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北美退伍军人节(Veterans Day),12 日无更新
arXiv 0809.5069cond-mat.str-el
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Ba $_{3}$ Cr $_{2}$ O $_{8}$中弱耦合$s = 1/2$量子自旋单态

Weakly coupled $s = 1/2$ quantum spin singlets in Ba$_{3}$Cr$_{2}$O$_{8}$

M. Kofu, J. -H. Kim, S. Ji, S. -H. Lee, H. Ueda, Y. Qiu, H. -J. Kang, M. Green, Y. Ueda

摘要:

利用单晶非弹性中子散射和粉末中子衍射,我们的特点是磁相互作用的Ba $_3$ Cr $_2$ O $_8$。在没有电场的情况下,我们发现在$(h,h,l)$散射面上存在三种单重态到三重态的激发模式。我们完整的分析表明,这三种模式是由于空间各向异性interdimer相互作用,是由周围的Jahn-Teller活性铬$^{5+} (3d^1)$的氧四面体的局部扭曲引起的。$J_0 = 2.38(2)$ meV的强二聚体内耦合和弱二聚体间相互作用($|J_{\rm inter}| \leq 0.52(2)$ meV)使得Ba $_3$ Cr $_2$ O $_8$成为弱耦合$s = 1/2$量子自旋二聚体的良好模型系统。

英文摘要:

Using single crystal inelastic neutron scattering with and without application of an external magnetic field and powder neutron diffraction, we have characterized magnetic interactions in Ba$_3$Cr$_2$O$_8$. Even without field, we found that there exist three singlet-to-triplet excitation modes in $(h,h,l)$ scattering plane. Our complete analysis shows that the three modes are due to spatially anisotropic interdimer interactions that are induced by local distortions of the tetrahedron of oxygens surrounding the Jahn-Teller active Cr$^{5+} (3d^1)$. The strong intradimer coupling of $J_0 = 2.38(2)$ meV and weak interdimer interactions ($|J_{\rm inter}| \leq 0.52(2)$ meV) makes Ba$_3$Cr$_2$O$_8$ a good model system for weakly-coupled $s = 1/2$ quantum spin dimers.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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