceptibility data and the energy dependence of the spin susceptibility at antiferromagnetic vector, Q = (p,p), can be interpreted by using the phase diagram for hole-doped cuprates. We analyze also the origin of the resonant peak which relates to the order parameter for long-range phase coherence in hole-doped cuprates. Thus, we present an interpretation of neutron data in LSCO, YBCO and Bi2212 p…
We amend ab initio strongly-correlated band structures by taking into account the band-tailing phenomenon in doped charge-transfer Mott-Hubbard insulators. We show that the photoemission from band tails accounts for sharp "quasi-particle" peaks, rapid loss of their intensities in some directions of the Brillouin zone ("Fermi-arcs") and high-energy "waterfall" anomalies as a consequence of matrix-element effects of disorder-localised states in the charge-transfer gap of doped cuprates.
Systematic analysis of the planar resistivity, Hall effect and cotangent of the Hall angle for the electron-doped cuprates reveals underlying Fermi-liquid behavior even deep in the antiferromagnetic part of the phase diagram. The transport scattering rate exhibits a quadratic temperature dependence, and is nearly independent of doping, compound and carrier type (electrons vs. holes), and hence universal. Our analysis moreover indicates that the material-specific resistivity upturn at low temperatures and low doping has the same origin in both electron- and hole-doped cuprates.
Recent quantum oscillation measurements on underdoped cuprates are shown to be consistent with the predictions of a mean field theory of the 1/8 magnetic antiphase stripe order proposed to occur in high-$T_c$ cuprates. In particular, for intermediate values of the stripe order parameter, the magneto-transport is found to be dominated by an electron pocket.
We study charge ordered d-wave resonating valence bond states (dRVB) in the doped cuprates, and estimate the energies of these states in a generalized $t-J $ model by using a renormalized mean field theory. The long range Coulomb potential tends to modulate the charge density in favor of the charge ordered RVB state. The possible relevance to the recently observed $4 \times 4$ checkerboard patterns in tunnelling conductance in high $T_c$ cuprates is discussed.
We present conductance-voltage (G-V) data for point contact junctions between a normal metal and the electron doped cuprate superconductor Pr{2-x}Ce{x}CuO4 (PCCO). We observe a zero bias conductance peak (ZBCP) for the under-doped composition of this cuprate (x=0.13) which is consistent with d-wave pairing symmetry. For optimally-doped (x=0.15) and over-doped (x=0.17) PCCO, we find that the G-V characteristics indicate the presence of an order parameter without nodes. We investigate this further by obtaining point contact spectroscopy data for different barrier strengths and as a function of m…
Recent experiments in underdoped hole-doped cuprates have shown the presence of two energy scales in the Raman spectrum in the superconducting state. This feature has a natural explanation in some models in which pseudogap and superconductivity compete. In electron-doped cuprates antiferromagnetic correlations are believed to survive in the superconducting state, and to produce a pseudogap above the critical temperature. Contrary to hole-doped systems, in electron-doped compounds only one energy scale appear since the pair breaking Raman intensity peaks in both B$_{1g}$ (antinodal) and B$_{2g}…
We report a tunneling study between Pr_2-xCe_xCuO_{4-delta} (PCCO) and Lead as a function of doping, temperature and magnetic field. The temperature dependence of the gap follows the BCS prediction. Our data fits a nonmonotonic d-wave order parameter for the whole doping range studied. From our data we are able to conclude that the electron-doped cuprate PCCO is a weak coupling, BCS, dirty superconductor.
Many important questions for high-$T_c$ cuprates are closely related to the insulating nature of parent compounds. While there has been intensive discussion on this issue, all arguments rely strongly on, or are closely related to, the correlation strength of the materials. Clear understanding has been seriously hampered by the absence of a direct measure of this interaction, traditionally denoted by $U$. Here, we report a first-principles estimation of $U$ for several different types of cuprates. The $U$ values clearly increase as a function of the inverse bond distance between apical oxygen a…
Superconductivity research is like running a marathon. Three decades after the discovery of high-Tc cuprates, there have been mass data generated from transport measurements, which bring fruitful information. In this review, we give a brief summary of the intriguing phenomena reported in electron-doped cuprates from the aspect of electrical transport as well as the complementary thermal transport. We attempt to sort out common features of the electron-doped family, e.g. the strange metal, negative magnetoresistance, multiple sign reversals of Hall in mixed state, abnormal Nernst signal, comple…
We study the quantum transition from an antiferromagnet to a superconductor in a model for electron- and hole-doped cuprates by means of a variational cluster perturbation theory approach. In both cases, our results suggest a tendency towards phase separation between a mixed antiferromagnetic-superconducting phase at low doping and a pure superconducting phase at larger doping. However, in the electron-doped case the energy scale for phase separation is an order of magnitude smaller than for hole doping. We argue that this can explain the different pseudogap and superconducting transition scal…
We investigate the electronic states in the antiferromagnetic (AF) phase of electron-doped cuprates by using numerically exact diagonalization technique for a t-t'-t''-J model. When AF correlation develops with decreasing temperature, a gaplike behavior emerges in the optical conductivity. Simultaneously, the coherent motion of carriers due to the same sublattice hoppings is enhanced. We propose that the phase is characterized as an AF state with small Fermi surface around the momentum k=(π,0) and (0,π). This is a remarkable contrast to the behavior of hole-doped cuprates.
We use the idea of the Wigner probability distribution (WPD) in a reduced scattering phase space (RPS) for the elastic scattering cross-section, with the help of a Tight-Binding (TB) numerical procedure allowing us to consider the anisotropic quantum effects, to phenomenologically predict several phases in these two novel unconventional superconductors. Unlike our previous works with pieces of evidence that these two compounds are in the unitary strong scattering regime and that superconductivity is suppressed by the atoms of strontium in both materials, several phases are built. In the case o…
The purpose of this paper is to discuss a phase diagram of hole-doped cuprates. Hole-doped cuprates have a very rich phase diagram as a function of doping. This is due to a charge inhomogeneity in CuO_2 planes: the charge distribution in CuO_2 planes is inhomogeneous both on a nanoscale and macroscale. Depending on doping level, the CuO_2 planes comprise at least four different types of clusters having a size of a few nanometers. Each type of clusters has its own features. As a consequence, the common phase diagram consists of, at least, seven different energy/temperature scales. As an example…
An antiferromagnetic (AF) spin fluctuation induced pairing model is proposed for the electron-doped cuprate superconductors. It suggests that, similar to the hole-doped side, the superconducting gap function is monotonic d_{x^2-y^2}-wave and explains why the observed gap function has a nonmonotonic d_{x^2-y^2}-wave behavior when an AF order is taken into account. Dynamical spin susceptibility is calculated and shown to be in good agreement with the experiment. This gives a strong support to the proposed model.
Pairing Correlations are studied numerically in the hole-doped spin-fermion model for cuprates. Simulations performed on up to 12x12 clusters provide robust indications of D-wave superconductivity away from half-filling. The pairing correlations are the strongest in the direction perpendicular to the dynamic stripe-like inhomogeneities that appear in the ground state at some densities. An optimal doping, where the correlations reach a maximum value, was observed at about 25% doping, in qualitative agreement with hight T_{c} cuprates' experiments. On the other hand, pairing correlations are sup…
We apply the spin-fermion model to study the normal state and pairing instability in electron-doped cuprates near the antiferromagnetic QCP. Peculiar frequency dependencies of the normal state properties are shown to emerge from the self-consistent equations on the fermionic and bosonic self-energies, and are in agreement with experimentally observed ones. We argue that the pairing instability is in the $d_{x^{2}-y^{2}}$ channel, as in hole-doped cuprates, but theoretical $T_{c}$ is much lower than in the hole-doped case. For the same hopping integrals and the interaction strength as in hole-d…
The electron-doped cuprates were studied by electronic Raman spectroscopy across the entire region of the superconducting (SC) phase diagram. We determined that the magnitude of the SC order parameter varies between 4.6 and 3.5 k_BT_c, consistent with weak coupling BCS theory. Using a ``Raman conductivity" sum rule, we found that doped carriers divide into coherent quasi-particles (QPs) and carriers that remain incoherent. The coherent QPs mainly reside in the vicinity of (pi/2a, pi/2a) regions of the Brillouin zone. The carriers doped beyond optimal doping remain incoherent. Only coherent QPs…
We report on the magnetic phase diagram of a hole-doped cuprate Ca$_{2-x}$Na$_{x}$CuO$_{2}$Cl$_{2}$, which is free from buckling of CuO$_2$ planes, determined by muon spin rotation and relaxation. It is characterized by a quasi-static spin glass-like phase over a range of sodium concentration ($0.05\leq x\leq 0.12$), which is held between long range antiferromagnetic (AF) phase ($x\leq 0.02$) and superconducting phase where the system is non-magnetic for $x\geq 0.15$. The obtained phase diagram qualitatively agrees well with that commonly found for hole-doped high-\tc cuprates, strongly sugges…
We report resistivity, Hall effect, Nernst effect, and magnetoresistance measurements on T'-phase La1.85Y0.15CuO (LYCO) films prepared by pulsed laser deposition under different oxygen conditions. Our results show that superconductivity in LYCO originates from an oxygen-doped Mott-like insulator and not from a weakly correlated, half-filled band metal as proposed previously.
We analyze high-resolution scanning tunneling spectra of the electron-doped cuprate Pr0.88LaCe0.12CuO4 (T_c = 24 K). We find that the spectral fine structure below 35 meV is consistent with strong coupling to a bosonic mode at 16 meV, in quantitative agreement with early tunneling spectra of Nd1.85Ce0.15CuO4. Since the energy of the bosonic mode is significantly higher than that (9.5-11 meV) of the magnetic resonance-like mode observed by inelastic neutron scattering, the coupling feature at 16 meV cannot arise from strong coupling to the magnetic mode. The present work thus demonstrates that …
Differentiation of electron doping and oxygen reduction in electron-doped cuprates
Institute for Solid State Physics, The University of Tokyo（东京大学固体离子体研究所）；Department of Engineering and Applied Sciences, Sophia University（上智大学理工学部）；Department of Applied Physics, Tohoku University（东北大学应用物理系）；UVSOR Synchrotron Facility, Institute for Molecular Science（分子科学研究所UVSOR同步辐射设施）
An understanding of the high-temperature copper oxide (cuprate) superconductors has eluded the physics community for over thirty years, and represents one of the greatest unsolved problems in condensed matter physics. Particularly enigmatic is the normal state from which superconductivity emerges, so much so that this phase has been dubbed a "strange metal." In this article, we will review recent research into this strange metallic state as realized in the electron-doped cuprates with a focus on their transport properties. The electron-doped compounds differ in several ways from their more tho…
